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Report on the international workshop on cold moderators for pulsed neutron sources. (open access)

Report on the international workshop on cold moderators for pulsed neutron sources.

The International Workshop on Cold Moderators for Pulsed Neutron Sources resulted from the coincidence of two forces. Our sponsors in the Materials Sciences Branch of DOE's Office of Energy Research and the community of moderator and neutron facility developers both realized that it was time. The Neutron Sources Working Group of the Megascience Forum of the Organization for Economic Cooperation and Development offered to contribute its support by publishing the proceedings, which with DOE and Argonne sponsorship cemented the initiative. The purposes of the workshop were: to recall and improve the theoretical groundwork of time-dependent neutron thermalization; to pose and examine the needs for and benefits of cold moderators for neutron scattering and other applications of pulsed neutron sources; to summarize experience with pulsed source, cold moderators, their performance, effectiveness, successes, problems and solutions, and the needs for operational data; to compile and evaluate new ideas for cold moderator materials and geometries; to review methods of measuring and characterizing pulsed source cold moderator performance; to appraise methods of calculating needed source characteristics and to evaluate the needs and prospects for improvements; to assess the state of knowledge of data needed for calculating the neutronic and engineering performance of cold moderators; …
Date: January 6, 1999
Creator: Carpenter, J. M.
System: The UNT Digital Library
Recycling of Advanced Batteries for Electric Vehicles (open access)

Recycling of Advanced Batteries for Electric Vehicles

The pace of development and fielding of electric vehicles is briefly described and the principal advanced battery chemistries expected to be used in the EV application are identified as Ni/MH in the near term and Li-ion/Li-polymer in the intermediate to long term. The status of recycling process development is reviewed for each of the two chemistries and future research needs are discussed.
Date: October 6, 1999
Creator: JUNGST,RUDOLPH G.
System: The UNT Digital Library
Comparison of the corrosion behaviors of the glass-bonded sodalite ceramic waste form and reference HLW glasses. (open access)

Comparison of the corrosion behaviors of the glass-bonded sodalite ceramic waste form and reference HLW glasses.

A glass-bonded sodalite ceramic waste form is being developed for the long-term immobilization of salt wastes that are generated during spent nuclear fuel conditioning activities. A durable waste form is prepared by hot isostatic pressing (HIP) a mixture of salt-loaded zeolite powders and glass frit. A mechanistic description of the corrosion processes is being developed to support qualification of the CWF for disposal. The initial set of characterization tests included two standard tests that have been used extensively to study the corrosion behavior of high level waste (HLW) glasses: the Material Characterization Center-1 (MCC-1) Test and the Product Consistency Test (PCT). Direct comparison of the results of tests with the reference CWF and HLW glasses indicate that the corrosion behaviors of the CWF and HLW glasses are very similar.
Date: May 6, 1999
Creator: Ebert, W. L. & Lewis, M. A.
System: The UNT Digital Library
Lessons learned from U.S. Department of Defense 911-Bio Advanced Concept Technology Demonstrations. (open access)

Lessons learned from U.S. Department of Defense 911-Bio Advanced Concept Technology Demonstrations.

The US Department of Defense (DoD), in cooperation with other federal agencies, has taken many initiatives to improve its ability to support civilian response to a domestic biological terrorism incident. This paper discusses one initiative, the 911-Bio Advanced Concept Technology Demonstrations (ACTDs), conducted by the Office of the Secretary of Defense during 1997 to better understand: (1) the capability of newly developed chemical and biological collection and identification technologies in a field environment; (2) the ability of specialized DoD response teams to use these new technologies within the structure of cooperating DoD and civilian consequence management organizations; and (3) the adequacy of current modeling tools for predicting the dispersal of biological hazards. This paper discusses the experience of the ACTDs from the civilian community support perspective. The 911-Bio ACTD project provided a valuable opportunity for DoD and civilian officials to learn how they should use their combined capabilities to manage the aftermath of a domestic biological terrorism incident.
Date: July 6, 1999
Creator: Baldwin, T.; Gasper, W.; Lacher, L.; Newsom, D. & Yantosik, G.
System: The UNT Digital Library
Developing solid state experiments on the Nova laser (open access)

Developing solid state experiments on the Nova laser

An x-ray drive has been developed to shock compress metal foils in the solid state using an internally shielded hohlraum with a high contrast shaped pulse from the Nova laser. The drive has been characterized and hydrodynamics experiments designed to study growth of the Rayleigh-Taylor (RT) instability in Cu foils at 3 Mbar peak pressures in the plastic flow regime have been started. Pre-imposed modulations with an initial wavelength of 20-50 {micro}m, and amplitudes of 1.0-2.5 {micro}m show growth consistent with simulations. In the Nova experiments, the fluid and solid states are expected to behave similarly for Cu. An analytic stability analysis is used to motivate an experimental design with an Al foil where the effects of material strength on the RT growth are significantly enhanced. The conditions reached in the metal foils at peak compression are similar to those predicted at the core of the earth.
Date: August 6, 1999
Creator: Chandler, E. A.; Colvin, J. D.; Failor, B. H.; Gold, D. M.; Hauer, A.; Kalantar, D. H. et al.
System: The UNT Digital Library
Precision fast kickers for kiloampere electron beams (open access)

Precision fast kickers for kiloampere electron beams

These kickers will be used to make fast dipoles and quadrupoles which are driven by sharp risetime pulsers to provide precision beam manipulations for high current kA electron beams. This technology will be used on the 2nd axis of the DARHT linac at LANL. It will be used to provide 4 micropulses of pulse width 20 to 120 nsec. selected from a 2 {micro}sec., 2kA, 20MeV macropulse. The fast pulsers will have amplitude modulation capability to compensate for beam-induced steering effects and other slow beam centroid motion to within the bandwidth of the kicker system. Scaling laws derived from theory will be presented along with extensive experimental data obtained on the test bed ETA-II.
Date: October 6, 1999
Creator: Caporaso, G. J.; Chen, Y. J. & Weir, J. T.
System: The UNT Digital Library
The National Facility physics and diagnostics (open access)

The National Facility physics and diagnostics

This paper presents a description of the National Ignition Facility, some of the physics experiments that will be performed on it and a description of some of the diagnostics needed to complete these experiments. Experiments are presented under the headings of: ignition physics, weapons physics or high-energy-density experimental science, weapons effects, and basic science and inertial fusion energy. The diagnostics discussed are primarily those that will be provided for early operation.
Date: August 6, 1999
Creator: Wooton, A
System: The UNT Digital Library
The national facility physics and diagnostics (open access)

The national facility physics and diagnostics

This paper presents a description of the National Ignition Facility, some of the physics experiments that will be performed on it and a description of some of the diagnostics needed to complete these experiments. Experiments are presented under the headings of: ignition physics, weapons physics or high-energy-density experimental science, weapons effects, and basic science and inertial fusion energy. The diagnostics discussed are primarily those that will be provided for early operation.
Date: August 6, 1999
Creator: Wootton, A
System: The UNT Digital Library
Cryogenic moderator simulations : confronting reality. (open access)

Cryogenic moderator simulations : confronting reality.

The Intense Pulsed Neutron Source (IPNS) at Argonne National Laboratory is a spallation neutron source dedicated to materials research. Its three cryogenic methane moderators provide twelve neutron beams to fourteen instruments and test facilities. This report concerns ongoing activities for benchmarking our Monte Carlo model of the IPNS neutron generation system. This paper concentrates on the techniques (both experimental and calculational) used in such benchmarking activities.
Date: January 6, 1999
Creator: Iverson, E. B.
System: The UNT Digital Library
Greenhouse-gas emissions from biofuel use in Asia. (open access)

Greenhouse-gas emissions from biofuel use in Asia.

Biomass is a primary fuel for much of the world's population. In some developing countries it can contribute 80-90% of total primary energy consumption. In Asia as a whole we estimate that biomass contributes about 22 EJ, almost 24% of total energy use. Much of this biomass is combusted in inefficient domestic stoves and cookers, enhancing the formation of products of incomplete combustion (PIC), many of which are greenhouse gases. An inventory of the combustion of biofuels (fuelwood, crop residues, and dried animal waste) in Asia is used to develop estimates of the emissions of carbon-containing greenhouse gases (CO{sub 2},CO, CH{sub 4}, and NMHC) in Asian countries. The data are examined from two perspectives: total carbon released and total global warming potential (GWP) of the gases. We estimate that blofuels contributed 573 Tg-C in 1990, about 28% of the total carbon emissions from energy use in Asia. China (259 Tg-C) and India (187 Tg-C) were the largest emitting countries by far. The majority of the emissions, 504 Tg-C, are in the form of CO{sub 2}; however, emissions of non-CO{sub 2} greenhouse gases are significant: 57 Tg-C as CO, 6.4 Tg-C as CH{sub 4}, and 5.9 Tg-C as NMHC. Because of …
Date: July 6, 1999
Creator: Streets, D. G. & Waldhoff, S. T.
System: The UNT Digital Library
The National Facility physics and diagnostics (open access)

The National Facility physics and diagnostics

This paper presents a description of the National Ignition Facility, some of the physics experiments that will be performed on it, and a description of some of the diagnostics needed to complete these experiments. Experiments are presented under the headings of: ignition physics, weapons physics or high-energy-density experimental science, weapons effects, and basic science and inertial fusion energy. The diagnostics discussed are primarily those that will be provided for early operation.
Date: August 6, 1999
Creator: Wootton, A.
System: The UNT Digital Library
Energy Transfer of Excitons Between Quantum Wells Separated by a Wide Barrier (open access)

Energy Transfer of Excitons Between Quantum Wells Separated by a Wide Barrier

We present a microscopic theory of the excitonic Stokes and anti-Stokes energy transfer mechanisms between two widely separated unequal quantum wells with a large energy mismatch ({Delta}) at low temperatures (T). Exciton transfer through dipolar coupling, photon-exchange coupling and over-barrier ionization of the excitons through exciton-exciton Auger processes are examined. The energy transfer rate is calculated as a function of T and the center-to-center distance d between the two wells. The rates depend sensitively on T for plane-wave excitons. For located excitons, the rates depend on T only through the T-dependence of the localization radius.
Date: December 6, 1999
Creator: LYO,SUNGKWUN K.
System: The UNT Digital Library
Field Balancing in the Real World: Part 2 (open access)

Field Balancing in the Real World: Part 2

This paper is a follow-up to an earlier paper, Field Balancing in the Real World, which was presented at CSI Reliability Week 1997 in Nashville. Case studies of excessive vibrations on fans at ORNL will be discussed. Except for a few small sections from the earlier paper, this paper is entirely new. The case studies are new. As in the first paper, all fans are rigid-rotor type fans. Normal operation, therefore, is at less than the shaft's first critical speed. The presentation of case studies with root cause problems other than unbalance is a major departure from the first paper. We believe they belong here, since unbalance is suspected most of the time when a fan is vibrating excessively, even when it is not the root cause. In reality, unbalance is the underlying cause of the excess vibration on fans we have fixed at ORNL only about half the time. Furthermore, the analyst's credibility could be called into question upon an unsuccessful attempt at field balancing when underlying causes are later discovered and fixed. A demonstration will follow the case study presentation. The additional tests described in this paper to confirm centrifugal force (probable unbalance) will be performed.
Date: October 6, 1999
Creator: Bracher, R. K. & Surrett, Clark L.
System: The UNT Digital Library
MPC and A enhancements for the Murmansk shipping company icebreaker fleet (open access)

MPC and A enhancements for the Murmansk shipping company icebreaker fleet

The United States and the Russian Federation entered into a cooperative agreement in 1994 that resulted in a nuclear weapons non-proliferation program within the United States (US) Department of Energy (DOE) currently known as the Russia/Newly Independent States (NIS) Nuclear Material Security Task Force. In 1996, a project was initiated with the Murmansk Shipping Company to enhance material protection, control, and accounting of highly enriched nuclear fuel assemblies used for the Icebreaker Fleet. The commissioning ceremony for this project is scheduled for August 1999. This paper describes the physical protection, material control, and accounting measures implemented for the Icebreaker Fleet.
Date: July 6, 1999
Creator: Bartoch, O.; Bondarev, N.; Caskey, D.; Forehand, M.; Lambert, D.; Maltsev, V. et al.
System: The UNT Digital Library
Criticality safety evaluation - an endusers's perspective (open access)

Criticality safety evaluation - an endusers's perspective

This paper presents criticality safety evaluations from an enduser's perspective. Overall issues related to a criticality safety evaluation in an operations support setting are discussed. A work flow process is presented which shows the key steps in conducting an effective criticality evaluation. Finally, a few suggestions are given to assist newcomers to this field.
Date: May 6, 1999
Creator: Huang, S T
System: The UNT Digital Library
The Effect of Laser Surface Reconstruction of Disordered Carbons on Performance (open access)

The Effect of Laser Surface Reconstruction of Disordered Carbons on Performance

The reconstruction of the surface of disordered carbons was examined by heating carbons derived from polymethacrylonitrile (PMAN) and divinylbenzene (DVB) with a pulsed infrared laser in an argon or helium atmosphere, both fluidized and under static conditions. By graphitizing the outer surface of the carbons, it was hoped to reduce the high first-cycle losses associated with such disordered materials in Li-ion cells. The power to the sample was varied to observed the effects on surface morphology and electrochemical performance in 1M LiPF{sub 6} ethylene carbonate-dimethyl carbonate. The use various reactive atmosphere such as ethylene, 2-vinylpyridine, pyrrole, and furfuryl alcohol were also evaluated as an alternative means of hopefully forming a thin graphitic layer on the carbon particles to reduce first-cycle irreversibility. While some improvement was realized, these losses were still unacceptably high. The laser heating did improve the rate capabilities of the carbons, however. More work in this area is necessary to fully understand surface and bulk effects.
Date: October 6, 1999
Creator: EVEN JR., WILLIAM R. & GUIDOTTI, RONALD A.
System: The UNT Digital Library
TEM investigation of a ceramic waste form for immobilization of process salts generated during electrometallurgical treatment of spent nuclear fuel. (open access)

TEM investigation of a ceramic waste form for immobilization of process salts generated during electrometallurgical treatment of spent nuclear fuel.

Transmission electron microscopy (TEM) examination is presented of the microstructure of a ceramic waste form developed at Argonne National Lab - West for immobilization of actinides and fission products present in an electrorefiner salt. The material is produced by occluding the salt in zeolite granules, followed by hot isostatic pressing of the occluded zeolite in a mixture with a borosilicate glass. The paper presents results from a cold surrogate ceramic waste form, as well as {sup 239}Pu and {sup 238}Pu loaded samples.
Date: May 6, 1999
Creator: Esh, D. W.; Frank, S. M.; Goff, K. M.; Johnson, S. G.; Moschetti, T. L.; O'Holleran, T. P. et al.
System: The UNT Digital Library
Towards standardizing the measurement of electrochemical properties of solid state electrolytes in lithium batteries. (open access)

Towards standardizing the measurement of electrochemical properties of solid state electrolytes in lithium batteries.

The purpose of this paper is to stimulate thought and discussion in the technical community on standardization of the experimental determination of the pertinent electrochemical properties of solid electrolytes in lithium batteries. This standardization is needed for comparison and modeling of solid electrolytes in a practical lithium battery. The appropriate electrochemical properties include transport, thermodynamic, and physical parameters that generally depend on concentration and temperature. While it is beyond the scope of this work to put forward definitive measurement techniques for all types of solid electrolytes, it is hoped that comparisons between various techniques to examine a dissolved binary lithium salt in a dry polymer solvent will lead to improved understanding and methodology for examining solid electrolytes.
Date: May 6, 1999
Creator: Dees, D. W. & Henriksen, G. L.
System: The UNT Digital Library
Push technology at Argonne National Laboratory. (open access)

Push technology at Argonne National Laboratory.

Selective dissemination of information (SDI) services, also referred to as current awareness searches, are usually provided by periodically running computer programs (personal profiles) against a cumulative database or databases. This concept of pushing relevant content to users has long been integral to librarianship. Librarians traditionally turned to information companies to implement these searches for their users in business, academia, and the science community. This paper describes how a push technology was implemented on a large scale for scientists and engineers at Argonne National Laboratory, explains some of the challenges to designers/maintainers, and identifies the positive effects that SDI seems to be having on users. Argonne purchases the Institute for Scientific Information (ISI) Current Contents data (all subject areas except Humanities), and scientists no longer need to turn to outside companies for reliable SDI service. Argonne's database and its customized services are known as ACCESS (Argonne-University of Chicago Current Contents Electronic Search Service).
Date: April 6, 1999
Creator: Noel, R. E. & Woell, Y. N.
System: The UNT Digital Library
Status of the BNL High Current EBIS Test Stand. (open access)

Status of the BNL High Current EBIS Test Stand.

As part of a new, compact heavy ion injector for AGS/RHIC complex at Brookhaven National Laboratory we are developing an Electron Beam Ion Source (EBIS) that would satisfy present and future requirements. Such a source should be capable of producing intensities of e.g. Al{sup 35+} ions of about 3 x 10{sup 9} particles/pulse or U{sup 45+} of about 2 x 10{sup 9} particles/pulse. To achieve this, the required e-beam intensity is 10A, at a pulse length of 100ms. An EBIS test stand has been constructed, designed for the full electron beam power and having close to 1/2 of the trap length of an EBIS for RHIC. Initial electron beam tests have resulted in a 50{micro}s, 13A electron beam. Ion production and extraction has been shown with a 3.1 A, 50 ms electron beam, achieving an ion yield of 19 nC/pulse (neutralization degree of 61%); fast extraction trials have yielded extracted ion pulses of 1mA peak current and 18{micro}s at FWHM. Details of the test stand construction, results of the electron beam studies, and properties of the extracted ion pulse are presented.
Date: September 6, 1999
Creator: Beebe, E.
System: The UNT Digital Library
A new approach in utilizing a computer data acquisition system for criticality safety control (open access)

A new approach in utilizing a computer data acquisition system for criticality safety control

A new approach in utilizing a computer data acquisition system is proposed to address many issues associated with criticality safety control. This Criticality Safety Support System (CSSS) utilizes many features of computer and information process technology such as digital pictures, barcodes, voice data entry, etc. to enhance criticality safety in an R and D environment. Due to on-line data retrieving, data recording, and data management offered by new technology, the CSSS would provide a framework to design new solutions to old problems. This pilot program is the first step in developing this application for the years to come.
Date: May 6, 1999
Creator: Hopkins, H; Song, H & Warren, F
System: The UNT Digital Library
Estimates if population inversion for deep-UV transitions in Kr-like Y,Zr,Nb and Mo in a high-current reflex discharge (open access)

Estimates if population inversion for deep-UV transitions in Kr-like Y,Zr,Nb and Mo in a high-current reflex discharge

Kr-like ions are good candidates for FUV lasing since they can be produced in plasmas quite easily. We present results from a spectroscopic investigation of Y IV emission from a high current density, cold cathode reflex discharge. The Y II to Y V emission is recorded in the 200-3000 {angstrom} range using photometrically calibrated spectrometers, while the emission of trace aluminum ions serves for plasma diagnostics. The intensities of the Y IV 4d - 5p and 5s - 5p transitions strongly increase relative to lines from Y II and Y III with increasing plasma current. The spectra studied here are obtained at a current density of 1.75 A/cm{sup 2}. Experimental Y IV intensity ratios spanning several excited configurations are compared with collisional radiative predictions of the HULLAC atomic physics package. Good agreement is found for the measured and predicted ratios of 4p{sup 5}5p to 4p{sup 5}5s level populations per statistical weight. Finally, the response of the Kr-like system to a fast, transient excitation pulse is examined using the RADEX code. Large transient gains are predicted for several 5s - 5p transitions in Y IV, Zr V, Nb VI and Mo VII.
Date: July 6, 1999
Creator: Finkenthal, M.; May, M. J.; Fournier, K.; Goldstein, W. H.; Shlyaptsev, V. N.; Soukhanovskii, V. et al.
System: The UNT Digital Library
Structural and magnetic properties of UCo{sub 1/3}T{sub 2/3}Al solid solutions (T = Ru, Pt, Rh). (open access)

Structural and magnetic properties of UCo{sub 1/3}T{sub 2/3}Al solid solutions (T = Ru, Pt, Rh).

We report on neutron diffraction studies of UCo{sub 1/3}T{sub 2/3}Al (T = Ru, Pt, Rh). All three solid solutions form in the hexagonal ZrNiAl structure. The Ru-containing compound is found to be chemically ordered, while the Pt-containing compound is nearly disordered and the Rh-containing compound is purely disordered. All three compounds exhibit long-range magnetic order with rather small U moments.
Date: August 6, 1999
Creator: Andreev, A. V.; Bordallo, H. N.; Chang, S.; Nakotte, H.; Schultz, A. J.; Sechovsky, V. et al.
System: The UNT Digital Library
Coupling various methods for convection-diffusion problems with applications to flows in porous media (open access)

Coupling various methods for convection-diffusion problems with applications to flows in porous media

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Date: May 6, 1999
Creator: Lazrov, R D; Pasciak, J E & Vassilevski, P S
System: The UNT Digital Library