Resource Type

ANL Critical Assembly Covariance Matrix Generation (open access)

ANL Critical Assembly Covariance Matrix Generation

This report discusses the generation of a covariance matrix for selected critical assemblies that were carried out by Argonne National Laboratory (ANL) using four critical facilities - all of which are now decommissioned.
Date: January 15, 2014
Creator: McKnight, R. D. & Grimm, K. N. (Nuclear Engineering Division)
System: The UNT Digital Library
KONGMING: Performance Prediction in the Cloud via Multidimensional Interference Surrogates (open access)

KONGMING: Performance Prediction in the Cloud via Multidimensional Interference Surrogates

None
Date: January 15, 2014
Creator: Bowen, Z; Bronevetsky, G; Casas-Guix, M & Bagchi, S
System: The UNT Digital Library
Investigation of WO{sub 3}-Based H{sub 2}S Sensor Materials for Coal Gasification Systems (open access)

Investigation of WO{sub 3}-Based H{sub 2}S Sensor Materials for Coal Gasification Systems

The aim of this project was to engineer the materials studied to enhance the so-called 3S criteria: Sensitivity, Selectivity, and Stability, by using the advantage of controlling structure and properties at nanometer dimensions. It targeted sensor materials that are able to detect poisonous gases resulting from coal-gasification processes, especially sulfur containing emissions. Research findings based on this award demonstrate that doping tungsten oxide (WO{sub 3}) with a small amount of Ti (e.g. 5% in our work) results in a new material that has a higher structural symmetry (e.g. tetragonal morphology) as well as narrower crystalline particle size distribution. As high quality materials with excellent ordered structure and narrower particle-size distributions (which can also withstand high-temperature technological environments such as those encountered in furnaces and coal gasification systems without their structure being affected by phase transformations) are needed for developing new, more sensitive sensor materials, W-Ti-O thin films grown by RF sputtering are valuable candidates for such roles. It is well known that pure WO{sub 3} will change its structure at elevated temperatures. Our work indicates that, Ti doping not only increases the stability of the resultant material by promoting structural phase modifications, but also increases its sensitivity by increasing the …
Date: December 15, 2013
Creator: Manciu, Felicia & Ramana, Chintalapalle
System: The UNT Digital Library
Final report for DOE Grant No. DE-SC0006609 - Persistence of Microbially Facilitated Calcite Precipitation as an in situ Treatment for Strontium-90 (open access)

Final report for DOE Grant No. DE-SC0006609 - Persistence of Microbially Facilitated Calcite Precipitation as an in situ Treatment for Strontium-90

Subsurface radionuclide and metal contaminants throughout the U.S. Department of Energy (DOE) complex pose one of DOE?s greatest challenges for long-term stewardship. One promising stabilization mechanism for divalent ions, such as the short-lived radionuclide Sr-90, is co-precipitation in calcite. We have previously found that nutrient addition can stimulate microbial ureolytic activity, that this activity accelerates calcite precipitation and co-precipitation of Sr, and that higher calcite precipitation rates can result in increased Sr partitioning. We have conducted integrated field, laboratory, and computational research to evaluate the relationships between ureolysis and calcite precipitation rates and trace metal partitioning under environmentally relevant conditions, and investigated the coupling between flow/flux manipulations and precipitate distribution. A field experimental campaign conducted at the Integrated Field Research Challenge (IFRC) site located at Rifle, CO was based on a continuous recirculation design; water extracted from a down-gradient well was amended with urea and molasses (a carbon and electron donor) and re-injected into an up-gradient well. The goal of the recirculation design and simultaneous injection of urea and molasses was to uniformly accelerate the hydrolysis of urea and calcite precipitation over the entire inter-wellbore zone. The urea-molasses recirculation phase lasted, with brief interruptions for geophysical surveys, for 12 days …
Date: November 15, 2013
Creator: Smith, Robert W. & Fujita, Yoshiko
System: The UNT Digital Library
UV Excited Photoacoustic Raman (open access)

UV Excited Photoacoustic Raman

None
Date: November 15, 2013
Creator: Carter, J; Chambers, D; Steele, P; Haugen, P & Heller, D
System: The UNT Digital Library
Alternatives to the Maroni Process for Tritium Recovery in Fusion Reactors: Avoiding Volatile Hydrogen Fluoride and High-Temperature High-Speed Rotating Machinery (open access)

Alternatives to the Maroni Process for Tritium Recovery in Fusion Reactors: Avoiding Volatile Hydrogen Fluoride and High-Temperature High-Speed Rotating Machinery

None
Date: October 15, 2013
Creator: Farmer, J.; El-Dasher, B.; Bandhauer, T.; Rubenchik, A.; Reyes, S.; Dunne, M. et al.
System: The UNT Digital Library
Architecture-Aware Algorithms for Scalable Performance and Resilience on Heterogeneous Architectures (open access)

Architecture-Aware Algorithms for Scalable Performance and Resilience on Heterogeneous Architectures

The goal of the Extreme-scale Algorithms & Software Institute (EASI) is to close the �application-architecture performance gap� by exploring algorithms and runtime improvements that will enable key science applications to better exploit the architectural features of DOE extreme-scale systems. For the past year of the project, our efforts at the University of Tennessee have concentrated on, and made significant progress related to, the following high-level EASI goals: � Develop multi-precision and architecture-aware implementations of Krylov, Poisson, Helmholtz solvers, and dense factorizations for heterogeneous multi-core systems; � Explore new methods of algorithm resilience, and develop new algorithms with these capabilities; � Develop runtime support for adaptable algorithms that are dealing with resilience, scalability; � Distribute the new algorithms and runtime support through widely used software packages; � Establish a strong outreach program to disseminate results, interact with colleagues and train students and junior members of our community.
Date: October 15, 2013
Creator: Dongarra, Jack
System: The UNT Digital Library
Final Report: Large-Scale Optimization for Bayesian Inference in Complex Systems (open access)

Final Report: Large-Scale Optimization for Bayesian Inference in Complex Systems

The SAGUARO (Scalable Algorithms for Groundwater Uncertainty Analysis and Robust Optimiza- tion) Project focuses on the development of scalable numerical algorithms for large-scale Bayesian inversion in complex systems that capitalize on advances in large-scale simulation-based optimiza- tion and inversion methods. Our research is directed in three complementary areas: efficient approximations of the Hessian operator, reductions in complexity of forward simulations via stochastic spectral approximations and model reduction, and employing large-scale optimization concepts to accelerate sampling. Our efforts are integrated in the context of a challenging testbed problem that considers subsurface reacting flow and transport. The MIT component of the SAGUARO Project addresses the intractability of conventional sampling methods for large-scale statistical inverse problems by devising reduced-order models that are faithful to the full-order model over a wide range of parameter values; sampling then employs the reduced model rather than the full model, resulting in very large computational savings. Results indicate little effect on the computed posterior distribution. On the other hand, in the Texas-Georgia Tech component of the project, we retain the full-order model, but exploit inverse problem structure (adjoint-based gradients and partial Hessian information of the parameter-to- observation map) to implicitly extract lower dimensional information on the posterior distribution; …
Date: October 15, 2013
Creator: Ghattas, Omar
System: The UNT Digital Library
Future Automotive Aftertreatment Solutions: The 150°C Challenge Workshop Report (open access)

Future Automotive Aftertreatment Solutions: The 150°C Challenge Workshop Report

With future fuel economy standards enacted, the U.S. automotive manufacturers (OEMs) are committed to pursuing a variety of high risk/highly efficient stoichiometric and lean combustion strategies to achieve superior performance. In recognition of this need, the U.S. Department of Energy (DOE) has partnered with domestic automotive manufacturers through U.S. DRIVE to develop these advanced technologies. However, before these advancements can be introduced into the U.S. market, they must also be able to meet increasingly stringent emissions requirements. A significant roadblock to this implementation is the inability of current catalyst and aftertreatment technologies to provide the required activity at the much lower exhaust temperatures that will accompany highly efficient combustion processes and powertrain strategies. Therefore, the goal of this workshop and report is to create a U.S. DRIVE emission control roadmap that will identify new materials and aftertreatment approaches that offer the potential for 90% conversion of emissions at low temperature (150°C) and are consistent with highly efficient combustion technologies currently under investigation within U.S. DRIVE Advanced Combustion and Emission Control (ACEC) programs.
Date: October 15, 2013
Creator: Zammit, Michael; DiMaggio, Craig L.; Kim, Chang H.; Lambert, Christine; Muntean, George G.; Peden, Charles HF et al.
System: The UNT Digital Library
Integrated Genome-Based Studies of Shewanella Ecophysiology (open access)

Integrated Genome-Based Studies of Shewanella Ecophysiology

This project had as its goals the understanding of the ecophysiology of the genus Shewanella using various genomics approaches. As opposed to other programs involving Shewanella, this one branched out into the various areas in which Shewanella cells are active, and included both basic and applied studies. All of the work was, to some extent, related to the ability of the bacteria to accomplish electron exchange between the cell and solid state electron acceptors and/or electron donors, a process we call Extracellular Electron Transport, or EET. The major accomplishments related to several different areas: Basic Science Studies: 1. Genetics and genomics of nitrate reduction, resulting in elucidation of atypical nitrate reduction systems in Shewanella oneidensis (MR-1)[2]. 2. Influence of bacterial strain and growth conditions on iron reduction, showing that rates of reduction, extents of reduction, and the formation of secondary minerals were different for different strains of Shewanella [3,4,9]. 3. Comparative genomics as a tool for comparing metabolic capacities of different Shewanella strains, and for predicting growth and metabolism [6,10,15]. In these studies, collaboration with ORNL, PNNL, and 4. Basic studies of electron transport in strain MR-1, both to poised electrodes, and via conductive nanowires [12,13]. This included the first …
Date: October 15, 2013
Creator: Nealson, Kenneth H.
System: The UNT Digital Library
Polarimetry at RHIC: RHIC polarized beam in Run 2011 (open access)

Polarimetry at RHIC: RHIC polarized beam in Run 2011

N/A
Date: October 15, 2013
Creator: Zelenski, A.
System: The UNT Digital Library
Radionuclide Retention in Concrete Wasteforms - FY13 (open access)

Radionuclide Retention in Concrete Wasteforms - FY13

Assessing long-term performance of Category 3 waste cement grouts for radionuclide encasement requires knowledge of the radionuclide-cement interactions and mechanisms of retention (i.e., sorption or precipitation); the mechanism of contaminant release; the significance of contaminant release pathways; how wasteform performance is affected by the full range of environmental conditions within the disposal facility; the process of wasteform aging under conditions that are representative of processes occurring in response to changing environmental conditions within the disposal facility; the effect of wasteform aging on chemical, physical, and radiological properties; and the associated impact on contaminant release. This knowledge will enable accurate prediction of radionuclide fate when the wasteforms come in contact with groundwater. Data collected throughout the course of this work will be used to quantify the efficacy of concrete wasteforms, similar to those used in the disposal of low-level waste and mixed low-level waste, for the immobilization of key radionuclides (i.e., uranium, technetium, and iodine). Data collected will also be used to quantify the physical and chemical properties of the concrete affecting radionuclide retention.
Date: October 15, 2013
Creator: Snyder, Michelle MV; Golovich, Elizabeth C.; Wellman, Dawn M.; Crum, Jarrod V.; Lapierre, Robert; Dage, Denomy C. et al.
System: The UNT Digital Library
The RHIC polarized source upgrade (open access)

The RHIC polarized source upgrade

N/A
Date: October 15, 2013
Creator: A., Zelenski; Atoian, G.; Ritter, J.; Steski, D.; Davydenko, V.; Ivanov, A. et al.
System: The UNT Digital Library
WET-NZ Multi-Mode Wave Energy Converter Advancement Project (open access)

WET-NZ Multi-Mode Wave Energy Converter Advancement Project

The overall objective of the project was to verify the ocean wavelength functionality of the WET-NZ through targeted hydrodynamic testing at wave tank scale and controlled open sea deployment of a 1/2 scale (1:2) experimental device. This objective was accomplished through a series of tasks designed to achieve four specific goals: Wave Tank Testing to Characterize Hydrodynamic Characteristics;  Open-Sea Testing of a New 1:2 Scale Experimental Model;  Synthesis and Analysis to Demonstrate and Confirm TRL5/6 Status;  Market Impact & Competitor Analysis, Business Plan and Commercialization Strategy.
Date: October 15, 2013
Creator: Kopf, Steven
System: The UNT Digital Library
Assessment of Energy Production Potential from Ocean Currents along the United States Coastline (open access)

Assessment of Energy Production Potential from Ocean Currents along the United States Coastline

Increasing energy consumption and depleting reserves of fossil fuels have resulted in growing interest in alternative renewable energy from the ocean. Ocean currents are an alternative source of clean energy due to their inherent reliability, persistence and sustainability. General ocean circulations exist in the form of large rotating ocean gyres, and feature extremely rapid current flow in the western boundaries due to the Coriolis Effect. The Gulf Stream system is formed by the western boundary current of the North Atlantic Ocean that flows along the east coastline of the United States, and therefore is of particular interest as a potential energy resource for the United States. This project created a national database of ocean current energy resources to help advance awareness and market penetration in ocean current energy resource assessment. The database, consisting of joint velocity magnitude and direction probability histograms, was created from data created by seven years of numerical model simulations. The accuracy of the database was evaluated by ORNL?s independent validation effort documented in a separate report. Estimates of the total theoretical power resource contained in the ocean currents were calculated utilizing two separate approaches. Firstly, the theoretical energy balance in the Gulf Stream system was examined …
Date: September 15, 2013
Creator: Haas, Kevin
System: The UNT Digital Library
High Efficiency Integrated Package (open access)

High Efficiency Integrated Package

Solid-state lighting based on LEDs has emerged as a superior alternative to inefficient conventional lighting, particularly incandescent. LED lighting can lead to 80 percent energy savings; can last 50,000 hours – 2-50 times longer than most bulbs; and contains no toxic lead or mercury. However, to enable mass adoption, particularly at the consumer level, the cost of LED luminaires must be reduced by an order of magnitude while achieving superior efficiency, light quality and lifetime. To become viable, energy-efficient replacement solutions must deliver system efficacies of ≥ 100 lumens per watt (LPW) with excellent color rendering (CRI > 85) at a cost that enables payback cycles of two years or less for commercial applications. This development will enable significant site energy savings as it targets commercial and retail lighting applications that are most sensitive to the lifetime operating costs with their extended operating hours per day. If costs are reduced substantially, dramatic energy savings can be realized by replacing incandescent lighting in the residential market as well. In light of these challenges, Cree proposed to develop a multi-chip integrated LED package with an output of > 1000 lumens of warm white light operating at an efficacy of at least 128 …
Date: September 15, 2013
Creator: Ibbetson, James
System: The UNT Digital Library
COMPARISON OF RESULTS FOR QUARTER 4 SURFACE WATER SPLIT SAMPLES COLLECTED AT THE NUCLEAR FUELS SERVICES SITE, ERWIN, TN (open access)

COMPARISON OF RESULTS FOR QUARTER 4 SURFACE WATER SPLIT SAMPLES COLLECTED AT THE NUCLEAR FUELS SERVICES SITE, ERWIN, TN

Oak Ridge Associated Universities (ORAU), under the Oak Ridge Institute for Science and Education (ORISE) contract, collected split surface water samples with Nuclear Fuel Services (NFS) representatives on June 12, 2013. Representatives from the U.S. Nuclear Regulatory Commission (NRC) and the Tennessee Department of Environment and Conservation were also in attendance. Samples were collected at four surface water stations, as required in the approved Request for Technical Assistance number 11-018. These stations included Nolichucky River upstream (NRU), Nolichucky River downstream (NRD), Martin Creek upstream (MCU), and Martin Creek downstream (MCD). Both ORAU and NFS performed gross alpha and gross beta analyses, and Table 1 presents the comparison of results using the duplicate error ratio (DER), also known as the normalized absolute difference. A DER ≤ 3 indicates at a 99% confidence interval that split sample results do not differ significantly when compared to their respective one standard deviation (sigma) uncertainty (ANSI N42.22). The NFS split sample report specifies 95% confidence level of reported uncertainties (NFS 2013). Therefore, standard two sigma reporting values were divided by 1.96. In conclusion, most DER values were less than 3 and results are consistent with low (e.g., background) concentrations. The gross beta result for sample …
Date: August 15, 2013
Creator: unknown
System: The UNT Digital Library
Development of Molten-Salt Heat Transfer Fluid Technology for Parabolic Trough Solar Power Plants - Public Final Technical Report (open access)

Development of Molten-Salt Heat Transfer Fluid Technology for Parabolic Trough Solar Power Plants - Public Final Technical Report

Executive Summary This Final Report for the "Development of Molten-Salt Heat Transfer Fluid (HTF) Technology for Parabolic Trough Solar Power Plants” describes the overall project accomplishments, results and conclusions. Phase 1 analyzed the feasibility, cost and performance of a parabolic trough solar power plant with a molten salt heat transfer fluid (HTF); researched and/or developed feasible component options, detailed cost estimates and workable operating procedures; and developed hourly performance models. As a result, a molten salt plant with 6 hours of storage was shown to reduce Thermal Energy Storage (TES) cost by 43.2%, solar field cost by 14.8%, and levelized cost of energy (LCOE) by 9.8% - 14.5% relative to a similar state-of-the-art baseline plant. The LCOE savings range met the project’s Go/No Go criteria of 10% LCOE reduction. Another primary focus of Phase 1 and 2 was risk mitigation. The large risk areas associated with a molten salt parabolic trough plant were addressed in both Phases, such as; HTF freeze prevention and recovery, collector components and piping connections, and complex component interactions. Phase 2 analyzed in more detail the technical and economic feasibility of a 140 MWe,gross molten-salt CSP plant with 6 hours of TES. Phase 2 accomplishments included …
Date: August 15, 2013
Creator: Grogan, Dylan C. P.
System: The UNT Digital Library
Hydrogen Concentration in the Inner-Most Container within a Pencil Tank Overpack Packaged in a Standard Waste Box Package (open access)

Hydrogen Concentration in the Inner-Most Container within a Pencil Tank Overpack Packaged in a Standard Waste Box Package

The purpose of this report is to evaluate hydrogen generation within Pencil Tank Overpacks (PTO) in a Standard Waste Box (SWB), to establish plutonium (Pu) limits for PTOs based on hydrogen concentration in the inner-most container and to establish required configurations or validate existing or proposed configurations for PTOs. The methodology and requirements are provided in this report.
Date: August 15, 2013
Creator: Marusich, Robert M.
System: The UNT Digital Library
Technoeconomic Evaluation of MEA versus Mixed Amines for CO2 Removal at Near-Commercial Scale at Duke Energy Gibson 3 Plant (open access)

Technoeconomic Evaluation of MEA versus Mixed Amines for CO2 Removal at Near-Commercial Scale at Duke Energy Gibson 3 Plant

None
Date: August 15, 2013
Creator: Jones, D. A.; McVey, T. & Friedmann, S. J.
System: The UNT Digital Library
THERMAL PERFORMANCE SENSITIVITY STUDIES IN SUPPORT OF MATERIAL MODELING FOR EXTENDED STORAGE OF USED NUCLEAR FUEL (open access)

THERMAL PERFORMANCE SENSITIVITY STUDIES IN SUPPORT OF MATERIAL MODELING FOR EXTENDED STORAGE OF USED NUCLEAR FUEL

The work reported here is an investigation of the sensitivity of component temperatures of a storage system, including fuel cladding temperatures, in response to age-related changes that could degrade the design-basis thermal behavior of the system. Three specific areas of interest were identified for this study. • degradation of the canister backfill gas from pure helium to a mixture of air and helium, resulting from postulated leakage due to stress corrosion cracking (SCC) of canister welds • changes in surface emissivity of system components, resulting from corrosion or other aging mechanisms, which could cause potentially significant changes in temperatures and temperature distributions, due to the effect on thermal radiation exchange between components • changes in fuel and basket temperatures due to changes in fuel assembly position within the basket cells in the canister The purpose of these sensitivity studies is to provide a realistic example of how changes in the physical properties or configuration of the storage system components can affect temperatures and temperature distributions. The magnitudes of these sensitivities can provide guidance for identifying appropriate modeling assumptions for thermal evaluations extending long term storage out beyond 50, 100, 200, and 300 years.
Date: August 15, 2013
Creator: Cuta, Judith M.; Suffield, Sarah R.; Fort, James A. & Adkins, Harold E.
System: The UNT Digital Library
ADVANCE System Requirements (open access)

ADVANCE System Requirements

N/A
Date: July 15, 2013
Creator: Brown, D. A.; Arcilla, R. & Herman, M.
System: The UNT Digital Library
Analysis Of 2H-Evaporator Scale Pot Bottom Sample [HTF-13-11-28H] (open access)

Analysis Of 2H-Evaporator Scale Pot Bottom Sample [HTF-13-11-28H]

Savannah River Remediation (SRR) is planning to remove a buildup of sodium aluminosilicate scale from the 2H-evaporator pot by loading and soaking the pot with heated 1.5 M nitric acid solution. Sampling and analysis of the scale material from the 2H evaporator has been performed so that the evaporator can be chemically cleaned beginning July of 2013. Historically, since the operation of the Defense Waste Processing Facility (DWPF), silicon in the DWPF recycle stream combines with aluminum in the typical tank farm supernate to form sodium aluminosilicate scale mineral deposits in the 2H-evaporator pot and gravity drain line. The 2H-evaporator scale samples analyzed by Savannah River National Laboratory (SRNL) came from the bottom cone sections of the 2H-evaporator pot. The sample holder from the 2H-evaporator wall was virtually empty and was not included in the analysis. It is worth noting that after the delivery of these 2H-evaporator scale samples to SRNL for the analyses, the plant customer determined that the 2H evaporator could be operated for additional period prior to requiring cleaning. Therefore, there was no need for expedited sample analysis as was presented in the Technical Task Request. However, a second set of 2H evaporator scale samples were expected …
Date: July 15, 2013
Creator: Oji, L. N.
System: The UNT Digital Library
Final Scientific/Technical Report Development of Large-Area Photo-Detectors (open access)

Final Scientific/Technical Report Development of Large-Area Photo-Detectors

This proposal requested ADR funds for two years to make measurements and detector proto-types in the context of planning a program in conjunction with Argonne National Laboratory to develop very large-area planar photodetectors. The proposed detectors have integrated transmission-line readout and sampling electronics able to achieve timing and position resolutions in the range of 1-50 psec and 1-10 mm, respectively. The capability for very precise time measurements is inherent in the design, and provides a �third� coordinate, orthogonal to the two in the plane, for the point of origin of photons or charged particles, allowing �tomographic� reconstruction in 3-dimensions inside a volume.
Date: July 15, 2013
Creator: Frisch, Henry J.
System: The UNT Digital Library