Neutrino physics today, important issues and the future (open access)

Neutrino physics today, important issues and the future

The status and the most important issues in neutrino physics will be summarized as well as how the current, pressing questions will be addressed by future experiments. Since the discovery of neutrino flavor transitions by the SuperKamiokande experiment in 1998, which demonstrates that neutrinos change and hence their clocks tick, i.e. they are not traveling at the speed of light and hence are not massless, the field of neutrino physics has made remarkable progress in untangling the nature of the neutrino. However, there are still many important questions to answer.
Date: October 1, 2010
Creator: Parke, Stephen J.
System: The UNT Digital Library
An Assessment of Molecular Dynamic Force Fields for Silica for Use in Simulating Laser Damage Mitigation (open access)

An Assessment of Molecular Dynamic Force Fields for Silica for Use in Simulating Laser Damage Mitigation

We compare force fields (FF's) that have been used in molecular dynamic (MD) simulations of silica in order to assess their applicability for use in simulating IR-laser damage mitigation. Although pairwise FF?s obtained by fitting quantum mechanical calculations such as the BKS and CHIK potentials have been shown to reproduce many of the properties of silica including the stability of silica polymorphs and the densification of the liquid, we show that melting temperatures and fictive temperatures are much too high. Softer empirical force fields give liquid and glass properties at experimental temperatures but may not predict all properties important to laser mitigation experiments.
Date: October 21, 2010
Creator: Soules, T F; Gilmer, G H; Matthews, M J; Stolken, J S & Feit, M D
System: The UNT Digital Library
Li+ alumino-silicate ion source development for the Neutralized Drift Compression Experiment (NDCX) (open access)

Li+ alumino-silicate ion source development for the Neutralized Drift Compression Experiment (NDCX)

We report results on lithium alumino-silicate ion source development in preparation for warmdense-matter heating experiments on the new Neutralized Drift Compression Experiment (NDCXII). The practical limit to the current density for a lithium alumino-silicate source is determined by the maximum operating temperature that the ion source can withstand before running into problems of heat transfer, melting of the alumino-silicate material, and emission lifetime. Using small prototype emitters, at a temperature of ~;;1275 oC, a space-charge-limited Li+ beam current density of J ~;;1 mA/cm2 was obtained. The lifetime of the ion source was ~;;50 hours while pulsing at a rate of 0.033 Hz with a pulse duration of 5-6 mu s.
Date: October 1, 2010
Creator: Roy, Prabir K.; Greenway, Wayne G.; Kwan, Joe W.; Seidl, Peter A.; Waldron, William L. & Wu, James K.
System: The UNT Digital Library
A truncated Levenberg-Marquardt algorithm for the calibration of highly parameterized nonlinear models (open access)

A truncated Levenberg-Marquardt algorithm for the calibration of highly parameterized nonlinear models

We propose a modification to the Levenberg-Marquardt minimization algorithm for a more robust and more efficient calibration of highly parameterized, strongly nonlinear models of multiphase flow through porous media. The new method combines the advantages of truncated singular value decomposition with those of the classical Levenberg-Marquardt algorithm, thus enabling a more robust solution of underdetermined inverse problems with complex relations between the parameters to be estimated and the observable state variables used for calibration. The truncation limit separating the solution space from the calibration null space is re-evaluated during the iterative calibration process. In between these re-evaluations, fewer forward simulations are required, compared to the standard approach, to calculate the approximate sensitivity matrix. Truncated singular values are used to calculate the Levenberg-Marquardt parameter updates, ensuring that safe small steps along the steepest-descent direction are taken for highly correlated parameters of low sensitivity, whereas efficient quasi-Gauss-Newton steps are taken for independent parameters with high impact. The performance of the proposed scheme is demonstrated for a synthetic data set representing infiltration into a partially saturated, heterogeneous soil, where hydrogeological, petrophysical, and geostatistical parameters are estimated based on the joint inversion of hydrological and geophysical data.
Date: October 15, 2010
Creator: Finsterle, S. & Kowalsky, M.B.
System: The UNT Digital Library
Photodetectors for Scintillator Proportionality Measurement (open access)

Photodetectors for Scintillator Proportionality Measurement

None
Date: October 22, 2010
Creator: Moses, William W.; Choong, W. -S.; Hull, G.; Payne, S.; Cherepy, N. & Valentine, J. D.
System: The UNT Digital Library
Importance of electronic relaxation for inter-coulombic decay in aqueous systems (open access)

Importance of electronic relaxation for inter-coulombic decay in aqueous systems

Inspired by recent photoelectron spectroscopy (PES) experiments on hydroxide solutions, we have examined the conditions necessary for enhanced (and, in the case of solutions, detectable) intercoulombic decay (ICD)--Auger emission from an atomic site other than that originally excited. We present general guidelines, based on energetic and spatial overlap of molecular orbitals, for this enhancement of ICDbased energy transfer in solutions. These guidelines indicate that this decay process should be exhibited by broad classes of biomolecules and suggest a design criterion for targeted radiooncology protocols. Our findings show that PES cannot resolve the current hydroxide coordination controversy.
Date: October 1, 2010
Creator: Schwartz, Craig P.; Fatehi, Shervin; Saykally, Richard J. & Prendergast, David
System: The UNT Digital Library
Top Quark Physics at the Tevatron (open access)

Top Quark Physics at the Tevatron

The authors review the field of top-quark physics with an emphasis on experimental techniques. The role of the top quark in the Standard Model of particle physics is summarized and the basic phenomenology of top-quark production and decay is introduced. They discuss how contributions from physics beyond the Standard model could affect the top-quark properties or event samples. The many measurements made at the Fermilab Tevatron, which test the Standard model predictions or probe for direct evidence of new physics using the top-quark event samples, are reviewed here.
Date: October 1, 2010
Creator: Deliot, Frederic; /DAPNIA, Saclay & Glenzinski, Douglas A.
System: The UNT Digital Library
The Role of Quench-back in the Passive Quench Protection of Uncoupled Solenoids in Series with and without Coil Sub-division (open access)

The Role of Quench-back in the Passive Quench Protection of Uncoupled Solenoids in Series with and without Coil Sub-division

This paper is the final paper in a series of papers that discusses passive quench protection for high inductance solenoid magnets. This report describes how passive quench protection system may be applied to superconducting magnets that are connected in series but not inductively coupled. Previous papers have discussed the role of magnet sub-division and quench back from a conductive mandrel in reducing the hot-spot temperature and the peak coil voltages to ground. When magnets are connected in series, quench-back from a conductive mandrel can cause other magnets in a string to quench even without inductive coupling between magnets. The magnet mandrels must be well coupled to the magnet circuit that is being quenched. When magnet circuit sub-division is employed to reduce the voltages-to-ground within magnets, the resistance across the subdivision becomes the most important factor in the successful quenching of the magnet string.
Date: October 15, 2010
Creator: Guo, Xing Long; Green, Michael A; Wang, Li; Wu, Hong & Pan, Heng
System: The UNT Digital Library
Results of applying a non-evaporative mitigation technique to laser-initiated surface damage on fused-silica (open access)

Results of applying a non-evaporative mitigation technique to laser-initiated surface damage on fused-silica

We present results from a study to determine an acceptable CO{sub 2} laser-based non-evaporative mitigation protocol for use on surface damage sites in fused-silica optics. A promising protocol is identified and evaluated on a set of surface damage sites created under ICF-type laser conditions. Mitigation protocol acceptability criteria for damage re-initiation and growth, downstream intensification, and residual stress are discussed. In previous work, we found that a power ramp at the end of the protocol effectively minimizes the residual stress (<25 MPa) left in the substrate. However, the biggest difficulty in determining an acceptable protocol was balancing between low re-initiation and problematic downstream intensification. Typical growing surface damage sites mitigated with a candidate CO{sub 2} laser-based mitigation protocol all survived 351 nm, 5 ns damage testing to fluences >12.5 J/cm{sup 2}. The downstream intensification arising from the mitigated sites is evaluated, and all but one of the sites has 100% passing downstream damage expectation values. We demonstrate, for the first time, a successful non-evaporative 10.6 {micro}m CO{sub 2} laser mitigation protocol applicable to fused-silica optics used on fusion-class lasers like the National Ignition Facility (NIF).
Date: October 26, 2010
Creator: Adams, J. J.; Bolourchi, M.; Bude, J. D.; Guss, G. M.; Matthews, M. J. & Nostrand, M. C.
System: The UNT Digital Library
Studies of non-proportionality in alkali halide and strontium iodide scintillators using SLYNCI (open access)

Studies of non-proportionality in alkali halide and strontium iodide scintillators using SLYNCI

Recently a collaboration of LLNL and LBNL has constructed a second generation Compton coincidence instrument to study the non-proportionality of scintillators. This device, known as SLYNCI (Scintillator Light-Yield Non-proportionality Characterization Instrument), has can completely characterize a sample with less than 24 hours of running time. Thus, SLYNCI enables a number of systematic studies of scintillators since many samples can be processed in a reasonable length of time. These studies include differences in nonproportionality between different types of scintillators, different members of the same family of scintillators, and impact of different doping levels. The results of such recent studies are presented here, including a study of various alkali halides, and the impact of europium doping level in strontium iodide. Directions of future work area also discussed.
Date: October 14, 2010
Creator: Ahle, Larry; Bizarri, Gregory; Boatner, Lynn; Cherepy, Nerine J.; Choong, Woon-Seng; Moses, William W. et al.
System: The UNT Digital Library
Transport and deposition of functionalized CdTe nanoparticles in saturated porous media (open access)

Transport and deposition of functionalized CdTe nanoparticles in saturated porous media

Comprehensive understanding of the transport and deposition of engineered nanoparticles (NPs) in subsurface is required to assess their potential negative impact on the environment. We studied the deposition behavior of functionalized quantum dot (QD) NPs (CdTe) in different types of sands (Accusand, ultrapure quartz, and iron-coated sand) at various solution ionic strengths (IS). The observed transport behavior in ultrapure quartz and iron-coated sand was consistent with conventional colloid deposition theories. However, our results from the Accusand column showed that deposition was minimal at the lowest IS (1 mM) and increased significantly as the IS increased. The effluent breakthrough occurred with a delay, followed by a rapid rise to the maximum normalized concentration of unity. Negligible deposition in the column packed with ultrapure quartz sand (100 mM) and Accusand (1 mM) rules out the effect of straining and suggests the importance of surface charge heterogeneity in QD deposition in Accusand at higher IS. Data analyses further show that only a small fraction of sand surface area contributed in QD deposition even at the highest IS (100 mM) tested. The observed delay in breakthrough curves of QDs was attributed to the fast diffusive mass transfer rate of QDs from bulk solution to …
Date: October 15, 2010
Creator: Torkzaban, S.; Wan, J.; Kim, Y.; Mulvihill, M. & Tokunaga, T. K.
System: The UNT Digital Library
Enhanced Magnetism of Fe3O4 Nanoparticles with Ga Doping (open access)

Enhanced Magnetism of Fe3O4 Nanoparticles with Ga Doping

Magnetic (Ga{sub x}Fe{sub 1-x}){sub 3}O{sub 4} nanoparticles with 5%-33% gallium doping (x = 0.05-0.33) were measured using x-ray absorption spectroscopy and x-ray magnetic circular dichroism to determine that the Ga dopant is substituting for Fe{sub 3+} as Ga{sub 3+} in the tetrahedral A-site of the spinel structure, resulting in an overall increase in the total moment of the material. Frequency-dependent alternating-current magnetic susceptibility measurements showed these particles to be weakly interacting with a reduction of the cubic anisotropy energy term with Ga concentration. The element-specific dichroism spectra show that the average Fe moment is observed to increase with Ga concentration, a result consistent with the replacement of A-site Fe by Ga.
Date: October 22, 2010
Creator: Pool, V. L.; Klem, M. T.; Chorney, C. L.; Arenholz, E. & Idzerda, Y.U.
System: The UNT Digital Library
Study of the neutron damage on electronics at the National Ignition Facility (open access)

Study of the neutron damage on electronics at the National Ignition Facility

The NIF environment is very complex leading to a large and non trivial radiation background. A shield surrounding the electronics is required to lower the neutron background to less than 1e7 n/cm{sup 2}. Moving electronics to behind the 6 foot-thick target bay wall is the best shield.
Date: October 28, 2010
Creator: Dauffy, L S; Mcnaney, J M & Khater, H Y
System: The UNT Digital Library
Nodal Diffusion Burnable Poison Treatment for Prismatic Reactor Cores (open access)

Nodal Diffusion Burnable Poison Treatment for Prismatic Reactor Cores

The prismatic block version of the High Temperature Reactor (HTR) considered as a candidate Very High Temperature Reactor (VHTR)design may use burnable poison pins in locations at some corners of the fuel blocks (i.e., assembly equivalent structures). The presence of any highly absorbing materials, such as these burnable poisons, within fuel blocks for hexagonal geometry, graphite-moderated High Temperature Reactors (HTRs) causes a local inter-block flux depression that most nodal diffusion-based method have failed to properly model or otherwise represent. The location of these burnable poisons near vertices results in an asymmetry in the morphology of the assemblies (or blocks). Hence the resulting inadequacy of traditional homogenization methods, as these “spread” the actually local effect of the burnable poisons throughout the assembly. Furthermore, the actual effect of the burnable poison is primarily local with influence in its immediate vicinity, which happens to include a small region within the same assembly as well as similar regions in the adjacent assemblies. Traditional homogenization methods miss this artifact entirely. This paper presents a novel method for treating the local effect of the burnable poison explicitly in the context of a modern nodal method.
Date: October 1, 2010
Creator: Ougouag, A. M. & Ferrer, R. M.
System: The UNT Digital Library
A luminescent nanocrystal stress gauge (open access)

A luminescent nanocrystal stress gauge

Microscale mechanical forces can determine important outcomes ranging from the site of material fracture to stem cell fate. However, local stresses in a vast majority of systems cannot be measured due to the limitations of current techniques. In this work, we present the design and implementation of the CdSe/CdS core/shell tetrapod nanocrystal, a local stress sensor with bright luminescence readout. We calibrate the tetrapod luminescence response to stress, and use the luminescence signal to report the spatial distribution of local stresses in single polyester fibers under uniaxial strain. The bright stress-dependent emission of the tetrapod, its nanoscale size, and its colloidal nature provide a unique tool that may be incorporated into a variety of micromechanical systems including materials and biological samples to quantify local stresses with high spatial resolution.
Date: October 25, 2010
Creator: Choi, Charina; Koski, Kristie; Olson, Andrew & Alivisatos, Paul
System: The UNT Digital Library
Post-Shot Radiation Environment Following Low-Yield Shots Inside the National Ignition Facility (open access)

Post-Shot Radiation Environment Following Low-Yield Shots Inside the National Ignition Facility

A detailed model of the Target Bay (TB) at the National Ignition Facility (NIF) has been developed to estimate the post-shot radiation environment inside the facility. The model includes large number of structures and diagnostic instruments present inside the TB. These structures and instruments are activated by the few nanosecond pulse of neutrons generated during a shot and the resultant gamma dose rates are estimated at various decay times following the shot. The results presented in this paper are based on a low-yield D-T shot of 10{sup 16} neutrons. General environment dose rates drop to below 3 mrem/h within three hours following a shot with higher dose rates observed at contact with some of the components. Dose rate maps of the different TB levels were generated to aid in estimating worker stay-out times following a shot before entry is permitted into the TB.
Date: October 29, 2010
Creator: Sitaraman, S.; Brereton, S.; Dauffy, L.; Hall, J.; Hansen, L.; Khater, H. et al.
System: The UNT Digital Library
Validation of two ribosomal RNA removal methods for microbial metatranscriptomics (open access)

Validation of two ribosomal RNA removal methods for microbial metatranscriptomics

The predominance of rRNAs in the transcriptome is a major technical challenge in sequence-based analysis of cDNAs from microbial isolates and communities. Several approaches have been applied to deplete rRNAs from (meta)transcriptomes, but no systematic investigation of potential biases introduced by any of these approaches has been reported. Here we validated the effectiveness and fidelity of the two most commonly used approaches, subtractive hybridization and exonuclease digestion, as well as combinations of these treatments, on two synthetic five-microorganism metatranscriptomes using massively parallel sequencing. We found that the effectiveness of rRNA removal was a function of community composition and RNA integrity for these treatments. Subtractive hybridization alone introduced the least bias in relative transcript abundance, whereas exonuclease and in particular combined treatments greatly compromised mRNA abundance fidelity. Illumina sequencing itself also can compromise quantitative data analysis by introducing a G+C bias between runs.
Date: October 1, 2010
Creator: He, Shaomei; Wurtzel, Omri; Singh, Kanwar; Froula, Jeff L; Yilmaz, Suzan; Tringe, Susannah G et al.
System: The UNT Digital Library
Towards Long-Term Corrosion Resistance in FE Service Environments (open access)

Towards Long-Term Corrosion Resistance in FE Service Environments

The push for carbon capture and sequestration for fossil fuel energy production has materials performance challenges in terms of high temperature oxidation and corrosion resistance. Such challenges will be illustrated with examples from several current technologies that are close to being realized. These include cases where existing technologies are being modified—for example fireside corrosion resulting from increased corrosivity of flue gas in coal boilers refit for oxy-fuel combustion, or steam corrosion resulting from increased temperatures in advanced ultra supercritical steam boilers. New technology concepts also push the high temperature corrosion and oxidation limits—for example the effects of multiple oxidants during the use of high CO2 and water flue gas used as turbine working fluids.
Date: October 1, 2010
Creator: Holcomb, G. R. & Wang, P.
System: The UNT Digital Library
The Importance of High Temporal Resolution in Modeling Renewable Energy Penetration Scenarios (open access)

The Importance of High Temporal Resolution in Modeling Renewable Energy Penetration Scenarios

Traditionally, modeling investment and dispatch problems in electricity economics has been limited by computation power. Due to this limitation, simplifications are applied. One common practice, for example, is to reduce the temporal resolution of the dispatch by clustering similar load levels. The increase of intermittent electricity from renewable energy sources (RES-E) changes the validity of this assumption. RES-E already cover a certain amount of the total demand. This leaves an increasingly volatile residual demand to be matched by the conventional power market. This paper quantifies differences in investment decisions by applying three different time-resolution residual load patterns in an investment and dispatch power system model. The model optimizes investment decisions in five year steps between today and 2030 with residual load levels for 8760, 288 and 16 time slices per year. The market under consideration is the four zone ERCOT market in Texas. The results show that investment decisions significantly differ across the three scenarios. In particular, investments into base-load technologies are substantially reduced in the high resolution scenario (8760 residual load levels) relative to the scenarios with lower temporal resolution. Additionally, the amount of RES-E curtailment and the market value of RES-E exhibit noteworthy differences.
Date: October 8, 2010
Creator: Nicolosi, Marco; Mills, Andrew D & Wiser, Ryan H
System: The UNT Digital Library
Photodetectors for Scintillator Proportionality Measurement (open access)

Photodetectors for Scintillator Proportionality Measurement

We evaluate photodetectors for use in a Compton Coincidence apparatus designed for measuring scintillator proportionality. There are many requirements placed on the photodetector in these systems, including active area, linearity, and the ability to accurately measure low light levels (which implies high quantum efficiency and high signal-to-noise ratio). Through a combination of measurement and Monte Carlo simulation, we evaluate a number of potential photodetectors, especially photomultiplier tubes and hybrid photodetectors. Of these, we find that the most promising devices available are photomultiplier tubes with high ({approx}50%) quantum efficiency, although hybrid photodetectors with high quantum efficiency would be preferable.
Date: October 18, 2010
Creator: Moses, William W.; Choong, Woon-Seng; Hull, Giulia; Payne, Steve; Cherepy, Nerine & Valentine, J. D.
System: The UNT Digital Library
Plutonium complexation by phosphonate-functionalized mesoporous silica (open access)

Plutonium complexation by phosphonate-functionalized mesoporous silica

MCM-41-type mesoporous silica functionalized with the CMPO-based 'Ac-Phos' silane has been reported in the literature (1) to show good capacity as an acftinide sorbent material, with potential applications in environmental sequestration, aqueous waste separation and/or vitrification, and chemical sensing of actinides in solution. The study explores the complexation of Pu(IV and VI) and other selected actinides and lanthanides by SBA-15 type mesoporous silica functionalized with Ac-Phos. The Pu binding kinetics and binding capacity were determined for both the Ac-Phos functionalized and unmodified SBA-15. They analyzed the binding geometry and redox behavior of Pu(VI) by X-ray absorption spectroscopy (XAS). They discuss the synthesis and characterization of the functionalized mesoporous material, batch sorption experiments, and the detailed analyses of the actinide complexes that are formed. Structural measurements are paired with high-level quantum mechanical modeling to elucidate the binding mechanisms.
Date: October 27, 2010
Creator: Parsons-Moss, T; Schwaiger, L K; Hubaud, A; Hu, Y J; Tuysuz, H; Yang, P et al.
System: The UNT Digital Library
Oxidative cleavage of erucic acid for the synthesis of brassylic acid (open access)

Oxidative cleavage of erucic acid for the synthesis of brassylic acid

The main focus of this work is to synthesize Brassylic Acid (BA) using oxidative cleavage of Erucic Acid (EA). Crambe (Crambe abyssinica) is an industrial oilseed grown in North Dakota. Crambe has potential as an industrial fatty acid feedstock as a source of Erucic acid (EA). It has approximately 50-60 % of EA, a C{sub 22} monounsaturated fatty acid. Oxidative cleavage of unsaturated fatty acids derived from oilseeds produces long chain (9, 11, and 13 carbon atoms) dibasic and monobasic acids. These acids are known commercial feedstocks for the preparation of nylons, polyesters, waxes, surfactants, and perfumes. Other sources of EA are Rapeseed seed oil which 50-60 % of EA. Rapeseed is grown outside USA. The oxidative cleavage of EA was done using a high throughput parallel pressure reactor system. Kinetics of the reaction shows that BA yields reach a saturation at 12 hours. H{sub 2}WO{sub 4} was found to be the best catalyst for the oxidative cleavage of EA. High yields of BA were obtained at 80 C with bubbling of O{sub 2} or 10 bar of O{sub 2} for 12 hours.
Date: October 29, 2010
Creator: Nasrullah, Mohammed J.; Thapliyal, Pooja; Pfarr, Erica N.; Dusek, Nicholas S.; Schiele, Kristofer L. & Bahr, James A.
System: The UNT Digital Library
ADVANCING REACTIVE TRACER METHODS FOR MONITORING THERMAL DRAWDOWN IN GEOTHERMAL ENHANCED GEOTHERMAL RESERVOIRS (open access)

ADVANCING REACTIVE TRACER METHODS FOR MONITORING THERMAL DRAWDOWN IN GEOTHERMAL ENHANCED GEOTHERMAL RESERVOIRS

Reactive tracers have long been considered a possible means of measuring thermal drawdown in a geothermal system, before significant cooling occurs at the extraction well. Here, we examine the sensitivity of the proposed method to evaluate reservoir cooling and demonstrate that while the sensitivity of the method as generally proposed is low, it may be practical under certain conditions.
Date: October 1, 2010
Creator: Plummer, Mitchell A.; Palmer, Carl D.; Mattson, Earl D.; Redden, George D. & Hull, Laurence C.
System: The UNT Digital Library
The Northwest Geysers EGS Demonstration Project Phase 1: Pre-stimulation coupled geomechanical modeling to guide stimulation and monitoring plans (open access)

The Northwest Geysers EGS Demonstration Project Phase 1: Pre-stimulation coupled geomechanical modeling to guide stimulation and monitoring plans

This paper presents activities and results associated with Phase 1 (pre-stimulation phase) of an Enhanced Geothermal System (EGS) demonstration project at the northwest part of The Geysers geothermal field, California. The paper presents development of a 3-D geological model, coupled thermal-hydraulic-mechanical (THM) modeling of proposed stimulation injection as well as current plans for stimulation and monitoring of the site. The project aims at creating an EGS by directly and systematically injecting cool water at relatively low pressure into a known High Temperature (about 280 to 350 C) Zone (HTZ) located under the conventional (240 C) steam reservoir at depths of {approx}3 km. Accurate micro-earthquake monitoring initiated before the start of the injection will be used as a tool for tracking the development of the EGS and monitoring changes in microseismicity. We first analyzed historic injection and micro-earthquake data from an injection well (Aidlin 11) located about 3 miles to the west of the new EGS demonstration area. Thereafter, we used the same modeling approach to predict the likely extent of the zone of enhanced permeability for a proposed initial injection in two wells (Prati State 31 and Prati 32) at the new EGS demonstration area. Our modeling indicates that the …
Date: October 20, 2010
Creator: Rutqvist, J.; Dobson, P. F.; Oldenburg, C. M.; Garcia, J. & Walters, M.
System: The UNT Digital Library