Infrared Spectra of High Pressure Carbon Monoxide (open access)

Infrared Spectra of High Pressure Carbon Monoxide

We report infrared (IR) spectroscopic measurements of carbon monoxide (CO) at high pressures. Although CO is one of the simplest heteronuclear diatomic molecules, it displays surprisingly complex behavior at high pressures and has been the subject of several studies [1-5]. IR spectroscopic studies of high pressures phases of CO provide data complementing results from previous studies and elucidating the nature of these phases. Though a well-known and widely utilized diagnostic of molecular systems, IR spectroscopy presents several experimental challenges to high pressure diamond anvil cell research. We present measurements of the IR absorption bands of CO at high pressures and experimentally illustrate the crucial importance of accurate normalization of IR spectra specially within regions of strong absorptions in diamond.
Date: September 21, 2001
Creator: Evans, W. J.; Lipp, M. J. & Lorenzana, H. E.
Object Type: Article
System: The UNT Digital Library
Experimental verification of caustic-side solvent extraction for removal of cesium from tank waste. (open access)

Experimental verification of caustic-side solvent extraction for removal of cesium from tank waste.

The objectives of this report are: to demonstrate complete CSSX process flowsheet (proof of concept)--decontamination factor {ge} 40,000, and concentration factor {approx}15; Scientific and technical issues evaluated--stage efficiency, temperature control, hydraulic performance, long time (multi-day) operation, short-term shutdown, effect of solids, and recovery from Cs moving through strip section.
Date: September 21, 2001
Creator: Leonard, R. A.; Aase, S. B.; Arafat, H. A.; Chamberlain, D. B.; Conner, C.; Regalbuto, M. C. et al.
Object Type: Article
System: The UNT Digital Library
Precision Measurement of MUON G-2 and Accelerator Related Issues (open access)

Precision Measurement of MUON G-2 and Accelerator Related Issues

A precision measurement of the anomalous g value, a{sub {mu}}=(g-2)/2, for the positive muon has been made using high intensity protons available at the Brookhaven AGS. The result based on the 1999 data a{sub {mu}}=11659202(14)(6) x 10{sup 10} (1.3ppm) is in good agreement with previous measurements and has an error one third that of the combined previous data. The current theoretical value from the standard model is a{sub {mu}} (SM)=11659159.6(6.7) x 10{sup 10} (0.57 ppm) and differ by over 2.5 standard deviation with experiment. Issues with reducing systematic errors and enhancing the injection and storage efficiencies are discussed.
Date: September 21, 2001
Creator: Brown, H. N.; Bunce, G.; Carey, R. M.; Cushman, P.; Danby, G. T.; Debevec, P. T. et al.
Object Type: Article
System: The UNT Digital Library
Oak Ridge Multiple Attribute System (ORMAS) for Pu, HEU, HE, Chemical Agents, and Drugs (open access)

Oak Ridge Multiple Attribute System (ORMAS) for Pu, HEU, HE, Chemical Agents, and Drugs

The concept for the Oak Ridge Multiple Attribute System (ORMAS) is a Nuclear Materials Identification System (NMIS) time-dependent coincidence processor that incorporates gamma ray spectrometry and utilizes a small, lightweight, portable DT neutron (14.1 MeV) generator (1 x 10{sup 8} n/s), proton recoil scintillation detectors, and a gamma ray detector (HPGe). ORMAS is based on detecting fission neutrons and gamma rays from inherent source fission, fission induced by the external DT source, gamma ray detection of natural emissions of uranium and Pu, and induced gamma ray emission by the interaction of the 14.1 MeV neutrons from the DT source. This system is uniquely suited for detection of shielded highly enriched uranium (HEU), plutonium and other special nuclear materials, and detection of high explosives (HE), chemical agents, and in some cases, drugs. It could easily be adjusted to utilize a trusted processor that incorporates information barrier and authentication techniques using open software and then be useful in some international applications for materials whose characteristics may be classified. Since it is based entirely on commercially available components, the entire system, including the NMIS data acquisition boards, can be built with commercial off the shelf components (COTS). ORMAS incorporates the PINS technology of …
Date: September 21, 2001
Creator: Mihalczo, J.T.
Object Type: Report
System: The UNT Digital Library
Modeling the acceleration field and objective lens for an aberration corrected photoemission electron microscope (open access)

Modeling the acceleration field and objective lens for an aberration corrected photoemission electron microscope

None
Date: September 21, 2001
Creator: Feng, J.; Padmore, H.; Wei, D.H.; Anders, S.; Wu, Y.; Scholl, A. et al.
Object Type: Article
System: The UNT Digital Library
Modification of the Coherence Properties of a Laser Beam by a Plasma (open access)

Modification of the Coherence Properties of a Laser Beam by a Plasma

Spatial and temporal coherence is a fundamental property of laser beams. This peculiar quality is a problem for laser fusion because it induces spatial non uniformities of the laser intensity in the focal spot and it generates coherent coupling between the electromagnetic laser wave and the plasma waves. In the past many years, it has been shown that laser beam smoothing using different techniques (random phase plate, smoothing by spectral dispersion, polarization smoothing, ...) can reduce parametric and hydrodynamic instabilities which are detrimental processes to Inertial Confinement Fusion (ICF). More recently, it has been predicted theoretically and numerically that the laser beam coherence properties can be modified by the propagation of the laser beam through an underdense plasma. Recent experiments with the six-beam LULI laser facility demonstrate the effectiveness of this process through different diagnostics, give insight on its origin, and show some of its consequences on parametric instabilities.
Date: September 21, 2001
Creator: Labaune, C.; Fuchs, J.; Depierreaux, S.; Bandulet, H.; Michel, P. & Baldis, H. A.
Object Type: Article
System: The UNT Digital Library
Applications using a Picosecond 14.7 nm X-Ray Laser (open access)

Applications using a Picosecond 14.7 nm X-Ray Laser

We report recent application experiments on the LLNL COMET tabletop facility using the picosecond, 14.7 nm Ni-like Pd x-ray laser. This work includes measurements of a laser-produced plasma density profile with a diffraction grating interferometer.
Date: September 21, 2001
Creator: Dunn, J.; Smith, R. F.; Nilsen, J.; Shlyaptsev, V. N.; Filevich, J.; Rocca, J. J. et al.
Object Type: Article
System: The UNT Digital Library
One-Dimensional Heat Transfer Analysis For Thin Films With Applications In Inertial Fusion Energy (open access)

One-Dimensional Heat Transfer Analysis For Thin Films With Applications In Inertial Fusion Energy

The x-rays from inertial fusion energy micro explosions deposited in a thin film will lead to a temperature rise dependent on penetration depth and time duration. This temperature rise is important to the study of surface tension driven flows and the surface quality of films for optics. A one-dimensional heat transfer analysis is used to estimate the film temperature rise for several different cases applicable to both final optical surfaces and renewable liquid first walls. Attenuating gas mixtures of xenon and krypton are considered to mitigate the deposition of x-ray energy.
Date: September 21, 2001
Creator: Durbin, S G & Moir, R W
Object Type: Report
System: The UNT Digital Library
Application of a Dynamic Fuzzy Search Algorithm to Determine Optimal Wind Plant Sizes and Locations in Iowa (open access)

Application of a Dynamic Fuzzy Search Algorithm to Determine Optimal Wind Plant Sizes and Locations in Iowa

This paper illustrates a method for choosing the optimal mix of wind capacity at several geographically dispersed locations. The method is based on a dynamic fuzzy search algorithm that can be applied to different optimization targets. We illustrate the method using two objective functions for the optimization: maximum economic benefit and maximum reliability. We also illustrate the sensitivity of the fuzzy economic benefit solutions to small perturbations of the capacity selections at each wind site. We find that small changes in site capacity and/or location have small effects on the economic benefit provided by wind power plants. We use electric load and generator data from Iowa, along with high-quality wind-speed data collected by the Iowa Wind Energy Institute.
Date: September 21, 2001
Creator: Milligan, M. R., National Renewable Energy Laboratory & Factor, T., Iowa Wind Energy Institute
Object Type: Article
System: The UNT Digital Library
Position Paper on Sludge Batch 2 Qualification Strategy and Simulant Composition (open access)

Position Paper on Sludge Batch 2 Qualification Strategy and Simulant Composition

This report targets the sludge compositions used for glass testing (the ''Variability Study''), cold process simulation and makes recommendations as to sampling and qualification strategy.
Date: September 21, 2001
Creator: Elder, H.H.
Object Type: Report
System: The UNT Digital Library
Description of Fracture Systems for External Criticality Reports (open access)

Description of Fracture Systems for External Criticality Reports

The purpose of this Analysis/Model Report (AMR) is to describe probabilistically the main features of the geometry of the fracture system in the vicinity of the repository. They will be used to determine the quantity of fissile material that could accumulate in the fractured rock underneath a waste package as it degrades. This AMR is to feed the geochemical calculations for external criticality reports. This AMR is done in accordance with the technical work plan (BSC (Bechtel SAIC Company) 2001 b). The scope of this AMR is restricted to the relevant parameters of the fracture system. The main parameters of interest are fracture aperture and fracture spacing distribution parameters. The relative orientation of the different fracture sets is also important because of its impact on criticality, but they will be set deterministically. The maximum accumulation of material depends primarily on the fracture porosity, combination of the fracture aperture, and fracture intensity. However, the fracture porosity itself is not sufficient to characterize the potential for accumulation of a fracture system. The fracture aperture is also important because it controls both the flow through the fracture and the potential plugging of the system. Other features contributing to the void space such as …
Date: September 21, 2001
Creator: Nicot, Jean-Philippe
Object Type: Report
System: The UNT Digital Library
New York City Transit Diesel Hybrid Electric Buses (open access)

New York City Transit Diesel Hybrid Electric Buses

A description of diesel hybrid electric buses used at NYC Transit, the largest public transportation system in the United States. Clean fuel buses represent about 5% of NYC Transit's fleet.
Date: September 21, 2001
Creator: Eudy, L.
Object Type: Book
System: The UNT Digital Library
AUTOMATION FOR THE SYNTHESIS AND APPLICATION OF PET RADIOPHARMACEUTICALS. (open access)

AUTOMATION FOR THE SYNTHESIS AND APPLICATION OF PET RADIOPHARMACEUTICALS.

The development of automated systems supporting the production and application of PET radiopharmaceuticals has been an important focus of researchers since the first successes of using carbon-11 (Comar et al., 1979) and fluorine-18 (Reivich et al., 1979) labeled compounds to visualize functional activity of the human brain. These initial successes of imaging the human brain soon led to applications in the human heart (Schelbert et al., 1980), and quickly radiochemists began to see the importance of automation to support PET studies in humans (Lambrecht, 1982; Langstrom et al., 1983). Driven by the necessity of controlling processes emanating high fluxes of 511 KeV photons, and by the tedium of repetitive syntheses for carrying out these human PET investigations, academic and government scientists have designed, developed and tested many useful and novel automated systems in the past twenty years. These systems, originally designed primarily by radiochemists, not only carry out effectively the tasks they were designed for, but also demonstrate significant engineering innovation in the field of laboratory automation.
Date: September 21, 2001
Creator: Alexoff, D. L.
Object Type: Book
System: The UNT Digital Library
Experimental Plan for the Cold Demonstration (Scoping Tests) of Glass Removal Methods from a DWPF Melter (open access)

Experimental Plan for the Cold Demonstration (Scoping Tests) of Glass Removal Methods from a DWPF Melter

SRS and WVDP currently do not have the capability to size reduce, decontaminate, classify, and dispose of large, failed, highly contaminated equipment. Tanks Focus Area Task 777 was developed to address this problem. The first activity for Task 777 is to develop and demonstrate techniques suitable for removing the solid HLW glass from HLW melters. This experimental plan describes the work that will be performed for this glass removal demonstration.
Date: September 21, 2001
Creator: Smith, M.E.
Object Type: Report
System: The UNT Digital Library
Mixing Envelope D Sludge with LAW Intermediate Products with and without Glass Formers (open access)

Mixing Envelope D Sludge with LAW Intermediate Products with and without Glass Formers

The Department of Energy (DOE) Office of River Protection is in the process of designing a waste treatment system to process the Hanford Reservation High Level Waste (HLW). Envelope D sludge slurries will be blended with the concentrated Cs/Ts eluates, and the Sr/TRU intermediates separated from Envelope A, B, and C feeds. This study produced two washed simulated sludges (representing tanks 241-AZ-101 and 241-AZ-102 sludge), a Sr/TRU washed precipitate produced from tank 241-AN-107 simulant, and a concentrated blended eluate simulant based upon eluates from processing 241-AZ-102 supernate.
Date: September 21, 2001
Creator: Hansen, E.K.
Object Type: Report
System: The UNT Digital Library
Short-Term Output Variations in Wind Farms--Implications for Ancillary Services in the United States: Preprint (open access)

Short-Term Output Variations in Wind Farms--Implications for Ancillary Services in the United States: Preprint

With the advent of competition in the electric power marketplace, this paper reviews changes that affect wind and other renewable energy technologies, and discusses the role of federal and state policies in the recent wind installations in the United States. In particular, it reviews the implications of ancillary service requirements on a wind farm and presents initial operating results of monitoring one Midwest wind farm. Under federal energy policy, each generator must purchase, or otherwise provide for, ancillary services, such as dispatch, regulation, operation reserve, voltage regulation, and scheduling required to move power to load. As a renewable technology that depends on the forces of nature, short-term output variations are inherently greater for a wind farm than for a gas-fired combined cycle or a supercritical coal-fired unit.
Date: September 21, 2001
Creator: Cadogan, J.; Milligan, M.; Wan, Y. & Kirby, B.
Object Type: Article
System: The UNT Digital Library
Neutronics studies for a long-wavelength target station at SNS. (open access)

Neutronics studies for a long-wavelength target station at SNS.

The Spallation Neutron Source (SNS), under construction at Oak Ridge National Laboratory, will be the premier facility for neutron scattering studies in the United States. From the outset the SNS can achieve additional flexibility and accommodate a broader range of scientific investigation than would be possible with only the High Power Target Station by utilizing two target stations, each operating under a separate set of conditions and optimized for a certain class of instruments. A second target station, termed the Long-Wavelength Target Station (LWTS), would operate at a lower pulse rate (e.g., 10 vs. 60 Hz) and utilize very cold moderators to emphasize low-energy (long wavelength) neutrons. The LWTS concept discussed here obtains the highest low-energy fluxes possible for neutron scattering instruments by using a heavy-water-cooled solid tungsten target with two moderators in slab geometry and one in a front wing position. The primary focus has been on solid methane moderators, with liquid methane and hydrogen also considered. We used MCNPX to conduct a series of optimization and sensitivity studies to help determine the optimal neutronic parameters of the LWTS. We compared different options based on the thermal and epithermal fluxes as determined by fitting the spectral intensity of the …
Date: September 21, 2001
Creator: Micklich, B. J.; Iverson, E. B. & Carpenter, J. M.
Object Type: Article
System: The UNT Digital Library
Preliminary Dynamic Modeling of the Hanford Waste Treatment Plant Melter Offgas (open access)

Preliminary Dynamic Modeling of the Hanford Waste Treatment Plant Melter Offgas

This report documents preliminary versions of the models that include the components of the offgas systems from the melters through the exhaust stacks and the vessel ventilation systems. The models consider only the two major chemical species in the offgas stream: air and steam or water vapor. Model mass and energy balance calculations are designed to show the dynamic behavior of gas pressure and flow throughout the offgas systems in response to transient driving forces.
Date: September 21, 2001
Creator: Smith, F. G., III
Object Type: Report
System: The UNT Digital Library