"The resonant frequencies of the magnet power supply are investigated. It is found that there are eleven resonant modes in addition to the desired mode of operation with six additional resonant frequencies. From measurements of the choke model, it appears that the frequencies of some of the spurious modes may lie in the same range as the desired mode of operation."

"The effect of correcting quadrupole lenses on the betatron oscillation characteristics of an AG synchrotron was studied, and general formulas are given for the fractional changes of the amplitude and phase functions. Calculations performed for different setups of different numbers of lenses for the CEA synchrotron structure point out that one may correct for sizable errors in the n- value by means of 8 pairs of quadrupole lenses in two consecutive straight sections with the focusing lens between defocusing sectors and vice versa. An increase of BETA /sub max/ of about 5% is obtained for DELTA n/n approximately 0.04. It was found that the necessary corrections can probably be obtained satisfactorily with lenses of 6 in. length. "

The purpose of the test was to obtain data on the decontamination factors for Cesium-136, Cesium-137, Strontium-92, one hour gross iodine and Iodine-131. This data will be used to determinate efficiency of lithium hydroxide resin for removing radioactive cations and anions. The denomination factors for a particular demineralizer using lithium hydroxide resign were found to vary for different radioisotopes. This variation was from 2.3 for Cesium136 to 77,000 for gross iodine.

The purpose of the test was to determine if the 1A Canal Water System Demineralizers can be satisfactorily charged with resin. The 1A Canal Water System Demineralizer was satisfactorily charged with resin and conductivity of the demineralizer effluent was less than 0.1 microbes as specified in the Test Procedure.

From the point of view of predicting melting behavior of fuel elements containing fission products after 50 percent burn-up, the fuel can be considered to consist of 2000 moles Th, 150 moles U, 55 moles of rate earth metal, 31 moles of Zr, 25 moles of Mo, 20 moles of Rh-Ru-Tc, and 15 moles of alkaline earth metal. All other fission products are present in too small amounts to have any important effect upon the melting point or will have vaporized. However, the presence of alkali metal vapor should be considered.

The purpose of the survey was to determine the radiation levels in the 1 D Boiler Chamber during plant operation. The conclusion of this survey is that the radiation level in the 1 D Boiler Compartment with the 1A, 1B, and 1C Main Coolant loops in service at approximately 100 per cent power ranged from .03 MR/HR to 6.0 MR/HR.

The statistical theory of pressure broadening is developed for any interaction law in which the potential energy is inversely proportional to some power of the distance between the molecules, including cases in which the forces change sign. This note is intended to prove two propositions: A. When a spectral line is broadened by single impacts of perturbing molecules and the half-width of the line is delta infinity, the statistical theory of broadening is applicable provided delta infinity . R >> 1. In this criterion T is a time comparable to the interval in which the perturbed traverses a distance equal to the impact parameter. B. Far in the wings of a line the statistical theory is always applicable.

Work was completed on the high-temperature, high efficiency air filter. Technical assistance was given at a large-scale, privately financed run of an all-glass medium. Full-size filers have been produced in quantity and are offered by manufacturers; it is considered that commercial manufacture has been established. A survey was made of air sampling practices at 37 laboratories. Analysis of the survey results indicated that 22 different kinds of air-sampling filer media were in use among the laboratories questioned. We have recommended that air-assay practice be simplified by use of fewer media. A group of five media has been proposed as adequate for meeting all requirements. Laboratory work was done on the development of a high-efficiency, low-ash, all-purpose, air-assay paper. Two methods of approach were tried. In one an effort was made to produce cellulose fibrils in sufficient quantity and quality to act as the fine-fiber component of a filter. Only moderate success was attained. Better promise was shown by combining synthetic organic microfibers with cellulose fibers in a wet-formed sheet. No plant work was undertaken on this item.

Studies are being made on the recovery of thorium (and uranium) from granitic rock, since this source represents a very large potential thorium reserve for the nuclear power industry. In preliminary leaching studies on 16 granite samples (containing 8-95 ppm thorium and 1.5-16 ppm uranium), maximum recoveries of thorium and uranium ranged 30-85% and 15-65% respectively, and sulfuric acid consumption was high (30-120 lbs H2SO4 per ton of granite). A relatively high acidity was needed to obtain rapid and efficient dissolution of the soluble thorium fraction. The cost of treating granite was estimated at $3.50-5.20 per ton, variations within this range being dependent primarily on differences in acid consumption for different granites. Estimated costs per pound of thorium plus uranium recovered ranged $30-500.

The attached memo by G. N. Krouse of Sturm-Krouse, Inc. gives results of a preliminary analysis of the deflections of beam holes due to thermal expansion and internal pressure in the vessel. A partial solution of the problem is suggested. Based on preliminary pressure-temperature data the following deflections were derived: Movement of horizontal beam tubes = 0.046 in. Movement of Engineering facility tubes = 0.117 in. Vertical motion of the vessel at the horizontal beam tubes due to thermal expansion may be eliminated by locating the supports in that plane. That also will reduce the expansion at the point where the slant tubes pierce the vessel wall.

The problem of controlling the surface temperatures of core vessels in two-region aqueous homogeneous reactors has been examined by analyzing several possible systems for cooling the wall: (1) direction of the inlet core fluid along the wall at a high velocity; (2) passage of heavy water through the wall of a double-wall core vessel; and (3) flow of cool blanket slurry past the wall.

The gamma dose rate in the motor region of the HRT fuel circulation pump was measured with the pump scroll full of radioactive solution. Extrapolation of the data to the solution activity expected in the pump under normal operation gives a dose rate well below that which would result in excessive gas production in the stator can within the life of the pump. The above dose rate does not include the effects of fast neutrons from the fuel solution or of the general cell radiation level in the vicinity of the pump. It appears that the possibility of gas production in the stator from the cell background radiation is sufficiently great to warrant the installation of a shield around the outside of the motor end of the fuel circulating pump.

Measurements of flow rate through the fuel high-pressure system sampler indicate that the average flow rates is about 0.29 gpm (145 lb/hr) plus or minus 50%, which affords an adequate purge of from 12 to 36 volumes through the sample line if the full fifteen minutes of purging is allowed before isolating the sample. The fuel sample cooler was fund to have adequate capacity to reduce the temperature of the fuel solution form about 275 to 70 C, using pre-heated cooling water at 70 C. Uncertainties in temperature measurements make it impossible to estimate an observed over-all heat transfer coefficient.

Preliminary results of tests wit the Westinghouse 100A pump indicate that Al2)3 and tungsten carbide coated bearing-journal assemblies prepared by the Linde process are not promising as substitutes for the graphitar-stellite combination. The front Al2O3 assembly failed at start-up with water and both front and rear tungsten carbide assemblies failed after 121 hours with water at 245 C.

The radiolytic decomposition of tributyl phosphate has been show by burr to product gases, acids, and polymers. the acids that are formed can limit the usefulness of tributyl phosphate for the processing of radioactive materials. The study of acid formation on radiolysis therefor becomes important to us for the understanding of the mechanism of acid formation, the influence of added materials and the effect of the structure of organo- phosphorous compounds. Samples of purified esters have been irradiated in the ORNL cobalt source. Conclusions: (1) The formation of acid from tributyl phosphate during irradiation with cobalt gamma rays involves a mechanism that is not a primary step. Evidence has been obtained for a secondary reaction that is minimized by the presence of certain compounds. (2) Toluene acting as an inhibitor for radiolytic formation of acid may indicate the usefulness of an aromatic hydrocarbon diluent in processing. (3) The aromatic hydrocarbon, when phenyl, was not effective when it was part of the molecule. (4) First tests revealed that dibutyl butyl-phosphonate produced less acid the TBP and may warrant further consideration for process application.

Section 9.0 is the "Chemical Processes for Fission Product Concentration, Removal or Fixation" section of the Status Report on the Disposal of Radioactive Wastes. The report is divided into four areas: (1) Introduction; (2) Summary of waste processes; (3) Concept of a multipurpose waste processing facility; and (4) Details of some of the waste processes.

A reference design of a large high power density core has been established representing the available technology as of August, 1960. Reference core performance and cost should improve considerably after incorporation of improvements now under study.

Uranium precipitates obtained from Congo leach liquors by an ion exchange process contained more than 0.1 percent chloride. Attempts were made to reduce the chloride content of typical precipitates by calcination of dried precipitate, releaching of dried precipitate with water, and washing of wet precipitate with water. Washing of wet precipitate with an aqueous solution of 0.25 percent Na2SO4, to prevent peptization, provided a simple solution to the problem.

In order that fairly accurate thermal stress calculations can be made on the ART, it is necessary to have a reasonable picture of the temperature distribution in the reactor. To get the temperature distributions, and to determine cooling requirements in various parts of the reactor, one must know the heat deposition rates due to alpha particles, beta rays, gamma rays, and neutrons in all parts of the reactor. The present report contains only the basic physical data necessary to determine the heat deposition rates due to gamma rays. Neutron fluxes in the core and reflector regions of the ART are to be obtained from two-dimensional multigroup calculations (performed by the Curtiss-Wright Corporation). These fluxes, in conjunction with the neutron absorption cross sections, determine the neutron capture and inelastic scattering rates in the core and in the reflector. The data in this report permit the calculation of the number of gamma rays originating at various energies at every point in the core and reflector.

Several potential hazards that have been recognized and anticipated in the design and fabrication of the pressure vessel in the Homogeneous Reactor Test are discussed. These hazards results from the high operating pressure and temperature of the reactor, the exposure of the reactor vessel material to potential embrittlement and other affects of fast-neutron irradiation, and the need for containment of corrosive flowing liquids. The steps taken in recognition of these hazards are also discussed. The applicability of present codes to the reactor vessel fabrication is considered. Additional fields are suggested where recommended practices developed by code writing bodies could assist in development-type reactor design and fabrication.

Technique used in deriving values of the linac ball tuner settings to produce various fields is discussed briefly, and tables showing ball tuner change numbers and values used in making up the ball tuner change numbers are given.

In the memorandum entitled "Stored Energy in BNL Reactor Graphite", dated February 25, 1953, there is described an experiment conducted by Gurinsky's group to determine the energy per gram of irradiated graphite released in a 200°C anneal. Similar experiments were subsequently conducted by W. Kosiba, differing from the original in two particulars: a) Instead of two graphite samples, one normal, and one irradiated, Kosiba used only an irradiated sample which he heated first to release the stored energy, and then again after the energy was released. In this way, he obtained time against temperature curves for both normal and irradiated graphite from the same sample. (These curves are graphed for each run in Figs. 1 thru 5.) b) The vycor tubing used in the original experiment was not used by Kosiba. Five runs of this experiment were selected, Runs 4P, 13, 36, and 40 at furnace temperatures of 200°C, and Run 45 at a furnace temperature of 400°C.

During the last year we have been attempting to increase our understanding of the significance of the various dilution methods used to measure the extra-cellular fluid. When the dilution methods were first proposed to obtain a measure of the extracellular fluid volume, it was hoped that an agent could be found which would distribute uniformly and exclusively throughout this compartment, which would approach equilibrium rapidly, and which could be measured by simple and accurate procedures. We have turned our attention chiefly to the methods themselves using dogs and non-edematous adults as subjects.

At the request of 234-5 Development, studies of a system for controlling plutonium powder transfer were undertaken by Process Equipment Development. This report presents details of equipment designed to fulfill requirements and proposes equipment for installation on additional Hot Button Line prototypes.