The development of ionic methods for the determination of corrosion products in the highly radioactive Homogeneous Reactor (HR) fuels has been of major interest in the work of the Ionic Analyses Laboratory. Methods for the spectrophotometric determination of aluminum and for the polarographic determination of iron in HR fuels have been developed. The polarographic determination of molybdenum in uranyl sulfate solutions was studied. A polarographic method for the determination of zinc was developed. A fluorometric method for the determination of microgram amounts of fluoride was studied. Three organic reagents were investigated as precipitants for microgram quantities of zirconium in HR fuel. The automatic photometric titration technique was applied to the determination of thorium and of sulfate. A method was developed for the ionexchange separation and potentiometric titration of cobalt. The ultraviolet absorption spectra of technetium and rhenium were studied.