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A Beamline for High Pressure Studies at the Advanced Light Source With a Superconducting Bending Magnet as the Source (open access)

A Beamline for High Pressure Studies at the Advanced Light Source With a Superconducting Bending Magnet as the Source

A new facility for high-pressure diffraction and spectroscopy using diamond anvil high-pressure cells has been built at the Advanced Light Source on Beamline 12.2.2. This beamline benefits from the hard X-radiation generated by a 6 Tesla superconducting bending magnet (superbend). Useful x-ray flux is available between 5 keV and 35 keV. The radiation is transferred from the superbend to the experimental enclosure by the brightness preserving optics of the beamline. These optics are comprised of: a plane parabola collimating mirror (M1), followed by a Kohzu monochromator vessel with a Si(111) crystals (E/{Delta}E {approx} 7000) and a W/B{sub 4}C multilayer (E/{Delta}E {approx} 100), and then a toroidal focusing mirror (M2) with variable focusing distance. The experimental enclosure contains an automated beam positioning system, a set of slits, ion chambers, the sample positioning goniometry and area detectors (CCD or image-plate detector). Future developments aim at the installation of a second end station dedicated for in situ laser-heating on one hand and a dedicated high-pressure single-crystal station, applying both monochromatic as well as polychromatic techniques.
Date: April 21, 2005
Creator: Kunz, M.; MacDowell, A. A.; Caldwell, W. A.; Cambie, D.; Celestre, R. S.; Domning, E. E. et al.
System: The UNT Digital Library
Laser System for Photoelectron and X-Ray Production in the PLEIADES Compton Light Source (open access)

Laser System for Photoelectron and X-Ray Production in the PLEIADES Compton Light Source

The PLEIADES (Picosecond Laser-Electron Interaction for the Dynamic Evaluation of Structures) facility provides tunable short x-ray pulses with energies of 30-140 keV and pulse durations of 0.3-5 ps by scattering an intense, ultrashort laser pulse off a 35-75 MeV electron beam. Synchronization of the laser and electron beam is obtained by using a photoinjector gun, and using the same laser system to generate the electrons and the scattering laser. The Ti Ti:Sapphire, chirped pulse amplification based 500 mJ, 50 fs, 810 nm scattering laser and the similar 300 {micro}J, 5 ps, 266 nm photoinjector laser systems are detailed. Additionally, an optical parametric chirped pulse amplification (OPCPA) system is studied as a replacement for part of the scattering laser front end. Such a change would significantly simplify the set-up the laser system by removing the need for active switching optics, as well as increase the pre-pulse contrast ratio which will be important when part of the scattering laser is used as a pump beam in pump-probe diffraction experiments using the ultrashort tunable x-rays generated as the probe.
Date: April 21, 2005
Creator: Gibson, D J; Barty, C J; Betts, S M; Crane, J K & Jovanovic, I
System: The UNT Digital Library
Estimation of (n,f) Cross-Sections by Measuring Reaction Probability Ratios (open access)

Estimation of (n,f) Cross-Sections by Measuring Reaction Probability Ratios

Neutron-induced reaction cross-sections on unstable nuclei are inherently difficult to measure due to target activity and the low intensity of neutron beams. In an alternative approach, named the 'surrogate' technique, one measures the decay probability of the same compound nucleus produced using a stable beam on a stable target to estimate the neutron-induced reaction cross-section. As an extension of the surrogate method, in this paper they introduce a new technique of measuring the fission probabilities of two different compound nuclei as a ratio, which has the advantage of removing most of the systematic uncertainties. This method was benchmarked in this report by measuring the probability of deuteron-induced fission events in coincidence with protons, and forming the ratio P({sup 236}U(d,pf))/P({sup 238}U(d,pf)), which serves as a surrogate for the known cross-section ratio of {sup 236}U(n,f)/{sup 238}U(n,f). IN addition, the P({sup 238}U(d,d{prime}f))/P({sup 236}U(d,d{prime}f)) ratio as a surrogate for the {sup 237}U(n,f)/{sup 235}U(n,f) cross-section ratio was measured for the first time in an unprecedented range of excitation energies.
Date: April 21, 2005
Creator: Plettner, C.; Ai, H.; Beausang, C. W.; Bernstein, L. A.; Ahle, L.; Amro, H. et al.
System: The UNT Digital Library
VACUUM WINDOW DESIGN FOR HIGH-POWER LASERS. (open access)

VACUUM WINDOW DESIGN FOR HIGH-POWER LASERS.

One of the problems in the high-power lasers design is in outcoupling of a powerful laser beam out of a vacuum volume into atmosphere. Usually the laser device is located inside a vacuum tank. The laser radiation is transported to the outside world through the transparent vacuum window. While considered transparent, some of the light passing through the glass is absorbed and converted to heat. For most applications, these properties are academic curiosities; however, in multi-kilowatt lasers, the heat becomes significant and can lead to a failure. The absorbed power can result in thermal stress, reduction of light transmission and, consequently, window damage. Modern optical technology has developed different types of glass (Silica, BK7, diamond, etc.) that have high thermal conductivity and damage threshold. However, for kilo- and megawatt lasers the issue still remains open. In this paper we present a solution that may relieve the heat load on the output window. We discuss advantages and issues of this particular window design.
Date: April 21, 2005
Creator: SHAFTAN, T.
System: The UNT Digital Library
CHEMICAL REACTIVITY TEST: Assessing Thermal Stability and Chemical Compatibility (open access)

CHEMICAL REACTIVITY TEST: Assessing Thermal Stability and Chemical Compatibility

The thermal stability of high explosive (HE) and its compatibility with other materials are of critical importance in storage and handling practices. These properties are measured at Lawrence Livermore National Laboratory using the chemical reactivity test (CRT). The CRT measures the total amount of gas evolved from a material or combination of materials after being heat treated for a designated period of time. When the test result is compared to a threshold value, the relative thermal stability of an HE or the compatibility of an HE with other materials is determined. We describe the CRT testing apparatus, the experimental procedure, and the comparison methodology and provide examples and discussion of results.
Date: April 21, 2005
Creator: Koerner, J.; Tran, T.; Gagliardi, F. & Fontes, A.
System: The UNT Digital Library
Fluctuation Results Fro PHENIX. (open access)

Fluctuation Results Fro PHENIX.

The PHENIX Experiment at the Relativistic Heavy Ion Collider has made measurements of event-by-event fluctuations in the net charge, the mean transverse momentum, and the charged particle multiplicity as a function of collision energy, centrality, and transverse momentum in heavy ion collisions. The results of these measurements will be reviewed and discussed.
Date: April 21, 2005
Creator: Mitchell, J. T.
System: The UNT Digital Library
PHOTOEMISSION AND SECONDARY ION MASS SPECTROMETRY STUDY OF URANIUM PASSIVATION BY C+ IMPLANTATION (open access)

PHOTOEMISSION AND SECONDARY ION MASS SPECTROMETRY STUDY OF URANIUM PASSIVATION BY C+ IMPLANTATION

Preventing the corrosion and oxidation of uranium is important to the continued development of advanced nuclear fuel technologies. Knowledge of the surface reactions of uranium metal with various environmental and atmospheric agents, and the subsequent degradation processes, are vitally important in 21st century nuclear technology. A review of the oxidation of actinide elements and their use in catalysis summarizes the present understanding of the kinetics and mechanisms of the reaction in dry and humid air. Researchers have recently used N{sub 2}{sup +} and C{sup +} ion implantation to modify the near surface region chemistry and structure of U to affect the nucleation and growth kinetics of corrosion and to passivate the surface. These researchers used Auger electron spectroscopy (AES) in conjunction with sputter depth profiling to show that the implanted surfaces had compositional gradients containing nitrides and carbides. In addition to chemical modification, ion implantation can create special reactive surface species that include defect structures that affect the initial absorption and dissociation of molecules on the surface, thus providing mechanical stability and protection against further air corrosion.
Date: April 21, 2005
Creator: Nelson, A J; Felter, T E; Wu, K J; Evans, C; Ferreira, J L; Siekhaus, W J et al.
System: The UNT Digital Library
Decontamination Techniques and Fixative Coatings Evaluated in the Building 235-F Legacy Source Term Removal Study (open access)

Decontamination Techniques and Fixative Coatings Evaluated in the Building 235-F Legacy Source Term Removal Study

Savannah River Site Building 235-F was being considered for future plutonium storage and stabilization missions but the Defense Nuclear Facilities Safety Board (DNFSB) noted that large quantities of Plutonium-238 left in cells and gloveboxes from previous operations posed a potential hazard to both the existing and future workforce. This material resulted from the manufacture of Pu-238 heat sources used by the NASA space program to generate electricity for deep space exploration satellites. A multi-disciplinary team was assembled to propose a cost- effective solution to mitigate this legacy source term which would facilitate future DOE plutonium storage activities in 235-F. One aspect of this study involved an evaluation of commercially available radiological decontamination techniques to remove the legacy Pu-238 and fixative coatings that could stabilize any residual Pu-238 following decontamination activities. Four chemical methods were identified as most likely to meet decontamination objectives for this project and are discussed in detail. Short and long term fixatives will be reviewed with particular attention to the potential radiation damage caused by Pu-238, which has a high specific activity and would be expected to cause significant radiation damage to any coating applied. Encapsulants that were considered to mitigate the legacy Pu-238 will also be …
Date: April 21, 2005
Creator: Farrell, Wayne
System: The UNT Digital Library
[After a Fashion, April 21, 2005] (open access)

[After a Fashion, April 21, 2005]

Article about the Women on their Toes benefit, the Austin Museum of Art's annual Art Ball, and other events around Austin, Texas.
Date: April 21, 2005
Creator: Moser, Stephen MacMillan
System: The UNT Digital Library