Technical report containing short reports on (1) Mass spectrometer studies; (2) Purification of heavy water; and (3) Equilibration studies.

Abstract: "Photographic plates have been used to measure the energy of neutrons from the fission of 25. The spectrum as inferred from the ranges of 850 protons recoiling in the forward direction shows a very wide maximum at ~1.5 Mev with an exponentially decreasing high energy tail which extends beyond 7 Mev. The minimum energy neutrons recorded were ~700 kv. If the spectrum is extrapolated to zero, one finds that this average neutron energy is about 1.85 Mev. The stopping power of the plates was calibrated by the use of monochromatic neutrons from the Li-7(pn) Be-7 reaction and the d-d reaction."

Abstract: The counting accuracy of the Chicago Scalers, Models 961A and 961B, is a function of the bias setting of the limiter (V2). this report gives quantitative data supporting this thesis. A method of making bias settings is suggested. These tests were run at the suggestion of Mr. V. C. Hanson.

From introduction: "The measurement of the thermal conductivity of liquid TF6 presented unusual difficulties because of two of its properties which necessitated working with a closed system. The properties were (1) the liquid can exist as such only above 64.05°C. at which temperature its saturated vapor pressure is 1140 mm. of mercury, and (2) the compound reacts rapidly with moist air. Also because of the liquid's extremely corrosive nature, it was necessary to design a cell of special corrosion resistant materials."

Abstract: Pure UO2F2 is made by reaction between anhydrous HF and pure UO3. Although it is difficult to prepare free of water, it is not very hygroscopic. Prolonged heating at 100-105 degrees releases 99.9% of the water in an aqueous solution; the rate of loss of water is very small after saturation is reached. X-ray diffraction data give a density of 6.2 for the solid. The density of a 1.004 M solution is 1.274; the density of a saturated solution (5.130 M) is 2.400. The densities of F-9 solutions have been calculated from the densities of ordinary aqueous solutions, and the values are compared graphically. Data on the solubility indicate that there is a small increase in the range 25-100 degrees. Recovery of pure F-9 from a solution is hampered by hydrolysis of U)2F2 to give HF. The HF may be held back by addition of UO3 or CaO; the use of the latter, however, makes more difficult the recovery of all the F-9. Molar conductivities of UO2F2 solutions at 25 degrees, as well as the specific conductivities of a 1 molar solution containing various concentrations of UO3, have been determined. The addition of UO3 lowers the conductivity. The low …