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Local Phase Manipulation for Multi-Beam Interference Lithography for the Fabrication of Two and Three Dimensional Photonic Crystal Templates (open access)

Local Phase Manipulation for Multi-Beam Interference Lithography for the Fabrication of Two and Three Dimensional Photonic Crystal Templates

In this work, we study the use of a spatial light modulator (SLM) for local manipulation of phase in interfering laser beams to fabricate photonic crystal templates with embedded, engineered defects. A SLM displaying geometric phase patterns was used as a digitally programmable phase mask to fabricate 4-fold and 6-fold symmetric photonic crystal templates. Through pixel-by-pixel phase engineering, digital control of the phases of one or more of the interfering beams was demonstrated, thus allowing change in the interference pattern. The phases of the generated beams were programmed at specific locations, resulting in defect structures in the fabricated photonic lattices such as missing lattice line defects, and single-motif lattice defects in dual-motif lattice background. The diffraction efficiency from the phase pattern was used to locally modify the filling fraction in holographically fabricated structures, resulting in defects with a different fill fraction than the bulk lattice. Through two steps of phase engineering, a spatially variant lattice defect with a 90° bend in a periodic bulk lattice was fabricated. Finally, by reducing the relative phase shift of the defect line and utilizing the different diffraction efficiency between the defect line and the background phase pattern, desired and functional defect lattices can be …
Date: December 2016
Creator: Lutkenhaus, Jeffrey Ryan
System: The UNT Digital Library
Low-Energy Electron Irradiation of Preheated and Gas-Exposed Single-Wall Carbon Nanotubes (open access)

Low-Energy Electron Irradiation of Preheated and Gas-Exposed Single-Wall Carbon Nanotubes

We investigate the conditions under which electron irradiation of single-walled carbon nanotube (SWCNT) bundles with 2 keV electrons produces an increase in the Raman D peak. We find that an increase in the D peak does not occur when SWCNTs are preheated in situ at 600 C for 1 h in ultrahigh vacuum (UHV) before irradiation is performed. Exposing SWCNTs to air or other gases after preheating in UHV and before irradiation results in an increase in the D peak. Small diameter SWCNTs that are not preheated or preheated and exposed to air show a significant increase in the D and G bands after irradiation. X-ray photoelectron spectroscopy shows no chemical shifts in the C1s peak of SWCNTs that have been irradiated versus SWCNTs that have not been irradiated, suggesting that the increase in the D peak is not due to chemisorption of adsorbates on the nanotubes.
Date: December 2016
Creator: Ecton, Philip
System: The UNT Digital Library
Ion Beam Synthesis of Binary and Ternary Transition Metal Silicide Thin Films (open access)

Ion Beam Synthesis of Binary and Ternary Transition Metal Silicide Thin Films

Among the well-known methods to form or modify the composition and physical properties of thin films, ion implantation has shown to be a very powerful technique. In particular, ion beam syntheses of binary iron silicide have been studied by several groups. Further, the interests in transition metal silicide systems are triggered by their potential use in advanced silicon based opto-electronic devices. In addition, ternary silicides have been by far less studied than their binary counterparts despite the fact that they have interesting magnetic and electronic properties. In this study, we investigate ion beam synthesis of Fe-Si binary structures and Fe-Co-Si ternary structures. This work involves fundamental investigation into development of a scalable synthesis process involving binary and ternary transitional metal silicide thin films and Nano-structures using low energy ion beams. Binary structures were synthesized by implanting Fe- at 50 keV energy. Since ion implantation is a dynamic process, Dynamic simulation techniques were used in these studies to determine saturation fluences for ion implantation. Also, static and dynamic simulation results were compared with experimental results. The outcome of simulations and experimental results indicate, dynamic simulation codes are more suitable than static version of the TRIM to simulate high fluence, low energy …
Date: December 2016
Creator: Lakshantha, Wickramaarachchige Jayampath
System: The UNT Digital Library
Charged Particle Transport and Confinement Along Null Magnetic Curves and in Various Other Nonuniform Field Configurations for Applications in Antihydrogen Production (open access)

Charged Particle Transport and Confinement Along Null Magnetic Curves and in Various Other Nonuniform Field Configurations for Applications in Antihydrogen Production

Comparisons between measurements of the ground-state hyperfine structure and gravitational acceleration of hydrogen and antihydrogen could provide a test of fundamental physical theories such as CPT (charge conjugation, parity, time-reversal) and gravitational symmetries. Currently, antihydrogen traps are based on Malmberg-Penning traps. The number of antiprotons in Malmberg-Penning traps with sufficiently low energy to be suitable for trappable antihydrogen production may be reduced by the electrostatic space charge of the positrons and/or collisions among antiprotons. Alternative trap designs may be needed for future antihydrogen experiments. A computational tool is developed to simulate charged particle motion in customizable magnetic fields generated by combinations of current loops and current lines. The tool is used to examine charged particle confinement in two systems consisting of dual, levitated current loops. The loops are coaxial and arranged to produce a magnetic null curve. Conditions leading to confinement in the system are quantified and confinement modes near the null curve and encircling one or both loops are identified. Furthermore, the tool is used to examine and quantify charged particle motion parallel to the null curve in the large radius limit of the dual, levitated current loops. An alternative to new trap designs is to identify the effects …
Date: May 2016
Creator: Lane, Ryan A.
System: The UNT Digital Library
A Search for Periodic and Quasi-Periodic Patterns in Select Proxy Data with a Goal to Understanding Temperature Variation (open access)

A Search for Periodic and Quasi-Periodic Patterns in Select Proxy Data with a Goal to Understanding Temperature Variation

In this work over 200 temperature proxy data sets have been analyzed to determine if periodic and or quasi-periodic patterns exist in the data sets. References to the journal articles where data are recorded are provided. Chapter 1 serves an introduction to the problem of temperature determination in providing information on how various proxy data sources are derived. Examples are given of the techniques followed in producing proxy data that predict temperature for each method used. In chapter 2 temperature proxy data spanning the last 4000 years, from 2,000 BCE to 2,000 CE, are analyzed to determine if overarching patterns exist in proxy data sets. An average of over 100 proxy data sets was used to produce Figure 4. An overview of the data shows that several “peaks” can be identified. The data were then subjected to analysis using a series of frequency modulated cosine waves. This analysis led to a function that can be expressed by equation 3. The literature was examined to determine what mathematical models had been published to fit the experimental proxy data for temperature. A number of attempts have been made to fit data from limited data sets with some degree of success. Some other …
Date: May 2016
Creator: Otto, James (James Robert)
System: The UNT Digital Library
Quantum Coherent Control and Propagation in Lambda System (open access)

Quantum Coherent Control and Propagation in Lambda System

Strong coherence in quasi-resonant laser driven system interferes with effective relaxations, resulting in behaviors like, coherent population trapping and Electromagnetically induced transparency. The Raman system can optimize this utilizing excited coherence in the lambda system when exposed to counter- intuitive pump-stokes pulses. The phenomenon can result in complete population transfer between vibrational levels called Stimulated Raman adiabatic passage(STIRAP). STIRAP and CHIRAP have been studied with Gaussian and chirped pulses. The optical propagation effects in dense medium for these phenomenon is studied to calculate the limitations and induced coherences. Further, the effect of rotational levels has been investigated. The molecular vibrational coherence strongly depends on the effect of rotational levels. The change in coherence interaction for ro-vibrational levels are reported and explained. We have considered the effects on the phase of radiation related to rotational mechanical motion of quantum system by taking advantages in ultra strong dispersion medium provided by quantum coherence in lambda system. The enhanced Fizeau effect on a single atom is observed.
Date: May 2016
Creator: Singh, Pooja, 1983-
System: The UNT Digital Library