Traditional safety performance requirements for nuclear reactors have been developed for critical reactors, whose kinetics characteristics differ significantly from sub-critical, accelerator-driven nuclear reactors. In a critical nuclear reactor, relatively small amounts of reactivity (negative or positive) can produce large changes in the fission rate. In sub-critical reactors, the self-multiplication (k) decreases as the sub-criticality (1-k) increases, and the responsiveness to small reactivity changes decreases. This makes sub-critical nuclear reactors less responsive to positive reactivity insertions than critical reactors. Also, larger negative reactivity insertions are needed in sub-critical reactors to shut down the fission chain if the neutron source remains. This paper presents the results from a computational analysis of the safety performance of sub-critical, accelerator-driven nuclear reactors. Coupled kinetics and thermal-hydraulics models are used to quantify the effectiveness of traditional protection and control system designs in sub-critical reactors. The analyses also quantify the role of inherent, passive reactivity feedback mechanisms in sub-critical reactors. Computational results are used to develop conclusions regarding the most favorable and effective means for reactor control and protection in sub-critical, accelerator-driven nuclear reactors.

High voltage, solid state, inductive adder, pulse generators have found increasing application as fast kicker pulse modulators for charged particle beams. The solid state, inductive adder, pulse generator is similar in operation to the linear induction accelerator. The main difference is that the solid state, adder couples energy by transformer action from multiple primaries to a voltage summing stalk, instead of an electron beam. Ideally, the inductive adder produces a rectangular voltage pulse at the load. In reality, there is usually some voltage variation at the load due to droop on primary circuit storage capacitors, or, temporal variations in the load impedance. Power MOSFET circuits have been developed to provide analog modulation of the output voltage amplitude of a solid state, inductive adder, pulse generator. The modulation is achieved by including MOSFET based, variable subtraction circuits in the multiple primary stack. The subtraction circuits can be used to compensate for voltage droop, or, to tailor the output pulse amplitude to provide a desired effect in the load. Power MOSFET subtraction circuits have been developed to modulate short, temporal (60-400 ns), voltage and current pulses. MOSFET devices have been tested up to 20 amps and 800 Volts with a band pass …

During this reporting period our project focused on (1) review of case studies of remediation of centralized and commercial drilling fluid disposal (CCDD) sites in Texas, and (2) information transfer with preparation of a proceedings paper and a workshop/short course. Texas remediation of certain drilling-fluid disposal sites includes examples at CCDD sites as well as commercial oil reclamation sites and saltwater disposal sites that also disposed of drilling fluids in pits. Site investigations range from qualitative visual inspection and assessment to comprehensive hydrodynamic, chemical, and geophysical analyses of wastes and groundwater. A range of techniques has been used to evaluate waste material, soil, groundwater, and surface water for potential contamination with hydrocarbons, chemicals, saltwater, and naturally occurring radioactive materials (NORM). Most constituents of concern measured in these studies are below regulatory action levels and established guidelines. A proceedings paper summarizes results presented in this and previous semi-annual progress reports will be part of the Transactions of the Gulf Coast Association of Geological Societies (GCAGS). A technology transfer workshop also was prepared as part of that Annual Meeting of the GCAGS to be held in November 2002.

The discovery of two high-temperature fumaroles, with gas geochemistry compatible with an economic geothermal system, established Apacheta as one of the most attractive geothermal exploration prospects in northern Chile. These remote fumaroles at 5,150 m elevation were first sampled in 1999 by ENAP and its partners, following up on the reports of a CODELCO water exploration well that flowed small amounts of dry steam at 4,540 m elevation in the valley 4.5 km east of the fumaroles. The prospect is associated with a Plio-Pleistocene volcanic complex located within a NW-trending graben along the axis of the high Andes. The regional water table is 4,200 masl. There are no hot springs, just the 88 degrees C steam well and the 109 degrees and 118 degrees C fumaroles with gas compositions that indicate reservoir temperatures of greater than or equal to 250 degrees C, using a variety of gas geothermometers. An MT-TDEM survey was completed in 2001-2002 by Geotermica del Norte (SDN), an ENAP-C ODELCO partnership, to explore the Apacheta geothermal concession. The survey results indicated that base of the low resistivity clay cap has a structural apex just west of the fumaroles, a pattern typically associated with shallow permeability within a …

Traditional techniques for performance analysis provide a means for extracting and analyzing raw performance information from applications. Users then reason about and compare this raw performance data to their performance expectations for important application constructs. This comparison can be tedious, difficult, and error-prone for the scale and complexity of today's architectures and software systems. To address this situation, we present a methodology and prototype that allows users to assert performance expectations explicitly in their source code using performance assertions. As the application executes, each performance assertion in the application collects data implicitly to verify the assertion. By allowing the user to specify a performance expectation with individual code segments, the runtime system can jettison raw data for measurements that pass their expectation, while reacting to failures with a variety of responses. We present several compelling uses of performance assertions with our operational prototype including raising a performance exception, validating a performance model, and adapting an algorithm to an architecture empirically at runtime.

Nuclear Materials Management Division (NMMD) has proposed that up to 100 kg of the plutonium (Pu) solutions stored in H-Canyon be precipitated with a nuclear poison and dispositioned to H-Area Tank Farm. The use of gadolinium (Gd) as the poison would greatly reduce the number of additional glass logs resulting from this disposition. This report summarizes the characteristics of the precipitation process and addresses criticality concerns in the Nuclear Criticality Safety Evaluation. No problems were found with the nature of the precipitate or the neutralization process.

Extremely high quality data was acquired using an experimental ultrasound scanner developed at Lawrence Livermore National Laboratory using a 2D ring geometry with up to 720 transmitter/receiver transducer positions. This unique geometry allows reflection and transmission modes and transmission imaging and quantification of a 3D volume using 2D slice data. Standard image reconstruction methods were applied to the data including straight-ray filtered back projection, reflection tomography, and diffraction tomography. Newer approaches were also tested such as full wave, full wave adjoint method, bent-ray filtered back projection, and full-aperture tomography. A variety of data sets were collected including a formalin-fixed human breast tissue sample, a commercial ultrasound complex breast phantom, and cylindrical objects with and without inclusions. The resulting reconstruction quality of the images ranges from poor to excellent. The method and results of this study are described including like-data reconstructions produced by different algorithms with side-by-side image comparisons. Comparisons to medical B-scan and x-ray CT scan images are also shown. Reconstruction methods with respect to image quality using resolution, noise, and quantitative accuracy, and computational efficiency metrics will also be discussed.

A synchrotron radiation-based X-ray scattering facility for materials research on complex fluids has been completed on Sector 09 at the Advanced Photon Source at Argonne National Laboratory. It consists of a beamline on an undulator magnet source with doubly focusing X-ray optics and endstation spectrometers for both small angle X-ray scattering and liquid surface X-ray scattering.

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We analyze the Sudbury Neutrino Observatory (SNO) and Super-Kamiokande (SK) data on charged current (CC), neutral current (NC) and neutrino electron elastic scattering (ES) reactions to constrain the leading weak axial two-body current parameterized by L{sub 1A}. This two-body current is the dominant uncertainty of every low energy weak interaction deuteron breakup process, including SNO's CC and NC reactions. Our method shows that the theoretical inputs to SNO's determination of the CC and NC fluxes can be self-calibrated, be calibrated by SK, or be calibrated by reactor data. The only assumption made is that the total flux of active neutrinos has the standard {sup 8}B spectral shape (but distortions in the electron neutrino spectrum are allowed). We show that SNO's conclusion about the inconsistency of the no-flavor-conversion hypothesis does not contain significant theoretical uncertainty, and we determine the magnitude of the active solar neutrino flux.

Describes linear optical activity which studies non linear optical activity of dimer-like chiral molecules.

Structural properties of single-phase films of {kappa}-In{sub 2}Se{sub 3} and {gamma}-In{sub 2}Se{sub 3} were investigated. Both films were polycrystalline but their microstructure differed considerably. The a-lattice parameter of {kappa}-In{sub 2}Se{sub 3} has been measured. Comparison between these two materials indicates that {kappa}-In{sub 2}Se{sub 3} has a significantly larger unit cell ({Delta}c = 2.5 {+-} 0.2 % and {Delta}a = 13.5 {+-} 0.5%) and a structure more similar to the {alpha}-phase of In{sub 2}Se{sub 3}.

The ability to extract particle beam bunches from a ring accelerator in arbitrary order can greatly extend an accelerator's capabilities and applications. A prototype solid-state kicker pulser capable of generating asynchronous bursts of 50 kV pulses has been designed and tested into a 50{Omega} load. The pulser features fast rise and fall times and is capable of generating an arbitrary pattern of pulses with a maximum burst frequency exceeding 5 MHz If required, the pulse-width of each pulse in the burst is independently adjustable. This kicker modulator uses multiple solid-state modules stacked in an inductive-adder configuration where the energy is switched into each section of the adder by a parallel array of MOSFETs. Test data, capabilities, and limitations of the prototype pulser are described.

The purpose of this project is to explore the feasibility of using surface X-ray diffraction (SXRD) to determine the structure of biomineral surfaces in electrolyte solutions and of the adsorbed layer of acidic amino acids that are believed to play a central role in the control of biomineral formation and function. The work is a critical component in the development of an integrated picture of the physical and chemical basis for deposition and dissolution at solid-liquid interfaces in biological systems, and brings a new and very powerful surface-sensitive capability to LLNL. We have chosen as our model systems calcium carbonate and calcium phosphate in aspartic and glutamic acid-bearing solutions. The calcium compounds are ubiquitous among biomineral structures, both those that are beneficial such as bones and teeth, and those that are pathological such as kidney stones, while the two acidic amino acids--both as simple and poly-amino acids--are the dominant constituents of protein mixtures implicated in the control of biomineralization. The goals of the work are: (1) to determine the surface structure of pure calcium phosphate and calcium carbonate surfaces in aqueous solution using SXRD; (2) to determine how those surfaces are modified by the presence of aspartic and glutamic acid, …

The US Heavy Ion Fusion Virtual National Laboratory is continuing research into ion sources and injectors that simultaneously provide high current (0.5-1.0 Amps) and high brightness (normalized emittance better than 1.0 {pi}-mm-mr). The central issue of focus is whether to continue pursuing the traditional approach of large surface ionization sources or to adopt a multiaperture approach that transports many smaller ''beamlets'' separately at low energies before allowing them to merge. For the large surface source concept, the recent commissioning of the 2-MeV injector for the High Current eXperiment has increased our understanding of the beam quality limitations for these sources. We have also improved our techniques for fabricating large diameter aluminosilicate sources to improve lifetime and emission uniformity. For the multiaperture approach, we are continuing to study the feasibility of small surface sources and a RF induced plasma source in preparation for beamlet merging experiments, while continuing to run computer simulations for better understanding of this alternate concept. Experiments into both architectures will be performed on a newly commissioned ion source test stand at LLNL called STS-500. This stand test provides a platform for testing a variety of ion sources and accelerating structures with 500 kV, 17-microsecond pulses. Recent progress …

The current work continues a project completed in 1999 by ReMaxCo Technologies in which a novel, microwave based, VLS Silicon Carbide Fibrils concept was verified. This project continues the process development of a pilot scale commercial reactor. Success will lead to sufficient quantities of fibrils to expand work by ORNL and others on heat exchanger tube development. A semi-continuous, microwave heated, vacuum reactor was designed, fabricated and tested in these experiments. Cylindrical aluminum oxide reaction boats are coated, on the inner surface, with a catalyst and placed into the reactor under a light vacuum. A series of reaction boats are then moved, one at a time, through the reactor. Each boat is first preheated with resistance heaters to 850 C to 900 C. Each reaction boat is then moved, in turn, to the microwave heated section. The catalyst is heated to the required temperature of 1200 C to 1300 C while a mixture of MTS (methyl trichlorosilane) and hydrogen are introduced into the annulus of the boat. The MTS is dissociated to allow the carbon and silicon components to be dissolved into the catalyst. The catalyst saturates and precipitates silicon carbide onto the surface of the reaction boat to grow …

Researchers at the Timken Company conceived a project to develop an on-line instrument for wall thickness measurement of steel seamless mechanical tubing based on laser ultrasonic technology. The instrument, which has been installed and tested at a piercing mill, provides data on tube eccentricity and concentricity. Such measurements permit fine-tuning of manufacturing processes to eliminate excess material in the tube wall and therefore provide a more precisely dimensioned product for their customers. The resulting process energy savings are substantial, as is lowered environmental burden. The expected savings are $85.8 million per year in seamless mechanical tube piercing alone. Applied across the industry, this measurement has a potential of reducing energy consumption by 6 x 10{sup 12} BTU per year, greenhouse gas emissions by 0.3 million metric tons carbon equivalent per year, and toxic waste by 0.255 million pounds per year. The principal technical contributors to the project were the Timken Company, Industrial Materials Institute (IMI, a contractor to Timken), and Oak Ridge National Laboratory (ORNL). Timken provided mill access as well as process and metallurgical understanding. Timken researchers had previously developed fundamental ultrasonic analysis methods on which this project is based. IMI developed and fabricated the laser ultrasonic generation and …

The purpose of this study was to investigate the Salt and Mud Slough tributaries as sources of oxygen demanding materials entering the San Joaquin River (SJR). Mud Slough and Salt Slough are the main drainage arteries of the Grasslands Watershed, a 370,000-acre area west of the SJR, covering portions of Merced and Fresno Counties. Although these tributaries of the SJR are typically classified as agricultural, they are also heavily influenced by Federal, State and private wetlands. The majority of the surface water used for both irrigation and wetland management in the Grassland Watershed is imported from the Sacramento-San Joaquin Delta through the Delta-Mendota Canal. In this study, they measured algal biomass (as chlorophyll a), organic carbon, ammonia, biochemical oxygen demand (BOD), and other measures of water quality in drainage from both agricultural and wetland sources at key points in the Salt Slough and Mud Slough tributaries. This report includes the data collected between June 16th and October 4th, 2001. The objective of the study was to compare agricultural and wetland drainage in the Grasslands Watershed and to determine the relative importance of each return flow source to the concentration and mass loading of oxygen demanding materials entering the SJR. Additionally, …

An experimental facility for conducting research on capillary pumped loop (CPL) systems was developed. In order to simulate shipboard cooling water encountered at various locations of the ocean, the heat sink temperature of the facility could be varied. A flat plate, CPL evaporator was designed and tested under various heat sink temperatures. The sink temperature ranged from 274.3 to 305.2 K and the heat input varied from 250 to 800 W which corresponds to heat fluxes up to 1.8 W/cm{sup 2}. The CPL flat plate evaporator performed very well under this range of heat input and sink temperatures. The main result obtained showed that a large degree of subcooling developed between the evaporator vapor outlet line and liquid return line. This condensate depression increased with increasing heat input.

Predicting structural radiated noise is a process that involves several steps, often including the development of a finite element (FE) model to provide structural response predictions. Limitations of these FE models often govern the success of overall noise predictions. The purpose of the present investigation is to identify the effects of real world attachments on edge-stiffened plates and identify advanced modeling methods to facilitate vibroacoustic analyses of such complex structures. A combination of experimental and numerical methods is used in the evaluation. The results show the effects of adding attachments to the edge-stiffened plate in terms of mode shape mass loading, creation of new mode shapes, modifications to original mode shapes, and variations in damping levels. A finite element model of the edge-stiffened plate with simplified attachments has been developed and is used in conjunction with experimental data to aid in the developments. The investigation presented here represents a necessary first step toward implementing an advanced modeling technique.

The report describes the analyses performed on core samples from the sludge region of the waste in Tank 241-AY-102 to determine the electrochemical corrosion potential.

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Although programming models and languages appear to be converging, the computational workloads and communication patterns for scientific applications vary dramatically, depending, in part, on the nature of the problem the applications are solving. In this paper, we investigate the scalability, architectural requirements, and inherent behavioral characteristics of eight scalable scientific applications. We provide a comparative analysis of these applications and isolate their performance characteristics using empirical measurements. We refine our analysis into precise explanations of the factors that influence performance and scalability for each application; we distill these factors into common traits and overall recommendations. Initially, we examine the overall scalability of each application. Then, based on these results, we iteratively investigate the primary factors that affect scalability and performance using a combination of measurement techniques, such as message tracing and monitoring hardware counters, until we can understand each application's primary performance properties and the root causes of those properties.

The effect on the filter flux of tributyl phosphate and normal paraffin hydrocarbon in a simulate AZ-101 3.5 wt percent insoluble, 28-30 wt percent total slurry was studied.