Raising Photoemission Efficiency with Surface Acoustic Waves (open access)

Raising Photoemission Efficiency with Surface Acoustic Waves

We are developing a novel technique that may help increase the efficiency and reduce costs of photoelectron sources used at electron accelerators. The technique is based on the use of Surface Acoustic Waves (SAW) in piezoelectric materials, such as GaAs, that are commonly used as photocathodes. Piezoelectric fields produced by the traveling SAW spatially separate electrons and holes, reducing their probability of recombination, thereby enhancing the photoemission quantum efficiency of the photocathode. Additional advantages could be increased polarization provided by the enhanced mobility of charge carriers that can be controlled by the SAW and the ionization of optically-generated excitons resulting in the creation of additional electron-hole pairs. It is expected that these novel features will reduce the cost of accelerator operation. A theoretical model for photoemission in the presence of SAW has been developed, and experimental tests of the technique are underway.
Date: July 1, 2012
Creator: A. Afanasev, F. Hassani, C.E. Korman, V.G. Dudnikov, R.P. Johnson, M. Poelker, K.E.L. Surles-Law
System: The UNT Digital Library
A CASE STUDY OF CHLORINE TRANSPORT AND FATE FOLLOWING A LARGE ACCIDENTAL RELEASE (open access)

A CASE STUDY OF CHLORINE TRANSPORT AND FATE FOLLOWING A LARGE ACCIDENTAL RELEASE

A train derailment that occurred in Graniteville, South Carolina during the early morning hours of 06 January, 2005 resulted in the prompt release of approximately 60 tons of chlorine to the environment. Comprehensive modeling of the transport and fate of this release was performed including the characterization of the initial three-phased chlorine release, a detailed determination of the local atmospheric conditions acting to generate, disperse, and deplete the chlorine vapor cloud, the establishment of physical exchange mechanisms between the airborne vapor and local surface waters, and local aquatic dilution and mixing.
Date: August 1, 2012
Creator: Buckley, R.; Hunter, C.; Werth, D.; Whiteside, M.; Chen, K. & Mazzola, C.
System: The UNT Digital Library
Importance of Final-State Fluctuations in Radiative Capture Reactions and Applications to Surrogate Reaction Measurements (open access)

Importance of Final-State Fluctuations in Radiative Capture Reactions and Applications to Surrogate Reaction Measurements

None
Date: October 10, 2012
Creator: Dietrich, F S
System: The UNT Digital Library
Full toroidal imaging of non-axisymmetric plasma material interaction in the National Spherical Torus eXperiment divertor (open access)

Full toroidal imaging of non-axisymmetric plasma material interaction in the National Spherical Torus eXperiment divertor

None
Date: May 7, 2012
Creator: Scotti, F; Roquemore, A L & Soukhanovskii, V A
System: The UNT Digital Library
Effects of grids in drift tubes (open access)

Effects of grids in drift tubes

In 2011, we upgraded a 201 MHz buncher in the proton injector for the alternating gradient synchrotron (AGS) - relativistic heavy ion collider (RHIC) complex. In the buncher we installed four grids made of tungsten to improve the transit time factor. The grid installed drift tubes have 32 mm of inner diameter and the each grid consists of four quadrants. The quadrants were cut out precisely from 1mm thick tungsten plates by a computerized numerically controlled (CNC) wire cutting electrical discharge machining (EDM). The 3D electric field of the grid was simulated.
Date: May 20, 2012
Creator: M., Okamura & Yamauchi, H.
System: The UNT Digital Library
Using a Research Simulator for Validating Control Room Modernization Concepts (open access)

Using a Research Simulator for Validating Control Room Modernization Concepts

The Light Water Reactor Sustainability Program is a research, development, and deployment program sponsored by the United States Department of Energy. The program is operated in close collaboration with industry research and development programs to provide the technical foundations for licensing and managing the long-term, safe, and economical operation of nuclear power plants that are currently in operation. Advanced instrumentation and control (I&C) technologies are needed to support the continued safe and reliable production of power from nuclear energy systems during sustained periods of operation up to and beyond their expected licensed lifetime. This requires that new capabilities to achieve process control be developed and eventually implemented in existing nuclear control rooms. It also requires that approaches be developed and proven to achieve sustainability of I&C systems throughout the period of extended operation. Idaho National Laboratory (INL) is working closely with nuclear utilities to develop technologies and solutions to help ensure the safe life extension of current reactors. One of the main areas of focus is control room modernization. Current analog control rooms are growing obsolete, and it is difficult for utilities to maintain them. Using its reconfigurable control room simulator adapted from a training simulator, INL serves as a …
Date: May 1, 2012
Creator: Boring, Ronald L.; Agarwal, Vivek; Persensky, Julius J. & Joe, Jeffrey C.
System: The UNT Digital Library
3D Equilibrium Effects Due to RMP Application on DIII-D (open access)

3D Equilibrium Effects Due to RMP Application on DIII-D

The mitigation and suppression of edge localized modes (ELMs) through application of resonant magnetic perturbations (RMPs) in Tokamak plasmas is a well documented phenomenon [1]. Vacuum calculations suggest the formation of edge islands and stochastic regions when RMPs are applied to the axisymmetric equilibria. Self-consistent calculations of the plasma equilibrium with the VMEC [2] and SPEC [3] codes have been performed for an up-down symmetric shot (142603) in DIII-D. In these codes, a self-consistent calculation of the plasma response due to the RMP coils is calculated. The VMEC code globally enforces the constraints of ideal MHD; consequently, a continuously nested family of flux surfaces is enforced throughout the plasma domain. This approach necessarily precludes the observation of islands or field-line chaos. The SPEC code relaxes the constraints of ideal MHD locally, and allows for islands and field line chaos at or near the rational surfaces. Equilibria with finite pressure gradients are approximated by a set of discrete "ideal-interfaces" at the most irrational flux surfaces and where the strongest pressure gradients are observed. Both the VMEC and SPEC calculations are initialized from EFIT reconstructions of the plasma that are consistent with the experimental pressure and current profiles. A 3D reconstruction using …
Date: June 20, 2012
Creator: Lazerson, S.; Lazarus, E.; Hudson, S.; Pablant, N. & Gates, D.
System: The UNT Digital Library
Coherent electron cooling proof of principle instrumentation design (open access)

Coherent electron cooling proof of principle instrumentation design

The goal of the Coherent Electron Cooling Proof-of-Principle (CeC PoP) experiment being designed at RHIC is to demonstrate longitudinal (energy spread) cooling before the expected CD-2 for eRHIC. The scope of the experiment is to longitudinally cool a single bunch of 40 GeV/u gold ions in RHIC. This paper will describe the instrumentation systems proposed to meet the diagnostics challenges. These include measurements of beam intensity, emittance, energy spread, bunch length, position, orbit stability, and transverse and temporal alignment of electron and ion beams.
Date: April 15, 2012
Creator: M., Gassner D.; Litvinenko, V.; Michnoff, R.; Miller, T.; Minty, M. & Pinayev, I.
System: The UNT Digital Library
Gas-Phase Molecular Dynamics: High Resolution Spectroscopy and Collision Dynamics of Transient Species (open access)

Gas-Phase Molecular Dynamics: High Resolution Spectroscopy and Collision Dynamics of Transient Species

This research is carried out as part of the Gas-Phase Molecular Dynamics program in the Chemistry Department at Brookhaven National Laboratory. Chemical intermediates in the elementary gas-phase reactions involved in combustion chemistry are investigated by high resolution spectroscopic tools. Production, reaction, and energy transfer processes are investigated by transient, double resonance, polarization and saturation spectroscopies, with an emphasis on technique development and connection with theory, as well as specific molecular properties.
Date: May 29, 2012
Creator: Hall, G. E. & Goncharov, V.
System: The UNT Digital Library
PHASE II VAULT TESTING OF THE ARGONNE RFID SYSTEM (open access)

PHASE II VAULT TESTING OF THE ARGONNE RFID SYSTEM

The U.S. Department of Energy (DOE) (Environmental Management [EM], Office of Packaging and Transportation [EM-45]) Packaging and Certification Program (DOE PCP) has developed a Radio Frequency Identification (RFID) tracking and monitoring system, called ARG-US, for the management of nuclear materials packages during transportation and storage. The performance of the ARG-US RFID equipment and system has been fully tested in two demonstration projects in April 2008 and August 2009. With the strong support of DOE-SR and DOE PCP, a field testing program was completed in Savannah River Site's K-Area Material Storage (KAMS) Facility, an active Category I Plutonium Storage Facility, in 2010. As the next step (Phase II) of continued vault testing for the ARG-US system, the Savannah River Site K Area Material Storage facility has placed the ARG-US RFIDs into the 910B storage vault for operational testing. This latest version (Mark III) of the Argonne RFID system now has the capability to measure radiation dose and dose rate. This paper will report field testing progress of the ARG-US RFID equipment in KAMS, the operability and reliability trend results associated with the applications of the system, and discuss the potential benefits in enhancing safety, security and materials accountability. The purpose of …
Date: June 25, 2012
Creator: Willoner, T.; Turlington, R. & Koenig, R.
System: The UNT Digital Library
An efficient modeling method for thermal stratification simulation in a BWR suppression pool (open access)

An efficient modeling method for thermal stratification simulation in a BWR suppression pool

The suppression pool in a BWR plant not only is the major heat sink within the containment system, but also provides major emergency cooling water for the reactor core. In several accident scenarios, such as LOCA and extended station blackout, thermal stratification tends to form in the pool after the initial rapid venting stage. Accurately predicting the pool stratification phenomenon is important because it affects the peak containment pressure; and the pool temperature distribution also affects the NPSHa (Available Net Positive Suction Head) and therefore the performance of the pump which draws cooling water back to the core. Current safety analysis codes use 0-D lumped parameter methods to calculate the energy and mass balance in the pool and therefore have large uncertainty in prediction of scenarios in which stratification and mixing are important. While 3-D CFD methods can be used to analyze realistic 3D configurations, these methods normally require very fine grid resolution to resolve thin substructures such as jets and wall boundaries, therefore long simulation time. For mixing in stably stratified large enclosures, the BMIX++ code has been developed to implement a highly efficient analysis method for stratification where the ambient fluid volume is represented by 1-D transient partial …
Date: September 1, 2012
Creator: Zhao, Haihua; Zou, Ling; Zhang, Hongbin; Li, Hua; Villanueva, Walter & Kudinov, Pavel
System: The UNT Digital Library
Setting Whole-Building Absolute Energy Use Targets for the K-12 School, Retail, and Healthcare Sectors: Preprint (open access)

Setting Whole-Building Absolute Energy Use Targets for the K-12 School, Retail, and Healthcare Sectors: Preprint

This paper helps owners' efficiency representatives to inform executive management, contract development, and project management staff as to how specifying and applying whole-building absolute energy use targets for new construction or renovation projects can improve the operational energy performance of commercial buildings.
Date: August 1, 2012
Creator: Leach, M.; Bonnema, E.; Pless, S. & Torcellini, P.
System: The UNT Digital Library
A VUV Photoionization Study of the Combustion-Relevant Reaction of the Phenyl Radical (C6H5) with Propylene (C3H6) in a High Temperature Chemical Reactor (open access)

A VUV Photoionization Study of the Combustion-Relevant Reaction of the Phenyl Radical (C6H5) with Propylene (C3H6) in a High Temperature Chemical Reactor

We studied the reaction of phenyl radicals (C6H5) with propylene (C3H6) exploiting a high temperature chemical reactor under combustion-like conditions (300 Torr, 1,200-1,500 K). The reaction products were probed in a supersonic beam by utilizing tunable vacuum ultraviolet (VUV) radiation from the Advanced Light Source and recording the photoionization efficiency (PIE) curves at mass-to-charge ratios of m/z = 118 (C9H10+) and m/z = 104 (C8H8+). Our results suggest that the methyl and atomic hydrogen losses are the two major reaction pathways with branching ratios of 86 10 percent and 14 10 percent. The isomer distributions were probed by fitting the recorded PIE curves with a linear combination of the PIE curves of the individual C9H10 and C8H8 isomers. Styrene (C6H5C2H3) was found to be the exclusive product contributing to m/z = 104 (C8H8+), whereas 3-phenylpropene, cis-1-phenylpropene, and 2-phenylpropene with branching ratios of 96 4 percent, 3 3 percent, and 1 1 percent could account for signal at m/z = 118 (C9H10+). Although searched for carefully, no evidence of the bicyclic indane molecule could be provided. The reaction mechanisms and branching ratios are explained in terms of electronic structure calculations nicely agreeing with a recent crossed molecular beam study on this …
Date: February 22, 2012
Creator: Manoa, University of Hawaii at; Laboratories, Sandia National; Zhang, Fangtong; Kaiser, Ralf I.; Golan, Amir; Ahmed, Musahid et al.
System: The UNT Digital Library
The 12 GeV Energy Upgrade at Jefferson Laboratory (open access)

The 12 GeV Energy Upgrade at Jefferson Laboratory

Two new cryomodules and an extensive upgrade of the bending magnets at Jefferson Lab has been recently completed in preparation for the full energy upgrade in about one year. Jefferson Laboratory has undertaken a major upgrade of its flagship facility, the CW re-circulating CEBAF linac, with the goal of doubling the linac energy to 12 GeV. I will discuss here the main scope and timeline of the upgrade and report on recent accomplishments and the present status. I will then discuss in more detail the core of the upgrade, the new additional C100 cryomodules, their production, tests and recent successful performance. I will then conclude by looking at the future plans of Jefferson Laboratory, from the commissioning and operations of the 12 GeV CEBAF to the design of the MEIC electron ion collider.
Date: September 2012
Creator: Pilat, Fulvia C.
System: The UNT Digital Library
Ultra-High Gradient Compact S-Band Linac for Laboratory and Industrial Applications (open access)

Ultra-High Gradient Compact S-Band Linac for Laboratory and Industrial Applications

There is growing demand from the industrial and research communities for high gradient, compact RF accelerating structures. The commonly used S-band SLAC-type structure has an operating gradient of only about 20 MV/m; while much higher operating gradients (up to 70 MV/m) have been recently achieved in X-band, as a consequence of the substantial efforts by the Next Linear Collider (NLC) collaboration to push the performance envelope of RF structures towards higher accelerating gradients. Currently however, high power X-band RF sources are not readily available for industrial applications. Therefore, RadiaBeam Technologies is developing a short, standing wave S-band structure which uses frequency scaled NLC design concepts to achieve up to a 50 MV/m operating gradient at 2856 MHz. The design and prototype commissioning plans are presented.
Date: July 3, 2012
Creator: Faillace, Luigi; Tech., /RadiaBeam; Agustsson, Ronald; Tech., /RadiaBeam; Frigola, Pedro; Tech., /RadiaBeam et al.
System: The UNT Digital Library
Searches for New Physics in Top Events at the Tevatron (open access)

Searches for New Physics in Top Events at the Tevatron

Recent results of searches for new physics in top events at the Tevatron are presented. In case of CDF three searches are discussed using 6 to 8.7 fb{sup -1} of data, with the latter being the final CDF data sample available for this kind of analysis. CDF carried out a search for Top + jet resonance production, dark matter production in association with single top and boosted tops. No signs of new physics are observed and instead upper limits are derived. D0 used 5.3 fb{sup -1} of data and searched for a narrow resonance in t{bar t} production and a time dependent t{bar t} cross section, which would reveal a violation of Lorentz invariance. However, no signs for deviations from standard model are seen and instead upper limits for non-standard model contributions are calculated.
Date: June 1, 2012
Creator: Jung, A.W.
System: The UNT Digital Library
Analog Video Authentication and Seal Verification Equipment Development (open access)

Analog Video Authentication and Seal Verification Equipment Development

Under contract to the US Department of Energy in support of arms control treaty verification activities, the Savannah River National Laboratory in conjunction with the Pacific Northwest National Laboratory, the Idaho National Laboratory and Milagro Consulting, LLC developed equipment for use within a chain of custody regime. This paper discussed two specific devices, the Authentication Through the Lens (ATL) analog video authentication system and a photographic multi-seal reader. Both of these devices have been demonstrated in a field trial, and the experience gained throughout will also be discussed. Typically, cryptographic methods are used to prove the authenticity of digital images and video used in arms control chain of custody applications. However, in some applications analog cameras are used. Since cryptographic authentication methods will not work on analog video streams, a simple method of authenticating analog video was developed and tested. A photographic multi-seal reader was developed to image different types of visual unique identifiers for use in chain of custody and authentication activities. This seal reader is unique in its ability to image various types of seals including the Cobra Seal, Reflective Particle Tags, and adhesive seals. Flicker comparison is used to compare before and after images collected with the …
Date: September 1, 2012
Creator: Lancaster, Gregory
System: The UNT Digital Library
Phase Competition in Trisected Superconducting Dome (open access)

Phase Competition in Trisected Superconducting Dome

None
Date: October 2, 2012
Creator: Vishik, I.M.; Hashimoto, M; He, Rui-Hua; Lee, Wei-Sheng; Schmitt, Felix; Lu, Donghui et al.
System: The UNT Digital Library
Cavity Beam Position Monitor System for ATF2 (open access)

Cavity Beam Position Monitor System for ATF2

The Accelerator Test Facility 2 (ATF2) in KEK, Japan, is a prototype scaled demonstrator system for the final focus required for a future high energy lepton linear collider. The ATF2 beam-line is instrumented with a total of 38 C and S band resonant cavity beam position monitors (CBPM) with associated mixer electronics and digitizers. The current status of the BPM system is described, with a focus on operational techniques and performance. The ATF2 C-band system is performing well, with individual CBPM resolution approaching or at the design resolution of 50 nm. The changes in the CBPM calibration observed over three weeks can probably be attributed to thermal effects on the mixer electronics systems. The CW calibration tone power will be upgraded to monitor changes in the electronics gain and phase. The four S-band CBPMs are still to be investigated, the main problem associated with these cavities is a large cross coupling between the x and y ports. This combined with the large design dispersion in that degion makes the digital signal processing difficult, although various techniques exist to determine the cavity parameters and use these coupled signals for beam position determination.
Date: July 9, 2012
Creator: Boogert, Stewart; /Oxford U., JAI; Boorman, Gary; /Oxford U., JAI; Swinson, Christina; /Oxford U., JAI et al.
System: The UNT Digital Library
Statistical Simulation of the Performance and Degradation of a PEMFC Membrane Electrode Assembly (open access)

Statistical Simulation of the Performance and Degradation of a PEMFC Membrane Electrode Assembly

A 1-D MEA Performance model was developed that considered transport of liquid water, agglomerate catalyst structure, and the statistical variation of the MEA characteristic parameters. The model was validated against a low surface area carbon supported catalyst across various platinum loadings and operational conditions. The statistical variation was found to play a significant role in creating noise in the validation data and that there was a coupling effect between movement in material properties with liquid water transport. Further, in studying the low platinum loaded catalyst layers it was found that liquid water played a significant role in the increasing the overall transport losses. The model was then further applied to study platinum dissolution via potential cycling accelerated stress tests, in which the platinum was found to dissolve nearest the membrane effectively resulting in reaction distribution shifts within the layer.
Date: July 1, 2012
Creator: Harvey, David; Bellemare-Davis, Alexander; Karan, Kunal; Jayansankar, Barath; Pharoah, Jon; Colbow, Vesna et al.
System: The UNT Digital Library
Hydrogenation of Dislocation-Limited Heteroepitaxial Silicon Solar Cells: Preprint (open access)

Hydrogenation of Dislocation-Limited Heteroepitaxial Silicon Solar Cells: Preprint

Post-deposition hydrogenation by remote plasma significantly improves performance of heteroepitaxial silicon solar cells. Heteroepitaxial deposition of thin crystal silicon on sapphire for photovoltaics (PV) is an excellent model system for the study and improvement of deposition on inexpensive Al2O3-coated (100) biaxially-textured metal foils. Without hydrogenation, PV conversion efficiencies are less than 1% on our model system. Performance is limited by carrier recombination at electrically active dislocations that result from lattice mismatch, and other defects. We find that low-temperature hydrogenation at 350 degrees C is more effective than hydrogenation at 610 degrees C. In this work, we use measurements such as spectral quantum efficiency, secondary ion mass spectrometry (SIMS), and vibrational Si-H spectroscopies to understand the effects of hydrogenation on the materials and devices. Quantum efficiency increases most at red and green wavelengths, indicating hydrogenation is affecting the bulk more than the surface of the cells. SIMS shows there are 100X more hydrogen atoms in our cells than dangling bonds along dislocations. Yet, Raman spectroscopy indicates that only low temperature hydrogenation creates Si-H bonds; trapped hydrogen does not stably passivate dangling-bond recombination sites at high temperatures.
Date: June 1, 2012
Creator: Bolen, M. L.; Grover, S.; Teplin, C. W.; Bobela, D.; Branz, H. M. & Stradins, P.
System: The UNT Digital Library
Emissivity Tuned Emitter for RTPV Power Sources (open access)

Emissivity Tuned Emitter for RTPV Power Sources

Every mission launched by NASA to the outer planets has produced unexpected results. The Voyager I and II, Galileo, and Cassini missions produced images and collected scientific data that totally revolutionized our understanding of the solar system and the formation of the planetary systems. These missions were enabled by the use of nuclear power. Because of the distances from the Sun, electrical power was produced using the radioactive decay of a plutonium isotope. Radioisotopic Thermoelectric Generators (RTGs) used in the past and currently used Multi-Mission RTGs (MMRTGs) provide power for space missions. Unfortunately, RTGs rely on thermocouples to convert heat to electricity and are inherently inefficient ({approx} 3-7% thermal to electric efficiency). A Radioisotope Thermal Photovoltaic (RTPV) power source has the potential to reduce the specific mass of the onboard power supply by increasing the efficiency of thermal to electric conversion. In an RTPV, a radioisotope heats an emitter, which emits light to a photovoltaic (PV) cell, which converts the light into electricity. Developing an emitter tuned to the desired wavelength of the photovoltaic is a key part in increasing overall performance. Researchers at the NASA Glenn Research Center (GRC) have built a Thermal Photovoltaic (TPV) system, that utilizes a …
Date: March 1, 2012
Creator: Stoots, Carl M.; O'Brien, Robert C. & Howe, Troy M.
System: The UNT Digital Library
Electronic Structure and Oxidation State Changes in the Mn (4) Ca Cluster of Photosystem II (open access)

Electronic Structure and Oxidation State Changes in the Mn (4) Ca Cluster of Photosystem II

Oxygen-evolving complex (Mn{sub 4}Ca cluster) of Photosystem II cycles through five intermediate states (S{sub i}-states, i = 0-4) before a molecule of dioxygen is released. During the S-state transitions, electrons are extracted from the OEC, either from Mn or alternatively from a Mn ligand. The oxidation state of Mn is widely accepted as Mn{sub 4}(III{sub 2},IV{sub 2}) and Mn{sub 4}(III,IV{sub 3}) for S{sub 1} and S{sub 2} states, while it is still controversial for the S{sub 0} and S{sub 3} states. We used resonant inelastic X-ray scattering (RIXS) to study the electronic structure of Mn{sub 4}Ca complex in the OEC. The RIXS data yield two-dimensional plots that provide a significant advantage by obtaining both K-edge pre-edge and L-edge-like spectra (metal spin state) simultaneously. We have collected data from PSII samples in the each of the S-states and compared them with data from various inorganic Mn complexes. The spectral changes in the Mn 1s2p{sub 3/2} RIXS spectra between the S-states were compared to those of the oxides of Mn and coordination complexes. The results indicate strong covalency for the electronic configuration in the OEC, and we conclude that the electron is transferred from a strongly delocalized orbital, compared to those in …
Date: August 17, 2012
Creator: Yano, J.; Pushkar, Y.; Messinger, J.; Bergmann, U.; Glatzel, P. & Yachandra, V. K.
System: The UNT Digital Library
Clinical Trials of ProxiScan Compact Gamma Camera in Prostate Cancer Diagnosis (open access)

Clinical Trials of ProxiScan Compact Gamma Camera in Prostate Cancer Diagnosis

N/A
Date: October 29, 2012
Creator: Y., Cui
System: The UNT Digital Library