Dominant Role of Hole Transport Pathway in Achieving Record High Photoconductivity in Two-Dimensional Metal-Organic Frameworks (open access)

Dominant Role of Hole Transport Pathway in Achieving Record High Photoconductivity in Two-Dimensional Metal-Organic Frameworks

Article describes how metal-organic frameworks with mobile charges have attracted significant attention due to their potential application in photoelectric devices, chemical resistance sensors, and catalysis. The authors report the mechanisms of photoinduced charge transport and electron dynamics in the conductive 2D M−HHTP MOFs and their correlation with photoconductivity using the combination of time-resolved terahertz spectroscopy, optical transient absorption spectroscopy, X-ray transient absorption spectroscopy, and density functional theory calculations.
Date: October 23, 2023
Creator: Wang, Denan; Ostresh, Sarah; Streater, Daniel; He, Peilei; Nyakuchena, James; Ma, Qiushi et al.
System: The UNT Digital Library