Report presenting seven distinct operations in the preparation of 2,2,4,4-tetramethylpentane, including the preparation of di-isobutylene hydrochloride, preparation of dimethylzinc, reaction of dimethylzinc in dry benzene with di-isobutylene hydrochloride, preliminary distillation of the reaction products, treatment of the first distillate with sodium and alcohol, final distillation after appropriate washing of the products, and recovery of the iodine in the zinc residues of II as methyl iodide.