Incorporation of high-level wastes in SYNROC: results from recent process-engineering studies at Lawrence Livermore National Laboratory (open access)

Incorporation of high-level wastes in SYNROC: results from recent process-engineering studies at Lawrence Livermore National Laboratory

In this paper, highlights from recent engineering research and development, in particular, results from fluidized bed calcination studies of SYNROC slurry are summarized. A schematic diagram of the envisioned SYNROC process (at this stage of development) is also presented. It shows the use of a fluidized bed calciner to prepare SYNROC powder that is then fed to a storage hopper. Bellows-type canisters are filled, evacuated, sealed and preheated. The preheated canisters are loaded into a hot isotactic pressing unit where they are densified, then removed and cooled and finally loaded into a waste storage container. After sealing, this container is decontaminated and transferred to the interim storage facility and then, ultimately, to an underground repository.
Date: April 15, 1982
Creator: Campbell, J. H.; Hoenig, C. L.; Ackerman, F. J.; Peters, P. E. & Grens, J. Z.
System: The UNT Digital Library
Immobilization of high-level defense wastes in SYNROC-D: recent research and development results on process scale-up (open access)

Immobilization of high-level defense wastes in SYNROC-D: recent research and development results on process scale-up

SYNROC is a titanate-based ceramic waste form being developed to immobilize high-level nuclear reactor wastes. SYNROC-D is a unique variation of SYNROC designed to contain high-level defense wastes, particularly those in storage at the Savannah River Plant (SRP). We review recent research and development on SYNROC-D processing options and report on work in progress on various unit operations. The overall immobilization process can be divided into three general parts: (1) slurry preparation (formulation, reactant addition and blending); (2) powder processing (spray drying, calcination/redox control); and (3) mineralization (densification). Powder processing research is directed toward development of a slurry-fed, fluidized-bed calciner based on the ICPP design. Densification research is focused on use of hot isostatic pressing (HIP) or hot uniaxial pressing (HUP). The successful use of both have been demonstrated.
Date: March 15, 1982
Creator: Campbell, J. H.; Rozsa, R. B. & Hoenig, C. L.
System: The UNT Digital Library
Application of Monte Carlo codes to neutron dosimetry (open access)

Application of Monte Carlo codes to neutron dosimetry

In neutron dosimetry, calculations enable one to predict the response of a proposed dosimeter before effort is expended to design and fabricate the neutron instrument or dosimeter. The nature of these calculations requires the use of computer programs that implement mathematical models representing the transport of radiation through attenuating media. Numerical, and in some cases analytical, solutions of these models can be obtained by one of several calculational techniques. All of these techniques are either approximate solutions to the well-known Boltzmann equation or are based on kernels obtained from solutions to the equation. The Boltzmann equation is a precise mathematical description of neutron behavior in terms of position, energy, direction, and time. The solution of the transport equation represents the average value of the particle flux density. Integral forms of the transport equation are generally regarded as the formal basis for the Monte Carlo method, the results of which can in principle be made to approach the exact solution. This paper focuses on the Monte Carlo technique.
Date: June 15, 1982
Creator: Prevo, C.T.
System: The UNT Digital Library
Evaluating Alternative Responses to Safeguards Alarms (open access)

Evaluating Alternative Responses to Safeguards Alarms

This paper describes a quantitative approach to help evaluate and respond to safeguards alarms. These alarms may be generated internally by a facility's safeguards systems or externally by individuals claiming to have stolen special nuclear material (SNM). This approach can be used to identify the most likely cause of an alarm - theft, hoax, or error - and to evaluate alternative responses to alarms. Possible responses include conducting investigations, initiating measures to recover stolen SNM, and replying to external threats. Based on the results of each alarm investigation step, the evaluation revises the likelihoods of possible causes of an alarm, and uses this information to determine the optimal sequence of further responses. The choice of an optimal sequence of responses takes into consideration the costs and benefits of successful thefts or hoaxes. These results provide an analytical basis for setting priorities and developing contingency plans for responding to safeguards alarms.
Date: April 15, 1982
Creator: Al-Ayat, R. A.; Judd, B. R. & McCord, R. K.
System: The UNT Digital Library
Current status of fast-neutron-capture calculations (open access)

Current status of fast-neutron-capture calculations

This work is primarily concerned with the calculation of neutron capture cross sections and capture gamma-ray spectra, in the framework of the Hauser-Feshbach statistical model and for neutrons from the resonance region up to several MeV. An argument is made that, for applied purposes such as constructing evaluated cross-section libraries, nonstatistical capture mechanisms may be completely neglected at low energies and adequately approximated at high energies in a simple way. The use of gamma-ray strength functions to obtain radiation widths is emphasized. Using the reaction /sup 89/Y + n as an example, the problems encountered in trying to construct a case that could be run equivalently on two different nuclear reaction codes are illustrated, and the effects produced by certain parameter variations are discussed.
Date: April 15, 1982
Creator: Gardner, D. G.
System: The UNT Digital Library
High-explosive-driven delay line pulse generator (open access)

High-explosive-driven delay line pulse generator

The inclusion of a delay line circuit into the design of a high-explosive-driven generator shortens the time constant of the output pulse. After a brief review of generator concepts and previously described pulse-shortening methods, a geometry is presented which incorporates delay line circuit techcniques into a coil generator. The circuit constants are adjusted to match the velocity of the generated electromagnetic wave to the detonation velocity of the high explosive. The proposed generator can be modeled by adding a variable inductance term to the telegrapher's equation. A particular solution of this equation is useful for exploring the operational parameters of the generator. The duration of the electromagnetic pulse equals the radial expansion time of the high-explosive-driven armature until it strikes the coil. Because the impedance of the generator is a constant, the current multiplication factor is limited only by nonlinear effects such as voltage breakdown, diffusion, and compression at high energies.
Date: November 15, 1982
Creator: Shearer, J.W.
System: The UNT Digital Library
High-temperature oxidation of ion-implanted tantalum. [At 500 and 1000/sup 0/C] (open access)

High-temperature oxidation of ion-implanted tantalum. [At 500 and 1000/sup 0/C]

The oxidation of ion-implanted Ta in two different high temperature regimes has been studied. Oxidations were carried out at 500/sup 0/C in Ar/O/sub 2/ mixtures, where oxide growth is known to follow a parabolic rate law in initial stages, and at 1000/sup 0/C in pure O/sub 2/, where a linear-rate behavior obtains. Implanted species include Al, Ce, Cr, Li, Si and Zr at fluences of the order of 10/sup 17//cm/sup 2/. Oxidized samples were studied using Rutherford backscattering, nuclear reaction analysis, Auger spectroscopy, secondary-ion mass spectroscopy, x-ray diffraction and optical microscopy. Significant differences among the specimens were noted after the milder 500/sup 0/C treatment, specifically, in the amount of oxide formed, the degree of oxygen dissolution in the metal beneath the oxide, and in the redistribution behavior of the implanted solutes. Under the severe 1000/sup 0/C treatment, indications of different solute distributions and of different optical features were found, whereas overall oxidation rate appeared to be unaffected by the presence of the solute. 7 figures.
Date: September 15, 1982
Creator: Kaufmann, E. N.; Musket, R. G.; Truhan, J. J.; Grabowski, K. S.; Singer, I. L. & Gossett, C. R.
System: The UNT Digital Library
Hafnium-implanted nickel studied with TDPAC and RBS/channeling before and after laser-surface melting and thermal annealing (open access)

Hafnium-implanted nickel studied with TDPAC and RBS/channeling before and after laser-surface melting and thermal annealing

The Hf implanted Ni system has been studied by the time-differential perturbed angular correlation (TDPAC) technique and by Rutherford backscattering (RBS)/channeling. Low fluence implants were thermally annealed in vacuum at increasing temperature in order to study the evolution of substitutional and defect-associated solutes using TDPAC. Both detrapping and precipitation (or segregation) effects have been observed. Higher fluence implants were studied by both TDPAC and RBS/channeling in as-implanted as well as laser-surface-melted regimes. 10 figures.
Date: September 15, 1982
Creator: Kaufmann, E. N.; Buene, L.; McDonald, M. L.; Kotthaus, J.; Freitag, K.; Vianden, R. et al.
System: The UNT Digital Library
Introduction to the magnet and vacuum systems of an electron storage ring (open access)

Introduction to the magnet and vacuum systems of an electron storage ring

An accelerator or storage ring complex is a concerted interplay of various functional systems. For the convenience of discussion we can divide it into the following systems: injector, magnet, RF, vacuum, instrumentation and control. In addition, the conventional construction of the building and radiation safety consideration are also needed and finally the beam lines, detector, data acquisition and analysis set-ups for research programs. Dr. L. Teng has given a comprehensive review of the whole complex and the operation of such a facility. I concentrate on the description of magnet and vacuum systems. Only the general function of each system and the basic design concepts will be introduced, no detailed engineering practice will be given which will be best done after a machine design is produced. For further understanding and references a table of bibliography is provided at the end of the paper.
Date: August 15, 1982
Creator: Weng, W. T.
System: The UNT Digital Library
Mechanical-engineering aspects of mirror-fusion technology (open access)

Mechanical-engineering aspects of mirror-fusion technology

The mirror approach to magnetic fusion has evolved from the original simple mirror cell to today's mainline effort: the tandem-mirror machine with thermal barriers. Physics and engineering research is being conducted throughout the world, with major efforts in Japan, the USSR, and the US. At least one facility under construction (MFTF-B) will approach equivalent energy breakeven in physics performance. Significant mechanical engineering development is needed, however, before a demonstration reactor can be constructed. The principal areas crucial to mirror reactor development include large high-field superconducting magnets, high-speed continuous vacuum-pumping systems, long-pulse high-power neutral-beam and rf-plasma heating systems, and efficient high-voltage high-power direct converters. Other areas common to all fusion systems include tritium handling technology, first-wall materials development, and fusion blanket design.
Date: July 15, 1982
Creator: Fisher, D. K. & Doggett, J. N.
System: The UNT Digital Library