Report documenting the progress of the Army Gas-Cooled Reactor Systems Program to develop a mobile nuclear power plant for military field operation.

Final design for the 30 megawatt intermediate heat exchanger and steam generator.

Abstract. The region where exact thermodynamic description of the state of matter at high pressure and high temperature is possible is located. In the remaining region various approximate theories and empirical relations are discussed. These considerations are applied to hydrogen to locate the density and pressure at which the diatomic bond collapses. Also the approximate conditions are determined at which no bound electron states exist.

From abstract: The fuel element assembly was successfully irradiated in the SRE to a maximum burnup of 5300 Mwd/MTU, at a peak fission rate of approximately 1.5 x 10E13 fissions/cm3-sec and a maximum central temperature near 1200F.

From introduction: This report covers the results of a study of a mobile irradiator for fruit grown in California.

Abstract. the direct and inert-gas radiolysis, as well as the vacuum ultra-violet photolysis of CD3CH2CD3, CH3CD2CH3 and C3H2+C3D3 mixtures have been investigated in the presence of radical scavengers. The major conclusions are : (a) at atmospheric pressures, neutral propane decomposition contributes to the observed products although to a lesser extent than parent ion decompositions ; (b) a variation in pressure has a pronounced effect on the fragmentation of the parent ion ; (c) the hydrogen atoms in the ethyl ion are randomized in the direct as well as in the inert-gas sensitized radiolysis ; (d) rearrangement in the parent ion is of minor importance in the radiolysis ; (e) although the formation of propylene is related to the propyl ion, it is not necessarily produced by the neutralization of this ion.

Description of 15 specific systems employing search-type selection principles.

Introduction. The phase diagram data reported in this paper were obtained during an investigation of the beryllium-metal compounds of the titanium group transition elements. Several compounds in these systems had been previously reported but their compositions and structures were not all known. In the course of this study many details of the phase diagrams of the system were observed. Tentative diagrams consistent with this data will be presented.

From summary: The design of a spectrometer with the requisite improvement in crystals facilitates X-ray tube fluorescence.

From Abstract: "The bibliography, a supplement to NBS Monograph 35, of the same title, covers the years 1960 to 1965, inclusive, and include 109 references for prior years not listed in Monograph 35. It contains 1787 references, 38 of which are to books. The references, besides those directly concerned with pressure measurement, include those on vacuum technology which may bear on the technique of vacuum measurement, such as on adsorption and desorption, diffusion of gases into solids, gas conductance and hardware such as pumps, seals and traps."

This report covers the S-I-5-B-M fuel irradiation in the GETR Maritime Loop during the second quarter of fiscal year 1962. The data are summarized in Section II. Discussions on fuel performance, fuel environment (water chemistry), problems with loop operations, and the crud deposition program are included.

This report follows an investigation made to determine creep-rupture data for three sheet materials. Fourteen of sixteen tests were made in an atmosphere of carbon dioxide within hermetically sealed capsules, analyzing the reaction of the three sheet metals: 347 stainless steel, iron-aluminum-chromium alloy designated 261C, and a zirconium-base alloy, AE1H. Minimum creep rate, per cent elongation, and rupture life were determined and reported.

The study which has been carried out under Contract AT(30-1)2477 has as its objective the review of all work which has been done on the application of radionuclear techniques to research in water resources and supply, the evaluation of this work, and the suggestions of specific experiments which must be performed if these applications are to be extended.

Previous studies have been made of the relationship among acceleration, specific power, payload fraction, and travel time for many interplanetary missions. These utilized tangential thrust and correspond to the high thrust Hohmann transfer orbits. In addition, a complete optimization of the one way Mars mission has been accomplished. Since the minimum Jupiter round trip time was six and a half years for tangential thrust, calculations were carried out using higher energy transfer orbits. It is shown that the orbit-matching problem cannot be solved with tangential thrust programming in this case. The initial period of acceleration away from the earth's orbit was accomplished using tangential thrust in order to minimize energy expenditure. This was followed by a period of coasting until the proper moment arrived for commencing the orbit-matching maneuver. This terminates when the velocity and spatial coordinates of Jupiter's orbit are matched. The technique used for accomplishing these various orbit matching conditions without iteration are described. Best results for the final maneuver were obtained with the thrust vector approximately normal to the velocity vector. By this technique it is shown that the round-trip Jupiter mission may be carried out in four and an half years with 16% payload and 0.10 …

Report covering progress regarding a study on radiation synthesis involving halogenated compounds. Experimental progress, results and discussion are included.

"Rates of acetylene polymerization induced by Kr/sup 85/ in d-c fields were up to 15 times greater than those observed when no fields were imposed. Work to determine the relations between acetylene pressure, Kr/sup 85/ concentration, and the field intensity is continuing. In other activities, equipment is being designed to study the effects of megacycle electric fields on radioinduced chemical reactions."

From abstract: A series of three multi-compartmented experiments was designed to investigate the irradiation behavior uranium carbide fuels, as a function of composition, temperature, and burn-up; and the mechanical properties of Type 304 stainless steel, as a function of temperature and integrated thermal neutron flux.

"In the following report, a new technology is discussed which was first proposed in 1959, but which has been developed mainly since 1964; the in situ production of oil from shale by large underground retorts created by nuclear explosives. The first part of the present report describes this new process; the second part gives an analysis of the United States and the world endowments with crude oil resources and oil shale deposits and finally, the third part deals with expected cost estimates of this new technology as compared with present crude oil prices and potential costs of conventional shale oil production."

"Progress is reported on: design of a continuous flow system for the irradiation of silane using a Cos5 source; pile irradiation of silane samples at elevated temperatures; investigation of materials other than silane, including nonsilicon compounds as well as those containing the silyl group; modification of the existing vacuum system for handling larger quantities of silane as well as increasing the accuracy of the pressure measurements; and use of an electric discharge for the decomposition of silane. The work performed during the period of this report consisted of the following: 1. Preparation of samples of trichlorosilane and hydrogen and subsequent thermal and irradiation studies, and analysis of these samples. 2. Preparation of mixed samples of silane and argon and subsequent thermal and irradiation studies and and analysis. 3. Outlining of future investigations to be conducted on this project."

From introduction: The purpose of this survey was to document the pre-event and post-event condition of all existing surface facilities within a 10-mile radius of ground zero for Project GNOME.

Report issued by the APDA over studies conducted on reactor meltdown accidents. The studies incorporated the use of simulation materials. Methods and results of the studies are presented and discussed. This report includes tables, illustrations, and photographs.

"As presented in the original proposal the project consisted essentially of three parts: Phase I, Development and refinement of a radiochemical flow counting technique for the study of kinetics of reactions in solution ; Phase II, The application of this technique to the detailed study of the mechanism of solvolysis of sulfonium salts in mixed solvents ; Phase II, The further application of this kinetic technique, as a longer term aim, to other reacting systems of biochemical or other interest. This report covers the work of the contractual period 1 Sept. 1959 to 31 Aug. 1960."

The absolute differential cross sections for elastic scattering of 31-Mev He3 ions on Be, Al, Cu, Sn(nat), Sn120, and Bi have been measured in the angular range of approximately 10 to 120 deg in the center-of-mass system. Thin self-supporting foil targets were chosen to span the parameter A 1/3, where A is the target mass number. The first excited states of the isotopes of the above elements had sufficient energy separation from the ground state to enable elastic scattering to be resolved from inelastic scattering. The detection system, consisting of Cal(Tl) scintillation crystals, was capable of 3%pulse-height resolution and 1 degree angular resolution. Characteristically, the light-element angular distributions show strong diffraction effects. The differential cross section divided by the Rutherford cross section decreases exponentially at large angles for the heavy elements, and the differential cross sections break away from Rutherford behavior at angles which increase almost linearly with increase of atomic number of the target nucleus. A comparison of the results for natural tin, and tin enriched to 85% in Sn120, indicated that within the experimental uncertainties over the measured angular interval, there were no pronounced isotopic effects. The data are presented both in tabular and graphical form to allow …

Abstract: Electrical resistance measurements and metallography were employed in a study of the kinetics of the gamma to gamma prime transformation in the uranium-molybdenum system at 16 wt% molybdenum.