The study of the interaction of the electromagnetic field with nuclei has proved very fruitful for the elucidation of many details of nuclear structure. The γ-ray transitions observed in either absorption or emission can be divided into three classes, depending on whether the matrix elements of the transition are (1) much larger, (2) approximately equal or (3) much smaller than those expected for single proton transitions which are usually taken as a norm. In class (1) we find (a) the broad transitions leading to the "giant resonances" in the nuclear photo-electric effect, and (b) the "fast" transitions between low lying states, especially for even-even nuclei far removed from magic numbers. The large matrix elements and the regular dependence of their magnitude on the atomic weight speak for cooperative phenomena in which many nucleons or the nuclei as a whole are involved. In class (2) we find the much studied M4 transitions which give strong support for the single particle model; they have rather uniform matrix elements. Some finer points remain to be understood, especially why some odd nuclei do not show the expected ratio for |M|^2 of ~ 2:1. The transitions belonging to class (3) require further selection rules and …

In this report we present solutions of the design problem in which a system of quadruple lenses is required to carry a particle beam from given focal lines in the x and y planes to other given focal lines. Particular attention will be given to the case of the anastigmatic lens system which takes a beam from one focal point to another focal point. Since the general problem is almost impossibly complicated a simplification is introduced by breaking the lens system into two parts. The first part of the lens system is required to bring the initial beam to the state where it is parallel to the z axis in both planes. The second part carries the initially parallel beam to the required final condition. Each part will involve two quadrupoles so that the complete system will consist of four quadruples; usually, however, the field gradients in the second and third quadrupoles can be made identical so that those quadrupoles can be combined into one and the system becomes a three quadrupole system. The configuration of the lens element will be as shown in the figures below. These figures indicate also the general character of the beam path in the …

The so-called Fluoride Volatility Processes refer to several proposed non-aqueous methods of processing irradiated fuel elements. In each of these methods, the uranium is fluorinated to UF6 and then decontaminated by distillation. One of those methods, involving the direct fluorination of the uranium by bromine trifluoride (BTF), has been under investigation at BNL since 1950. In 1952, it was demonstrated at BNL that uranium, as UF6, could be satisfactorily decontaminated by distillation in small-scale pilot plant equipment; end in 1953, BNL undertook the job of determining the technical feasibility of a continuous dissolver on a pilot-plant scale. The reason for the project was that the economic superiority of the process seemed to depend upon its amenability to continuous operation.

We consider here the accuracy of relaxation lengths measured during the water-uranium lattice experiments. Since such an analysis for all measurements would take a great deal of time, we have applied it to just one lattice. This one (2:1 water-to-metal ratio) was chosen completely at random.

In the memorandum entitled "Stored Energy in BNL Reactor Graphite", dated February 25, 1953, there is described an experiment conducted by Gurinsky's group to determine the energy per gram of irradiated graphite released in a 200°C anneal. Similar experiments were subsequently conducted by W. Kosiba, differing from the original in two particulars: a) Instead of two graphite samples, one normal, and one irradiated, Kosiba used only an irradiated sample which he heated first to release the stored energy, and then again after the energy was released. In this way, he obtained time against temperature curves for both normal and irradiated graphite from the same sample. (These curves are graphed for each run in Figs. 1 thru 5.) b) The vycor tubing used in the original experiment was not used by Kosiba. Five runs of this experiment were selected, Runs 4P, 13, 36, and 40 at furnace temperatures of 200°C, and Run 45 at a furnace temperature of 400°C.

Report issued by the Brookhaven National Laboratory discussing data collected from two BNL meteorological towers. As stated in the introduction, "results are presented in graphic form rather than tabular form" (p. 1). This report includes tables, maps, illustrations, and photographs.

The method of spherical harmonic tensors developed Mark for solving the Boltzmann transport equation in isotropic media is herein extended to anisotropic media for cylindrical geometry. A formal solution is given for the case of two concentric cylindrical media, A and B, but no numerical work has yet been done. The following treatment differs from a similar one by the H. K. Ferguson Co. in that the external medium B is assumed to be both a neutron absorber and finite in extent rather than a non-absorber and infinite in extent.

Preliminary data are enclosed in Tables I, II, II, IV, V, and VI. Tables I to V are data for round nickel tubes in a vertical and inclined (45°) position. Table VI contains some preliminary data for nickel rectangular channels (0.060" and 0.050" spacings) in a vertical position.

The following report concerns the application of a relaxation mesh method for the determination of the average flux within the moderator of a light water moderated, 1.027 per cent U-235, hexagonal lattice with a volume ratio (V_H2O + V_Al)/V_Uranium of 4:1. It was hoped that the calculation would enable one to determine any differences in flux which might result from the fact that the unit cell is a hexagon instead of a cylinder. Because we were primarily interested in the effect due to geometry we applied the same theory, diffusion theory, to the hexagon by means of the mesh method and to the equivalent cylinder.

In recent months, experiments investigating the total, non-elastic, transport, etc., cross-sections of U-238 have been performed. It is the purpose of this memo to examine these data and to obtain from them information which will be of use in refinements pile calculations. In cases, e.g. transport cross-sections, where experimental data do not suffice, the theory developed pertaining to the continuum model of the nucleus has been depended upon. One of the fundamental requirements of this model is that the spacings of the energy levels in the compound nucleus are small compared to their widths and that consequently many levels are excited by the incoming particles. As a result there are many more modes of decay and the continuum model is an average over these levels.

The absorption bands induced in α-Al2O3 by gamma and reactor irradiation have been studied. The slight coloration due to γ-rays saturates. Bands specific to reactor irradiation have been found and their growth studied.

The proton beam in the Cosmotron is accelerated to an energy of 2.3 billion electron volts by a radio frequency voltage which is impressed across an insulated gap in the ferrite loaded accelerating cavity of the vacuum chamber. To maintain a constant orbit radius as the beam is accelerated, the frequency of the accelerating voltage must increase from the initial value of 370 kc/sec to 4200 kc/sec during the one second magnet pulse. Over the entire 11:1 frequency range, a minimum gap voltage of 2000 volts rms must be maintained. At every instant throughout the magnet pulse, the frequency of this voltage must be a predetermined function of the magnet field to a high degree of accuracy. Frequency errors greater than about .2 percent result in loss of beam due to excessive radius changes. Smaller errors than this however, can excite fatal phase oscillations in the beam if they occur rapidly. As little as .005 percent frequency modulation can result in total beam loss if it occurs at a rate of several kc/sec, where the beam is most sensitive to such disturbances.

This report is the culmination of a year of progress and planning in the high-energy particle field. During this year the Brookhaven Cosmotron has been successfully completed and brought into operation for research at 2.3 Bev. Preliminary experimental results with the copious output of π-mesons are in process of publication. Multiple production of mesons has been observed, a few V-particles detected, and the interactions of π-mesons in hydrogen have been studied. Yet it already appears that higher energies will be needed to produce and study the several new heavy particles detected in cosmic ray observations.

A new colorimetric method for the determination of cholesterol has been investigated. It makes use of the relatively stable green color given by a purified digitonin precipitate with the anthrone reagent of Dreywood. Equal precision can be obtained with the new method using 1/10 or less of the quantity of material required for present colorimetric methods.

Recently, there has been some evidence to point to possible ordering in the α-brasses. Masumoto et al. have concluded from their specific heat measurements that there is a possibility of ordering in the α-brasses. In particular they observed an anomaly in the specific heat curves for the α-brasses for the temperature range from 200 to 260°C and explained these results upon the basis of a change in local or short range order in α-brasses at these temperatures. In connection with the study of radiation damage effects in α-brass ordering has been suspected. Rosenblatt has annealed 70-30 α-brass previously annealed at 350°C and cooled to room temperature at 190°C for six weeks. He observed a decrease of .90 ± .03% in the electrical resistivity of α-brass measured at -196°C after the anneal at 190°C.

Selective incorporation of radioactivity from proteins of labeled chorio-allantoic grafts of adult chicken tissues into proteins of homologous tissues of host chick embryos.

A study of the effects of gamma radiation with respect to the formation of nitro-hydrocarbons on the Purex and Redox systems shows that no appreciable formation of nitro-paraffins occurs.

The rapid development of the field of atomic energy during the past few years now permits the exploration of applications to medicine involving new concepts in the treatment of cancer. One such has been the study of neutron capture therapy which is being developed at the Brookhaven National Laboratory.

The polymerization of vinyl monomers can be initiated by heat, ultraviolet radiation, and various catalysts. More recently, ionizing radiation has been shown to effectively initiate vinyl polymerization. However, polymerization in the solid state by ionizing radiation is not reported in the literature, although several papers have been published that describe briefly the thermal polymerization of divinyldiphenyl, Leuch's anhydride and in greater detail the peroxide catalyzed polymerization of acetaldehyde. The purpose of this note is to describe some experiments which demonstrate that crystalline acrylamide undergoes polymerization upon irradiation with γ-rays from an intense Co-60 source. Below its melting point the monomer shows little or no tendency to polymerize thermally.

As a result of unreported information, it was suspected by some people that a change in dimension was experienced by 2S Aluminum due to a sudden change in neutron flux impinging on it. This was thought to be of the order of 500 microinches per inch in magnitude. Such an effect, if present, could help explain some of the creep phenomena reported lately (i.e. change in creep rate due to cyclotron bombardment.)

Summary of miscellaneous updates related to the project. This includes information on the following. Simplified equations for modeling reactor conditions. Solubility tests involving thorium, bismuth, and protactinium. various other measurements and tests involving thorium, uranium, protactinium, bismuth, aluminum, and various other salts.

In a third run with the fluorine torch, the settling chamber wells were kept hotter than before (≥ 625°C); the flame was cooled by diluting the fluorine with helium. In the analysis of the products, 99% of the thorium fluoride fed in was accounted for, but only 64% of the protactinium activity. Part of this was carried in the exhaust gases past the cold trap and into the soda line disposal column, where it was detected by survey meters. The stripping of protactinium from the solid was somewhat more efficient than before; 77% of the feed which was recovered from the settling chamber had lost 72% of its original specific activity. About 15% of the input activity was trapped on the cold fingers with very little thorium fluoride.

Summary of miscellaneous updates related to the project. This includes information on the following: the declassification of a relevant paper, solubility measurements, static corrosion tests, various other tests involving bismuth, magnesium, uranium, protactinium, and thorium.

This memorandum clarifies the present status of ξ measurements in the uranium-water lattices.