Report on solving problems with shell-and-tube heat exchangers resulting from recent trends toward higher flowrates, larger size, and optimized designs.

Typical industrial shell-and-tube heat exchanger configurations are investigated systematically for the occurrence of potentially damaging tube vibration as a function of flow-rate. In continuation of an ongoing experimental program, results from shell-side water flow tests of twenty-two additional test exchanger configurations are reported. The test cases include single- and double-segmentally baffled tube bundles having various combinations of triangular and square tube layout patterns, baffle arrangements, and baffle edge orientations. All layouts had a tube pitch-to-diameter ratio of 1.25. The testing focused on identification of the lowest critical flow-rates to initiate fluid-elastic instability and/or large amplitude tube motion and the location within the bundle of the tubes which first experience these responses. The threshold flow-rates are determined from a combination of methods based on sensory observations, vibration amplitude data, and frequency response information. Instability criteria are preliminarily evaluated. Also reported are the measured overall shell-side pressure drop and the incremental pressure drops across sections of the exchanger for all configurations.

A set of programs, gathered from major Argonne computer users, was run on the current generation of supercomputers: the CRAY X-MP-4, Fujitsu VP-200, and Hitachi S-810/20. The results show that a single processor of a CRAY X-MP-4 is a consistently strong performer over a wide range of problems. The Fujitsu and Hitachi excel on highly vectorized programs and offer an attractive opportunity to sites with IBM-compatible computers.

In this document we present the characteristics of the electromagnetic radiation from various types of sources on a 6-GeV storage ring. The sources include bending magnets, undulators and wigglers. The characteristics are compared with those of other synchrotron sources when operated at their design specifications. The influence of positron beam size on the brilliance is discussed, along with the power distribution from these sources. The goal of this document is to provide users with enough information on the behavior of radiation from a 6-GeV storage ring so that a dialogue can be established with the accelerator physicists and engineers to achieve an optimal design.

As multiprocessors become commercially available, a great deal of concern is being focused on the problems involved in writing and debugging software for such machines. Earlier work described the use of monitors implemented by macro processors to attain portable code. This work formulates a general-purpose monitor which simplifies the programming of a wide class of numeric algorithms. We believe that the approach of describing a set of schedulable units of computation advocated by Brown offers a real simplification for the applications programmer. In this paper, we propose a straight-forward programming paradigm for describing schedulable units of computation that allows the description of many algorithms with very little effort.

A generic three-dimensional thermal model was developed for analyzing the thermal behavior of electric-vehicle batteries. The model calculates temperature distribution and excursion of a battery during discharge, change, and open circuit. The model takes into account the effects of heat generation, internal conduction and convection, and external heat dissipation on the temperature distribution in a battery. The three-dimensional feature of the model permits incorporation of various asymmetric boundary conditions; thus the effects of cell orientation and packaging on thermal behavior can be analyzed for a multiple-cell battery pack. Various modes of boundary heat transfer such as radiation, insulation, and natural and forced convections were also included in the model.

This report summarizes the work done to date on the application of the TRUEX solvent extraction process for removing and separately recovering plutonium and americium from a nitric acid waste solution containing these elements, uranium, and a complement of inert metal ions. This simulated waste stream is typical of a raffinate from a tributyl phosphate (TBP)-based solvent extraction process for removing uranium and plutonium from dissolved plutonium-containing metallurgical scrap. The TRUEX process solvent in these experiments was a solution of TBP and octyl(phenyl)-N,N-diisobutylcarbamoylmethylphosphine oxide (CMPO) dissolved in carbon tetrachloride. A flowsheet was designed on the basis of measured batch distribution ratios to reduce the TRU content of the solidified raffinate to less than or equal to 10 nCi/g and was tested in a countercurrent experiment performed in a 14-stage Argonne-model centrifugal contractor. The process solvent was recycled without cleanup. An unexpectedly high evaporative loss of CCl4 resulted in concentration of the active extractant, CMPO, to nearly 0.30M in the solvent. Results are consistent with this higher CMPO concentration. The raffinate contained only 2 nCi/g of TRU, but the higher CMPO concentration resulted in reduced effectiveness in the stripping of americium from the solvent. Conditions can be easily adjusted to give …

Fluid forces are important in the assessment of vibration of the Space Shuttle Main Engine liquid oxygen posts. This report summarizes the available data on fluid excitation forces acting on tube arrays in turbulent crossflow, and test results for an array of tubes subject to turbulent flow. The fluctuating drag and lift forces are measured as a function of Reynolds number, incoming flow conditions, and tube location in an array.

A general theory of fluid-elastic instability for a tube array in crossflow is presented for application to the space shuttle main engine liquid oxygen (SSME LOX) posts. Various techniques to obtain the motion-dependent fluid-force coefficients are discussed and the general instability characteristics are summarized. The theory is also used to evaluate the results of other mathematical models for crossflow-induced instability.

Report of the activities of the physics division at Argonne including the successful completion of Argonne Tandem-Linac Accelerator System.

Measurements are described for determining average values of fission rates in uranium-235, uranium-238 and plutonium-239 and capture rates in uranium-238 for heterogeneous cells used to construct fast critical assemblies. The measurements are based on irradiations of foils of uranium-238, uranium-235 and plutonium-239 with counting of fission and capture products using gamma-ray spectroscopy. Both plate and pin cells are considered. Procedures are described for inferring cell-average reaction rate values from a single foil location based on a cell using a quantity called a cell factor. Cell factors are determined from special measurements in which several foils are irradiated within a cell. Comparisons are presented between cell factors determined by measurements and by Monte Carlo calculations which lend credibility to the measurement procedures.

Eccentricity of a specific slip-joint design separating two cantilevered, telescoping tubes did not create any self-excited lateral vibrations that had not been observed previously for a concentric slip joint. In fact, the eccentricity made instabilities less likely to occur, but only marginally. Most important, design rules previously established to avoid instabilities for the concentric slip joint remain valid for the eccentric slip joint.

This report provides a summary of theoretical and experimental studies of actinide spectra in condensed phases. Much of the work was accomplished at Argonne National Laboratory, but references to related investigations by others are included. Spectroscopic studies of the trivlent actinides are emphasized, as is the use of energy level parameters, evaluated from experimental data, to investigate systematic trends in electronic structure and other properties. Some reference is made to correlations with atomic spectra, as well as with spectra of the (II), (IV), and higher valence states.

Report on research in carcinogenesis, human radiobiology, low-level radiation, molecular biology, and toxicology.

When calculations of flux are done in less than three dimensions, leakage-absorption cross sections are normally used to model leakages (flows) in the dimensions for which the flux is not calculated. Since the neutron flux is axially dependent, the leakages, and hence the leakage-absorption cross sections, are also axially dependent. Therefore, to obtain axial flux profiles (or reaction rates) for individual subassemblies, an XY-geometry calculation delineating each subassembly has to be done at several axial heights with space- and energy-dependent leakage-absorption cross sections that are appropriate for each height. This report discusses homogeneous and heterogeneous XY-geometry calculations at various axial locations and using several differing assumptions for the calculation of the leakage-absorption cross section. The positive (outward) leakage-absorption cross sections are modeled as actual leakage absorptions, but the negative (inward) leakage-absorption cross sections are modeled as either negative leakage absorptions (+-B² method) or positive downscatter cross sections (the ..sigma../sub s/(1 ..-->.. g) method).

Section I introduces the material contained in the rest of the report. Section II presents the origin and characteristics of humic materials as we understand them today and outlines the methods that have been used to separate and analyze these substances. Section III focuses on the general problem of metal-organic interactions and treats some of the factors that are important in chelating and complexing of metal ions by humic substances. Section IV deals specifically with the complexing of radionuclides by organic substances, treated from the standpoint of both empirical and experimental studies.

This report contains historical information on the Li-alloy/FeS system that will be useful in its future applications. This document includes the following: (1) the chemical and electrochemical reactions for the Li-alloy/FeS system, accomplishments in past cell development efforts, and performance attained by state-of-the-art cells vs performance goals; (2) detailed drawings of state-of-the-art cell designs, documentation of cell fabrication techniques, and comparisons of alternative types of cell components (such as BN felt vs MgO powder separators, stainless vs low-carbon steel cell housings) and fabrication techniques (such as charged vs uncharged electrodes); (3) results of post-test cell analyses, including cell failure mechanisms, electrode morphology and active material distribution, and in-cell corrosion rates; (4) data from trade-off studies between specific power and energy; (5) discussion of battery design considerations (e.g., volumetric energy density, battery charger, and high-efficiency thermal insulation); (6) results of cost studies, which include materials and manufacturing costs of cells and batteries and heating costs involved in battery operation; and (7) projections of cell designs having the greatest potential for meeting electric-vehicle performance requirements.

Quarterly report on activities of Argonne National Laboratory's Nuclear Technical Programs, including a review of studies of the ability of backfill to inhibit groundwater flow in a nuclear waste repository.

Quarterly report discussing fuel cell research and development work at Argonne National Laboratory (ANL). This report describes studies directed toward seeking alternative cathode materials to NiO for molten carbonate fuel cells.

This report summarizes the flow-induced vibration of circular cylinders in quiescent fluid, axial flow, and crossflow, and applications of the analytical methods and experimental data in design evaluation of various system components consisting of circular cylinders.

Fluid excitation forces are measured in a water loop for two circular cylinders arranged in tandem and normal to flow. The Strouhal number and fluctuating drag and lift coefficients for both cylinders are presented for various spacings and incoming flow conditions. Results show the effects of Reynolds number, pitch ratio, and upstream turbulence on the fluid excitation forces.

Tutorial description of the Warren machine with a basic introduction to the motivation of the machine and the instructions that define it. Discussion of the fairly limited extensions required to extend the machine for more general use outside of implementations of logic programming. Substantial speedups will occur due to improvements in the implementation of the basic algorithms.

A set of macro libraries has been developed that allows programmers to write portable FORTRAN code for multiprocessors. This document presents, in tutorial form, the macros used to implement three common synchronization patterns: self-scheduling DO-loops, barrier synchronization, and the askfor monitor.

Pre and postprocessors have been written for an established hydraulic program (COMMIX-IHX) which enables prediction of the internal crossflow field for each tube of Argonne's Test Heat Exchanger and identification of those tubes most likely to experience fluid-elastic instability, together with the instability vibration mode. While the direct use of the HXVA method is limited to single pass, single-segmentally baffled tube bundle configurations, its algorithms and methods can be applied to any type of heat exchanger which can be analyzed by COMMIX-IHX. The processors are explained and an example problem is given along with comparisons of experimental results.