Dissolution experiments were performed on actual samples of NWCF Run H-4 radioactive calcine in fiscal years 1998 and 1999. Run H-4 is an aluminum/sodium blend calcine. Typical dissolution data indicates that between 90-95 wt% of H-4 calcine can be dissolved using 1gram of calcine per 10 mLs of 5-8M nitric acid at boiling temperature. Two liquid raffinate solutions composed of a WM-188/aluminum nitrate blend and a WM-185/aluminum nitrate blend were converted into calcine at the NWCF. Calcine made from each blend was collected and transferred to RAL for dissolution studies. The WM-188/aluminum nitrate blend calcine was dissolved with resultant solutions used as feed material for separation treatment experimentation. The WM-185/aluminum nitrate blend calcine dissolution testing was performed to determine compositional analyses of the dissolved solution and generate UDS for solid/liquid separation experiments. Analytical fusion techniques were then used to determine compositions of the solid calcine and UDS from dissolution. The results from each of these analyses were used to calculate elemental material balances around the dissolution process, validating the experimental data. This report contains all experimental data from dissolution experiments performed using both calcine blends.

The report presents calculation results of isotopic composition of irradiated fuel performed for the Quad Cities-1 reactor bundle with UO{sub 2} and MOX fuel. The MCU-REA code was used for calculations. The code is developed in Kurchatov Institute, Russia. The MCU-REA results are compared with the experimental data and HELIOS code results.

Drilling activities were conducted in FY97 and FY98 in the A/M Area to further identify areas of pure phase DNAPL below the water table. The purpose of the work was to further understand the subsurface contaminant distribution and to identify locations below the water table where aggressive DNAPL remediation technologies should be pursued.