In the separation of mixtures of radioactive iron and cobalt from neutron irradiated targets and in the removal of iron from cobalt targets for cyclotron production of radioiron, it is desirable to have a method superior to extraction from isopropyl ether in efficiency and ease of manipulation. Recent studies by Moore and Kraus on the separation of cobalt and nickel and on the behavior of iron in hydrochloric acid on Dowex-l resin in relation to the selective adsorption of chloride complexes of these elements have suggested the use of resin for the separation of iron and cobalt.