Abstract: The caustic permanganate-rinse decontamination treatment was investigated. Loop and metallurgical studies were performed to determine optimum operating conditions as well as the metallurgical effects of the treatment. A treatment with 10 percent sodium hydroxide and 5 percent potassium permanganate solution followed by a rinse with a 5 percent ammonium citrate, 2 percent citric acid and 1/2 percent Versene solution was chosen for the decontamination of a stainless steel steam generator. Decontamination factors of greater than 50 were obtained in loop tests using the above treatment. Corrosion and metallurgical results indicated a total penetration of less than 0.01 mil on annealed Type 304 stainless steel with no evidence of any deleterious effects.

Abstract: A survey of the problem of reactor system contamination by radioactive material and methods that have been employed to remove the material was carried out. Following this survey, an investigation of chemical solutions was undertaken to find one which might be successfully employed in the decontamination of a stainless steel steam generator. From a preliminary screening, the most promising chemical method from the view point of minimum corrosion and maximum decontamination is a caustic permanganate treatment followed by and acid rinse.

Abstract: A decontamination procedure for a stainless steel steam generator similar to the APPR-1 using a fill-flush application of a caustic permanganate-citrate combination solution is recommended. The isolation of the steam generator is to be accomplished by means of specially designed plugs at the reactor vessel outlet and at the primary coolant pumps. Anticipated results, including corrosion rates and decontamination factors, are presented.

Abstract: The primary coolant of the SM-1 (APPR-1) was analyzed for short-lived and fission product activities. Manganese-56 was found to be the predominant non-fission product nuclide contributing to the short lived activity. Fission products were found in the coolant. It is concluded these fission products originate from a defects in the cladding and from surface contamination of the fuel elements.

Introduction: Seldom does the actual arrangement of control elements in a nuclear reactor confers to the ideal and convenient mathematical array. In order to achieve shim control. safety and regulation, it is desirable to design with rods of different sizes and materials. With given fuel element arrangement, typically in square or hexagonal lattice spacing, there will be rods located at different distances form the center of the core and from each other. As the reactor operates, absorbers will be withdrawn, leaving further asymmetries in the location of those remaining. It is the purpose of this report to develop in detail a two-group diffusion theory with as complete generality as possible. The method is as yet restricted to the unreflected core, or to the reflected core by use of reflector savings and bare equivalent geometries.

Abstract: Fission product measurements were made on the SM-1 primary coolant. The airborne activity observed during the sampling of the primary system was identified. An analysis was made on the primary coolant for alpha activity and on the secondary water for fission production iodine.

Abstract: The results of activity buildup studies in the SM-1 (APPR-1) performed from February 1958 to January 1959 are reported. Data are presented on the extent, nature, and mechanism of the buildup of long-lived gamma emitting nuclides in the reactor primary system. Mathematical equations to describe the activity buildup are derived. Radiation levels after reactor shutdown are presented, as well as the predicted radiation levels at the end of core life.

Abstract: Critical experiment studies were performed, varying the parameters U235, B10 and metal to water ratio, in the SM-2 7 x 7 core configuration with 38 stationary elements and seven control rods of the SM-1 (APPR-1) type. An experimental mock-up of the SM-1 was assembled using the basic SM-2 fuel plates. Excellent agreement between the SM-1 boron loading, determined by chemical analysis, and the SM-1 mock-up boron loading, for equivalent bank positions, was noted. Several SM-2 mock-ups, cold clean and midlife, were assembled and studied with regard to reflector effects, flow divider effects, relative control rod array worths, critical rod configurations, and relative power distributions. The results of these experiments indicate as satisfactory a U235 loading of 36.4 Kg and a B10 loading of 63.4 grams for the SM-2. Attention is drawn to numerous power peaks present in the active core. The open seven control rod array has a slight reactivity advantage over the closed seven array and consequent minor disadvantage with respect to "stuck rod" criteria.

Abstract: This technical report contains a description and results of a second series of critical experiments performed on the SM-2 core mock-up, as additional to the first series of experiments reported in APAE No. 54. The SM-2 core mock-up contains 36.4 kg U-235 and and estimated 67.9 gm B-10. The equivalent diameter and the active height are about 22 in.; the metal-to-water volume ration is 0.344. Data is presented on activation, reactivity, and stuck rod measurements. All measurements were conducted on the open seven control rod array employing 38 stationary fuel elements. Activation measurements consisted of neutron flux measurements using uranium fission foils for relative power distribution studies, the effect of flux suppressors on reducing power peaks, blocked coolant channel measurements, and gamma ray dose distribution. Reactivity measurements were performed to determine the effect f flow divider, flux suppressors and stimulated high temperature and pressure operation; b-10 loading in the SM-2 core; and core material coefficients. For the later, the worth in cents per gm or cents per cc was determined at simulated temperature of 510 degree F for B-10, U-235, stainless steel, and void. Stuck rod measurements were made to obtain an indication of the criticality margin in the …

Abstract: This technical report is concerned with the program and results of the SM-1 reactor vessel head removal and core inspection at Fort Belvoir, Virginia from the period March 7, 1969 to May 17, 1959. It covers the operating procedures in detail and records the conditions found and problems encountered in order to make a record for reference in future work of this nature. The major objective of the program, to obtain irradiation data on the SM-1 type core, has been met. The boron control rod elements were found unsatisfactory for full core life, and europium oxide elements were placed in the core for future irradiation stability data. A major problem was experienced with the cracked pressure vessel head studs. The methods developed for the removal of the broken studs are presented. The complete metallurgical study of the stud failure from stress corrosion is included as Appendix B.

Summary: Prototype testing of the safety and control rod drives indicated that both units functioned properly. No major problems were encountered during testing. Seal leakage data collected indicated that the seal units were performing satisfactorily. Scram times during both cold and hot testing were excellent and actually better than expected.

Abstract: This technical report summarizes the data obtained in a recent literature survey conducted to determine the effects of neutron irradiation on the impact and other mechanical properties of both ferritic steels and austenitic stainless steels. The survey was primarily aimed at obtaining sufficient data on the behavior of pressure vessel steels at high integrated neutron flux levels in order that a reference material of construction could be selected for the SM-2 (APPR-1B) reactor vessel. Materials studied in this literature survey included carbon and low alloy steels such as: ASTM A-212B, ASTM A-201, ASTM A-301B (CR-Mo), ASTM A-106 (coarse and fine grained), ASTM A-285, ASTM A-302B (Mn-Mo), ASTM A-353, ASTM A-203 Grade D, E-7016 carbon steel weld metal, USS Carilloy T-1, HY-65 and HY-80. In addition, Types 304 and 347 stainless steels were also investigated as representative austenitic materials which might be used in pressure vessel construction. A careful evaluation was made of the irradiation induced changes in the mechanical properties of the above materials. The ferritic steels were evaluated primarily on the basis of increases in transition temperature due to irradiation and decreases in the amount of maximum energy absorbed prior to ductile failure. Factors such as industrial experience, …

Introduction: Objectives and Method of Approach. High plant efficiencies can be realized without excessively high core temperatures and high coolant pressures by the use of liquid metal coolant. In an attempt to prove the feasibility of liquid sodium as a reactor coolant ALCO Products, Inc., under sponsorship of the Atomic Energy Commission, is undertaking a design study of three vital system components: the intermediate exchanger, the boiler, and the superheater. Since, in the past programs, the nuclear reactor had been the major focus of attention, the development of the sodium cooled reactor and sodium pumps for this application are thought to need the less development than the heat exchanger equipment. Consequently, parallel design studies of the reactor, pumps, and other system components have not yet been initiated.

Preface. This technical report is an updated and revised version of the original SM-1 (APPR-1) Hazards Summary Report. The original report was issued July 1955, almost two years before construction of the SM-1 plant was completed. During that time interval there were numerous design changes. Consequently, the original report does not accurately describe the plant as built. This revision is written after the SM-1 has been operated 3 years. It describes the as-build plant and includes plant modifications and experience obtained during the first 3 years of SM-1 operation.

Abstract. The design, selection, and calculation of the Army Package Power Reactor shielding are described. The APPR-1, a prototype of a package reactor for remote locations, has a primary shield of iron and water. this shield has been adopted to permit fast erection and to provide low transported weight. economically, including transportation cost, the iron water shield is better than a lead water shield and is competitive with a concrete shield for a remote site. Because of the location at Fort Belvoir,Va., the shielding requirements for the APR-1 are considerably more stringent than those for a reactor at a remote base. Since the secondary shielding which surrounds the entire primary system must provide protection for personnel at any location outside the vapor container, concrete is provided for this need.

Abstract: The reactor analysis of the critical experiment and the APPR-1 resulted in a loading of the APPR-1 of 31.096 gm of B-10 with 22.5 kg U-335. This loading will result in adequate reactivity for a core life of 13 MWYR based on uniform burnup of U-335 and B-10. Calculations indicate that five of the seven control rods provided are more than adequate to shut the reactor down at any time. The temperature coefficient of reactivity should be at least -2 x 10-4 [delta] K/0F.

Abstract: The reactor analysis of the critical experiment and the APPR-1 resulted in a loading of the APPR-1 of 31.096 gm of B-10 with 22.5 kg U-335. This loading will result in adequate reactivity for a core life of 13 MWYR based on uniform burnup of U-335 and B-10. Calculations indicate that five of the seven control rods provided are more than adequate to shut the reactor down at any time. The temperature coefficient of reactivity should be at least -2 x 10-4 [delta] K/0F.

Abstract: A study has been made of the radiochemical composition and the specific activity of insoluble corrosion products (crud) removed from the primary system of the APPR-1. This report presents the results of analysis of twelve crud samples collected during the interval from September 3, 1957 to December 1, 1957. The samples were radiochemically analyzed for long-lived gamma emitting nuclides only. Data are presented on the measured values of the specific activity of crud, the ratios of the nuclide specific activities, and the concentration of crud (crud level) in the circulating primary water. Also included in data, based on the analysis of a single sample, comparing the specific activity of the deposited and circulating corrosion products.

Abstract: The removal of both SM-1 Core I high burnup elements from the SM-1 Core II and the insertion of two SM-1 Core I spare elements i their places are discussed. Nuclear and thermal characteristics of Core II with the change are presented and conclusion related to the change in hazard potential are made. If the core change indicated by this report is made, local peaking factors will be decreased and burnout ratios will be increased. This, of course, in itself leads to a more conservative estimate of core safety. There is no conceivable reason why this perturbation may not be safely made in the SM-1 Core II.

Abstract: Development of welding processes for stainless steel fuel elements, previously initiated by Alco Products, was continued in Task 5. Three objectives were accomplished; (1) development of a suitable reference welding process, (2) evaluation by out-of-pile tests of the structural integrity of reference welded fuel elements, and (3) preparation of specifications and fabrication procedures for the reference welding process.

Abstract: This technical report contains a comprehensive analysis of the nuclear characteristics of the SM-1 Core I. Comparison of analytical and experimental results for neutron ages and core reactivities of a variety of cases investigated shows that the MUFT III with P-1 slowing down approximation gives the best results. At startup the core reactivity and rod bank worth under various operating conditions are investigated and compared to experiment. Core lifetime was calculated to be 16.8 MWYR compared to 16.4 MWYR experimental. The temperature coefficient has been calculated and compared to experiment as function of burnup. In Appendix A, flux distribution, temperature coefficient, effective delayed neutron fraction and core life are analyzed by Dr. R. L. Murray by one and two group modified theory series expansion calculations.

Abstract: The results of activity buildup studies in the SM-1 performed during Core I lifetime (June 3, 1957 to April 28, 1960) are reported. Data are presented on the extent, nature, and mechanism of the buildup of long-lived gamma emitting nuclides in the reactor primary system. Radiation levels after reactor shutdown are presented, as well as mathematical equations used to account for the observed activity levels. The data have shown that Co60 is the major contributor to radiation levels in the SM-1. Co60 activity arises from the cobalt in Haynes 25 alloy flux suppressors, and the cobalt impurity in stainless steel. After 35 months operation at an average power level of 55%, deposited Co60 activity accounted for approximately 83% of the total radiation level (mr/hr) contributed by the long-lived gamma emitting nuclides. The contribution of the primary coolant activity to the total radiation level is insignificant when compared to the contribution of the activity deposited on the walls of the system. The radiation level on the super-heater side of the steam generator was about 1400 mr/hr after 35 months of reactor operation. The percentages of Co60 activity in the coolant and in the deposits were not the same. This indicates …

Abstract: A zero power experiment on the SM-1 Core II included an element by element reactivity check of fuel elements and control rod absorber sections, and an estimate of burnable nuclear poison loading in stationary fuel elements. An approach to criticality was made by the inverse multiplication method, and critical rod bank position obtained as a function fuel loading up to full core loading. Minimum and maximum core reactivity measurements were obtained by selective loading of stationary fuel elements, and total excess K of the core was established. Power distribution measurements were taken in the regions of the core-reflector interface and the fuel-absorber interface in the control rod assemblies. The effectiveness of europium flux suppressors in the top of control rod fuel elements was determined, and power peaking was measured in stationary elements adjacent to control rod assembly water gaps. Survey measurements established the work of spiking clean, cold SM-1 cores with SM-2 elements and the work of water holes in the SM-1 Core. The reduced scope zero power experiment performed on SM-1A core I included an element by element uniformity check of stationary fuel elements, a core assembly test, comparison of Eu2O3 and B4C absorber sections, and development of …

Abstract: An element by element reactivity check for SM-1 Core II fuel elements and control rod absorber sections was performed and the burnable nuclear poison loading in the SM-1 Core II stationary fuel elements was established. An approach to criticality of the SM-1 Core II was performed by the inverse multiplication method and the critical rod bank position obtained as a function of fuel loading up to the full SM-1 Core II loading. Maximum and minimum core reactivity measurements were obtained by selective loading of stationary fuel elements and the total "excess K" for the core established. Power distribution measurements in the region of the core-reflector interface and the fuel-absorber interface in the control rod assemblies were performed. The effectiveness of europium flux suppressors in the top of control rod fuel elements and the power peaking in stationary elements adjacent to water gaps in control rod assemblies were measured. Survey measurements established the worth of spiking cold clean SM-1 cores with SM-2 elements, and of water holes in the SM-1 core which might be utilized as flux traps for materials irradiation.