The acceleration of charged particles in the Berkeley 60-inch and 184-inch cyclotrons has made it possible to study a large variety of nuclear reactions. The characterization of the products from these reactions is done by chemical separations of elemental fractions and subsequent identification of the nuclides formed.

The state of polonium in aqueous solutions was investigated by means of ion exchange equilibrium studies. The distribution of the polonium between the solid and liquid phases was determined for solutions of various compositions using both a cation and an anion exchanges. These studies show that in the absence of a complexing agent polonium is hydrolyzed to such a degree that it forms monovalent cations and anions whose charge was not investigated in this study.

The fission and spallation reactions caused in uranium by bombardment with high energy protons (340 to 350 Mev) were investigated. The reaction products were separated from the target by chemical processes and identified by their radioactive properties. The relative yields of the observed fission products were measured, and the results plotted as a function of mass number. Several of the spallation products were identified and their yields estimated.