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Experience base for Radioactive Waste Thermal Processing Systems: A preliminary survey
In the process of considering thermal technologies for potential treatment of the Idaho National Engineering Laboratory mixed transuranic contaminated wastes, a preliminary survey of the experience base available from Radioactive Waste Thermal Processing Systems is reported. A list of known commercial radioactive waste facilities in the United States and some international thermal treatment facilities are provided. Survey focus is upon the US Department of Energy thermal treatment facilities. A brief facility description and a preliminary summary of facility status, and problems experienced is provided for a selected subset of the DOE facilities.
Date:
April 1, 1992
Creator:
Mayberry, J.; Geimer, R.; Gillins, R.; Steverson, E.M.; Dalton, D. (Science Applications International Corp., Idaho Falls, ID (United States)) & Anderson, G.L. (EG and G Idaho, Inc., Idaho Falls, ID (United States))
System:
The UNT Digital Library
The development of precipitated iron catalysts with improved stability
The objective of this program is to identify the chemical principles governing the deactivation of precipitated iron catalysts during Fischer-Tropsch synthesis and to use these chemical principles in the design of catalysts suitable for slurry reactors. The performance targets are 88% CO+H{sub 2} conversion with less than 1% deactivation/day for 1 month and a methane and ethane selectivity of no more than 7% (based on hydrocarbons and oxygenates only) at a space velocity of at least 2 normal liters per hr per gram iron (NL/hr/gFe) using a synthesis gas with 0.5-1.0 H{sub 2}:CO ratio in a slurry reactor.
Date:
May 6, 1992
Creator:
Abrevaya, H.
System:
The UNT Digital Library
Brookhaven highlights for fiscal year 1991, October 1, 1990--September 30, 1991
This report highlights Brookhaven National Laboratory's activities for fiscal year 1991. Topics from the four research divisions: Computing and Communications, Instrumentation, Reactors, and Safety and Environmental Protection are presented. The research programs at Brookhaven are diverse, as is reflected by the nine different scientific departments: Accelerator Development, Alternating Gradient Synchrotron, Applied Science, Biology, Chemistry, Medical, National Synchrotron Light Source, Nuclear Energy, and Physics. Administrative and managerial information about Brookhaven are also disclosed. (GHH)
Date:
January 1, 1991
Creator:
Rowe, M.S.; Cohen, A.; Greenberg, D.; Seubert, L. & Kuper, J.B.H.
System:
The UNT Digital Library
A unified theory of resonant excitation of kinetic ballooning modes by energetic ions/alpha particles in tokamaks
A complete theory of wave-particle interactions is presented whereby both circulating and trapped energetic ions can destabilize kinetic ballooning modes in tokamaks. Four qualitatively different types of resonances, involving wave-precessional drift, wave-transit, wave-bounce, and precessional drift-bounce interactions, are identified, and the destabilization potential of each is assessed. For a characteristic slowing-down distribution function, the dominant interaction is that which taps those resonant ions with the highest energy. Implications of the theory for present and future generation fusion experiments are discussed. 16 refs.
Date:
October 1, 1991
Creator:
Biglari, H. & Chen, L.
System:
The UNT Digital Library
Electrochemistry of Thiobacillus ferrooxidans reactions with pyrite
The objective of this project is to provide the fundamental information on the mechanisms of bacterial leaching of pyrite. The knowledge of how bacterial leaching of pyrite functions is essential for design and development of a technology for coal cleaning with bacteria. The features of major electrochemical techniques will be examined to find out if any of them can provide a diagnostic information on the mechanisms of related reactions.
Date:
January 1, 1992
Creator:
Pesic, B.
System:
The UNT Digital Library
Photoinduced Charge Separation by Polymer-Bound Chromophores
This project has examined the photodynamic behavior of water-soluble polymers that have covalently linked hydrophobic chromophores spaced along the chains. These polymeric systems have been examined for photoinduced charge separation with electron-accepting ions having different total charge. Focus has been on the excited singlet (S{sub 1}) state formed by laser flash absorption. The effects of pH and ionic strength -- factors that govern the conformational nature of the polymer in solution -- have been studied. A second major effort has been to study photoinduced redox processes involving excited states of water-soluble variants of anthracene and acridine. 27 refs., 16 figs., 2 tabs.
Date:
September 1, 1991
Creator:
Rodgers, M. A. J.
System:
The UNT Digital Library
Physical fitness training reference manual for security force personnel at fuel cycle facilities possessing formula quantities of special nuclear materials
The recommendations contained throughout this NUREG are being provided to the Nuclear Regulatory Commission (NRC) as a reference manual which can be used by licensee management as they develop a program plan for the safe participation of guards, Tactical Response Team members (TRTs), and all other armed response personnel in physical fitness training and in physical performance standards testing. The information provided in this NUREG will help licensees to determine if guards, TRTs, and other armed response personnel can effectively perform their normal and emergency duties without undue hazard to themselves, to fellow employees, to the plant site, and to the general public. The recommendations in this NUREG are similar in part to those contained within the Department of Energy (DOE) Medical and Fitness Implementation Guide which was published in March 1991. The guidelines contained in this NUREG are not requirements, and compliance is not required. 25 refs.
Date:
September 1, 1991
Creator:
Arzino, P. A.; Caplan, C. S. & Goold, R. E. (California State Univ., Hayward, CA (United States). Foundation)
System:
The UNT Digital Library
A Novel Coal Feeder for Production of Low Sulfur Fuel
During the past three months, the coal feeding system has been tested and currently undergoing evaluation at the University of Cincinnati. The system consists primarily of an auger feed tube which is used to both convey and provide desulfurization of a high sulfur coal feedstock. The coal is conveyed at temperatures ranging from 350 to 550{degrees}C and under normal atmospheric pressure. Under these mild processing conditions, the coal partially pyrolizes and emits sulfur in the form of hydrogen sulfide while maintaining a relatively high heating value in the char product. The evolved gases are evacuated from the reactor (the feed tube) to another absorbing bed where H{sub 2}S reacts with the sorbent, usually lime or limestone. The resultant sorbent utilization is substantially higher than the values found in current dry scrubbing system and the produced low-sulfur char may then be used in a conventional steam boiler.
Date:
January 1, 1990
Creator:
Khang, S. J. & Keener, T. C.
System:
The UNT Digital Library
Fuel performance annual report for 1989
This annual report, the twelfth in a series, provides a brief description of fuel performance during 1989 in commercial nuclear power plants and an indication of trends. Brief summaries of fuel design changes, fuel surveillance programs, fuel operating experience, fuel problems, high-burnup fuel experience, and items of general significance are provided. References to more detailed information and related US Nuclear Regulatory Commission evaluations are included.
Date:
June 1, 1992
Creator:
Bailey, W.J.; Berting, F.M. (Pacific Northwest Lab., Richland, WA (United States)) & Wu, S. (Nuclear Regulatory Commission, Washington, DC (United States). Div. of Systems Technology)
System:
The UNT Digital Library
Continuum damping of low-n toroidicity-induced shear Alfven eigenmodes
The effect of resonant continuum damping is investigated for the low-mode-number, toroidicity-induced, global shear Alfven eigenmodes, which can be self-excited by energetic circulating alpha particles in an ignited tokamak plasma. Resonant interaction with the shear Alfven continuum is possible for these eigenmodes, especially near the plasma periphery, leading to significant dissipation, which is typically larger than direct bulk plasma dissipation rates. Two perturbation methods are developed for obtaining the Alfven resonance damping rate from the ideal fluid zeroth-order shear Alfven eigenvalue and eigenfunction. In both methods the real part of the frequency is estimated to zeroth order, and the imaginary part, which includes the damping rate, is then obtained by perturbation theory. One method, which is applicable when the eigenfunction is nearly real, can readily be incorporated into general MHD codes. In the second method, the zeroth-order eigenfunctions may be complex; however, the application of this method to general MHD codes needs more detailed development. Also, an analytical estimate is found for the next-order real frequency shift of the fluid global Alfven mode. Analytical and numerical studies of this continuum damping effect indicate that it can substantially reduce the alpha particle-induced growth rate. Thus, either it is possible to prevent …
Date:
September 1, 1991
Creator:
Berk, H.L.; Van Dam, J.W.; Guo, Z. & Lindberg, D.M.
System:
The UNT Digital Library
Safety rod latch inspection
During an attempt to raise control rods from the 100 K reactor in December, one rod could not be withdrawn. Subsequent investigation revealed that a small button'' in the latch mechanism had broken off of the lock plunger'' and was wedged in a position that prevented rod withdrawal. Concern that this failure may have resulted from corrosion or some other metallurgical problem resulted in a request that SRL examine six typical latch mechanisms from the 100 L reactor by use of radiography and metallography. During the examination of the L-Area latches, a failed latch mechanism from the 100 K reactor was added to the investigation. Fourteen latches that had a history of problems were removed from K-Area and sent to SRL for inclusion in this study the week after the original seven assemblies were examined, bringing the total of latch assemblies discussed in this report to twenty one. Results of the examination of the K-Area latch that initiated this study is not included in this report.
Date:
February 1, 1992
Creator:
Leader, D.R.
System:
The UNT Digital Library
An update on passive correctors for the SSC dipole magnets
The concept of correction of the magnetization sextupole became a topic of discussion as soon as it was realized that superconductor magnetization could have a serious effect on the SSC beam during injection. Several methods of correction were proposed. These included (1) correction with active bore tube windings like those on the HERA machine which correct out magnetization sextupole and the sextupole due to iron saturation, (2) correction with persistent sextupole windings mounted on the bore tube (3) correction using passive superconductor (4) correction using ferromagnetic material, and (5) correction using oriented magnetized materials. This report deals with the use of passive superconductor to correct the magnetization sextupole. Two basic methods are explored in this report: (1) One can correct the magnetization sextupole by changing the diameter of the superconductor filaments in one or more blocks of the SSC dipole. (2) One can correct the magnetization sextupole and decapole by mounting passive superconducting wires on the inside of the SSC dipole coil bore. In addition, an assessment of the contribution of each conductor in the dipole to the magnetization sextupole and decapole is shown. 38 refs, 25 figs., 15 tabs.
Date:
May 1, 1991
Creator:
Green, Michael A.
System:
The UNT Digital Library
Geothermal Materials Development, Annual Report FY 1991
Advances in the development of new materials, the commercial availabilities of which are essential for the attainment of Hydrothermal Category Level I and II Objectives, continue to be made in the Geothermal Materials Development Project. Many successes have already been accrued and the results used commercially. In FY 1991, utility company sponsored full cost'' recovery programs based upon materials technology developed in this project were initiated on topics such as condensing heat exchangers, high temperature composites for utility vaults used in district heating systems, and corrosion resistant coatings for use in oil-fired electric generating processes. In FY 1991 the DOE/GD-sponsored R D project was focused on reducing well drilling, fluid transport and energy conversion costs. Specific activities being performed included lightweight CO{sub 2}- resistant well cements, chemical systems for lost circulation control, thermally conductive and scale resistant protective linear systems, corrosion mitigation in process components at The Geysers, and elastomer-metal bonding systems needed for use in high temperature well drilling and safety related applications.
Date:
December 1, 1991
Creator:
Kukacka, L. E.
System:
The UNT Digital Library
Sonic enhanced ash agglomeration and sulfur capture
The major objective of the Phase 1 test program is to confirm the feasibility of the Manufacturing and Technology Conversion International, Inc. bimodal particle size approach to enhance particulate control by acoustic ash agglomeration. An ancillary objective of the Phase 1 effort is to demonstrate and confirm the feasibility of an acoustic field to enhance sulfur capture by increasing sorbent reactivity. Phase 1 tests are designed to cover the frequency range between 50 and 1400 Hz, establish monomodal baseline performance as a benchmark from which to measure the degree of enhancement expected from the bimodal approach, and, finally, to confirm the effectiveness of low-frequency fields over high-frequency fields for realistic particulate streams. The program will demonstrate the effectiveness of a unique approach which uses a bimodal distribution composed of large sorbent particles and fine fly ash particles to enhance ash agglomeration and sulfur capture at conditions found in direct coal-fired turbines. Under the impact of high-intensity sound waves, sorbent reactivity and utilization, it is theorized, will increase while agglomerates of fly ash and sorbents are formed which are readily collected in commercial cyclones. The work will extend the concept from the demonstration of feasibility (Phase 1), through proof-of-concept (Phase 2) …
Date:
January 1, 1991
Creator:
unknown
System:
The UNT Digital Library
(Environmental investigation of ground water contamination at Wright-Patterson Air Force Base, Ohio)
This report presents information concerning field procedures employed during the monitoring, well construction, well purging, sampling, and well logging at the Wright-Patterson Air Force Base. Activities were conducted in an effort to evaluate ground water contamination.
Date:
October 1, 1991
Creator:
unknown
System:
The UNT Digital Library
Configuration Management Program Plan
Westinghouse Savannah River Company (WSRC) has established a configuration management (CM) plan to execute the SRS CM Policy and the requirements of the DOE Order 4700.1. The Reactor Restart Division (RRD) has developed its CM Plan under the SRS CM Program and is implementing it via the RRD CM Program Plan and the Integrated Action Plan. The purpose of the RRD CM program is to improve those processes which are essential to the safe and efficient operation of SRS production reactors. This document provides details of this plan.
Date:
September 25, 1991
Creator:
unknown
System:
The UNT Digital Library
Health effects models for nuclear power plant accident consequence analysis: Low LET radiation
This report describes dose-response models intended to be used in estimating the radiological health effects of nuclear power plant accidents. Models of early and continuing effects, cancers and thyroid nodules, and genetic effects are provided. Weibull dose-response functions are recommended for evaluating the risks of early and continuing health effects. Three potentially lethal early effects -- the hematopoietic, pulmonary, and gastrointestinal syndromes -- are considered. In addition, models are included for assessing the risks of several nonlethal early and continuing effects -- including prodromal vomiting and diarrhea, hypothyroidism and radiation thyroiditis, skin burns, reproductive effects, and pregnancy losses. Linear and linear-quadratic models are recommended for estimating cancer risks. Parameters are given for analyzing the risks of seven types of cancer in adults -- leukemia, bone, lung, breast, gastrointestinal, thyroid, and other.'' The category, other'' cancers, is intended to reflect the combined risks of multiple myeloma, lymphoma, and cancers of the bladder, kidney, brain, ovary, uterus and cervix. Models of childhood cancers due to in utero exposure are also developed. For most cancers, both incidence and mortality are addressed. The models of cancer risk are derived largely from information summarized in BEIR III -- with some adjustment to reflect more recent …
Date:
January 1, 1990
Creator:
Evans, J. S.
System:
The UNT Digital Library
NQR-NMR studies of higher alcohol synthesis Cu-Co catalysts
Copper and cobalt are the key elements in syngas conversion catalyst systems used for higher alcohol synthesis. Their proximity and synergy sensitively control the selectivity and efficiency of the process. It is believed that their outer electronic charge distribution which is responsible for their electrical and magnetic properties might be governing their catalytic properties also. To examine the correlation between catalytic and magnetic properties, a series of copper cobalt catalysts (Co/Cu ratio 5:1 to 5:5) with and without a support were prepared. The nuclear quadrupole resonance spectrum of copper and (zero-field) nuclear magnetic resonance spectrum of cobalt and magnetization and hysteresis character of the catalyst were analyzed. Similar to the catalytic results, the magnetic results also were found to be very sensitive to the preparation technique. The results indicate possible electron exchange between copper and cobalt, and cobalt and the support Titania.
Date:
January 14, 1991
Creator:
unknown
System:
The UNT Digital Library
High temperature ceramic membrane reactors for coal liquid upgrading
In this project we intend to study a novel process concept, i.e, the use of ceramic membranes reactors in upgrading of coal derived liquids. Membrane reactors have been used in a number of catalytic reaction processes in order to overcome the limitations on conversion imposed by thermodynamic equilibrium. They have, furthermore, the inherent capability for combining reaction and separation in a single step. Thus they offer promise for improving and optimizing yield, selectivity and performance of processes involving complex liquids, as those typically found in coal liquid upgrading. Ceramic membranes are a new class of materials, which have shown promise in a variety of industrial applications. Their mechanical and chemical stability coupled with a wide range of operating temperatures and pressures make them suitable for environments found in coal liquid upgrading. In this project we will evaluate the performance of Sol-Gel alumina membranes in coal liquid upgrading processes under realistic temperature and pressure conditions and investigate the feasibility of using such membranes in a membrane reactor based coal liquid upgrading process. In addition, the development of novel ceramic membranes with enhanced catalytic activity for coal-liquid upgrading applications, such as carbon-coated alumina membranes, will be also investigated.
Date:
January 1, 1992
Creator:
Tsotsis, T.T.
System:
The UNT Digital Library
A Program of FRC Theory Research Annual Report
At the request of the Office of Fusion Energy, a group of experts was convened on February 6--8, 1990. This group met to assess the world data base on Reversed Field Pinch (RFP) physics, and, further, to assess the role of the ZTH experiment in providing reactor relevant physics understanding for that confinement geometry. This group met, analyzed some of the relevant literature, and heard extensive presentations on the physics of the RFP and the plans for the ZTH and RFX devices. The conclusions of this group of experts are contained in this report.
Date:
May 18, 1990
Creator:
Krall, Nicholas A.
System:
The UNT Digital Library
Exploring novel silicon-containing polymers---From preceramic polymers to conducting polymers with nonlinear optical properties
Several new types of silicon-containing preceramic polymers, i.e., poly(diorganosilacetylene) and poly(diorganosilvinylene) have been synthesized with molecular weights from 10,000 to 120,000. These polymers could be thermally converted to SiC with a moderate to high char yields. Ready solubility and good processability made these types of polymers attractive in their applications to ceramics. The thermal polymerization of diethynyldiphenyl-silane, which was reported in 1968 to afford poly(diphenylsilyldiacetylene) via dehydrogenation, was reinvestigated. Spectroscopic studies showed that the polymer had a structure of polyacetylene type not diacetylene. Diphenyldiethynylgermane and a series of diorganodiethynylsilances were synthesized. These could be polymerized in the presence of MoCl{sub 5} or WCl{sub 6} to afford a soluble, violet material with Mw as high as 108,000. 100 refs., 56 figs., 16 tabs.
Date:
October 7, 1991
Creator:
Pang, Yi.
System:
The UNT Digital Library
Liquefaction of coals using ultra-fine particle, unsupported catalysts: In situ generation by rapid expansion of supercritical fluid solutions
The program objective is to generate ultra-fine catalyst particles (20 to 400 {Angstrom} in size) and quantify their potential for improving coal dissolution in the solubilization stage of two-stage catalytic-catalytic liquefaction systems. In the first quarterly report for this program the concept behind our approach was detailed, the structure of the program was presented, key technical issues were identified, preliminary designs were outlined, and technical progress was discussed. All progress made during the second quarter of this program related to experiment design of the proposed supercritical expansion technique for generating ultra-fine, iron compound, catalyst particles. This second quarterly report, therefore, presents descriptions of the final designs for most system components; diagnostic approaches and designs for determining particles size and size distributions, and the composition of the pre-expansion supercritical solution; and the overall technique progress made during this reporting period. 6 refs., 15 figs., 1 tab.
Date:
September 1, 1991
Creator:
unknown
System:
The UNT Digital Library
Impact of Nonequilibrium Particle Temperature Considerations on Seeded Coal Combustion Plasma Properties
This past quarter ending 12/30/91, the linear MHD channel simulation model has not only been completely specified but also fully modified to incorporate considerations for nonequilibrium particle temperatures. Testing of the modified model with the initial values from the first submodel (Richter's combustion zone model) and evaluation of the non-equilibrium particle temperature effect on the overall MHD performance is being held up. Reasons for the holdup is the lack of adequate response from Dr. Richter on questions about his nonequilibrium particle temperature model. These questions relate to our insistence to know precisely how the model works and also some review of the source code to ascertain that it is synchronization with our overall analytical development. We have decided to generate initial generator inlet particle parameter values by modifying the CEC code to provide particle parameter values.
Date:
January 1, 1991
Creator:
Oni, A. A.
System:
The UNT Digital Library
Site Specific Verification Guidelines.
The Bonneville Power Administration (BPA) and the Northwest region have moved from energy surplus to a time when demand for energy is likely to exceed available supplies. The Northwest Power Planning Council is calling for a major push to acquire new resources.'' To meet anticipated loads in the next decade, BPA and the region must more than double that rate at which we acquire conservation resources. BPA hopes to achieve some of this doubling by programs independently designed and implemented by utilities and other parties without intensive BPA involvement. BPA will accept proposals for programs using performance-based payments, in which BPA bases its reimbursement to the sponsor on measured energy savings rather than program costs. To receive payment for conservation projects developed under performance-based programs, utilities and other project developers must propose verification plans to measure the amount of energy savings. BPA has traditionally used analysis of billing histories, before and after measure installation, adjusted by a comparison group on non-participating customers to measure conservation savings. This approach does not work well for all conversation projects. For large or unusual facilities the comparison group approach is not reliable due to the absence of enough comparable non-participants to allow appropriate statistical …
Date:
May 1, 1992
Creator:
Harding, Steve; Gordon, Frederick M. & Kennedy, Mike
System:
The UNT Digital Library