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The Status of De-Inventory of Security Category I/II Nuclear Materials at Lawrence Livermore National Laboratory (LLNL) (open access)

The Status of De-Inventory of Security Category I/II Nuclear Materials at Lawrence Livermore National Laboratory (LLNL)

None
Date: May 13, 2010
Creator: Riley, D C & Dodson, K
System: The UNT Digital Library
Polarization-selective vortex-core switching by tailored orthogonal Gaussian-pulse currents (open access)

Polarization-selective vortex-core switching by tailored orthogonal Gaussian-pulse currents

We experimentally demonstrate low-power-consumption vortex-core switching in magnetic nanodisks using tailored rotating magnetic fields produced with orthogonal and unipolar Gaussian-pulse currents. The optimal width of the orthogonal pulses and their time delay are found, from analytical and micromagnetic numerical calculations, to be determined only by the angular eigenfrequency {omega}{sub D} for a given vortex-state disk of polarization p, such that {sigma}=1/{omega}{sub D} and {Delta}t={pi}/2 p/{omega}{sub D} . The estimated optimal pulse parameters are in good agreement with the experimental results. This work lays a foundation for energy-efficient information recording in vortex-core cross-point architecture.
Date: October 13, 2010
Creator: Jung, H.; Choi, Y. S.; Yoo, M. W.; Im, M. Y. & Kim, S. K.
System: The UNT Digital Library
The National Ignition Facility and the Promise of Inertial Fusion Energy (open access)

The National Ignition Facility and the Promise of Inertial Fusion Energy

The National Ignition Facility (NIF) at the Lawrence Livermore National Laboratory (LLNL) in Livermore, CA, is now operational. The NIF is the world's most energetic laser system capable of producing 1.8 MJ and 500 TW of ultraviolet light. By concentrating the energy from its 192 extremely energetic laser beams into a mm{sup 3}-sized target, NIF can produce temperatures above 100 million K, densities of 1,000 g/cm{sup 3}, and pressures 100 billion times atmospheric pressure - conditions that have never been created in a laboratory and emulate those in planetary interiors and stellar environments. On September 29, 2010, the first integrated ignition experiment was conducted, demonstrating the successful coordination of the laser, cryogenic target system, array of diagnostics and infrastructure required for ignition demonstration. In light of this strong progress, the U.S. and international communities are examining the implication of NIF ignition for inertial fusion energy (IFE). A laser-based IFE power plant will require a repetition rate of 10-20 Hz and a laser with 10% electrical-optical efficiency, as well as further development and advances in large-scale target fabrication, target injection, and other supporting technologies. These capabilities could lead to a prototype IFE demonstration plant in the 10- to 15-year time frame. …
Date: December 13, 2010
Creator: Moses, E I
System: The UNT Digital Library
kt-factorization for Hard Processes in Nuclei (open access)

kt-factorization for Hard Processes in Nuclei

Two widely proposed kt-dependent gluon distributions in the small-x saturation regime are investigated using two particle back-to-back correlations in high energy scattering processes. The Weizsacker-Williams gluon distribution, interpreted as the number density of gluon inside the nucleus, is studied in the quark-antiquark jet correlation in deep inelastic scattering. On the other hand, the unintegrated gluon distribution, defined as the Fourier transform of the color-dipole cross section, is probed in the direct photon-jet correlation in pA collisions. Dijet-correlation in pA collisions depends on both gluon distributions through combination and convolution in the large Nc limit. We calculate these processes in two approaches: the transverse momentum dependent factorization approach and the color-dipole/color glass condensate formalism, and they agree with each other completely.
Date: September 13, 2010
Creator: Dominguez, Fabio; Xiao, Bo-Wen & Yuan, Feng
System: The UNT Digital Library
2010 Water & Aqueous Solutions (open access)

2010 Water & Aqueous Solutions

Water covers more than two thirds of the surface of the Earth and about the same fraction of water forms the total mass of a human body. Since the early days of our civilization water has also been in the focus of technological developments, starting from converting it to wine to more modern achievements. The meeting will focus on recent advances in experimental, theoretical, and computational understanding of the behavior of the most important and fascinating liquid in a variety of situations and applications. The emphasis will be less on water properties per se than on water as a medium in which fundamental dynamic and reactive processes take place. In the following sessions, speakers will discuss the latest breakthroughs in unraveling these processes at the molecular level: Water in Solutions; Water in Motion I and II; Water in Biology I and II; Water in the Environment I and II; Water in Confined Geometries and Water in Discussion (keynote lecture and poster winners presentations).
Date: August 13, 2010
Creator: Ben-Amotz, Dor
System: The UNT Digital Library
MIDAS (Material Implementation, Database, and Analysis Source): A comprehensive resource of material properties (open access)

MIDAS (Material Implementation, Database, and Analysis Source): A comprehensive resource of material properties

MIDAS is aimed to be an easy-to-use and comprehensive common source for material properties including both experimental data and models and their parameters. At LLNL, we will develop MIDAS to be the central repository for material strength related data and models with the long-term goal to encompass other material properties. MIDAS will allow the users to upload experimental data and updated models, to view and read materials data and references, to manipulate models and their parameters, and to serve as the central location for the application codes to access the continuously growing model source codes. MIDAS contains a suite of interoperable tools and utilizes components already existing at LLNL: MSD (material strength database), MatProp (database of materials properties files), and MSlib (library of material model source codes). MIDAS requires significant development of the computer science framework for the interfaces between different components. We present the current status of MIDAS and its future development in this paper.
Date: December 13, 2010
Creator: Tang, M.; Norquist, P.; Barton, N.; Durrenberger, K.; Florando, J. & Attia, A.
System: The UNT Digital Library
Evolution of Static Physical Properties in Plutonium by Self-irradiation Damage (open access)

Evolution of Static Physical Properties in Plutonium by Self-irradiation Damage

The alpha-decay of plutonium leads to the age-related change in physical properties. This paper presents updated results of age-related effects on enriched and reference alloys measured from immersion density, dilatometry, and mechanical tests. After nearly 100 equivalent years of aging, both the immersion density and dilatometry show that the enriched alloys are decreasing in density by less than 0.02% per year and now exhibit a near linear density decrease, without void swelling. The tensile tests show that the aging process increases the strength of plutonium alloys, followed by possible saturation past 70 equivalent years of age. The ultimate goal of this work is to develop capabilities to predict physical properties changed by aging effects.
Date: April 13, 2010
Creator: Chung, B W; Lema, K E & Hiromoto, D S
System: The UNT Digital Library
ROCK DEFORMATION 2010 GORDON RESEARCH CONFERENCE, AUGUST 8-13, 2010 (open access)

ROCK DEFORMATION 2010 GORDON RESEARCH CONFERENCE, AUGUST 8-13, 2010

Creep in the crust and mantle is commonly considered a steady-state process. This view prevails despite the fact that earthquakes do not represent steady-state and at the base of the seismogenic zone, for example, the stresses that drive creep must vary with the earthquake cycle. The contribution of transient versus steady-state behavior is not easy to determine from naturally-deformed brittle or plastic rocks and our view of steady-state depends on whether we consider geological or shorter time-scales. Perhaps we avoid a non steady-state picture because we lack appropriate descriptive or quantitative tools. The aim of the 2010 Gordon Research Conference (GRC) in rock deformation is to explore what we know about non steady-state deformation and how we might advance our understanding through geological and geophysical field investigations, laboratory experiments and modeling. This will require an appraisal of the applicability of steady-state concepts as well as an exploration of transient behavior, in which processes and physical properties cycle between different states as might be the case during earthquake cycles, and transitions in behavior, where finite strain or changing environmental conditions lead to changes in processes and properties. Conference sessions will cover seven broad and interlinked topics. (1) What is steady state?; …
Date: August 13, 2010
Creator: Prior, David
System: The UNT Digital Library
Rhodium-Catalyzed C-C Bond Formation via Heteroatom-Directed C-H Bond Activation (open access)

Rhodium-Catalyzed C-C Bond Formation via Heteroatom-Directed C-H Bond Activation

Once considered the 'holy grail' of organometallic chemistry, synthetically useful reactions employing C-H bond activation have increasingly been developed and applied to natural product and drug synthesis over the past decade. The ubiquity and relative low cost of hydrocarbons makes C-H bond functionalization an attractive alternative to classical C-C bond forming reactions such as cross-coupling, which require organohalides and organometallic reagents. In addition to providing an atom economical alternative to standard cross - coupling strategies, C-H bond functionalization also reduces the production of toxic by-products, thereby contributing to the growing field of reactions with decreased environmental impact. In the area of C-C bond forming reactions that proceed via a C-H activation mechanism, rhodium catalysts stand out for their functional group tolerance and wide range of synthetic utility. Over the course of the last decade, many Rh-catalyzed methods for heteroatom-directed C-H bond functionalization have been reported and will be the focus of this review. Material appearing in the literature prior to 2001 has been reviewed previously and will only be introduced as background when necessary. The synthesis of complex molecules from relatively simple precursors has long been a goal for many organic chemists. The ability to selectively functionalize a molecule with …
Date: May 13, 2010
Creator: Colby, Denise; Bergman, Robert & Ellman, Jonathan
System: The UNT Digital Library
Discharge Physics of High Power Impulse Magnetron Sputtering (open access)

Discharge Physics of High Power Impulse Magnetron Sputtering

High power impulse magnetron sputtering (HIPIMS) is pulsed sputtering where the peak power exceeds the time-averaged power by typically two orders of magnitude. The peak power density, averaged over the target area, can reach or exceed 107 W/m2, leading to plasma conditions that make ionization of the sputtered atoms very likely. A brief review of HIPIMS operation is given in a tutorial manner, illustrated by some original data related to the self-sputtering of niobium in argon and krypton. Emphasis is put on the current-voltage-time relationships near the threshold of self-sputtering runaway. The great variety of current pulse shapes delivers clues on the very strong gas rarefaction, self-sputtering runaway conditions, and the stopping of runaway due to the evolution of atom ionization and ion return probabilities as the gas plasma is replaced by metal plasma. The discussions are completed by considering instabilities and the special case of ?gasless? self-sputtering.
Date: October 13, 2010
Creator: Anders, Andre
System: The UNT Digital Library
Thermal Degradation Behavior of Siloxane Elastomer Impregnated Carbon Nanotube Areogel Networks (open access)

Thermal Degradation Behavior of Siloxane Elastomer Impregnated Carbon Nanotube Areogel Networks

A novel class of nanoporous graphitic carbon foams has been synthesized. Unprecedented properties - electrically conductive, thermally stable (> 1000 C), and mechanically robust. Improved transport properties (DWNT-CA, SWNT-CA) - greater than 100% enhancement in thermal conductivity, 100-400% improvement in electrical conductivity. Rich mechanical deformation behavior (SWNT-CA) - stiff ({approx}100% improvement of elastic modulus), energy dissipation, fracture toughness, and fatigue behavior. Implications for energy-related technologies - hydrogen storage, fusion and fission energy, catalysis, electrochemical energy storage, and composites with foam scaffolds.
Date: December 13, 2010
Creator: Lewicki, J P & Worsley, M A
System: The UNT Digital Library
Mechanical design and analysis of an eight-pole superconducting vector magnet for soft x-ray magnetic dichroism measurements (open access)

Mechanical design and analysis of an eight-pole superconducting vector magnet for soft x-ray magnetic dichroism measurements

An eight-pole superconducting magnet is being developed for soft x-ray magnetic dichroism (XMD) experiments at the Advanced Light Source, Lawrence Berkley National Laboratory (LBNL). Eight conical Nb{sub 3}Sn coils with Holmium poles are arranged in octahedral symmetry to form four dipole pairs that provide magnetic fields of up to 5 T in any direction relative to the incoming x-ray beam. The dimensions of the magnet yoke as well as pole taper, diameter, and length were optimized for maximum peak field in the magnet center using the software package TOSCA. The structural analysis of the magnet is performed using ANSYS with the coil properties derived using a numerical homogenization scheme. It is found that the use of orthotropic material properties for the coil has an important influence in the design of the magnet.
Date: January 13, 2010
Creator: Arbelaez, D.; Black, A.; Prestemon, S.O.; Wang, S.; Chen, J. & Arenholz, E.
System: The UNT Digital Library
DEVELOPMENT OF ASME SECTION X CODE RULES FOR HIGH PRESSURE COMPOSITE HYDROGEN PRESSURE VESSELS WITH NON-LOAD SHARING LINERS (open access)

DEVELOPMENT OF ASME SECTION X CODE RULES FOR HIGH PRESSURE COMPOSITE HYDROGEN PRESSURE VESSELS WITH NON-LOAD SHARING LINERS

The Boiler and Pressure Vessel Project Team on Hydrogen Tanks was formed in 2004 to develop Code rules to address the various needs that had been identified for the design and construction of up to 15000 psi hydrogen storage vessel. One of these needs was the development of Code rules for high pressure composite vessels with non-load sharing liners for stationary applications. In 2009, ASME approved new Appendix 8, for Section X Code which contains the rules for these vessels. These vessels are designated as Class III vessels with design pressure ranging from 20.7 MPa (3,000 ps)i to 103.4 MPa (15,000 psi) and maximum allowable outside liner diameter of 2.54 m (100 inches). The maximum design life of these vessels is limited to 20 years. Design, fabrication, and examination requirements have been specified, included Acoustic Emission testing at time of manufacture. The Code rules include the design qualification testing of prototype vessels. Qualification includes proof, expansion, burst, cyclic fatigue, creep, flaw, permeability, torque, penetration, and environmental testing.
Date: April 13, 2010
Creator: Rawls, G.; Newhouse, N.; Rana, M.; Shelley, B. & Gorman, M.
System: The UNT Digital Library
Environmental Reactivity of Solid-State Hydrogen Systems: Fundamental Testing and Evaluation (open access)

Environmental Reactivity of Solid-State Hydrogen Systems: Fundamental Testing and Evaluation

In order to enable the commercial acceptance of solid state hydrogen storage materials and systems it is important to understand the risks associated with the environmental exposure of various materials. In some instances, these materials are sensitive to the environment surrounding the material and the behavior is unique and independent to each material. The development of testing procedures to evaluate a material's behavior with different environmental exposures is a critical need. In some cases material modifications may be needed in order to reduce the risk of environmental exposure. We have redesigned two standardized UN tests for clarity and exactness; the burn rate and self-heating tests. The results of these and other UN tests are shown for ammonia borane, NH{sub 3}BH{sub 3}, and alane, AlH{sub 3}. The burn rate test showed a strong dependence on the preparation method of aluminum hydride as the particle size and trace amounts of solvent greatly influence the test results. The self-heating test for ammonia borane showed a failed test as low as 70 C in a modified cylindrical form. Finally, gas phase calorimetry was performed and resulted in an exothermic behavior within an air and 30%RH environment.
Date: December 13, 2010
Creator: James, C.; Cortes-Concepcion, J.; Anton, D. & Tamburello, D.
System: The UNT Digital Library
Automatic Model Order Reduction (open access)

Automatic Model Order Reduction

None
Date: December 13, 2010
Creator: White, D. A.
System: The UNT Digital Library
National Ignition Facility (NIF) Neutron time-of-flight (nTOF) Measurements (open access)

National Ignition Facility (NIF) Neutron time-of-flight (nTOF) Measurements

The first three of eighteen neutron time-of-flight (nTOF) channels have been installed at the National Ignition Facility (NIF). The role of these detectors includes yield, temperature, and bang time measurements. This article focuses on nTOF data analysis and quality of results obtained for the first set of experiments to use all 192 NIF beams. Targets produced up to 2 x 10{sup 10} 2.45-MeV neutrons for initial testing of the nTOF detectors. Differences in neutron scattering at the OMEGA laser facility where the detectors were calibrated and at NIF result in different response functions at the two facilities. Monte Carlo modeling shows this difference. The nTOF performance on these early experiments indicates the nTOF system with its full complement of detectors should perform well in future measurements of yield, temperature, and bang time.
Date: May 13, 2010
Creator: Lerche, R. A.; Glebov, V. Y.; Moran, M. J.; McNaney, J. M.; Kilkenny, J. D.; Eckart, M. et al.
System: The UNT Digital Library
Simulation of e-cloud driven instability and its attenuation using a simulated feedback system in the CERN SPS (open access)

Simulation of e-cloud driven instability and its attenuation using a simulated feedback system in the CERN SPS

Electron clouds have been shown to trigger fast growing instabilities on proton beams circulating in the SPS, and a feedback system to control the single-bunch instabilities is under active development. We present the latest improvements to the WARP-POSINST simulation framework and feedback model, and its application to the self-consistent simulations of two consecutive bunches interacting with an electron cloud in the SPS. Simulations using an idealized feedback system exhibit adequate mitigation of the instability providing that the cutoff of the feedback bandwidth is at or above 450 MHz. Artifacts from numerical noise of the injected distribution of electrons in the modeling of portions of bunch trains are discussed, and benchmarking of WARP against POSINST and HEADTAIL are presented.
Date: December 13, 2010
Creator: Vay, J. L. & Furman, M. A.
System: The UNT Digital Library
Quark mass variation constraints from Big Bang nucleosynthesis (open access)

Quark mass variation constraints from Big Bang nucleosynthesis

We study the impact on the primordial abundances of light elements created of a variation of the quark masses at the time of Big Bang nucleosynthesis (BBN). In order to navigate through the particle and nuclear physics required to connect quark masses to binding energies and reaction rates in a model-independent way we use lattice QCD data and an hierarchy of effective field theories. We find that the measured {sup 4}He abundances put a bound of {delta}-1% {approx}< m{sub q}/m{sub 1} {approx}< 0.7%. The effect of quark mass variations on the deuterium abundances can be largely compensated by changes of the baryon-to-photon ratio {eta}. Including the bounds on the variation of {eta} coming from WMAP results and some additional assumptions narrows the range of allowed values of {delta}m{sub q}/m{sub q} somewhat.
Date: December 13, 2010
Creator: Bedaque, P.; Luu, T. & Platter, L.
System: The UNT Digital Library
Application of a Multiscale Model of Tantalum Deformation at Megabar Pressures (open access)

Application of a Multiscale Model of Tantalum Deformation at Megabar Pressures

A new multiscale simulation tool has been developed to model the strength of tantalum under high-pressure dynamic compression. This new model combines simulations at multiple length scales to explain macroscopic properties of materials. Previously known continuum models of material response under load have built upon a mixture of theoretical physics and experimental phenomenology. Experimental data, typically measured at static pressures, are used as a means of calibration to construct models that parameterize the material properties; e.g., yield stress, work hardening, strain-rate dependence, etc. The pressure dependence for most models enters through the shear modulus, which is used to scale the flow stress. When these models are applied to data taken far outside the calibrated regions of phase space (e.g., strain rate or pressure) they often diverge in their predicted behavior of material deformation. The new multiscale model, developed at Lawrence Livermore National Laboratory, starts with interatomic quantum mechanical potential and is based on the motion and multiplication of dislocations. The basis for the macroscale model is plastic deformation by phonon drag and thermally activated dislocation motion and strain hardening resulting from elastic interactions among dislocations. The dislocation density, {rho}, and dislocation velocity, {nu}, are connected to the plastic strain rate …
Date: May 13, 2010
Creator: Cavallo, R. M.; Park, H.; Barton, N. R.; Remignton, B. A.; Pollaine, S. M.; Prisbrey, S. T. et al.
System: The UNT Digital Library
Bragg Diffraction Using a 100ps 17.5 Kev X-Ray Backlighter and the Bragg Diffraction Imager (open access)

Bragg Diffraction Using a 100ps 17.5 Kev X-Ray Backlighter and the Bragg Diffraction Imager

A new diagnostic for measuring Bragg diffraction from a laser-driven crystal using a 100ps 17.5 kV x-ray backlighter source is designed and tested successfully at the Omega EP laser facility on static Mo and Ta single crystal samples using a Mo Ka backlighter. The Bragg Diffraction Imager (BDI) consists of a heavily shielded enclosure and a precisely positioned beam block, attached to the main enclosure by an Aluminum arm. Image plate is used as the x-ray detector. The diffraction lines from Mo and Ta <222> planes are clearly detected with a high signal-to-noise using the 17.5 keV and 19.6 keV characteristic lines generated by a petawatt-driven Mo foil. This technique will be applied to shock and ramp-loaded single crystals on the Omega EP laser. Pulsed x-ray diffraction of shock- and ramp-compressed materials is an exciting new technique that can give insight into the dynamic behavior of materials at ultra-high pressure not achievable by any other means to date. X-ray diffraction can be used to determine not only the phase and compression of the lattice at high pressure, but by probing the lattice compression on a timescale equal to the 3D relaxation time of the material, information about dislocation mechanics, including …
Date: May 13, 2010
Creator: Maddox, B. R.; Park, H.; Hawreliak, J.; Comley, A.; Elsholz, A.; Van Maren, R. et al.
System: The UNT Digital Library
The Effect of Bad-Faith Laws on First-Party Insurance Claims Decisions (open access)

The Effect of Bad-Faith Laws on First-Party Insurance Claims Decisions

This article describes a study of the legal distinctions among bad-faith laws and provides a theoretical foundation for the authors' hypotheses that bad-faith laws affect both economic and noneconomic damage amounts.
Date: May 13, 2010
Creator: Browne, Mark J.; Pryor, Ellen S. & Puelz, Bob
System: The UNT Digital Library
Diamond anvil cell experiments applied to the geochemistry of Earth's core formation (open access)

Diamond anvil cell experiments applied to the geochemistry of Earth's core formation

None
Date: September 13, 2010
Creator: Siebert, J; Ryerson, F; Antonangeli, D; Corgne, A; Ricolleau, A; Badro, J et al.
System: The UNT Digital Library
Surface Kinetic Model for the Fractionation of Trace Elements and Isotopes in Calcite Precipitated from Aqueous Solution (open access)

Surface Kinetic Model for the Fractionation of Trace Elements and Isotopes in Calcite Precipitated from Aqueous Solution

None
Date: September 13, 2010
Creator: DePaolo, D J; Ryerson, F; Watkins, J M; Bourg, I C; Yang, W; Nielsen, L et al.
System: The UNT Digital Library
QMDS: A File System Metadata Management Service Supporting a Graph Data Model-Based Query Language (open access)

QMDS: A File System Metadata Management Service Supporting a Graph Data Model-Based Query Language

Proposes QMDS: a file system metadata management service that integrates all file system metadata and uses a graph model with attributes on nodes and edges.
Date: September 13, 2010
Creator: Ames, S; Gokhale, M B & Maltzahn, C
System: The UNT Digital Library