Report presenting research and development papers from the Oak Ridge National Laboratory's Analytical Chemistry Division.

Report covering the development of a set of difference equations for machine solution. In addition, this report serves as user's manual for Corn Pone, which is a code for the Oracle, the Oak Ridge National Laboratory computer.

Report regarding the structural evaluations made of the upper head of the Experimental Gas Cooled Reactor (EGCR). This report includes descriptions of the model, experimental procedures, and analyses of the results. Appendix begins on page 139.

Report documenting the research and development of the Oak Ridge National Laboratory's Gas-Cooled Reactor Project.

Report documenting ongoing research and developments at the Oak Ridge National Laboratory's Gas-Cooled Reactor Project.

Report documenting the ongoing research and developments at the Oak Ridge National Laboratory's Gas-Cooled Reactor Program.

Report containing the ongoing research and developments at the Oak Ridge National Laboratory's Gas-Cooled Reactor Program.

Report containing a preliminary chemical flowsheet "for the preparation of feed and two solvent extraction cycles for the processing of silicon-containing aluminum-uranium alloy, 20% enriched, fuel elements" (p. 2).

Report describing an "investigation of steady-state counter-flow of gases in a large pore graphite" by exposing it to streams of helium and argon.

Startup accident and pump run-down on the ORR have been simulated on the Reactor Controls Analog Facility. At full flow the 150% level scram (45 Mv) easily terminates the startup accident before the metal temperature gets above 180°F. For very low flows typical of criticality runs, temperature coefficients turn the excursion before it reaches 150% of full power, and temperatures climb to boiling, a potentially hazardous condition. (This same behavior can occur at full flow is the power is increased to the point where the level scram must be set above 50 Mw).

Simulated reactor fuel solutions were circulated at temperatures as high as 365°C in a small titanium pump loop. A hydroclone separator separated heavy phases formed at high temperatures. As the temperature of the solution was increased beyond the two-liquid-phase temperature (327°C), the salt concentration of the light phase decreased and the acid concentration increased. The mole ratios of uranium to sulfate, uranium to copper, and uranium to nickel in the light phase decreased in the same proportion in the temperature range of 330 to 365°C. Corrosion of titanium and Zircaloy-2 specimens was insignificant during the relatively short exposure periods.

A nonnuclear explosion involving an evaporator occurred in a shielded cell in the Radiochemical Processing Pilot plant at Oak Ridge National Laboratory. Plutonium released from the processing cell contaminated areas in the pilot plant building and nearby streets and building surfaces. The explosion is considered the result of rapid reaction of nitrated organic compounds formed by the inadvertent nitration of about 14 liters of a proprietary decontaminating reagent.

A carrier containing 138.99 liters of solution, uranium concentration 202.04 g/liter with an isotopic concentration of 97.3% U-233, was prepared for shipment. The total uranium was 28,062 +/- 60 g (95% confidence level) and the U-233, 27,305 +/- 66 g (95% confidence level).

The absorption in lead of Bremsstrahlung X radiation from a Sr^90 TiO3 pellet in the proximity of Hastelloy "C" was measured. The tenth value layer of the more energetic components of the X-ray continuum was determined to be 1.60 inches.

From Introduction: "The present semiannual progress report introduces more active consideration than has been given in the past (by us, at least) to the importance of energy degradation in DCX-like devices. The following pages introduce also a new major apparatus designated as DCX-2. Some of these concepts cannot as yet be released publicly and therefore Chap. 3 of this report, covering the DCX-EP-B design, is being issued separately, with restricted distribution, as ORNL-3044."

A listing and description is given of the experiments associated with the HFIR Critical Experiment-2. The primary experiments concern the reactivity of the bare core, reactivity worth of "gray" control plates, core-power distribution, reactivity. The secondary experiments concern the reactivity of the fuel, and the reactivity worth of a "partial" gray plate.

Report issued by the Oak Ridge National Laboratory discussing studies conducted on corrosion by fluorides. Equipment, procedures, results, and analysis is presented. This report includes tables, illustrations, and photographs.

THOROBRED is an IBM-704 code for the calculation of nuclear and economic characteristics of two-region homogeneous reactors operating on a U-Th fuel cycle in the steady state. The major input variables are reactor dimensions, power level, thorium concentration, chemical and purification systems cycle times, corrosion rates, fraction of Pa loss, and nuclear and economic data. The output includes equilibrium isotope concentrations, neutron balance, and a breakdown of fuel cost. Running times are normally less than one minute per case.

Analyses are generally made at the ORR with a view toward determining the surface temperatures of fuel plates.

A review of helium sources, availability, consumption, and future production capacity indicates that the helium consumed in the operation of 100 helium-cooled reactors for 300-Mwe power plants over a 20-year period will run no more than a few per cent of the helium consumed in the U. S. in the next 25 years and less than 1% of the helium that is to be stored during that period under the helium conservation act of 1960 (Public Law 86-777).

The equilibrium and maximum override values for xenon and samarium poisoning have been computed using the recently issued effective cross sections of C. H. Westcott. Values are given as a function of specific power, neutron temperature, and epithermal flux content.

"An analysis is presented of the accidental release of activity following the operation of the NS "Savannah" at the New York Shipbuilding Corporation docks in Camden, New Jersey. Although a number of accidents are considered, the report is primarily concerned with the environmental activity levels and subsequent exposures which would result from the "maximum credible accident" (p. v).

A cross section tape has been prepared containing data for elements of most interest for aqueous homogeneous reactor multigroup diffusion calculations involving combinations of 150, 200, 240, 260, and 280°C temperatures. This tape permits multigroup analysis of a reactor in which two or more regions are at different temperatures.

A multiple controller system for a single process is formulated in block diagram form. It is shown that for the general case of n controllers and one type of cross coupling, the system equations can be reduced to the standard forms of servomechanism theory. The effects of failure in individual controllers are examined, and it is demonstrated that the system shows considerable promise for both reliability and maintenance without process interruption.