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3,4,3-LI(1,2-HOPO): In Vitro Formation of Highly Stable Lanthanide Complexes Translates into Efficacious In Vivo Europium Decorporation
The spermine-based hydroxypyridonate octadentate chelator 3,4,3-LI(1,2-HOPO) was investigated for its ability to act as an antennae that sensitizes the emission of Sm{sup III}, Eu{sup III}, and Tb{sup III} in the Visible range (Φ{sub tot} = 0.2 - 7%) and the emission of Pr{sup III}, Nd{sup III}, Sm{sup III}, and Yb{sup III} in the Near Infra-Red range, with decay times varying from 1.78 μs to 805 μs at room temperature. The particular luminescence spectroscopic properties of these lanthanide complexes formed with 3,4,3-LI(1,2-HOPO) were used to characterize their respective solution thermodynamic stabilities as well as those of the corresponding La{sup III}, Gd{sup III}, Dy{sup III}, Ho{sup III}, Er{sup III}, Tm{sup III}, and Lu{sup III} complexes. The remarkably high affinity of 3,4,3-LI(1,2-HOPO) for lanthanide metal ions and the resulting high complex stabilities (pM values ranging from 17.2 for La{sup III} to 23.1 for Yb{sup III}) constitute a necessary but not sufficient criteria to consider this octadentate ligand an optimal candidate for in vivo metal decorporation. The in vivo lanthanide complex stability and decorporation capacity of the ligand were assessed, using the radioactive isotope {sup 152}Eu as a tracer in a rodent model, which provided a direct comparison with the in vitro thermodynamic results …
Date:
July 13, 2011
Creator:
Sturzbecher-Hoehne, Manuel; Ng Pak Leung, Clara; Daleo, Anthony; Kullgren, Birgitta; Prigent, Anne-Laure; Shuh, David K. et al.
Object Type:
Article
System:
The UNT Digital Library
A 4.2 GS/sec. Synchronized Vertical Excitation System for SPS Studies - Steps Toward Wideband Feedback
A 4.2 GS/sec. beam excitation system with accelerator synchronization and power stages is described. The system is capable of playing unique samples (32 samples/bunch) for 15,000 turns on selected bunch(es) in the SPS in syn- chronism with the injection and acceleration cycle. The purpose of the system is to excite internal modes of single-bunch vertical motion, and study the bunch dynamics in the presence of developing Electron cloud or TMCI effects. The system includes a synchronized master oscillator, SPS timing functions, an FPGA based arbitrary waveform generator, 4.2 GS/sec. D/A system and four 80W 20-1000 MHz amplifiers driving a tapered stripline pickup/kicker. A software GUI allows specification of various modulation signals, selection of bunches and turns to excite, while a remote control interface allows simple control/monitoring of the RF power stages located in the tunnel. The successful use of this system for SPS MD measurements in 2011 is a vital proof-of-principle for wideband feedback using similar functions to correct the beam motion.
Date:
July 10, 2012
Creator:
Fox, John
Object Type:
Article
System:
The UNT Digital Library
12 GeV Upgrade Project - Cryomodule Production
The Thomas Jefferson National Accelerator Facility (Jefferson Lab) is producing ten 100+MV SRF cryomodules (C100) as part of the CEBAF 12 GeV Upgrade Project. Once installed, these cryomodules will become part of an integrated accelerator system upgrade that will result in doubling the energy of the CEBAF machine from 6 to 12 GeV. This paper will present a complete overview of the C100 cryomodule production process. The C100 cryomodule was designed to have the major components procured from private industry and assembled together at Jefferson Lab. In addition to measuring the integrated component performance, the performance of the individual components is verified prior to being released for production and assembly into a cryomodule. Following a comprehensive cold acceptance test of all subsystems, the completed C100 cryomodules are installed and commissioned in the CEBAF machine in preparation of accelerator operations. This overview of the cryomodule production process will include all principal performance measurements, acceptance criterion and up to date status of current activities.
Date:
July 1, 2012
Creator:
J. Hogan, A. Burrill, G.K. Davis, M.A. Drury, M. Wiseman
Object Type:
Article
System:
The UNT Digital Library
A 12 GHz RF Power Source for the CLIC Study
The CLIC RF frequency has been changed in 2008 from the initial 30 GHz to the European X-band 11.9942 GHz permitting beam independent power production using klystrons for CLIC accelerating structure testing. A design and fabrication contract for five klystrons at that frequency has been signed by different parties with SLAC. France (IRFU, CEA Saclay) is contributing a solid state modulator purchased in industry and specific 12 GHz RF network components to the CLIC study. RF pulses over 120 MW peak at 230 ns length will be obtained by using a novel SLED-I type pulse compression scheme designed and fabricated by IAP, Nizhny Novgorod, Russia. The X-band power test stand is being installed in the CLIC Test Facility CTF3 for independent structure and component testing in a bunker, but allowing, in a later stage, for powering RF components in the CTF3 beam lines. The design of the facility, results from commissioning of the RF power source and the expected performance of the Test Facility are reported.
Date:
July 3, 2012
Creator:
Schirm, Karl; Curt, Stephane; Dobert, Steffen; McMonagle, Gerard; Rossat, Ghislain; Syratchev, Igor et al.
Object Type:
Article
System:
The UNT Digital Library
A 14 MeV Fusion Neutron Source for Material and Blanket Development and Fission Fuel Production
None
Date:
July 30, 2012
Creator:
Simonen, T. C.; Moir, R. W.; Molvik, A. W. & Ryutov, D. D.
Object Type:
Article
System:
The UNT Digital Library
17 GHz High Gradient Accelerator Research
This is a report on the MIT High Gradient Accelerator Research program which has included: Operation of the 17 GHz, 25 MeV MIT/Haimson Research Corp. electron accelerator at MIT, the highest frequency, stand-alone accelerator in the world; collaboration with members of the US High Gradient Collaboration, including the design and test of novel structures at SLAC at 11.4 GHz; the design, construction and testing of photonic bandgap structures, including metallic and dielectric structures; the investigation of the wakefields in novel structures; and the training of the next generation of graduate students and postdoctoral associates in accelerator physics.
Date:
July 10, 2013
Creator:
Temkin, Richard J. & Shapiro, Michael A.
Object Type:
Report
System:
The UNT Digital Library
25 Year Lifetime for Flexible Buildings Integrated Photovoltaics
Although preliminary proof-of-principle of the efficacy of barrier materials and processes, first developed by Battelle at PNNL and commercialized by Vitex, has been demonstrated at the laboratory scale, there are several challenges to the practical commercial implementation of these developments in the Buildings Integrated Photovoltaics (BIPV) market. Two important issues that are addressed in this project are identifying a low cost substrate material that can survive in the outside environment (rain, heat, dust, hail, etc.) for 25 years and developing an encapsulation method for the photovoltaic (PV) cells that can meet the required barrier performance without driving the cost of the total barrier package out of range (remaining below $3.00/Wp). Without these solutions, current encapsulation technologies will limit the use of PV for BIPV applications. Flexible, light-weight packaging that can withstand 25 years in the field is required for a totally flexible integrated PV package. The benefit of this research is to make substantial progress in the development of a cost-effective, viable thin film barrier package which will be a critical enabling technology to meet the Solar America Initiative cost and device reliability goals, and to make photovoltaics (PV) more cost-competitive with electricity generated using fossil fuels. Increased PV installations …
Date:
July 10, 2010
Creator:
Gross, Mark E.
Object Type:
Report
System:
The UNT Digital Library
50% Advanced Energy Design Guides: Preprint
This paper presents the process, methodology, and assumptions for the development of the 50% Energy Savings Advanced Energy Design Guides (AEDGs), a design guidance document that provides specific recommendations for achieving 50% energy savings above the requirements of ANSI/ASHRAE/IESNA Standard 90.1-2004 in four building types: (1) Small to medium office buildings, (2) K-12 school buildings, (3) Medium to big box retail buildings, (4) Large hospital buildings.
Date:
July 1, 2012
Creator:
Bonnema, E.; Leach, M.; Pless, S.; Liu, B.; Wang, W.; Thornton, B. et al.
Object Type:
Article
System:
The UNT Digital Library
112-pixel arrays of high-efficiency STJ X-ray detectors
None
Date:
July 15, 2013
Creator:
Friedrich, S; Harris, J; Warburton, W K; Carpenter, M H; Hall, J A & Cantor, R
Object Type:
Article
System:
The UNT Digital Library
241-AZ Tank Farm Construction Extent of Condition Review for Tank Integrity
This report provides the results of an extent of condition construction history review for tanks 241-AZ-101 and 241-AZ-102. The construction history of the 241-AZ tank farm has been reviewed to identify issues similar to those experienced during tank AY-102 construction. Those issues and others impacting integrity are discussed based on information found in available construction records, using tank AY-102 as the comparison benchmark. In the 241-AZ tank farm, the second DST farm constructed, both refractory quality and tank and liner fabrication were improved.
Date:
July 30, 2013
Creator:
Barnes, Travis J.; Boomer, Kayle D.; Gunter, Jason R. & Venetz, Theodore J.
Object Type:
Report
System:
The UNT Digital Library
241-SY Tank Farm Construction Extent of Condition Review for Tank Integrity
This report provides the results of an extent of condition construction history review for tanks 241-SY-101, 241-SY-102, and 241-SY-103. The construction history of the 241-SY tank farm has been reviewed to identify issues similar to those experienced during tank 241-AY-102 construction. Those issues and others impacting integrity are discussed based on information found in available construction records, using tank 241-AY-102 as the comparison benchmark. In the 241-SY tank farm, the third DST farm constructed, refractory quality and stress relief were improved, while similar tank and liner fabrication issues remained.
Date:
July 25, 2013
Creator:
Barnes, Travis J.; Boomer, Kayle D.; Gunter, Jason R. & Venetz, Theodore J.
Object Type:
Report
System:
The UNT Digital Library
500 MW X-Band RF System of a 0.25 GeV Electron LINAC for Advanced Compton Scattering Source Application
A Mono-Energetic Gamma-Ray (MEGa-Ray) Compton scattering light source is being developed at LLNL in collaboration with the SLAC National Accelerator Laboratory. The electron beam for the Compton scattering interaction will be generated by a X-band RF gun and a X-band LINAC at the frequency of 11.424 GHz. High power RF in excess of 500 MW is needed to accelerate the electrons to energy of 250 MeV or greater for the interaction. Two high power klystron amplifiers, each capable of generating 50 MW, 1.5 msec pulses, will be the main high power RF sources for the system. These klystrons will be powered by state of the art solid-state high voltage modulators. A RF pulse compressor, similar to the SLED II pulse compressor, will compress the klystron output pulse with a power gain factor of five. For compactness consideration, we are looking at a folded waveguide setup. This will give us 500 MW at output of the compressor. The compressed pulse will then be distributed to the RF gun and to six traveling wave accelerator sections. Phase and amplitude control are located at the RF gun input and additional control points along the LINAC to allow for parameter control during operation. This …
Date:
July 3, 2012
Creator:
Chu, Tak Sum; Anderson, Scott; Barty, Christopher; Gibson, David; Hartemann, Fred; Marsh, Roark et al.
Object Type:
Article
System:
The UNT Digital Library
The 2001 and 2003 Bush Tax Cuts and Deficit Reduction
This report uses the context of the current and long-term economic environment to examine the tax cuts implemented by the George W. Bush Administration, including the Economic Growth and Tax Relief Reconciliation Act of 2001 and the Jobs and Growth Tax Relief Reconciliation Act of 2003.
Date:
July 23, 2012
Creator:
Hungerford, Thomas L.
Object Type:
Report
System:
The UNT Digital Library
The 2001 and 2003 Bush Tax Cuts and Deficit Reduction
This report uses the context of the current and long-term economic environment to examine the tax cuts implemented by the George W. Bush Administration, including the Economic Growth and Tax Relief Reconciliation Act of 2001 and the Jobs and Growth Tax Relief Reconciliation Act of 2003.
Date:
July 18, 2012
Creator:
Hungerford, Thomas L.
Object Type:
Report
System:
The UNT Digital Library
2009 Y-12 National Security Complex Annual Illness and Injury Surveillance Report
The U.S. Department of Energy’s (DOE) commitment to assuring the health and safety of its workers includes the conduct of epidemiologic surveillance activities that provide an early warning system for health problems among workers. The Illness and Injury Surveillance Program monitors illnesses and health conditions that result in an absence of workdays, occupational injuries and illnesses, and disabilities and deaths among current workers.
Date:
July 9, 2010
Creator:
United States. Department of Energy. Office of Illness and Injury Prevention Programs.
Object Type:
Report
System:
The UNT Digital Library
2010 Atomic & Molecular Interactions Gordon Research Conference
The Atomic and Molecular Interactions Gordon Conferences is justifiably recognized for its broad scope, touching on areas ranging from fundamental gas phase and gas-condensed matter collision dynamics, to laser-molecule interactions, photophysics, and unimolecular decay processes. The meeting has traditionally involved scientists engaged in fundamental research in gas and condensed phases and those who apply these concepts to systems of practical chemical and physical interest. A key tradition in this meeting is the strong mixing of theory and experiment throughout. The program for 2010 conference continues these traditions. At the 2010 AMI GRC, there will be talks in 5 broadly defined and partially overlapping areas of intermolecular interactions and chemical dynamics: (1) Photoionization and Photoelectron Dynamics; (2) Quantum Control and Molecules in Strong Fields; (3) Photochemical Dynamics; (4) Complex Molecules and Condensed Phases; and (5) Clusters and Reaction Dynamics. These areas encompass many of the most productive and exciting areas of chemical physics, including both reactive and nonreactive processes, intermolecular and intramolecular energy transfer, and photodissociation and unimolecular processes. Gas phase dynamics, van der Waals and cluster studies, laser-matter interactions and multiple potential energy surface phenomena will all be discussed.
Date:
July 23, 2010
Creator:
Martinez, Todd
Object Type:
Article
System:
The UNT Digital Library
2010 CATALYSIS GORDON RESEARCH CONFERENCE, JUNE 27 - JULY 2, 2010, NEW LONDON, NEW HAMPSHIRE
Catalysis is a key technology for improving the quality of life while simultaneously reducing the adverse impact of human activities on the environment. The discovery of new catalytic processes and the improvement of existing ones are also critically important for securing the nation's energy supply. The GRC on Catalysis is considered one the most prestigious conference for catalysis research, bringing together leading researchers from both academia, industry and national labs to discuss the latest, most exciting research in catalysis and the future directions for the field. The 2010 GRC on Catalysis will follow time-honored traditions and feature invited talks from the world's leading experts in the fundamentals and applications of catalytic science and technology. We plan to have increased participation from industry. The extended discussions in the company of outstanding thinkers will stimulate and foster new science. The conference will include talks in the following areas: Alternative feedstocks for chemicals and fuels, Imaging and spectroscopy, Design of novel catalysts, Catalyst preparation fundamentals, Molecular insights through theory, Surface Science, Catalyst stability and dynamics. In 2010, the Catalysis conference will move to a larger conference room with a new poster session area that will allow 40 posters per session. The dorm rooms …
Date:
July 2, 2010
Creator:
Datye, Abhaya
Object Type:
Article
System:
The UNT Digital Library
The 2010 Deepwater Horizon Oil Spill: Natural Resource Damage Assessment Under the Oil Pollution Act
Report that examines the Natural Resources Damage Assessment (NRDA) process under the Oil Pollution Act (OPA) in the context of the Deepwater Horizon spill.
Date:
July 24, 2013
Creator:
Vann, Adam & Meltz, Robert
Object Type:
Report
System:
The UNT Digital Library
2010 GORDON RESEARCH CONFERENCE ON MITOCHONDRIA & CHLOROPLASTS, LUCCA, ITALY, JULY 11-16, 2010
The 2010 GRC on Mitochondria & Chloroplasts will assemble an international group of molecular, structural and cellular biologists, biochemists and geneticists investigating a broad spectrum of fundamental problems related to the biology of these organelles in animal, plant and fungal cells. This field has witnessed an extraordinary expansion in recent years, fueled by the discovery of the role of mitochondria in human disease and ageing, and of the synergy of chloroplasts and mitochondria in energetic output, the identification of novel factors involved in organelle division, movement, signaling and acclimation to changing environmental conditions, and by the powerful tools of organelle proteomics. The 2010 GRC will highlight advances in the elucidation of molecular mechanisms of organelle biogenesis including regulation of genome structure, evolution and expression, organellar protein import, assembly and turnover of respiratory and photosynthetic complexes, bidirectional signaling between organelles and nucleus, organelle morphology and dynamics, and the integration of cellular metabolism. We will also explore progress in mechanisms of disease and ageing/ senescence in animals and plants. The organellar field has forged new fronts toward a global and comprehensive understanding of mitochondrial and chloroplast biology at the molecular level. Many of the molecules under study in model organisms are responsible …
Date:
July 16, 2010
Creator:
Barkan, Alice
Object Type:
Article
System:
The UNT Digital Library
2010 Honda Civic Hybrid UltraBattery Conversion 5577 - Hybrid Electric Vehicle Battery Test Results
The U.S. Department of Energy Advanced Vehicle Testing Activity Program consists of vehicle, battery, and infrastructure testing on advanced technology related to transportation. The activity includes tests on hybrid electric vehicles (HEVs), including testing the HEV batteries when both the vehicles and batteries are new and at the conclusion of on-road fleet testing. This report documents battery testing performed for the 2010 Honda Civic HEV UltraBattery Conversion (VIN JHMFA3F24AS005577). Battery testing was performed by the Electric Transportation Engineering Corporation dba ECOtality North America. The Idaho National Laboratory and ECOtality North America collaborate on the AVTA for the Vehicle Technologies Program of the DOE.
Date:
July 1, 2013
Creator:
Gray, Tyler; Shirk, Matthew & Wishart, Jeffrey
Object Type:
Report
System:
The UNT Digital Library
2010 Membranes: Materials & Processes Gordon Research Conference
The GRC series on Membranes: Materials and Processes have gained significant international recognition, attracting leading experts on membranes and other related areas from around the world. It is now known for being an interdisciplinary and synergistic meeting. The next summer's edition will keep with the past tradition and include new, exciting aspects of material science, chemistry, chemical engineering, computer simulation with participants from academia, industry and national laboratories. This edition will focus on cutting edge topics of membranes for addressing several grand challenges facing our society, in particular, energy, water, health and more generally sustainability. During the technical program, we want to discuss new membrane structure and characterization techniques, the role of advanced membranes and membrane-based processes in sustainability/environment (including carbon dioxide capture), membranes in water processes, and membranes for biological and life support applications. As usual, the informal nature of the meeting, excellent quality of the oral presentations and posters, and ample opportunity to meet many outstanding colleagues make this an excellent conference for established scientists as well as for students. A Gordon Research Seminar (GRS) on the weekend prior to the GRC meeting will provide young researchers an opportunity to present their work and network with outstanding experts. …
Date:
July 30, 2010
Creator:
Lin, Jerry
Object Type:
Article
System:
The UNT Digital Library
2010 MICROBIAL STRESS RESPONSE GORDON RESEARCH CONFERENCE, JULY 18-23, 2010
The 2010 Gordon Research Conference on Microbial Stress Responses provides an open and exciting forum for the exchange of scientific discoveries on the remarkable mechanisms used by microbes to survive in nearly every niche on the planet. Understanding these stress responses is critical for our ability to control microbial survival, whether in the context of biotechnology, ecology, or pathogenesis. From its inception in 1994, this conference has traditionally employed a very broad definition of stress in microbial systems. Sessions will cover the major steps of stress responses from signal sensing to transcriptional regulation to the effectors that mediate responses. A wide range of stresses will be represented. Some examples include (but are not limited to) oxidative stress, protein quality control, antibiotic-induced stress and survival, envelope stress, DNA damage, and nutritional stress. The 2010 meeting will also focus on the role of stress responses in microbial communities, applied and environmental microbiology, and microbial development. This conference brings together researchers from both the biological and physical sciences investigating stress responses in medically- and environmentally relevant microbes, as well as model organisms, using cutting-edge techniques. Computational, systems-level, and biophysical approaches to exploring stress responsive circuits will be integrated throughout the sessions alongside the …
Date:
July 23, 2011
Creator:
Ades, Sarah
Object Type:
Article
System:
The UNT Digital Library
2010 Plant Molecular Biology Gordon Research Conference
The Plant Molecular Biology Conference has traditionally covered a breadth of exciting topics and the 2010 conference will continue in that tradition. Emerging concerns about food security have inspired a program with three main themes: (1) genomics, natural variation and breeding to understand adaptation and crop improvement, (2) hormonal cross talk, and (3) plant/microbe interactions. There are also sessions on epigenetics and proteomics/metabolomics. Thus this conference will bring together a range of disciplines, will foster the exchange of ideas and enable participants to learn of the latest developments and ideas in diverse areas of plant biology. The conference provides an excellent opportunity for individuals to discuss their research because additional speakers in each session will be selected from submitted abstracts. There will also be a poster session each day for a two-hour period prior to dinner. In particular, this conference plays a key role in enabling students and postdocs (the next generation of research leaders) to mingle with pioneers in multiple areas of plant science.
Date:
July 23, 2010
Creator:
Sussman, Michael
Object Type:
Article
System:
The UNT Digital Library
2010 POLYMER PHYSICS - JUNE 27 - JULY 2, 2010
The 2010 Gordon Research Conference on Polymer Physics will provide outstanding lectures and discussions in this critical field that impacts every industrial sector from electronics to transportation to medicine to textiles to energy generation and storage. Fundamental topics range from mechanical properties of soft gels to new understanding in polymer crystallization to energy conversion and transmission to simulating polymer dynamics at the nanoscale. This international conference will feature 22 invited lectures, wherein the opening 10 minutes are specifically designed for a general polymer physics audience. In addition, poster sessions and informal activities provide ample opportunity to discuss the latest advances in polymer physics. The technical content of the meeting will include new twists on traditional polymer physics topics, recent advances in previously underrepresented topics, and emerging technologies enabled by polymer physics. Here is a partially listing of targeted topics: (1) electrically-active and light-responsive polymers and polymer-based materials used in energy conversion and storage; (2) polymers with hierarchical structures including supramolecular assemblies, ion-containing polymers, and self-assembled block polymers; (3) mechanical and rheological properties of soft materials, such as hydrogels, and of heterogeneous materials, particularly microphase separated polymers and polymer nanocomposites; and (4) crystallization of polymers in dilute solutions, polymer melts, and …
Date:
July 2, 2010
Creator:
Winey, Karen
Object Type:
Article
System:
The UNT Digital Library