This document overviews an entirely new approach to determining the composition--the chemical-elemental, isotopic and molecular make-up--of complex, highly structured objects, moreover with microscopic spatial resolution in all 3 dimensions. The front cover depicts the new type of pulsed laser system at the heart of this novel technology under adjustment by Alexis Wynne, and schematically indicates two of its early uses: swiftly analyzing the 3-D composition governed structure of a transistor circuit with both optical and mass-spectrometric detectors, and of fossilized dinosaur and turtle bones high-speed probed by optical detection means. Studying the composition-cued 3-D micro-structures of advanced composite materials and the microscopic scale composition-texture of biological tissues are two near-term examples of the rich spectrum of novel applications enabled by this field-opening analytic tool-set.

This report provides information about the Background and Legislative Issues on Export-Import Bank. The import-export bank is the U.S chief government agency that helps finance American exports.

The problem of stopping nuclear smuggling of terrorist nuclear devices is a complex one, owing to the variety of pathways by which such a device can be transported. To fashion new detection systems that improve the chances of detecting such a device, it is important to know the various requirements and conditions that would be imposed on them by both the types of devices that might be smuggled and by the requirement that it not overly interfere with the transportation of legitimate goods. Requirements vary greatly from low-volume border crossings to high-volume industrial container ports, and the design of systems for them is likely to be quite different. There is also a further need to detect these devices if they are brought into a country via illicit routes, i.e., those which do not pass through customs posts, but travel overland though open space or to a smaller, unguarded airport or seaport. This paper describes some generic uses of detectors, how they need to be integrated into customs or other law enforcement systems, and what the specifications for such detectors might be.

The collateral damage caused by fallout from shallow-buried nuclear devices is of considerable interest. In this paper, we present results for ''standard'' calculations using the KDFOC4 fallout computer code. Results are presented for a parametric range of yields from 0.1 kt to 1 Mt in equally-spaced logarithmic increments and for emplacement depths of 5 meters in hard, dry rock and 20 meters in moist soil. We will see that for low yields, this emplacement depth has a marked influence on the shape of the fallout patterns but for the highest yields, the fallout patterns are insensitive to the emplacement medium and depth. We look at two categories of doses: (1) Those for which health effects begin to be serious and range upward to lethal, and (2) Doses that are politically very sensitive but for which any deleterious health effects are difficult to prove.

This report describes executive and legislative activities relating to research and development budgets and priority-setting that occurred primarily during FY1993 to FY2001, the period of the two Clinton Administrations.

The scope of the project was to conduct experimental and computer modeling studies of the launching, flight characteristics and impacts of thin flyer plates driven by laser ablation under drive conditions where the plate remains a solid and retains its strength. Motivation for the work was to provide the scientific underpinnings for advanced development work on new detonators that will be needed within the next ten years for use in the Laboratory's national security mission. Areas of study were to be coupling of laser energy into the flyer plate during the launch phase, melting and instability growth in the flyer during launch, and an explosive-grain-scale understanding of the shock-to-detonation transition when the flyer plate impacts an explosive target. Knowledge and modeling capability, developed from this study, were to enable us to tailor the launching and acceleration conditions of thin flyer plates to produce an optimum impact for initiating high explosives. Experimental and computational studies of the shock-to-detonation transition were to aid us in developing more efficient initiating explosives for use in future detonators.

Second order optical nonlinearities were induced in commercial phosphate glasses (Schott, IOG-1) by the thermal poling technique. The induced {chi}{sup (2)} was measured via second harmonic generation using a fundamental beam from a 1064 nm mode-locked Nd:YAG laser. The nonlinear regions were characterized using the Maker-Fringe technique, in which the second harmonic signals were observed as a function of incident angle of the fundamental beam. The results show that the {chi}{sup (2)} profile has contributions from two distinct regions: a near-anodic surface region and a bulk. We have modeled the induced profile to fit our experimental results. The dependence of the induced nonlinearity on applied poling fields, temperatures and poling time is discussed.

Developed equipment consisted of a high magnetic field solenoid with supporting instrumentation for electron plasma confinement. The solenoid was designed and delivered in year 1. In year 2, it was mapped and the trap was created and commissioned. In parallel, an ongoing program of beam-plasma interaction studies was carried out with a lower field trap developed earlier. The trap was placed in the IUCF Coolor (an intermediate-energy electron-cooled storage ring) and the effects of the beam on the plasma were investigated, including energy and angular momentum transfer. Student projects carried out within the beam-plasma group also included development of a diagnostic with high spatial resolution, and preparation for extension of the beam-plasma interaction study to much lower beam energy. This became the principal group activity during the latter part of the project.

There were 5 laser experiments conducted to date in FY-01 under the ongoing project to study the response of single crystal fcc materials under shock compression. An additional 10 laser shots are planned for August, 2001. This work has focused on developing capability to record diffraction from multiple lattice planes during the passage of a shock through a thin foil of single crystal copper, while simultaneously performing separate shock sample recovery experiments to study the residual deformation structure in the recovered samples.

OAK-B135 Monitoring the Durability Performance of Concrete in Nuclear Waste Containment

Absolute partial {gamma}-ray cross sections for production of discrete {gamma} rays in the {sup 239}Pu(n,2n{gamma}i){sup 238}Pu reaction have been measured. The experiments were performed at LANSCE/WNR on the 60R flight line. Reaction {gamma}-rays were measured using the large-scale Compton-suppressed array of Ge detectors, GEANIE. The motivation for this experiment, an overview of the partial {gamma}-ray cross-section measurement, and an introduction to the main experimental issues will be presented. The energy resolution of the Ge detectors allowed identification of reaction {gamma} rays above the background of sample radioactivity and fission {gamma} rays. The use of planar Ge detectors with their reduced sensitivity to neutron interactions and improved line shape was also important to the success of this experiment. Absolute partial {gamma}-ray cross sections are presented for the 6{sub 1}{sup +} {yields} 4{sub 1}{sup +} member of the ground state rotational band in {sup 238}Pu, together with miscellaneous other {gamma}-ray partial cross sections. The n,2n reaction cross section shape and magnitude as a function of neutron energy was extracted from these partial cross sections using nuclear modeling (enhanced Hauser-Feshbach) to relate partial {gamma}-ray cross sections to the n,2n cross section. The critical nuclear modeling issue is the ratio of a partial cross …

T*e, which is an elastic-plastic fracture parameter based on incremental theory of plasticity, was determined numerically and experimentally. The T*e integral of a tunneling crack in 2024-T3 aluminum, three point bend specimen was obtained through a hybrid analysis of moire interferometry and 3-D elastic-plastic finite element analysis. The results were verified by the good agreement between the experimentally and numerically determined T*e on the specimen surface.

In this paper we study the behavior of a premixed turbulent methane flame in three dimensions using numerical simulation. The simulations are performed using an adaptive time-dependent low Mach number combustion algorithm based on a second-order projection formulation that conserves both species mass and total enthalpy. The species and enthalpy equations are treated using an operator-split approach that incorporates stiff integration techniques for modeling detailed chemical kinetics. The methodology also incorporates a mixture model for differential diffusion. For the simulations presented here, methane chemistry and transport are modeled using the DRM-19 (19-species, 84-reaction) mechanism derived from the GRIMech-1.2 mechanism along with its associated thermodynamics and transport databases. We consider a lean flame with equivalence ratio 0.8 for two different levels of turbulent intensity. For each case we examine the basic structure of the flame including turbulent flame speed and flame surface area. The results indicate that flame wrinkling is the dominant factor leading to the increased turbulent flame speed. Joint probability distributions are computed to establish a correlation between heat release and curvature. We also investigate the effect of turbulent flame interaction on the flame chemistry. We identify specific flame intermediates that are sensitive to turbulence and explore various correlations …

Major radionuclide emissions from the Department of Energy's Y-12 National Security Complex are nuclides of uranium which are emitted as a particulate. The radionuclide NESHAP regulation requires stack sampling to be conducted in accordance with ANST Standard N13.1, 1969. Appendix B of this standard requires in every case where sampling delivery lines are used that an evaluation should be made of deposition in these lines. A number of Y-12 Complex stacks are fitted with continuous samplers which draw particulate laden air through a probe and across a sample filter. One approach to evaluate line loss as required by the ANSI standard is to establish a representative factor that is used for all subsequent sampling efforts. Another approach is to conduct a routine probe wash procedure on an ongoing basis to account for line losses. In 1991, Y-12 National Security Complex personnel began routine probe washes as part of their sample collection procedure. Since then, 50-80 stacks have been sampled on a near continuous basis and probe washes have been conducted quarterly. Particulate collection in probes versus particulate collection on filters is recorded as a probe factor and probe factor trends for a 10-year period are available.

On October 7, 1994, President Clinton transmitted to the Senate the 1982 United Nations Convention on the Law of the Sea and the 1994 Agreement relating to the Implementation of Part XI of the United Nations Convention. The package was referred to the Senate Committee on Foreign Relations. On November 16, 1994, the U.N. Law of the Sea Convention entered into force but without accession by the United States. The 1994 Agreement entered into force on July 28, 1996, again without U.S. ratification.

This report examines three fundamental points implicit in the "engine of growth" argument. First, it questions whether the current account deficit is caused by strong U.S. growth and weak foreign growth. Second, it examines whether foreign growth is dependent on U.S. imports and the maintenance of a large U.S. current account deficit. Finally, it reviews the proposition that a U.S. recession would cause a world recession by lowering U.S. import demand. The report concludes that to make the final argument persuasive, other factors need to come into play, such as deteriorating expectations, financial crisis, or slow economic adjustment. These other factors seem unlikely to occur in the context of slowing U.S. growth, but they are possible in a recession.

The 107th Congress is considering legislation that would amend federal pipeline safety law, which directs the U.S. Secretary of Transportation to regulate pipeline transportation and storage of natural gases and hazardous liquids. Those bills also would authorize funding for the Office of Pipeline Safety (OPS) of the U.S. Department of Transportation (DOT), which is charged with implementing federal pipeline safety law. Among the topics discussed as part of the process of reauthorizing the OPS program are: state versus federal roles in pipeline safety, increased community involvement, funding amounts to support OPS, and new regulatory directives and authorities intended to improve the OPS program and associated state activities. S. 235, as amended, the "Pipeline Safety Improvement Act of 2001," passed the Senate on February 8, 2001. This report will be updated as necessary.

Sub-Saharan Africa has been far more severely affected by AIDS than any other part of the world. The United Nations reports that 25.3 million adults and children are infected with the HIV virus in the region, which has about 10% of the world's population but more than 70% of the worldwide total of infected people. This report discusses this issue in detail, including the cause of the African AIDS epidemic, the social and economic consequences, response and treatment, and U.S. policy.

This report discusses one of the major trade issues in the 107th Congress: whether or not Congress approves authority for the President to negotiate trade agreements with expedited, or "fast track" procedures. Under this authority, Congress agrees to consider legislation to implement the nontariff trade agreements under a procedure with mandatory deadlines, no amendment, and limited debate. The President is required to consult with congressional committees during negotiation of nontariff trade agreements and notify Congress before entering into any such agreement. The President was granted fast-track authority almost continuously from 1974 to 1994, but the authority lapsed and has not been renewed.

This report explores the authority of BLM personnel regarding unauthorized cattle by reviewing the statutory authorities of BLM over the federal rangelands under its administration, and the regulations and administrative materials implementing those authorities in the context of grazing, trespass, impoundment and sale of unauthorized livestock.

Solar Electricity - The Power of Choice (formerly NREL PV Working With Industry) is a quarterly newsletter devoted to the photovoltaics (PV) research and development activities performed by NREL staff in concert with their industry and university partners. This issue is devoted to demonstrating that PV R and D is a valuable investment for the United States. The editorialist for this issue is Larry Kazmerski, director of the National Center for Photovoltaics.

This report describes the results achieved during Phase I of a three-phase subcontract to develop and understand thin-film solar cell technology associated with CuInSe2 and related alloys, a-Si and its alloys, and CdTe. Modules based on all these thin films are promising candidates to meet DOE long-range efficiency, reliability, and manufacturing cost goals. The critical issues being addressed under this program are intended to provide the science and engineering basis for developing viable commercial processes and to improve module performance. The generic research issues addressed are: (1) quantitative analysis of processing steps to provide information for efficient commercial-scale equipment design and operation; (2) device characterization relating the device performance to materials properties and process conditions; (3) development of alloy materials with different bandgaps to allow improved device structures for stability and compatibility with module design; (4) development of improved window/heterojunction layers and contacts to improve device performance and reliability; and (5) evaluation of cell stability with respect to illumination, temperature, and ambient, and with respect to device structure and module encapsulation.

The 120 GeV primary proton beamline for the NuMI-MINOS [1] experiment at Fermilab will transport one of the most intense high-energy beams ever constructed. in parallel operation with the Collider program, 80% of the intensity capability of the Fermilab Main Injector can be sent to NuMI. Radiation safety pertaining to residual activity, damage of equipment and irradiation of groundwater is a primary concern. A particular challenge is that this beam will be transported to and targeted in a cavern excavated in rock in an aquifer region. A model of the beamline, including transport elements and excavated enclosures, has been built in the radiation simulation program MARS. This model has been used to determine limits for allowable beam loss, and to study effects of instabilities and of various failure types. Some results obtained with this model are presented.

It is not unusual to place multiple accelerators in a common enclosure to save on civil construction costs. This often complicates operations, especially if accelerators are affecting each other. At Fermilab, the influence of a rapidly cycling Main Injector (MI) synchrotron on an antiproton storage ring (Recycler), placed in a common tunnel, was initially found to be unacceptable for a reliable operation of the Recycler. Initial closed orbit excursions in the Recycler ring during the MI ramp were in excess of 5 mm (rms). This paper describes a shielding technique, used to reduce these orbit excursions by a factor of five.