The work described was undertaken to provide data for nuclear safety studies concerning NPF reprocessing equipment. The original objective was to determine the uranium density and water (hydrogen) content of UO2-H2O mixtures ranging from compact centrifuge cakes to dilute slurries. The scope was later expanded to include mixtures of UO2 with hydrocarbon oil and mixtures of UO3-H2O.

This report follows the study of the oxidation of plutonium III and IV to the plutonyl state.

This report discusses methods for preparing thin films of plutonium on metallic disks, which are used for alpha energy analysis, fission counting, and preparation of geometry standards in ordinary counting. Various methods of preparation were tested and analyzed, but electrodeposition was the most effective method. Deposition was then tested, but the yields were "somewhat erratic".

This report discusses properties of the Redox process. Density, apparent molar volumes and viscosity are all described.

Below Richland, Washington there is a gradual decrease in the concentration of beta particle emitters in the Columbia River water. The concentration of alpha particle emitters in Columbia River water averages 5 X 10⁻⁹ μl/ml at all locations. The activity of alpha particle emitters in mud samples was less than the detection limit of 3 x 10⁻⁶ μl/gm; the average activity density of beta particle emitters approximates those reported for the previous quarter.