Water that forms the Florida Current, and eventually the Gulf Stream, coalesces in the Caribbean from both subtropical and equatorial sources. The equatorial sources are made up of, in part, South Atlantic water moving northward and compensating for southward flow at depth related to meridional overturning circulation. Subtropical surface water contains relatively high amounts of radiocarbon ({sup 14}C), whereas equatorial waters are influenced by the upwelling of low {sup 14}C water and have relatively low concentrations of {sup 14}C. We use a 250-year record of {Delta}{sup 14}C in a coral from southwestern Puerto Rico along with previously published coral {Delta}{sup 14}C records as tracers of subtropical and equatorial water mixing in the northern Caribbean. Data generated in this study and from other studies indicate that the influence of either of the two water masses can change considerably on interannual to interdecadal time scales. Variability due to ocean dynamics in this region is large relative to variability caused by atmospheric {sup 14}C changes, thus masking the Suess effect at this site. A mixing model produced using coral {Delta}{sup 14}C illustrates the time varying proportion of equatorial versus subtropical waters in the northern Caribbean between 1963 and 1983. The results of the …

Silicon carbide (SiC) fibers made by chemical vapor deposition (CVD) are of interest for organic, ceramic, and metal matrix composite materials due their high strength, high elastic modulus, and retention of mechanical properties at elevated processing and operating temperatures. The properties of SCS-6{trademark} silicon carbide fibers, which are made by a commercial process and consist largely of stoichiometric SiC, were compared with an experimental carbon-rich CVD SiC fiber, to which excess carbon was added during the CVD process. The concentration, homogeneity, and distribution of carbon were measured using energy dispersive x-ray spectroscopy (SEM/EDS). The effect of excess carbon on the tensile strength, elastic modulus, and the crystallographic and microstructural properties of CVD silicon carbide fibers was investigated using tensile testing, x-ray diffraction, scanning electron microscopy (SEM), and transmission electron microscopy (TEM).

Laboratory studies demonstrate that fractional crystallization is a viable process for separating Hanford medium-curie waste into high-curie and low-curie fractions. The product salt from the crystallization process qualifies as low-curie feed to a supplemental treatment system (e.g., bulk vitrification). The high-curie raffinate is returned to the double-shell tank system, eventually to be sent as feed to the Waste Treatment and Immobilization Plant. Process flowsheet tests were designed with the aid of thermodynamic chemical modeling. Laboratory equipment design and test procedures were developed using simulated tank waste samples. Proof-of-concept flowsheet tests were carried out in a shielded hot cell using actual tank waste samples. Data from both simulated waste tests and actual tank waste tests demonstrate that the process exceeded all of the separation criteria established for the program.

We present a set of UBV RIzJHKs photometry for 745 J +H band selected objects in a 22:5{prime} x 29:2{prime} region centered on the core of the Coma cluster. This includes 516 galaxies and is at least 80% complete to H = 16, with a spectroscopically complete sample of 111 cluster members (nearly all with morphological classification) for H < 14:5. For each object we present total Kron (1980) magnitudes and aperture photometry. As an example, we use these data to derive color-magnitude relations for Coma early-type galaxies, measure the intrinsic scatter of these relations and its dependence on galaxy mass, and address the issue of color gradients. We find that the color gradients are mild and that the intrinsic scatter about the color-magnitude relation is small ({approx} 0:05 mag in U-V and less than {approx} 0:03 in B-R, V-I, or J-K). There is no evidence that the intrinsic scatter varies with galaxy luminosity, suggesting that the cluster red sequence is established at early epochs over a range of {approx} 100 in stellar mass.

In theories with multiple vacua, reheating to a temperature greater than the height of a barrier can stimulate transitions from a desirable metastable vacuum to a lower energy state. We discuss the constraints this places on various theories and demonstrate that in a class of supersymmetric models this transition does not occur even for arbitrarily high reheating temperature.

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During the last 50 years, a large amount of information on radionuclide accumulators or 'sentinel-type' organisms in the environment has been published. Much of this work focused on the risks of food-chain transfer of radionuclides to higher organisms such as reindeer and man. However, until the 1980's and 1990's, there has been little published data on the radiocesium ({sup 134}Cs and {sup 137}Cs) accumulation by mushrooms. This presentation will consist of a review of the published data for {sup 134,137}Cs accumulation by mushrooms in nature. The review will consider the time of sampling, sample location characteristics, the radiocesium source term and other aspects that promote {sup 134,137}Cs uptake by mushrooms. This review will focus on published data for mushrooms that demonstrate a large propensity for use in the environmental biomonitoring of radiocesium contamination. It will also provide photographs and descriptions of habitats for many of these mushrooms to facilitate their collection for biomonitoring.

If the cosmic dark matter consists of weakly-interacting massive particles, these particles should be produced in reactions at the nextgeneration of high-energy accelerators. Measurements at these accelerators can then be used to determine the microscopic properties of the dark matter. From this, we can predict the cosmic density, the annihilation cross sections, and the cross sections relevant to direct detection. In this paper, we present studies in supersymmetry models with neutralino dark matter that give quantitative estimates of the accuracy that can be expected. We show that these are well matched to the requirements of anticipated astrophysical observations of dark matter. The capabilities of the proposed International Linear Collider (ILC) are expected to play a particularly important role in this study.

The complexation of plutonium(IV) with sulfate at variable temperatures has been investigated by solvent extraction method. A NaBrO{sub 3} solution was used as holding oxidant to maintain the plutonium(IV) oxidation state throughout the experiments. The distribution ratio of Pu(IV) between the organic and aqueous phases was found to decrease as the concentrations of sulfate were increased. Stability constants of the 1:1 and 1:2 Pu(IV)-HSO{sub 4}{sup -} complexes, dominant in the aqueous phase, were calculated from the effect of [HSO{sub 4}{sup -}] on the distribution ratio. The enthalpy and entropy of complexation were calculated from the stability constants at different temperatures using the Van't Hoff equation.

A dual-cathode arc plasma source was combined with acomputer-controlled bias amplifier such as to synchronize substrate biaswith the pulsed production of plasma. In this way, bias can be applied ina material-selective way. The principle has been applied to the synthesismetal-doped diamond-like carbon films, where the bias was applied andadjusted when the carbon plasma was condensing, and the substrate was atground when the metal was incorporated. In doing so, excessive sputteringby too-energetic metal ions can be avoided while the sp3/sp2 ratio can beadjusted. It is shown that the resistivity of the film can be tuned bythis species-selective bias. The principle can be extended tomultiple-material plasma sources and complex materials

The National Spherical Torus Experiment (NSTX) has made considerable progress in advancing the scientific understanding of high performance long-pulse plasmas needed for ITER and future low-aspect-ratio Spherical Torus (ST) devices. Plasma durations up to 1.6s (5 current redistribution times) have been achieved at plasma currents of 0.7 MA with non-inductive current fractions above 65% while achieving {beta}{sub T} and {beta}{sub N} values of 16% and 5.7 (%mT/MA), respectively. Newly available Motional Stark Effect data has allowed systematic study and validation of current drive sources and improved the understanding of ''hybrid''-like scenarios. In MHD research, six mid-plane ex-vessel radial field coils have been utilized to infer and correct intrinsic error fields, provide rotation control, and actively stabilize the n=1 resistive wall mode at ITER-relevant low plasma rotation values. In transport and turbulence, the low aspect ratio and wide range of achievable {beta} in NSTX provide unique data for confinement scaling studies. A new high-k scattering diagnostic is investigating turbulent density fluctuations with wavenumbers extending from ion to electron gyro-scales. In the area of energetic particle research, cyclic neutron rate drops have been associated with the destabilization of multiple large Toroidal Alfven Eigenmodes (TAEs) similar to the ''sea-of-TAE'' modes predicted for ITER. …

CDX-U has been operated with the vacuum vessel wall and limiter surfaces nearly completely coated with lithium, producing dramatic improvements to plasma performance. Discharges achieved global energy confinement times up to 6 ms, exceeding previous CDX-U results by a factor of 5, and ITER98P(y,1) scaling by 2-3. Lithium wall coatings up to 1000 {angstrom} thick were applied between discharges by electron-beam-induced evaporation of a lithium-filled limiter and vapor deposition from a resistively heated oven. The e-beam power was modest (1.6 kW) but it produced up to 60 MW/m2 power density in a 0.3 cm{sup 2} spot; the duration was up to 300 s. Convective transport of heat away from the beam spot was so effective that the entire lithium inventory (140 g) was heated to evaporation (400-500 C) and there was no observable hot spot on the lithium surface within the beam footprint. These results are promising for use of lithium plasma-facing components in reactor scale devices. Lithium coating has also been applied to NSTX carbon plasma-facing surfaces, to control the density rise during long-duration H-modes for non-inductive current sustainment. First, lithium pellets were injected into sequences of Ohmically heated helium plasmas in both center stack limiter (CSL) and lower …

Ultrafast excited state structural dynamics of [Cu{sup I}(dmp){sub 2}]{sup +} (dmp = 2,9-dimethyl-1,10-phenanthroline) have been studied to identify structural origins of transient spectroscopic changes during the photoinduced metal-to-ligand-charge-transfer (MLCT) transition that induces an electronic configuration change from Cu(I) (3d{sup 10}) to Cu(II) (3d{sup 9}). This study has important connections with the flattening of the Franck-Condon state tetrahedral geometry and the ligation of Cu(II)* with the solvent observed in the thermally equilibrated MLCT state by our previous laser-initiated time-resolved x-ray absorption spectroscopy (LITR-XAS) results. To better understand the structural photodynamics of Cu(I) complexes, we have studied both [Cu{sup I}(dmp){sub 2}]{sup +} and [Cu{sup I}(dpp){sub 2}]{sup +} (dpp = 2,9-diphenyl-1,10-phenanthroline) in solvents with different dielectric constants, viscosities and thermal diffusivities by transient absorption spectroscopy. The observed spectral dynamics suggest that a solvent-independent inner-sphere relaxation process is occurring despite the large amplitude motions due to the flattening of the tetrahedral coordinated geometry. The singlet fluorescence dynamics of photoexcited [Cu{sup I}(dmp){sub 2}]{sup +} were measured in the coordinating solvent acetonitrile, using the fluorescence upconversion method at different emission wavelengths. At the bluest emission wavelengths, a prompt fluorescence lifetime of 66 fs is attributed to the excited state deactivation processes due to the internal conversion …

In order to stabilize the beams at the interaction point, the X-band linear collider proposes to use a combination of techniques: inter-train and intra-train beam-beam feedback, passive vibration isolation, and active vibration stabilization based on either accelerometers or laser interferometers. These systems operate in a technologically redundant fashion: simulations indicate that if one technique proves unusable in the final machine, the others will still support adequate luminosity. Experiments underway for all of these technologies have already demonstrated adequate performance.

Characterization of transuranic waste is needed to makedecisions about waste site remediation. Soil-gas sampling for xenonisotopes can be used to define the locations of spent fuel andtransuranic wastes. Radioxenon in the subsurface is characteristic oftransuranic waste and can be measured with extreme sensitivity usinglarge-volume soilgas samples. Measurements at the Hanford Site showed133Xe and 135Xe levels indicative of 240Pu spontaneous fission. Stablexenon isotopic ratios from fission are distinct from atmospheric xenonbackground. Neutron capture by 135Xe produces an excess of 136Xe inreactor-produced xenon providing a means of distinguishing spent fuelfrom separated transuranic materials.

We present a comprehensive wavelength survey of Fe L-shell X-ray lines between 7 and 11 {angstrom} measured using flat crystal spectrometers and the EBIT-I and EBIT-II electron beam ion traps at the Lawrence Livermore National Laboratory. This survey includes all significant emission lines produced by over 200 n {yields} 2 transitions in Fe XIX-XXIV, with n = 4-10. The identification and assignment of transitions are made with the help of detailed theoretical modeling using the Flexible Atomic Code (FAC).

Using 230.2 fb{sup -1} of e{sup +}e{sup -} annihilation data collected with the BABAR detector at and near the peak of the {Upsilon}(4S) resonance, 489 {+-} 55 events containing the pure leptonic decay D{sub s}{sup +} {yields} {mu}{sup +}{nu}{sub {mu}} have been isolated in charm-tagged events. The ratio of partial widths {Lambda}(D{sub s}{sup +} {yields} {mu}{sup +}{nu}{sub {mu}})/{Lambda}(D{sub s}{sup +} {yields} {phi}{pi}{sup +}) is measured to be 0.143 {+-} 0.018 {+-} 0.006 allowing a determination of the pseudoscalar decay constant f{sub D{sub 2}} = (283 {+-} 17 {+-} 7 {+-} 14) MeV. The errors are statistical, systematic, and from the D{sub s}{sup +} {yields} {phi}{pi}{sup +} branching ratio, respectively.

At high currents and small bunch lengths beam line components in the PEP-II B-factory experience RF induced heating from higher order RF modes (HOMs) produced by scattered intense beam fields. A design for a passive HOM water cooled absorber for the PEP-II low energy ring is presented. This device is situated near HOM producing beamline components such as collimators and provide HOM damping for dipole and quadrupole modes without impacting beam impedance. We optimized the impedance characteristics of the device through the evaluation of absorber effectiveness for specific modes using scattering parameter and wakefield analysis. Operational results are presented and agree very well with the predicted effectiveness.

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We present the first collective x-ray scattering measurements of plasmons in solid-density plasmas. The forward scattering spectra of a laser-produced narrow-band x-ray line from isochorically heated beryllium show that the plasmon frequency is a sensitive measure of the electron density. Dynamic structure calculations that include collisions and detailed balance match the measured plasmon spectrum indicating that this technique will enable new applications to determine the equation of state and compressibility of dense matter.

Background: The distribution of the chromatin-associatedproteins plays a key role in directing nuclear function. Previously, wedeveloped an image-based method to quantify the nuclear distributions ofproteins and showed that these distributions depended on the phenotype ofhuman mammary epithelial cells. Here we describe a method that creates ahierarchical tree of the given cell phenotypes and calculates thestatistical significance between them, based on the clustering analysisof nuclear protein distributions. Results: Nuclear distributions ofnuclear mitotic apparatus protein were previously obtained fornon-neoplastic S1 and malignant T4-2 human mammary epithelial cellscultured for up to 12 days. Cell phenotype was defined as S1 or T4-2 andthe number of days in cultured. A probabilistic ensemble approach wasused to define a set of consensus clusters from the results of multipletraditional cluster analysis techniques applied to the nucleardistribution data. Cluster histograms were constructed to show how cellsin any one phenotype were distributed across the consensus clusters.Grouping various phenotypes allowed us to build phenotype trees andcalculate the statistical difference between each group. The resultsshowed that non-neoplastic S1 cells could be distinguished from malignantT4-2 cells with 94.19 percent accuracy; that proliferating S1 cells couldbe distinguished from differentiated S1 cells with 92.86 percentaccuracy; and showed no significant difference between the variousphenotypes of T4-2 …

The multi-group discrete-ordinate equations of radiation transfer is solved for the first time by Newton's method. It is a photon free method because the photon variables are eliminated from the radiation equations to yield a N{sub group}XN{sub direction} smaller but equivalent system of equations. The smaller set of equations can be solved more efficiently than the original set of equations. Newton's method is more stable than the Semi-implicit Linear method currently used by conventional radiation codes.

The accurate measurement of neutron-capture cross sections of the Eu isotopes is important for many reasons including nuclear astrophysics and nuclear diagnostics. Neutron capture excitation functions of {sup 151,153}Eu targets were measured recently using a 4{pi} {gamma}-ray calorimeter array DANCE located at the Los Alamos Neutron Science Center for E{sub n} = 0.1-100 keV. The progress on the data analysis efforts is given in the present paper. The {gamma}-ray multiplicity distributions for the Eu targets and Be backing are significantly different. The {gamma}-ray multiplicity distribution is found to be the same for different neutron energies for both {sup 151}Eu and {sup 153}Eu. The statistical simulation to model the {gamma}-ray decay cascade is summarized.

Adenosine deaminases that act on RNA (ADARs) catalyze the site-specific conversion of adenosine to inosine in primary mRNA transcripts. These re-coding events affect coding potential, splice-sites, and stability of mature mRNAs. ADAR is an essential gene and studies in mouse, C. elegans, and Drosophila suggest its primary function is to modify adult behavior by altering signaling components in the nervous system. By comparing the sequence of isogenic cDNAs to genomic DNA, we have identified and experimentally verified 27 new targets of Drosophila ADAR. Our analyses lead us to identify new classes of genes whose transcripts are targets of ADAR including components of the actin cytoskeleton, and genes involved in ion homeostasis and signal transduction. Our results indicate that editing in Drosophila increases the diversity of the proteome, and does so in a manner that has direct functional consequences on protein function.