A preliminary study has been made of a solid homogeneous reactor for stationary power plant application. The core consists of graphite spheres impregnated with uranium and thorium, and the coolant is bismuth. This concept possible offers advantages over other solid fuel reactor systems with respect to simplification of core structure, fuel fabrication and fuel handling, and reduction of fuel inventory external to the reactor. From the results of this preliminary study, it appears that the potential cost of electric power from this reactor is competitive with that from other reactor systems which have been proposed for the same application. The Po210 produced in the coolant presents a decontamination problem, but is also possibly a valuable by-producgt.

"General Chemistry investigations reported herein includes: (1) the Organic Coolant-Moderator Program, (2) investigations on zirconium hydride, and (3) analytical chemistry."

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"Heat production resulting from the absorption of gamma ray photons in thermal shields and the leakage of neutrons and photons from ferritic thermal shields are investigated. The gamma rays considered arise from three types of reactor radiation -- thermal neutrons, fast neutrons, and core and reflector gammas. The energy spectra of the fast neutron leakage and absorption have been investigated in some detail because of the significant contribution of fast neutrons to the heating of the concrete biological shield."

"A study has been made of the distribution of tracer fission products and plutonium between small samples of molten uranium and solid uranium oxide, carbine, and nitride. The distribution showed the same behavior i general for all three materials: 1. The rare earth elements, Cs, Ba, and Sr were extracted primarily into the solid scrub phase. 2. Zirconium and Nb partially concentrated in the scrub phase. 3. Plutonium, Mo, and Ru tended to remain completely in the metal phase. The distribution of activities agreed with trends predicted from the thermodynamic data. Uranium oxide appeared to be the most desirable scrub material for removing large amounts of fission products from the uranium while leaving beind the Pu. In addition the uranium metal was not severley contaminated by dissolved oxide."

"A series of thermal neutron diffusion length measurements has been made on non-multiplying lattice of lead-cadmium alloy rods in D2O. One-inch diameter rods in square lattice spacing of 4, 9, 6, 9, and 12 inches were used. Excellent agreement was found between theoretical and experimental values of the diffusion length. The analysis o the diffusion length measurement required a correction for the epithermal neutrons entering the exponential tank. These epithermal neutrons provided a distributed source of thermal neutrons upon slowing down in the lattice."

"Measurements of the intra-cell neutron flux distributing for a proposed Uranium Production Reactor have been made using a mock-up of a portion of the reactor core. Thermal neutron and thorium resonance neutron flux-distributions were investigated. As a result of the experimental measurements on the first mock-up, a decrease in thorium content appeared necessary in the reactor design studies. Experiments are now in progress on a second mock-up in which this change has been made."

"A method for solving multi-group reactor equations which arise in the diffusion approximation is outlined. Considerable work has been done on this problem at KAPL and ORNL. Their approach is to replace the differential equations by difference equations. Complications arise in this method where more than one slowing down medium is present since the fluxes are discontinuous at the interfaces. The primary purpose of this article is to develop an exact integral expression for the neutron flux which automatically satisfies the boundary conditions. An iterative method for obtaining the fluxes and critical neutron multiplication ratio based upon the above-mentioned integral expression is given. The only approximation used in obtaining the fluxes, in addition to the use of multi-group diffusion theory as the basic model, is the use of numerical integration to evaluate the analytic expression. The equations for a two region, two group spherical reactor are given in a form suitable for machine programing. The extension to more than two regions is also considered.

Introduction - The work of the Chemical Development Group has included studies on the thermal and radiation stability of organic materials suitable for reactor coolants, the thermal and radiation stability of zirconium hydride, reactor safety devices involving chemical systems, and general analytical development.

"Iodide-processed thorium foils were irradiated with 9-Mev protons at temperatures below -140 degrees C. the recover of electrical resistance upon annealing was studied in the range 0 degrees to 75 degrees where tempering curves showed rapid changes taking place. Determinations of the activation energy associated with this process were made and the mean value obtained was 1.22 ev. Correlations of this result have been made with those found previously for copper. From these comparisons, a tentative assignment of the motion of interstitial atoms in thorium has been made for this process. In addition, some evidence has been found which illustrates the corrosive action that water has on thorium at temperaturs as low as 0 degrees C."

"A design study is presented for a sodium cooked, graphite moderated power reactor utilizing low enrichment uranium fuel. The design is characterized by dependence on existing technology and the use of standard, or nearly standard, components. The reactor has a nominal rating of 167 thermal megawatts, and a plant comprising three such reactors for a total output of 500 thermal megawatts is described. Sodium in a secondary, non-radioactive, circulation system carries the heat to a steam generator at 910 degrees F and is returned at 420 degrees F. Steam conditions at the turbine throttle are 600 psig and 825 degrees F. Cost of the complete reactor power plant, consisting of the three reactors, and on 150-megawatt turbogenerator, is estimated to be approximately $43,165,000."