Attached are the impurity data for 20-liter growth runs N. Zaitseva/L. Carman made in the 1996-1997 time frame for which we have both solution and crystal data. The 5 impurities added for the runs are AI(III), Cr(III), Fe(III), Mo(VI), and Sb(V). As an explanation of the tables, I report all impurity concentrations as ppb (ng/g{sub KDP}) with respect to dry KDP (even solution data.) ''MDL'' stands for ''Method Detection Limit.'' Nominal uncertainties are 1 MDL or 10% of the quoted value, whichever is greater. If the measured value is less than the MDL, I report ''ND,'' for ''Not Detected.'' If the value is greater than the MDL, but less than twice the MDL, I report ''D,'' for ''Detected.'' If the value is more than twice the MDL, I report two significant figures. The values come from ICP-ES and ICP-MS measurements. I give the detection limit for the more sensitive technique in the table under the ''MDL'' heading. In case where only one technique was used, I give the MDL for that technique in parentheses after the impurity value in the table. Since these measurements were made, changes in instrumentation have resulted in significant improvements in many of the detection limits. …

The efficient representation of volumetric meshes is a central problem in scientific visualization. The difference in performance between most visualization algorithm for rectilinear grids and for unstructured mesh is mostly due to fundamental difference in efficiency of their representations. In Computer Graphics the gap in performance between 2D rectilinear grids and unstructured mesh has been overcome with the development of representation schemes based on the concept of subdivision surfaces. This gap has not been bridged in the volumetric cases which is fundamental interest for Scientific Visualization. In this paper we introduce a slow-growing volumetric subdivision scheme for meshes of any topology, any intrinsic dimension d and composed of a general type of polyhedral cells (topological balls). The main feature of this approach is the ability to split in different stages cells of different dimensions. This allows to increase the resolution of the mesh slowly using small stencils for the smoothing rules. ''Sharp features'' of dimension lower than d are embedded naturally in the subdivision procedure. Automatic adaptation is provided for variable resolution. In the uniform case the slow subdivision doubles the number of vertices in the mesh at each refinement independent of its dimension d. The bisection of all the …

Recently, new cross section measurements by the GEANIE collaboration have been published for {sup 239}Pu(n, 2n{gamma}) [Ber00] and {sup 235}U(n, 2n{gamma}) [You00] from threshold to 20 MeV. When combined with nuclear reaction calculations [Che00, Cha99, Cha01], these measurements provide the most accurate information available on the shape and magnitude of the {sup 239}Pu(n, 2n) cross section for incident neutron energies, E{sub n} {approx}< 14 MeV. This new data has prompted a re-evaluation of the {sup 239}Pu(n, 2n) {sup 238}Pu reaction cross section considering all available experimental data. The data prior to the measurement of Bernstein et al. [Ber00] is illustrated in Figure 1a. These data sets were considered by previous evaluations [ENDL] of the {sup 239}Pu(n, 2n) cross section. The most precise experiment was an activation measurement done by Lougheed et al. [Lou00] for incident neutron energies, E{sub n}, between 13-15 MeV. In addition, there were two neutron-counting experiments, one by Mather et al. [Mat72] and one by Frehaut et al. [Fre85]. These two measurements cover a wide incident neutron range, with data points from threshold to E{sub n} {approx} 14 MeV. The available data sets are in poor agreement with each other and in some cases do not meet …

We have developed an improved computational theory of condensed matter in the regime where T {le} T{sub Fermi}. Previous methods of calculating the equation of state (EOS) relied on interpolation between low-temperature (solid) and high-temperature (plasma) limits, or employed severe approximations. Recent theoretical and experimental developments have highlighted the need for accurate EOS and opacity data in the intermediate temperature range and offer the opportunity to test theoretical models. We describe our results for EOS and optical properties for temperatures up to 10{sup 6} K, and describe directions for future work.

This report provides year end status of PNNL performance against the FY01 critical outcomes.

This report describes the results obtained from deployment of the Enhanced Site Characterization System (ESCS) at the Hanford Site's 618-4 Burial Ground. The objective of this deployment was to use advanced geostatistical methods to integrate and interpret geophysical and ground truth data, to map the physical types of waste materials present in unexcavated portions of the burial ground. One issue of particularly interest was the number of drums (containing depleted uranium metal shavings or uranium-oxide powder) remaining in the burial ground and still requiring removal.Fuzzy adaptive resonance theory (ART), a neural network classification method, was used to cluster the study area into 3 classes based on their geophysical signatures. Multivariate statistical analyses and discriminant function analysis (DFA) indicated that the drum area as well as a second area (the SW anomaly) had similar geophysical signatures that were different from the rest of the burial ground. Further analysis of the drum area suggested that as many as 770 drums to 850 drums may remain in that area. Similarities between the geophysical signatures of the drum area and the SW anomaly suggested that excavation of the SW anomaly area also proceed with caution.Deployment of the ESCS technology was successful in integrating multiple …

This 2001 Facility Work Plan (FWP) has been prepared as required by Module VII, Section VII.M.1 of the Waste Isolation Pilot Plant (WIPP) Hazardous Waste Facility Permit, NM4890139088-TSDF (the Permit); (NMED, 1999a), and incorporates comments from the New Mexico Environment Department (NMED) received on December 6, 2000 (NMED, 2000a). This February 2001 FWP describes the programmatic facility-wide approach to future investigations at Solid Waste Management Units (SWMUs) and Areas of Concern (AOCs) specified in the Permit. The permittees are evaluating data from previous investigations of the SWMUs and AOCs against the newest guidance proposed by the NMED. Based on these data, the permittees expect that no further sampling will be required and that a request for No Further Action (NFA) at the SWMUs and AOCs will be submitted to the NMED. This FWP addresses the current Permit requirements. It uses the results of previous investigations performed at WIPP and expands the investigations as required by the Permit. As an alternative to the Resource Conservation and Recovery Act (RCRA) Facility Investigation (RFI) specified in Module VII of the Permit, current NMED guidance identifies an Accelerated Corrective Action Approach (ACAA) that may be used for any SWMU or AOC (NMED, 1998). This …

The goal of this research was to develop epidermal growthfactor receptor (EGFR) nuclear medicine breast cancer imaging agents. Ourapproach was to synthesize small molecule inhibitors of the EGFR tyrosinekinase (tk) suitable for labeling with single photon or positron-emittingradioisotopes and evaluate the imaging potential of these new molecules.We have synthesized and fully characterized 22 quinazoline compounds. Allcompounds inhibit EGFR tk phosphorylation activity in the nanomolarrange. All compounds tested exhibited specificity for the EGFR tk versusthe ErbB2 and ErbB4 tyrosine kinases. A radiometric binding assay usingan iodine-125 labeled quinazoline was developed to determine the affinityof the quinazolines for the EGFR tk ATP binding site. The affinitiesranged from 0.4-51 nM. The octanol/water partition coefficients (Log P;lipophilicity) of the new compounds ranged from 2.2-5.5. Six compoundshave been labeled with fluorine-18. Biodistribution in EGFRoverexpressing tumor bearing mice demonstrated tumor uptake buthighlighted delivery and metabolism issues. The 2-fluoro quinazoline wasnot metabolized in an in vitro hepatocyte study. From this work a breadthof agent characteristics was created establishing the foundation forfuture research toward the optimal EGFR imaging agent.

The objective of this calculation is to develop a time dependent in-drift effective thermal conductivity parameter that will approximate heat conduction, thermal radiation, and natural convection heat transfer using a single mode of heat transfer (heat conduction). In order to reduce the physical and numerical complexity of the heat transfer processes that occur (and must be modeled) as a result of the emplacement of heat generating wastes, a single parameter will be developed that approximates all forms of heat transfer from the waste package surface to the drift wall (or from one surface exchanging heat with another). Subsequently, with this single parameter, one heat transfer mechanism (e.g., conduction heat transfer) can be used in the models. The resulting parameter is to be used as input in the drift-scale process-level models applied in total system performance assessments for the site recommendation (TSPA-SR). The format of this parameter will be a time-dependent table for direct input into the thermal-hydrologic (TH) and the thermal-hydrologic-chemical (THC) models.

This Hanford Site environmental report is prepared annually to summarize environmental data and information, to describe environmental management performance, to demonstrate the status of compliance with environmental regulations, and to highlight major environmental programs and efforts.

There are nine separate zones of high sensitivity smoke detection (HSSD) at Dzero. These zones, their coverage, their condition thresholds, and their response to conditions are described in the table in the 'Zones & Responses' section of this document. This is an 'air-sampling' smoke detection system. Each zone is formed of a network of pipes which contain strategically sized and located air sampling holes. Each zone has a fanbox/detector head that continuously draws air into the holes and through the pipes to the detector head where it is evaluated for combustion products. The fanbox/detector heads are located on the Dzero detector platform and in the trusses. Each fanbox/detector head has a remotely located display control card (DCC) for monitoring the level of obscuration of the air sample. This remote equipment is located on the roof of the moving counting house. The DCC for each zone is networked to a single intelligent interface module (11M), also on the roof of the MCH, that collects the information from all nine zones and delivers it to the Dzero control room via an isolated RS-485 link to an operators console. This console is replicated via a 'remote video, keyboard, mouse system' in the DAB …

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This report discusses the Social Security recipients that receive a costof- living adjustment (COLA) in January of each year. An automatic Social Security benefit increase reflects the rise in the cost of living over roughly a 1-year period

This report considers the events of Chandler v. James in 1997. The case was a federal district court ruling in Alabama holding up a statute to violate the establishment of religion of the First amendment. The Governor attempted to appeal the court's position to both the Supreme Court and the circuit court but was denied.

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This report covers the status and legislative issues of the coastal non-point program.

This report analyzes four instruments and provides rough estimates of the relative magnitude of each.

This report describes types of CRS products and a selection of the most frequently used printed and online reference sources available in the reading room and research centers for use by congressional staff.

This report discusses the market-based strategies to reduce greenhouse gases for global climate change.

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The myriad of human activities including strategic and energy development at various DOE installations have resulted in the contamination of soils and waterways that can seriously threaten human and ecosystem health. Development of efficacious and economical remediation technologies is needed to ameliorate these immensely costly problems. Bioremediation (both plant and microbe-based) has promising potential to meet this demand but still requires advances in fundamental knowledge. For bioremediation of heavy metals, the three-way interaction of plant root, microbial community, and soil organic matter (SOM)1 in the rhizosphere is critically important for long-term sustainability but often underconsidered. Particularly urgent is the need to understand processes that lead to metal ion stabilization in soils, which is crucial to all of the goals of bioremediation: removal, stabilization, and transformation. This project will build on the knowledge that we have generated on the role of root exudation and metabolism for metal mobilization and accumulation, to address the following objectives: (1) Identify molecular markers and characterize the chemical nature of recalcitrant SOM pools that are involved in below ground metal ion interactions, which are likely to be markers for sustainable sequestration; (2) Utilize (1) to determine plant and microbial factors that contribute to sustainable metal sequestration …

This report summarizes the accomplishment made during the second year of this cooperative research effort between Washington University, Ohio State University and Air Products and Chemicals. The technical difficulties that were encountered in implementing Computer Automated Radioactive Particle Tracking (CARPT) in high pressure SBCR have been successfully resolved. New strategies for data acquisition and calibration procedure have been implemented. These have been performed as a part of other projects supported by Industrial Consortium and DOE via contract DE-2295PC95051 which are executed in parallel with this grant. CARPT and Computed Tomography (CT) experiments have been performed using air-water-glass beads in 6 inch high pressure stainless steel slurry bubble column reactor at selected conditions. Data processing of this work is in progress. The overall gas holdup and the hydrodynamic parameters are measured by Laser Doppler Anemometry (LDA) in 2 inch slurry bubble column using Norpar 15 that mimic at room temperature the Fischer Tropsch wax at FT reaction conditions of high pressure and temperature. To improve the design and scale-up of bubble column, new correlations have been developed to predict the radial gas holdup and the time averaged axial liquid recirculation velocity profiles in bubble columns.