Left unprotected, both transmissive and reflective final optics in a laser-driven inertial fusion power plant would quickly fail from melting, pulsed thermal stress, or degradation of optical properties as a result of ion implantation. One potential option for mitigating this threat is to magnetically deflect the ions such that they are directed to a robust energy dump. In this paper we detail integrated studies that have been carried out to assess the viability of this approach for protecting final optics.

The standard non-photochemical hole burning (NPHB) mechanism, which involves phonon-assisted tunneling in the electronically excited state, was originally proposed to explain the light-induced frequency change of chemically stable molecules in glassy solids at liquid helium temperatures by this research group more than two decades ago. The NPHB mechanism was then further elucidated and the concept of intrinsic to glass configurational relaxation processes as pre-mediating step to the hole burning process was introduced. The latter provided the theoretical basis for NPHB to evolve into a powerful tool probing the dynamics and nature of amorphous media, which aside from ''simple'' inorganic glasses may include also ''complex'' biological systems such as living cells and cancerous/normal tissues. Presented in this dissertation are the experimental and theoretical results of hole burning properties of aluminum phthalocyanine tetrasulphonate (APT) in several different matrices: (1) hyperquenched glassy water (HGW); (2) cubic ice (I{sub c}); and (3) water confined into poly(2-hydroxyethylmethacrylate) (poly-HEMA). In addition, results of photochemical hole burning (PHB) studies obtained for phthalocyanine tetrasulphonate (PcT) in HGW and free base phthalocyanine (Pc) in ortho-dichlorobenzene (DCB) glass are reported. The goal of this dissertation was to provide further evidence supporting the NPHB mechanism and to provide more insight that …

The goal of this project is to provide the capability for simulating fluid flow on complicated geometries, such as in the Bahia de Todos Santos. The Bahia de Todos Santos is a bay situated in the northwest corner of Mexico, off the coast of Ensenada and south of San Diego, California, USA. Figure 1.1 shows the Bahia de Todos Santos. It is part of an image taken from the Moderate Resolution Imaging Spectroradiometer (MODIS) sensors on the Aqua and Terra satellites in late June and early July 2003 [8]. Roughly 200 square kilometers in size, the bay also contains two islands off the peninsula of Punta Banda. Characteristics of flow in this bay are driven by the moon tide (M2) and wind forcing [9].

A collocation method using cubic splines is developed and applied to simulate steady and time-dependent, including turbulent, thermally convecting flows for two-dimensional compressible fluids. The state variables and the fluxes of the conserved quantities are approximated by cubic splines in both space direction. This method is shown to be numerically conservative and to have a local truncation error proportional to the fourth power of the grid spacing. A ''dual-staggered'' Cartesian grid, where energy and momentum are updated on one grid and mass density on the other, is used to discretize the flux form of the compressible Navier-Stokes equations. Each grid-line is staggered so that the fluxes, in each direction, are calculated at the grid midpoints. This numerical method is validated by simulating thermally convecting flows, from steady to turbulent, reproducing known results. Once validated, the method is used to investigate many aspects of thermal convection with high numerical accuracy. Simulations demonstrate that multiple steady solutions can coexist at the same Rayleigh number for compressible convection. As a system is driven further from equilibrium, a drop in the time-averaged dimensionless heat flux (and the dimensionless internal entropy production rate) occurs at the transition from laminar-periodic to chaotic flow. This observation is …

A study has been made of the generation of particles during laser ablation and has included size distribution measurements and observation of the formation processes. The particle size distribution with respect to different laser parameters was obtained in-line using a differential mobility analyzer (DMA) and a particle counter. The experimental results show that the particle size varies with laser energy, laser pulsewidth, ambient gas flow rate and sample properties. The results serve as a basis for controlling the size of nanoparticles generated by laser ablation. Laser shadowgraph imaging was used to study mass ejection processes and mechanisms. At higher laser irradiance, some particles were ejected in the liquid and even in the solid phase. Time-resolved images show the propagation of the shockwaves: external shockwaves propagate outward and decelerate, and internal shockwaves reflect back and forth between the gas contact surface and the sample surface. The internal shockwave is proposed to cause the ejection of liquid particles when the internal shockwave strikes the liquid molten layer. A simulation based on vapor plume expansion was carried out and provides satisfactory agreement with experimental results. Different material properties result in different particle ejection behavior:particle ejection for most materials including metals result in a …