"The effect of correcting quadrupole lenses on the betatron oscillation characteristics of an AG synchrotron was studied, and general formulas are given for the fractional changes of the amplitude and phase functions. Calculations performed for different setups of different numbers of lenses for the CEA synchrotron structure point out that one may correct for sizable errors in the n- value by means of 8 pairs of quadrupole lenses in two consecutive straight sections with the focusing lens between defocusing sectors and vice versa. An increase of BETA /sub max/ of about 5% is obtained for DELTA n/n approximately 0.04. It was found that the necessary corrections can probably be obtained satisfactorily with lenses of 6 in. length. "

"A summary is presented of a preliminary study of the application of pole- face windings to the Cambridge Electron Accelerator. Estimates are made of the currents required, the forces on the wibdings and the voltages induced by the magnetic flux. The possibility of automatic control of the pole-face currents in explored, and feasible control systems are suggested."

Since the inauguration of the Off-Site Animal Investigation project n 1957, there has been one annual report rendered as of 30 June 1958. this is the second annual report dated as of 30 June 1959. The objectives of the project have been unchanged during the past year. These are (1) to enhance the Nevada Test Site/off-site rancher relationship through an active investigation project in their interests, and (2) to provide further information as to the status of the off-site animals in their environment, with special emphasis on their radioactive isotope uptake from fall-out. isotope uptake of the animals is being emphasized as well as the gross and microscopic histopathological examinations. Two year's existence in an area of radio-contamination where a full fission spectrum of isotopes can be found, where radiation background reading range from 1/2 mr per hour to 1 = per hour, has produced no noticeable effect on the animals.

To summarize one finds that for diffusion in a temperature gradient by a vacancy mechanism one must have E(M) < E(F). No such restrictions occur for interstitial diffusion. The spatial vacancy distribution is very nearly the equilibrium distribution if dislocations are present. If no dislocations are present then one could obtain E(M) by measurement of the spatial distribution.

A simple non-destructive chemical method for the identification of cadmium plating is presented. The test requires no special techniques or equipment and may be conducted in less than fifteen seconds.

Fused uranium dioxide was separated into fractions of varying particle size by air separation. Specimens of the nominal size of 1/8 by 1/4 by 1½ in. were formed by hydrostatic pressing, firing, and lapping. Specimens prepared from the 0 to 5 μ fraction were the strongest and most dense. The room-temperature density was about 92% of theoretical and the room-temperature flexural strength was about 12,000 1b. per sq. in. When tested at 1000°C., the strength was about 18,000 1b. per sq. in. The flexural strength of specimens decreased and their density decreased as the starting particle size was increased. The crystallization of the urania fragments which had occurred during the firing treatment was observed.

This technical report represents a brief survey of work by this project on the effects of ultraviolet radiation (UV) on certain of the photochemical and metabolic properties of rhubarb chard and sugar beet (Beta vulgaris). These plants were selected for this work because for some years they have been used as sources of chloroplasts for Hill reaction studies in this laboratory. Some of this work has appeared as a brief paper.

The primary purpose of this contract is to develop and exploit techniques for the precision measurement of nuclear energy levels by the spectroscopic study of gamma-rays emitted during the decay of radioisotopes, (1) by the use of a high resolving power curved crystal focusing spectrometer to study wavelengths and intensities of gamma-rays themselves, (2) by means of a precision beta-ray spectrometer to study the conversion lines from gamma-rays both by internal conversion and with external converters.

Most of the publications in the open literature available to us agree that sodium does not readily react with graphite, though potassium, rubidium, and cesium readily enter between the planes of the graphite lattice. In view of the conflicting evidence available, it seems inadvisable without very extensive further study to consider the use of graphite in direct contact with liquid sodium, except under very mild conditions of temperature and irradiation, and then only with very pure sodium and completely graphitized graphite.

Part A. The major effort during the past year has been the construction of a suitable vacuum furnace for studying the effects of temperature and pressure on the wettability of metals by glass. A systems was completed that was capable of subjecting test combinations up to temperatures of 1400 degree C at a working pressure of 1 x 10(-5) mm. of Hg. Part B. A compound, identified by X-ray analysis as sodium meta tantalate (na2Ta2O6), was found at the interface between a sodium silicate glass and tantalum metal which had been heated in vacuum to 1000 degree C. thermodynamic calculations, followed by further experimental evidence, were used to determine the chemical reaction between tantalum and sodium silicate which resulted in the formation of Na2Ta3O6. the compound was synthesized by other methods, and its structure investigated.

1) The technical details of controlled experiments with iontophoresis of thorium X solutions are described. 2) Experiments carried out on living human skin in situ demonstrate that Iontophoresis of weak solutions of thorium X will increase its biologic effects as judged by erythema and pigmentation, and cause greater penetration as shown by autoradiography. 3) The possible relationship between increased penetration of thorium X and increased clinical biologic effects is discussed. 4) Some possible clinical applications of the Iontophoresis of thorium X to enhance its therapeutic effectiveness are mentioned.

The object of the work performed under this contract was to investigate the possibility of gas plating copper base metal with (a) pure chromium metal from chromium hexacarbonyl vapor; (b) chromium-nickel plating from a mixture of chromium hexacarbonyl and nickel tetracarbonyl. The object of the work performed during the final month was to confirm the fact that the gas plating of chromium metal and chromium-nickel laminates free from nitrides, oxides and carbides was practical.

During this period a prototype gamma ray detection system was assembled and data was obtained on samples of beryllium salts on filter paper under a variety of conditions. Ordinarily either a scaler-register combination or the CRM-recorder combination would be sufficient for obtaining data. Both units have been used here in order to utilize the particular advantages of each system. The scaler-register unit was employed for obtaining precise data over short intervals while the CRM-recorder was used to maintain a check on stability over longer intervals of time.

The non-project literature concerning the chemistry of vanadium has been summarized through November, 1952. The report is presented in terms of izo- and heteropoly vanadates and cationic forms of pentavalent vanadium, complexes of di-, tri-, and pentavalent vanadium, and oxidation potentials of various vanadium systems. A bibliography of 93 references is included.

An ion exchange testing program was completed on Gunnar acid leach liquors and pulps. A standard column system and a resin-in-pulp system, both using anion exchange resins, were investigated. The Gunnar leach liquors are readily amenable to the recovery of uranium by ion exchange.

Uranium ore from Radium Hill, South Australia was leached with hot sulfuric acid solutions and the uranium recovered from solution by uranous phosphate precipitation or by use of anion exchange resins.

Leaching tests indicated high recoveries could be obtained by use of large quantities of sulfuric acid and boiling for relatively long periods. Filtration rates were satisfactory but large settling areas would be required to wash and thicken before filtering.

"The quantum theory problem of constructing explicitly a local Lorentz invariant model field theory which has an asymptotic particle interpretation and gives rise to an S matrix different from unity is discussed. It is proved that if a local covariant field H(x) has a complete current, the S matrix associated with this field is identically equal to unity. Results show that in order to get an interaction, the current is not allowed to have a terminating expansion in terms of a free field. The absence of a finite connection between a free field and an interacting field tended to confirm the belief that in local quantum field theories with particle interpretation the requirement of the existence of scattering forces in the physical states are such that it is not pos sible to identify them with a linear space spanned by ""free'' particle states."

"Results of tests indicate that the nucerite-bearium seal system is compatible. This combination was operated as long as 9 hours without serious damage. In other work, the test rig was modified to eliminate pressure fluctuations and extraneous dirt, and Type IIA seal parts were designed."

"A series of high urania-content glasses were fiberized and examined for high-temperature strength properties. One glass, RX360 containing 60% U/sub 3/O/ sub 8/ by weight, had better high-temperature tensile properties than any glass previously reported. It was observed that many of the glasses studied separated into immiscible phases and that the fiberizable glass phase had lower U/sub 3/O/ sub 8/ content than the base compositions. A physical analysis of crystal structures of the devitrification products from the nuclear fuel glasses indicated that most of the crystals consisted of uranium oxide in a reduced state. By adding O/sub 2/ to molten glass, it was possible to eliminate most of this devitrification. By elimination of crystals, the fiberizing of the glass was more uniform and the glasses produced had more consistent physical properties."

"Mixed Fission Products (MFP) for use as a heat source for thermoelectric generators will become increasingly available in the coming years. The Atomic Energy Commission sponsored program on solidification of nuclear wastes is now entering the hot-bench scale test phase. During this phase approximately 5000 thermal watts of two year old MFP could be produced monthly. Two different types of hot calcination pilot plants are planned for installation at the Hanford National Laboratories in the 1964 to 1966 time period. Each of these plants should be able to produce 160,000 thermal watts of two year MFP and 16,000 thermal watts of ten year MFP on a monthly basis. A full scale plant for a 15,000 Mw(e) nuclear economy is estimated to produce four to five times as much MFP as either of the pilot plants. Costs will be dependent upon AEC policy in effect at the time the plant is operating."

"The diffusivities of Fe, Co, and Al in otherwise pure Au were determined by a residual activity technique. It was found that the frequency factors and activation energies of the transition elements into Au are normal relative to the values for Au self-diffusion, and suggest that lattice diffusion is operative, in contrast to the corresponding situation for the diffusion of these elements in Al. This difference in behavior is explained in terms of the marked difference in solid solubilities in the two series."

The self-diffusivities of Co60 and Ni63 in cobalt--nickel solid solutions exhibit a greater activation energy below the Curie temperature (T/sub c/) than above. Values of DELTA Q = Q (ferromagnetic) -- Q (paramagnetic) are approximately equal to RT/sub c/. This observation is interpreted to indicate that the increment in activation energy arises from an increase in the formation energy of a vacancy in the ferromagnetic lattice, with the additional binding energy arising from the interaction of a spin with the Weiss field."

"Properly designed and fitted respirators have been effective devices for reducing the inhalation of toxic aerosols. The degree of protection afforded by these devices has not been quantitatively measured under actual work conditions except by bioassay or other elaborate techniques. This report describes a new quantitative technique for evaluating over-all respiratory performance under conditions comparable to exposure to highly toxic radioactive materials such as plutonium and non-radioactive materials such as beryllium."