It has previously been shown that the polymer formed in solid state polymerization of acrylamide is amorphous in spite of the fact that the reaction takes place within a crystalline solid. The stage at which it becomes amorphous is not known at present. Work with dilute solid solutions of acrylamide in propionamide suggests that this occurs after the addition of, at most, a very few monomer units.

Preliminary experiments using acetylacetone in the presence of ethylenediaminetetraacetic acid to separate major quantities of beryllium from fission products are reported. Using 2M beryllium solutions, decontamination factors of the order of 10/sup 3/ were obtained with trace quantities of the more important fission products. This is sufficiently encouraging for the work to be repeated at higher activity levels.

This technical report describes development work done on zonal centrifuge systems at the Oak Ridge National Laboratory and the Oak Ridge Gaseous Diffusion Plant during the period July 1 to December 31, 1962 under the Joint National Institute for Health-Atomic Energy Commission Zonal Centrifuge Development Program. A basic purpose of this project is to develop new methods for isolating virus particles associated with cancerous cells and tissues. Three classes of rotor systems capable of separating particles ranging in size from whole animal or plant cells to protein or nucleic acid molecules on the basis of either sedimentation rate or density alone have been developed. Experiments with phage particles indicate the feasibility of large-scale virus isolation by continuous-flow centrifugation, followed by isopycnic banding in cesium chloride and velocity sedimentation in sucrose - all steps being carried out sequentially in the same rotor. Zonal rotors using the reorienting gradient principle for molecular separations have been tested to 141,000 rpm (formula). Previous work on zonal centrifugation and future plans for this program are discussed.

In calculating diffusion coefficients for gases diffusing from solids, the numerical solutions tabulated by Darken and Gurry, were found to lack the required precision, and the intervals between the arguments were too great to permit precise interpolations. Consequently the diffusion equation solutions of interest (diffusion from a sphere, cylinder, and plate, for the condition that the concentration of the diffusing species initially uniform) were re-evaluated. Computer programs for the three cases were written in FORTRAN for the IBM 7090. The solutions programmed are given in Crank. Values of the fractional completion were computed at approximately 0.01 increments, to the nearest 0.00001, and are tabulated in Table 1 to the nearest 0.0001. The table covers the fractional range from about 0.04 to 0.99. For smaller fractions satisfactory approximations are available. The table may be conveniently interpolated by plotting points about the region of interest and drawing a curve.

From introduction: "Evaluations to determine cause of fuel rods breakage following irradiation."

Report regarding an airborne radioactivity survey that took place in the 10,000 square mile area surrounding the National Reactor Testing Station in Idaho Falls, Idaho. Topics include the types of bedrock noted in the area as well as their levels of radioactivity.

From Introduction: "The principal objective of this study is to digest the experience accumulated in the operation of the demonstration plants, and from this information, to arrive at the cost of fresh water when produced on a large scale. It is important to recognize that the costs, as calculated in this report, are based upon the state of development of the processes as exemplified and proven in the demonstration plants. The field is new, and the rate of development is such that further cost reductions may be expected."

The angle by which a magnet deflects the trajectory of a particle in the x-z plane is proportional to the integral [integral not transcribed] taken over the trajectory wherever B≠0. Alternating gradient focusing is achieved by designing magnets so that I=I(x) varies linearly with x over a suitable x interval. Usually this is done by shaping the poles to give a linear variation of By with x while keeping the length of the magnet constant for different x. Certain advantaged may be gained by varying the effective length of the magnet with x and keeping By constant so that the integral varies properly with x. Figure 1 shows several such poles for which the trajectory length, and hence the integral (1), varies approximately from 2/3 to 4/3 of the mean value.

The amount by which the field of a magnet bends the path of a charged particle is proportional to the integral of Btds along the trajectory. Instead of making tedious point by point measurements of B in magnets and performing the integrations numerically, it has been found useful to measure directly, by using a search coil whose winding consists of long and narrow turns extending through the magnet gap from z1 and z2 in the direction of the trajectory. It should be noted that the integral Iy is taken along a straight x=constant, y=constant lines and not along the actual curved trajectory path; for small curvature the difference is small.

In discussing this subject, data on radiation induced mammary gland neoplasia in the rat indicating that direct interaction between the radiation and target tissue is necessary for maximum neoplasia induction will be presented mainly. Other types of radiation induced neoplasia, in which little or no information on the mechanisms involved is available, will be discussed briefly. In particular, investigations on radiation induced mouse lymphoma will be reviewed, in which neoplasia appears to be an abscopal effect. Implications of these data will be discussed, particularly with regard to possible mechanisms involved, and extrapolation to man.

The spectra of KHF2, KH2F3, NaH2F3, liquid and solid HF were measured between 1200 and 30 cm-1 by the inelastic scattering of "cold neutrons" (0.005e.v.). The spectrum of KHF2 is in agreement with previous infrared measurements and shows a peak at 147 mV corresponding to a deformation frequency v2 of the F-H-F group and a broad peak at 13 mV due to a libration of this group. The observed spectra for KH2F3, NaH2F3 solid and liquid HF were compared with that for KHF2 considering the known results that the F-F distance increases, the position of the H atom between the two fluorines becomes more asymmetrical, and the strength of the hydrogen bond decreases in going from the HF2- ion to H2F3- ion to HF. In this comparison the known structure of the H2F3- ion is considered as being intermediate between that of HF2- and the zig-zag hydrogen bonded chains in solid HF. As a result, the lines observed at 112 mV and 67 mV in the H2F3- spectra and in HF respectively are associated with the deformation frequency v2 of the H-F-H group in these compounds. In addition the spectra of H2F3- ions show a peak at a 15 mV …

Studies carried on since 1956 indicate that the prosaic breeding procedure of sibbing among the most perennial segregates in the hybrid of 4n maize x 4n perennial teosinte quickly restores perennialism to 50% maize tetraploids through increasing the expression of the rhizomatous habit under selection pressure. Similarly, only two generations of selection at the 75% maize level have resulted in a progressive recovery of the perennial expressive. A high degree of maize-likeness therefore appears to be compatible with the perennial expression at the 4n level.

From introduction: The main objective of the AGCRSP is to develop plans and specifications for a mobile nuclear power plant suitable for military field use.

Report investigating the compatibility of uranium carbide with tungsten, tantalum, molybdenum, Zircaloy-2, AISI 304L SS, Inconel, Hastelloy F, niobium-1% Zr, and niobium-33% Ta-1% Zr. These pairs were heated together at 1000 C and above for ten minutes.

Introduction: This is the third Quarterly Status Report of work under AEC Contract AT(04-3)-400, held by Stanford University. This contract provides for the construction of the Stanford Linear Accelerator Center (SLAC), a laboratory that will have as its chief instrument a two-mile-long linear electron accelerator.

Before discussing personnel monitoring of high energy radiations, it is appropriate to comment briefly on two basic methods of dosimetry applicable to such situations. In the first of these methods, one measures the rad dose in air with a tissue-equivalent ionization chamber that is operated with enough voltage on the collecting electrode to insure saturation even when the radiation is concentrated in short pulses, as is frequently the case. The linear energy transfer (LET) spectrum of the radiation is then determined and an average value of relative biological effectiveness (RBE) is determined. An experimental evaluation of the depth dose situation completes the data necessary for a full evaluation of the biological hazards. The method is completely general but is most applicable to situations where a substantial proportion of high energy components is present in the mixed radiation. It should be noted that the detailed composition of the radiation need not be known. Thus, components of dosage to which an RBE of 1 is assigned may be due to X-rays, gamma rays, or the ionization tracks produced by protons in the Gev energy range as well as by many other types of radiation. This method is applied frequently to the situation …

"Results of the continuing stratospheric flight test evaluation program for the Del Model I Electrostatic Precipitator Sampler and the Del Electrical Discharge Altimeter are described and discussed. Only one of four balloon launches reached floating altitude. The altimeter obtained an altitude recording consistent with concurrent aneroid barocoder readings. The reported gross gamma concentration for the precipitator sampler was approximates 25 and 80% higher than those of the two simultaneous direct flow filter samples. The completion of the design and construction of two prototype units of the Del Electrical Discharge Altimeter and their laboratory evaluation are described. A preliminary design concept is presented for an operational high volume electrostatic precipitator sampler to operate with high collection efficiency at an ambient flowrate of 500 cfm throughout the altitude range 100,000 to 150,000 ft."

From introduction: "Report summarizing all work completed during the preparation of design criteria for thermal flux loop."

From Summary: "The strains in the walls and ceiling of Cell No. 5 were recorded with 39 SR-4 strain gages strategically placed on reinforcing steel. Table I summarizes the comparative results without including correction for stress concentrations. The general pattern of cell behavior at 10 psig, as summarized in Table I, is shown in Figs. 10, 11, 12."

Map with graded color shading to show levels of naturally-occurring gamma aeroradioactivity within the Idaho National Reactor Texting Station Area. Details about the survey and map creation are printed at right. Scale 1:250,000.

It is appropriate that a conference devoted to the interactions of fast neutrons with nuclei begin with a survey of the available sources of such neutrons. Since its discovery in 1932, the neutron has provided a highly useful tool in attempts to understand the nucleus, and the types of nuclear phenomenon which could be studied and the nature of the results obtained are very dependent on the sources available.

Vacuum technology is germaine to and is utilized in an extroardinarily widespread scope of the scientific disciplines. From the medical technician freeze drying hog cholera vaccine to the solid state physicist studying thin film phenomena, vacuum technology is an important auxiliary. When one visits the NASA center at Langley and sees the clustered space environmental chambers, looking like a field of grotesque mushrooms, one realizes that vacuum technology is a vital adjunct in this most recent section of our total national scientific effort.

The major long lived activity induced in irradiated Pechiney and Brush BeO specimens is due to Se-46 arising from scandium present to the extent of about 1 p.p.m. The Brush specimens showed additional activities due to Fe-59 and Co-60 and to Cr-51. The levels of Cr-51 found are considerably higher than would be expected on the basis of stated chromium impurity levels suggesting that the chromium is introduced during handling of the samples on site. Approximate values of the dose rate are included.

The pioneer study by Benjamin and Sluka in 1908 on inhibition of antibody formation by X-rays revealed the importance of the temporal relationship between exposure to radiation and injection of antigen. X-radiation delivered three days before injection of beef serum inhibited precipitin formation in rabbits. A similar exposure to X-rays delivered three days after injection of the antigen failed to repress production of specific antibody. These observations were partially confirmed in 1915 when Hektoen reported inhibition of hemolysin production in the rat when X-radiation was delivered either before or after injection of sheep red cells. Although an absolute difference in radiosensitivity was not evident, the depressant effect of radiation on antibody production appeared to be less effective when radiation was given after injection of the antigen.