The following document describes data collected from a 14-month period of analyzing crustaceans containing radioactivity. Provided is information based on the change of radioactivity through seasonal changes.

Report describing the results of the cupferron extraction-copper spark method in determining the impurity elements in plutonium metal. This was required the 234-5 Project analytical program.

Report describing methods of determining trace impurities in plutonium in connection with the Metal Fabrication Process. The methods included are the cupferron extraction-copper spark method and the direct copper spark method.

In early July, 1958, it appeared that Columbia River temperature at HAPO would be near 24.5ºC by the end of August. River temperature were averaging 4º to 5º above 1957 figures and were 3º to 4º above the ten year highs. It seemed desirable to examine the problem to determine if any corrective measure could be taken, since it was apparent that production losses were imminent.

Apparent excessive concentrations of atmospheric contamination which were reported to be associated with an inert-gas-shielded consumable electrode arc wielding operation were studied to evaluate the potential health hazards. A study was made of the concentrations of metal fume and gaseous products of the operation as well as the spectrum of ultraviolet radiation. Recommendations for necessary controls were made.

The following report covers a test with the objective to demonstrate that the plutonium and uranium losses associated with the aluminum jacket dissolution could be reduced by substituting a water wash for the 5 per cent nitric acid wash following the coating removal and that this change would not adversely effect the product yield of decontamination in subsequent process steps.

In some engineering applications it has become necessary to operate equipment containing small diameter rods or tubes oriented parallel to flow stream. In the case of several nuclear reactors such as the Plutonium Recycle Test Reactor and the S. S. Savannah Maritime Reactor, bundles of small diameter rods are used as the fuel elements. The situation also has application to heat exchangers. A method for accurately predicting the pressure drop characteristics of various bundle configurations would be helpful in the design and selection of equipment. Some progress has been made toward gaining a greater knowledge of the bundle characteristics under low temperature conditions. This report includes the development of relationship for the effect of temperature on pressure drop.

Introduction: "A laboratory investigation of the relative corrosion resistance of several austenitic stainless steels to the RAW stream of the Tributyl Phosphate Waste Metal Recovery Process was made during the first quarter of 1950. The results of this investigation are reported herein; all original data are recorded in laboratory notebook HW-3282-T."

Introduction: "Room temperature and elevated temperature, static immersion and vapor suspicion, corrosion tests were conducted with Duriron, Hastelloy C, and tantalum in hydriotic acid and 234-5 project process supernatant solution (synthetic environments. The data relevant to these tests are contained herein."

The first series of tests in the KER-REP-1 loop proved that a fission product contaminated loop could be decontaminated to a safe level for contact maintenance. Since a good decontamination process was available, there was much that could be improved about this process. Further testing of this process and several variations of other processes have been scheduled. The evaluation of these processes includes specific decontamination factors, process corrosion, and loop activity reduction factors (loop decontamination factors).

The purpose of this procedure is to present a detailed, chronological presentation of the preliminary decontamination and post decontamination steps necessary to fulfill the requirements of the Production Test Authorization IP-239-N. The procedure attempts to present the required operation in sufficient detail to successfully accomplish the intent of the test. Certain procedures involve operations of a standard nature and have not been elaborated upon to any great extent, as it is expected that the reactor operations and radiation monitoring personnel will implement these instructions according to standard operating procedures.

The following report describes the process of the determination of nitrous oxide with the infrared spectrometer.

Objective: "Production Test 235-1 and an amendment, were written to outline the procedures for reducing the outgassing time and evaluating the effects of these reductions."

Introduction: "The problem of determining the properties and necessary controls on the TBP Plant waste disposal to eliminate transport line plugging and to permit higher concentration prior to return of this to the tank farms was studied. A report of preliminary findings was made to L. W. Finsh on January 31, 1953. This report compiles information in the aforementioned report and findings since its issuance. Previous studies related to this problem are summarized in the U. R. Technical Manual, HW-19140."

Hastelloy F is a prime contender as a material of construction for plant dissolvers in the power fuel reprocessing program. Consequently, the fabrication and installation of dissolver was undertaken to delineate any unknown problems associated with the use of Hastelloy F; and, at the same time, to provide a vessel for development studies on the Niflex or the Sulfex processes. The purpose of this report is to describe the actual basis for design as well as to present the problems encountered during the fabrication of the vessels.

Series of isothermal transformation studies for improvement in fabrication and reactor performance of uranium fuel elements.

In considering the problems associated with the measurement of SSNM content of Non-Production Fuels, two distinct problems are apparent. The first is the technical problem of obtaining highly accurate measurements in a complicated chemical and physical system. The second is the administrative problem of choosing a measurement system which provides a basic of financial settlement acceptable to both the seller (reactor operator) and the buyer (Commission).

Neutron attenuation in the old pile shields is dependent more and more on the slowing down characteristics of the iron as the hydrogen is baked out of the masonite. For neutrons above 1 or 2 Mev, iron does a good job by inelastic scattering. However, below this energy attenuation can be done only by the gradual moderation by elastic scattering to thermal energies with subsequent capture in the iron. Since iron is heavy and thus a poor moderator, there is a good possibility that many neutrons of intermediate energy will leak out of a burned out shield. Also, iron has a large dip in its cross section at 25 Kev which might allow a large burst of neutrons at this energy to leak out. Measurements using a lucite moderator with gold foil detectors indicate a large leakage of neutrons of intermediate energy, but interpretation of these measurements is difficult. These considerations prompted an attempt to get a rough idea of the energy distribution of the leakage neutrons through pure iron using a simple qualitative theory.

This report follows studies of the accumulation of beta omitting radioactive elements in Columbia River fish.

During normal operation the NPR will function as a closed system and the coolant will be maintained at a high degree of purity. Periodically, however, the system will have to be opened for fuel element discharge and/or decontamination. During these periods the reactor will be operated on single pass cooling. The use of deionized and deoxygenated water as the single pass coolant is not economically feasible due to the large quantities of coolant that will be required. At present it appears that filtered water will be used for this purpose. Since filtered water contains substantial amounts of dissolved solids (approximately 100 parts per million), and since it is saturated with air, this type of operation will have to be investigated with regard to corrosion problems. A particularly serious problem will be present after the system has been decontaminated, since the high temperature oxide films will have been removed and the bars metal surfaces will be exposed to the coolant.

A correlation between the optical densities if the Pb-Sn alloy system and UO2 with respect to Co^60 gamma radiation has been determined. This enables one to fabricate density standards of whatever geometry may be desired for one in the gamma absorptiometer by simply casting a Pb-Sn alloy of the proper composition to correspond to the density required.

The primary purpose of a cleanup system in a recirculating water loop is to maintain the best possible water quality conditions. This is normally accomplished by continuously purifying all or a portion of the coolant. A secondary objective of the cleanup system is to help maintain the system pH at a constant value. A system that will satisfactorily accomplish both of these objectives is at times difficult to obtain. Generally the pH control characteristics are sacrificed in favor of the more important cleanup requirements. A somewhat new approach to the problem pf cleanup system design appears to offer a solution to this problem for high pH systems.

This report follows work with the purposes of determining the minimum amount of nitric acid required to dissolve slurries of stored metal waste, determining the stability of such metastable solutions as a function of their chemical compositions - primarily acidity - versus time and temperature, and to define a feed suitable for a low-acid TBP process flowsheet, and to indicate the range of variations in composition which can be tolerated for plant operation.

The spatial distribution of thermal neutrons in a reactor lattices cell is of fundamental importance for many reasons. First of all, this information allows the determination of the relative absorption rates in each component of the cell which in turn enables a determination of the thermal utilization, and the diffusion length of the lattice. In addition, the observed spatial distributions of thermal neutrons in the lattice cell is of major interest in testing various approximations to the solution of the transport equation such as the P1 and P3 solutions.