A research program is being conducted to obtain experimental data in the irradiation of plutonium-enriched fuel to confirm a theoretical model for predicting isotopic composition and reactivity changes in plutonium-enriched, light-water-moderated reactors. Quarterly progress: Work has begun in the Radioactive Materials Laboratory to sample the project fuel from the pins irradiated to 1800 and 5000 MWT/T. Some delay has been experienced due to preemption of the hot cells by priority work. Examination of the autoradiographs of the un-irradiated project fuel showed that in a volume of fuel approximately equivalent to a pellet there were 13 hot spots larger than 15 mils. Evaluation of these spots with the fuel analyzer showed that they contained about 14 mg of PuO2 or about 9% of the total present. The EPITHERMOS code is being modified to automatically normalize the epithermal scattering to the correct value for all moderators. Calibration of the flux wires has been made and the reduction of the data from the VBWR irradiation is nearly complete. A similar resonance activation was made in the water reflector of the Stanford Pool Reactor to obtain the relative activity in a well-defined pure water spectrum. Reduction of these data is also in progress.

Work performed during the quarter is summarized by direct measurement of fission gas pressure, loop operations, performance of UO2 fuel.

Work performed during the quarter is summarized by: direct measurement of fission gas pressure, loop operations, performance of UO2 fuel, UO2 grain growth and melting studies.

This is a report of work completed during the period January 1, 1962, to March 31, 1962. Work was done on fuel irradiation, activation studies and UO2 scattering experiment