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Nuclear Resonance Fluorescence Excitations Near 2 MeV in 235U and 239Pu (open access)

Nuclear Resonance Fluorescence Excitations Near 2 MeV in 235U and 239Pu

A search for nuclear resonance fluorescence excitations in {sup 235}U and {sup 239}Pu within the energy range of 1.0- to 2.5-MeV was performed using a 4-MeV continuous bremsstrahlung source at the High Voltage Research Laboratory at the Massachusetts Institute of Technology. Measurements utilizing high purity Ge detectors at backward angles identified 9 photopeaks in {sup 235}U and 12 photopeaks in {sup 239}Pu in this energy range. These resonances provide unique signatures that allow the materials to be non-intrusively detected in a variety of environments including fuel cells, waste drums, vehicles and containers. The presence and properties of these states may prove useful in understanding the mechanisms for mixing low-lying collective dipole excitations with other states at low excitations in heavy nuclei.
Date: December 27, 2006
Creator: Bertozzi, W.; Caggiano, J. A.; Hensley, W. K.; Johnson, M. S.; Korbly, S. E.; Ledoux, R. J. et al.
System: The UNT Digital Library
Elevated Concentrations of Primordial Radionuclides in Sediments from the Reedy River and Surrounding Creeks in Simpsonville, South Carolina (open access)

Elevated Concentrations of Primordial Radionuclides in Sediments from the Reedy River and Surrounding Creeks in Simpsonville, South Carolina

A gamma-ray survey and analysis of sixteen riverbed samples from the Reedy River watershed near Simpsonville, SC were conducted and compared with national and international studies of primordial radionuclides. The study reported here follows on a recent discovery of anomalously high uranium concentrations in several private well waters in the area near Simpsonville, SC. A HPGe spectrometer was used for quantification of gamma emitting radionuclides in the sediments. All sediments contained radionuclides from the uranium and thorium series as well as {sup 40}K. Uranium-238 concentrations in sediment samples ranged from 11.1 to 74.2 Bq kg{sup -1}. The measured radionuclide concentrations were compared with data from UNSCEAR and NURE reports. The river and stream sediment data were augmented by in situ NaI(Tl) gamma-ray spectrometer measurements. Comparisons between the ex-situ and in-situ measurements indicate equivalently distributed uranium in the surface soils and stream sediments, the source of which is likely attributed to the monazite belts that are known to exist in the area.
Date: December 27, 2006
Creator: Powell, B. A.; Hughes, L. D.; Soreefan, A. M.; Falta, D.; Wall, M. & DeVol, T. A.
System: The UNT Digital Library