Report discussing a study testing features of the absorption spectra of different oxidation states of neptunium and perchloric acid concentration's effects on the spectra. Data regarding a disproportionation reaction present in neptunium(V) solutions in concentrated acid is included.

The following report analyzes experiments on urinary samples of personnel who were exposed to radioactive materials. This report describes the procedure employed for this assay, and data to show its performance and reasons for its present course are presented.

The following report measures a shield mockup in three regions: the first made almost entire of iron; the second, transition, region is made of various thicknesses of B4C; and the third region was borated water. The iron samples used in the experiments were made in the form of rectangular plates and place in the lid tank; however, the plates were not completely flat and created a water gap that was measured in this report.

A two-group approximation of the fission ratios and Pu production in an infinite hollow matrix is developed

We investigate the possibilities of using another reagent than glue as a filtration aid in South African ore treatment.

Report discussing calutron charge materials that can be used for the stable separation of isotopes.

From introduction: "This report summarizes the experimental data obtained at the San Pablo Laboratory on the corrosion of 5% Cr - 0.5% Mo steel by bismuth under conditions that allow mass transfer to occur. The bismuth is circulated through a temperature gradient by means of a thermosiphon loop."

Report summarizing corrosion tests meant to determine the corrosion rates of bronze, mild steel, T-304 stainless steel and 2S aluminum in 10% potassium tetraborate solution. Tests were completed under the boiling point of each solution except for 2S aluminum, which was tested at 40C, the approximate temperature in a pile.

Quarterly technical report including reports on chemistry of source, fissionable, and structural elements, nuclear chemistry, radio-organic chemistry, chemistry of separations processes, chemical physics, radiation chemistry, and instrumentation of the Chemistry Division of the Oak Ridge National Laboratory (ORNL). [From Abstract]

The following document describes observations from tests on neptunium metal and their reactions to different room temperatures.

Radioactive decay data are used to calculate the atomic masses of the heavy isotopes, A> 203. The four radioactive families are then connected by means of neutron binding energies known from reactions on various isotopes. Finally all the masses are collectively adjusted for the best fit with mass spectrographic information available in this region. The masses so calculated are presented. Differences between masses of isotopes are estimated to have an of (plus/minus) 0.00020 mas units or about 200 Kev; the position of the masses taken collectively is in doubt by about 1.5 Mev.

This report describes corrosion rate of uranium in hydrogen-saturated water appears to be constant with respect to time after a brief induction period and to involve only one type of over-all reaction, in which pitting effects are slight or nonexistent.

Report discussing the effects of xenon-135 and samarium-149 on the reactivity of nuclear reactors. The findings are presented in a "general manner, so as to be applicable to both the Converter and PuP Reactors."

Abstract: The radiations of U²³⁷ have been studied using a magnetic lens beta ray spectrometer and scintillation spectrometers for betas and gammas singly and in coincidence. A beta with an end point energy of 245 keV was found along with evidence for the existence of lower energy components. Gammas of energy 27, 42, 49, 59, 166, 208, 269, 354, 431, and 467 keV were found, and probably a gamma of 102 keV. The decay scheme constructed gives a total decay energy for this isotope of 512 keV.

Analysis of the problem of accelerating ions in a Thomas cyclotron has been confined almost entirely to the integration of various equations of motion (for single particles) for which a complete field description is necessary. In contrast, the problem of principal interest to rf system engineers concerns the gross transfer of electrical energy from an rf generator into an accelerated beam.

The following report describes the crystal structures of NpC and Pu2O3 identified by x-ray diffraction.

From abstract: "The variation of the reactivity of a pile as a function of width of a transverse gap is obtained. The method involves first finding the boundary condition satisfied by the flux at the gap face. This, in principle, provides enough information for a complete solution of the pile equations. A method for calculating the reactivity change is presented. The calculated reactivity is compared with experiment and a brief discussion of the validity of the approximations is given."

This quarterly progress report details the ongoing research happening at the Oak Ridge National Laboratory. In particular, this report discusses the current status of the Homogenous Reactor Experiment, boiling reactor and slurry studies, and general homogenous reactor studies.

From summary: "The influence of the structure of phosphate esters on the distribution coefficient of uranium between solutions of these esters in carbon tetrachloride and aqueous nitrate solutions has been studied. Esters of secondary alcohols showed higher distribution coefficients than primary alcohols. Phenyl esters extracted less uranium than alkyl esters, and the presence of other negative groups also resulted in less extraction. Compounds containing carbon to phosphorus bonds gave higher distribution coefficients than the corresponding esters, and the distribution coefficients increased with the number of such carbon to phosphorus bonds. Tributyl phosphine oxide (with three carbon to phosphorus bonds) showed high distribution coefficients with many salts, including uranyl nitrate, uranyl sulfate, uranyl chloride, thorium nitrate, plutonium (IV) nitrate and some of the fission products in nitrate solution. It is planned to study these and similar compounds further."

From abstract: "On the 86-inch cyclotron a 41-kw beam has been calorimetered at a net ion loading efficiency of 40%; the average proton current was 1.85 ma at 22.5 Mev. Practical specific yields have been determined for (p,2n) reactions on zinc and bismuth. The investigation of products of proton-induced fission of uranium has been continued and new techniques are being used in measuring angular distribution of reaction products. The 63-inch heavy particle cyclotron is now in operation; N+++ particles have been accelerated to ~25 Mev. In preliminary tests, induced activities have been detected in carbon, nitrogen, and oxygen targets. A hot-cathode ion source is ready for test operation. The 22-inch cyclotron is being used in an investigation of the problems associated with the use of rf and dc electrodes for the acceleration of protons from the ion source into the dees. Radiation-induced corrosion in Inconel tubing containing #21 eutectic (ANP) has been produced by proton irradiation in the 86-inch cylclotron; it is shown that the corrosion was not due to thermal effects. Approximately 150 grams of highly purified U 238 (< 5 ppm U 235) have been prepared, and two grams of thorium 230 (ionium) has been enriched to 90.6%."

Introduction: "In the early operation of the WTR severe canal corrosion of dummy fuel assemblies and a beryllium A-piece caused a great deal of concern as to the possible effects of long-time canal storage on such elements. A short-term experimental program was started to determine the causes of this corrosion and to correct them before any irradiated fuel elements had to be stored in the canal. The results of this program are presented here."

The following report introduces the aquadag, a part of the stellarator with the purposes to prevent the non-uniform accumulation of electrostatic charges on the walls of the stellerator and to free the electrons of the stellerator and provide accelerations, achieving a uniform field distribution.

Research progress on projects: Landau Effect with 32 Mev Protons, n - p Scattering of "300" Mev Neutrons, Geologic History of the Earth's Magnetic Field.

Corrosion rates of present reactor grade uranium were measured in boiling distilled water and were found to have higher values almost by a factor of two then previously reported corrosion rates of uranium. Mallinckrodt biscuit metal showed corrosion rates in the same medium somewhat lower than reactor grade uranium, and high purity metal prepared at Argonne National Laboratory corroded considerably less rapidly than the biscuit metal.