Laboratory studies have shown that the double salt, CaF2-PuF4, can be precipitated by rapid addition of hydro-fluoric acid to solutions containing 25 to 75 g Pu/1, caleium equimolar to plutonium, and 1 to 10 M HNO3. The precipitate, which is subsequently washed with water and dried to 300 degrees C in dehumidified, deoxygenated argon, can be reduced thermally by calcium to give high yields of plutonium metal.

Technical report describing that the pressure drop along an annular channel with dimensions D(1) = 0.375 inch; D(2) = 0.875 inch, L = 70 inches. Flow was vertical and upward, and only the internal surface was heated. Subcooled conditions existed at the inlet, with two-phase conditions at the exit. Groups of three radial spacer pins on 18-inch centers along the channel, held the inner surface concentric with the outer surface. The single phase loss coefficient for each spacer group is K(8) = 0.21. The single phase friction factor for the annual channel is given by f = 0.16 N(R)(-0.16). The two phase pressure drop increases as the quality increases for G [over] 10(6) = 0.5 ;b/hr ft(2). The effect of heat flux on the pressure drop is very is very slight over the range of fluxes tested (0.55 less than or equal to Q over 10(6).\ less than or equal to 0.8). The two-phase pressure drop gradient in the same annulus, with no heat addition is qualitatively the same as for a 1/4-inch by 1-3/4 inches rectangular channel but is quantitatively greater than for the rectangular channel.

In regard to the production of ozone and various nitrogen oxides in air by action of x-rays or gamma rays, thre seems to be no direct experimental data which can be used. There is some data on the action of alpha particles on air and some on the action of cathode rays.

The objective of the Accurate Nuclear Fuel Burnup Analyses program is to develop more accurate methods for burnup analysis for general use than the current method of analysis of Ca-137 or Sr-90. The program will require from three to five years of effort.

Thirty gram patches of plutonium dioxide can be readily chlorinated by reaction with phosgene or carbon tetrachloride at temperatures of 350 and 450 C respectively. Plutonium trichloride prepared by either method can be reduced to the metal in a hermetically sealed bomb by reaction with calcium. On a twenty gram scale yields of approximately 97 per cent are obtained when a calcium-iodine booster is employed. It has been demonstrated that a method for reduction of plutonium trichloride to the metal without the use of a booster can be development.