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Decoupling of self-diffusion and structural relaxation during afragile-to-strong cross-over in a kinetically constrained latticegas
We present an interpolated kinetically constrained lattice gas model which exhibits a transition from fragile to strong supercooled liquid behavior. We find non-monotonic decoupling that is due to this crossover and is seen in experiment.
Date:
January 30, 2005
Creator:
Pan, Albert C.; Garrahan, Juan P. & Chandler, David
System:
The UNT Digital Library