A 19-rod Zircaloy-clad half-length PRTR spike element successfully irradiated to high plutonium burnout at full power in the ETR shoved partial bonding of the core and cladding. Unsatisfactory autoclave films on the Zircaloy cladding of the PRTR Al-Pu fuel elements are delaying final assembly of the first 30 clusters. Further conditioning of the autoclaves and the availability of permanent etching facilities are expected to correct the present difficulties.

The evaluation of the inductance of an electrical component is often important in understanding and operating an electrical circuit. Inductance is defined by several equations, the most common being e= -L d1/dt . This equation defines inductance as the constant which relates the back emf produced in an element to the time-rate-of-change of current.

Investigation of aqueous and steam corrosion at elevated temperature has been carried on at Hanford for several tears. A number of reports have been published on various phases of the corrosion program but, except for monthly reports, little has been written on the progress of the Corrosion and Coatings Operation alloy development program. This interim report will outline the more important current phases of the aluminum alloy program.

In the continuing search for better methods of effecting the secondary fusion welded closure in Alsi bonded aluminum clad uranium metal fuel element, an article on "The Twin-Argon Welding Process" by J. A. Donellon was recently found in the September 1954 issue if the British Welding Journal. From a review of the article, the process appeared to have enough possibilities to warrant exploring it. Communication were established with the General Electric Company, Ltd..

The measurements reported here are companion measurements to those reported earlier in HW-63585. The only significant difference between the measurements is that 1.8 w/o enrichment UO2 fuel was used for the first set, and 2.6 w/o enrichment UO2 fuel was used for the measurements described in this report. The new results will be presented graphically, and for completeness, the details of the measurement will be included here as well as in HW-63585.

The development of a miniature probe was desired for measuring approximate single nuclide beta dose rate in solution and in various animal organs. This probe designed for biological experiments, was to have maximum possible sensitivity to detect low levels of nuclide concentrations. The desired dimensions of the light pipe were to be approximately one-fourth-inch diameter with lengths of three to twelve inches.

Pressurized water nuclear reactors may be designed based upon either of two concepts: (1) pressure vessel, wherein the entire core is placed in a large, high strength fuel channels within a low pressure container. The Plutonium Recycle Test Reactor is a pressure tube type reactor. Selection of this basic type of pressurized water reactor depended to an appreciable extent upon the availability of suitable pressure tubing.

A correlation between the optical densities if the Pb-Sn alloy system and UO2 with respect to Co^60 gamma radiation has been determined. This enables one to fabricate density standards of whatever geometry may be desired for one in the gamma absorptiometer by simply casting a Pb-Sn alloy of the proper composition to correspond to the density required.

The wrist badge provides a dosimeter that is useful in estimating the radiation dose to the hands and forearms. Its new shield system gives good gamma and slow neutron dose discrimination with duPont 552 film packets. The film can be evaluated using the present technique and equipment. Several attempts to develop hand dosimeters have been made. Finger rings using film have been used routinely but have not been entirely satisfactory for all situations. The wrist badge was developed to provide improved gamma and slow neutron dose measurement of the upper extremities under certain appropriate conditions. The wrist badge dosimeter is not a substitute or alternate for finger ring dosimeters but is a necessary dosimeter for some extremity exposure situations.

Ultrasonic cleaning uses high-frequency sound waves to induce cavitation within a cleaning, medium. During cavitation, millions of small bubbles form and collapse, resulting in agitation proportional to the energy put into the solution. The making and breaking of these bubbles produce the scrubbing action associated with ultrasonic cleaning.

In October 1959, a combination testing station developed at HAPO was reported to the Sheath committee. This testing station consisted of electronic instrumentation and mechanical scanning equipment to check coextruded fuel elements (rod and tube) for clad thickness, clad integrity, bond, and core integrity. The clad tests are performed by eddy current methods and the other are ultrasonic.

The Plutonium Recycle Test Reactor is heavy water moderated with a heavy or light water reflector contained by a complex aluminum vessel called a Calandria. ( See Figure 1). Construction of this vessel started in August, 1958, at a large West Coast vendor's plant and was completed at Hanford in December, 1959. The fabrication problems associated with a high integrity welded aluminum vessel were generally unrealized prior to this period. This report covers the fabrication of the Calandria and lists recommendations for improving the design and reducing the cost.

Facilities shall be provided in the 221-U Building for storing the metal solution product of the dissolution step in existing tankage from U, T, and B Plants until a reprocessing campaign is scheduled through Redox. This section shall provide a sampling tank for fuel accountability sampling and a pump tank from which the solution will be pumped via a cross-country pipeline to Redox for further processing.

The large scale application of Zircaloy-2 pressure tubes for structural use either in or out of reactor service, is without precedent. For more common materials, there normally are adequate data and long operating histories on which to base design and service limits. In the absence of such information for Zr-2, several investigative programs have been devised to provide much of the information from which design and service limits may be defined for Zr-2 pressure tubes. These investigations encompass in-and-out-of-reactor creep and stress-rupture testing, pre-and-post irradiation testing, and bust strength, as well as the effect of flaws or defects (from both fabrication and service origins) on burst strength and fracture characteristics. Already creep and stress rupture testing of unirradiated Zircaloy-2 is well advanced, and some experimental pre-irradiation burst testing has been carried out and will be extended rapidly as improved equipment becomes available. One irradiated KER tube sample has been burst tested and the requirement for post irradiation burst testing equipment have been defined.

In the past several years the use of neutron monitors for Pu concentration monitoring has been expanded in the Chemical Processing Department. Most of these monitors have been quite successful, and considerable effort is being made to improve the operation of both existing and future monitoring systems. One of the major improvements has been the development and use of a transistorized pre-amplifier or impedance matching circuits. This unit solves several problems associated with the use of boron trifluoride (BF3) neutron detectors in process monitoring; e.g., vacuum tube pre-amp failure because heat is not being conducted away.

A brief series of experiments was performed to study the high temperature reaction of the Zircaloy-uranium-aluminum system at the request of Reactor Engineering Operation, Irradiation Processing Department. Knowledge of the high temperature behavior of this combination of materials is important to the evaluation of reactor behavior during possible accidental over-heating of a fuel channel.

Calcination of liquid radioactive wastes, the process of converting metal nitrates and sulfates to oxides by heat, is under development at Hanford as a means of reducing these liquids to a dry powder or solid which can be stored safely. Radiant-heat spray calcination, one of the methods under study, was first investigated at the Oak Ridge K-25 Plant (1) as a possible method of calcining uranyl nitrate to uranium trioxide. The process has also been under extensive development at the Pulp and Paper Research Institute of Canada (2) and is designated by them as the Atomized Suspension Technique.

Limitations on the service life of a fuel element imposed by degradation of the fissile core during irradiation have been a matter of great concern. Limitations imposed by changes in cladding properties during irradiation should be evaluated with equal care. Zircaloy-2, stainless steel, and aluminum alloys have been irradiated in the form of cladding on metallic and ceramic fuel elements. Several aspects of fuel behavior as influenced by these clad materials will be discussed. All observations related to irradiation behavior in this paper have been made on fuel specimens irradiated in water coolant.

The feasibility of removing and recovering cesium-137 from various HAPO process solutions by precipitation of Cs2ZnFe(CN)6 has been demonstrated previously. Pilot plant studies of calcination and steam hydrolysis of non-radioactive Cs2ZnFe(CN)6 precipitates by members of the Process Equipment Development Operation are currently in progress. In support of these pilot plant studies, experiments were performed to determine the extent, if any, to which cesium volatilizes during calcination and hydrolysis of Cs2ZnFe(CN)6 precipitates containing cesium-137. Experimental procedures and results are presented in this report.

This report discusses the mathematical and statistical questions concerned with the estimation of a leak rate from data collected during a reactor containment vessel pressure test such as that performed on the PRTR vessel in May, 1959. A mathematical method is suggested in Section 3 for the construction of a total number of gas molecules in the containment vessel time series using vessel absolute pressure and temperature readings at several positions within the vessel. A formula for the precision of the series is given in terms of the individual instrument precisions. The question of accuracy and its relationship to the temperature gradient within the vessel is also considered.

The work described was undertaken to provide data for nuclear safety studies concerning NPF reprocessing equipment. The original objective was to determine the uranium density and water (hydrogen) content of UO2-H2O mixtures ranging from compact centrifuge cakes to dilute slurries. The scope was later expanded to include mixtures of UO2 with hydrocarbon oil and mixtures of UO3-H2O.

The need for criticality control in the proposed reprocessing of slightly enriched non-production fuels at Hanford has led to the development of a geometrically "safe", vertical tube, recirculating dissolver. A study of the nitric acid dissolution of uranium dioxide in a pilot plant dissolver of this type is reported here. The study was pointed toward the comparison of uranium dioxide dissolution rates in a batch and a recirculating dissolver and the definition of hydraulic problems associated with the recirculation of nitric acid, by air lift, technique through beds of reacting uranium dioxide.

The primary purpose of a cleanup system in a recirculating water loop is to maintain the best possible water quality conditions. This is normally accomplished by continuously purifying all or a portion of the coolant. A secondary objective of the cleanup system is to help maintain the system pH at a constant value. A system that will satisfactorily accomplish both of these objectives is at times difficult to obtain. Generally the pH control characteristics are sacrificed in favor of the more important cleanup requirements. A somewhat new approach to the problem pf cleanup system design appears to offer a solution to this problem for high pH systems.

The result of a leak in a PRTR process tube between the flow monitor and the heated section would be to increase the flow through the monitor, but to decrease the flow through the heated section. The concern for the case of small leaks is whether the increase in flow through the flow monitor is sufficient to cause a high flow tip and a reactor scram for the condition where the flow through the heated section is reduced to the point to cause excessive fuel element temperatures.