This report summarizes progress on investigation into improving the technological limits of boiling water reactors, Vallecitos Boiling Water Reactor and other facilities.

The primary purpose of this joint USAEC-Euratom program is to obtain a better understanding if the maximum achievable operating characteristics of UO2 as a reactor fuel. During the program work will be performed in two areas that have been of concern to reactor core designers for a long time, namely fission gas release and central melting in fuel rods.

Introduction: The objective of Project Agreement 22 is to determine the feasibility of covering the complete reactor neutron flux start range from 10(3) - 5 x 10(13) nv by using in-core chambers. The counting mode of operating will be used at low neutron fluxes and the root mean square voltage fluctuation mode will be used at high neutron flux levels. Experiments have been run utilizing various ion chambers, gases, gas pressures, voltage, and cables to measure sensitivities and range operating in the counting and RMS voltage modes. Theoretical discussions are presented showing how the RMS voltage is related to individual pulse at both amplifier input and output. Noise is also compared at amplifier output so that the optimum bandwidth can be selected. Spectral shifts with changes in applied voltage causing signal variations have been examined and can be eliminated by appropriate selection of amplifier bandwidth. In the counting mode, all experiments have been conducted with unterminated cable. The chamber has been designed with geometry, gas, and pressure to completely stop fission fragments in the gas and hence maximize the charge generated in the chamber. Cables have been selected to minimize capacity. Various gases, pressures, and voltages have been used to …

A research program is being conducted to obtain experimental data in the irradiation of plutonium-enriched fuel to confirm a theoretical model for predicting isotopic composition and reactivity changes in plutonium-enriched, light-water-moderated reactors. Quarterly progress: The densitometry procedure (for measurement of alpha autoradiographs of fuel pellets) has been modified to eliminate the need for a second emulsion. The existence of a problem of latent image fading and non-reciprocity of the high-resolution emulsion has been recognized. A tentative procedure has been worked out to correct these emulsion difficulties. the number of polished pellets has been increased to thirteen. The number of hot spots per pellet has not changed appreciably. The largest spot seen is irregular with an estimated volume equivalent to that of a sphere of 35 mil diameter with a PuO2 concentration in the neighborhood of 60%. The VBWR irradiation run now under way is not scheduled to end until October. To the end of the last run the cumulative exposure reached 3703 MWD/T, as logged by VBWR operating personnel. Applying the same scale factor between logged exposure and Ce-Cs analysis of the first fuel sample gives a corrected exposure of 4416 MWD/T. Further debugging of EPITHERMOS, the epithermal extension of …

Work performed during the quarter is summarized by; direct measurement of fission gas pressure, loop operations, performance of UO2 fuel, UO2 grain growth and melting studies.

Summary: Fundamental studies in support of the alloy design work are complete except for the experimental determination of the diffusion of oxygen in alloy-doped non-stoichiometric ZrO2. Over 100 oxidation runs have now been made on samples of ZrO2 doped with 1 mole percent of the oxides of Al, Y, Fe, Cr, and Ni. The first round testing of 31 alloys is now essentially complete. Analysis of the steam corrosion rate and hydriding raw data taken at 300, 400, and 500 degrees C indicates that Zr-Cr and Zr-Cu-Fe alloys show the most promise for development for service in steam over the entire temperature range 300-500 degrees C. Maximum resistance to corrosion hydrogen embrittlement requires high initial ductility and thus low, perhaps less than ~2.5 a/o total alloy content. For any composition, susceptibility to hydrogen embrittlement depends on crystallographic texture of the component; under certain circumstances hydrogen embrittlement may be high anisotropic. The second-round testing of 10 selected Zr-Cr and Zr-Cu base alloys is now about 50% complete. Three alternate fabrication schedules were evaluated; and the preliminary results indicate that the Zr-Cu alloy tested is less sensitive to heat treatment than is the Zr-Cr alloy tested. Raising the final alpha annealing temperature …

Quarterly report discussing progress on the Fast Ceramic Reactor Development Program. Information is reported on vented fuel production, fuel testing in TREAT, fuel performance evaluation, fast-flux irradiation of fuel, and reactor dynamics and design.

Quarterly progress report discussing activities related to the Vallecitos Boiling Water Reactor (VBWR) and related facilities

Activities in a program to develop techniques in the use of pulsed neutron sources to measure shutdown parameters related to large thermal power reactors are reported. The development of pulsed neutron source techniques for large power reactors has led to a new theoretical model recently developed by E. Garelis and J.L. Russell, Jr. The theory is presently based on a bare, one-group model with m-delayed precursors and takes all spatial modes into account. Results indicate, however, that the application of this model is much broader. Experiments were designed and carried out to both verify this new theory and to demonstrate the performance of the experimental hardware in a large power reactor.

The United States and the European Atomic Energy Community (Euratom), on May 29, and June 18, 1958, signed an agreement which provides a basis for co-operation in programs for the advancement of the peaceful applications of atomic energy. The work described in this report represents the Joint U.S.-Euratom effort. The over-all development program is designed to obtain the test data and operating experience necessary to eventually realize a 50 percent increase in the output of the Garigliano Nuclear Power Station located at Sessa Aurunca (Campania, Italy). Two tasks are in progress: Task III-F involves the preparation of test specimens of reactor vessel material for irradiation; Task IV consists of the formulation of specification for a complete data logging and computer system.

Summary: Initial critical heat flux, transition boiling temperature fluctuation, and film boiling coefficient data have been obtained on a two-rod cluster assembly at 1000 psia and 25 to 90 percent steam qualities. A representation showing the range of critical heat flux data is presented. Typical temperature recordings which indicate transition and film boiling behavior are shown. Fabrication of a new high pressure observational test section is nearly complete. An optical table and illumination system has been build and operationally tested for photographic use on the new observational section.

Development of nuclear reactor cores having high power density, long fuel life, and low fabrication costs is the objective of this program sponsored by the AEC. Five tasks are in progress: (1) Task 1A-High Power Density Fuel Development. The number of assemblies has been reduced to seven as a result of the failure of two pellet fuel assemblies. The average burnup of the group operating as of September 1 is 7500 MWD/T. (2) Task 1B-Fuel Fabrication Development. Assembly. Assembly 12S gave positive signals of being a leaker under the multi-type in-core sampler and was declared failed based on the in-core results and visual observation of a cracked rod. Modifications to the instrumented fuel assembly probes were made by removing the failed flow meter rotors to allow continued use of the flux detectors and thermocouples. Flux detectors and thermocouples performed properly after reactor start up. Flux wire tubes were found to be kinked such that their use was prohibited. (3) Task II-Stability, Heat Transfer and Fluid Flow. A series of noise recordings of fluxes, flows, and temperatures has been made at 91 MWt at the Big Rock Point plant. Preliminary analyses of some of the these records were made to obtain …

Abstract; Technical report describing a low-flow autoclave system developed for out-of-pile corrosion testing of materials in controlled environment steam up to 500 C. The system has been set up in triplicate to provide for the exposure of various zirconium alloys to steam at 300, 400, and 500 C. The oxygen and hydrogen of the steam were controlled at 25 ppm and 3 ppm, respectively, to simulate the gas conditions from radiolytic water decomposition found in a boiling water reactor. The autoclave internals were so designed to result in a temperature variation between specimens under test of less than 2C.

Technical report describing sixteen fuel rods clad with thin type 304 stainless steel and filled with vibratory compact powder UO2 that were fabricated and incorporated into a bundle for irradiation testing in the VBWR. The UO2 powders were tested for gas content. N2, CO, and H2 were the principal gases evolved by both type of UO2, but the arc-fused UO2 released about ten times as much gas as the Dyna Pak UO2. The amount of gas released was also a function of particle size and temperature. The gas evolution data were used to design the gas plenum to accommodate the absorbed gases along with the fission gases.

Technical report of a proposal of an analytical model to predict two-phase critical flow rate. The model is based upon thermal equilibrium, a "lumped" treatment of the two-phase velocity (each phase is represented by a single mean velocity), and upon the neglect of frictional and hydrostatic pressure losses. A comparison, of the proposed predictions with available test results and previous analyses shows that: (1) The present model agrees very well with the published test data. (2) In contrast to all other analyses, the model requires no assumption about the gas void fraction.

Summary: A prototype control rod containing absorber plates made from an electro- deposited dispersion of boron carbide in nickel was tested in the VBWR. It was exposed to the reactor environment of 545 degree F boiling water and thermal neutron fluxes (perturbed) which ranged from 0.6 to 1.1 x 10/sup 13/ nv for 2236 hours over a period of six months. The maximum B/sup 10/ burnup achieved during the test period was 1.8 percent. After irradiation, the rod was examined. The results of the examination are summarized below: (1) The B/sub 4/C-- Ni plate assembly did not undergo significant dimensional changes during irradiation. (2) Numerous blisters developed on both the outer and inner surfaces of three of the four plates. Blistering was more severe on the outer surface than on the inner, and was most severe in a large region located in the lower half of plate 4. Metallographic examination revealed that the blisters were located only in the 2- mil protective nickel overlay covering the B/sub 4/C-- Ni dispersion. It was concluded that they formed from the buildup of gas pressure at the Ni: Ni-- B/sub 4/C interfaces, rather than from corrosion attack. Helium from the B/sup 10/(n alpha …

GE is amending its application of 6/5/57 to construct and operate the Nuclear Test Reactor in order to incorporate changes in procedure and equipment.

A method of determining enclosure pressure in the event of a reactor rupture is presented and a sample calculation is shown. This method was used in calculating the design pressure of the Dresden Nuclear Power Station enclosure.

Methods for analyzing chemical impurities in sodium metal samples are presented. Chemical analysis was used to determine the following impurities: Calcium, Carbon, Chromium, Iron, Lithium, Nickel, Oxygen, Potassium, and Zirconium. Spectrographic analysis was used to determine many other impurities. Sodium samples obtained from experimental apparatus operated as part of the work being conducted for Atomics International were analyzed by these methods.

Experimental results on the effect of periodic acceleration on a natural circulation, 1000 psia, two-phase flow loop are presented, and related to the topic of marine reactor design. The initial results of this work were given previously in GEAP 3397.

Development of nuclear reactor cores having high power density, long fuel life, and low fabrication costs is the objective of this program sponsored by the AEC. It will be achieved by extensive development and testing carried out in conjunction with the design, construction and operation of the Big Rock Point plant of the Consumers Power Company in Michigan. This second quarterly report describes the progress achieved from July through September 1960.

Three thin-wall stainless steel fuel specimens made using fabrication processes and materials similar to the Consumers Big Rock Plant research and development fuel rods were power cycled 3000 times between 500,000 and 75,000 BTU/hr-ft2 in the General Electric Test Reactor (GETR) Trail Cable facility. The fuel specimens were exposed to 1000 psi boiling water. All of the fuel specimens withstood the test without failing or without any significant changes in the clad characteristics.

The work described in this report represents progress toward an agreement signed by the United States and the European Atomic Energy Community which provides a basis for cooperation in programs for the advancement of peaceful applications of atomic energy.

Work has continued on the development of accurate nuclear fuel burnup analysis. Work performed by the third quarter of 1962 is summarized.