Charm Mixing at BaBar (open access)

Charm Mixing at BaBar

We report on searches for D{sup 0}-{bar D}{sup 0} mixing using decay-time distributions of D{sup 0} {yields} K{pi} and D{sup 0} {yields} K{sup (*)}e{nu} decays and a lifetime ratio analysis of D{sup 0} {yields} K{sup +}K{sup -}, {pi}{sup +}{pi}{sup -} decays using 91 fb{sup -1} of e{sup +}e{sup -} data taken at the PEP-II asymmetric-energy storage ring at energies near 10.6 GeV. Searches for CP-violation in D{sup 0} mixing and decay are also reported, as well as a measurement of R{sub D}, the ratio of the doubly Cabibbo-suppressed decay rate to the Cabibbo-allowed decay rate.
Date: July 5, 2006
Creator: Cowan, Ray F.
Object Type: Article
System: The UNT Digital Library
Application of a New Method for Analyzing Images: Two-Dimensional Non-Linear Additive Decomposition (open access)

Application of a New Method for Analyzing Images: Two-Dimensional Non-Linear Additive Decomposition

This paper documents the application of a new image processing algorithm, two-dimensional non-linear additive decomposition (NLAD), which is used to identify regions in a digital image whose gray-scale (or color) intensity is different than the surrounding background. Standard image segmentation algorithms exist that allow users to segment images based on gray-scale intensity and/or shape. However, these processing techniques do not adequately account for the image noise and lighting variation that typically occurs across an image. NLAD is designed to separate image noise and background from artifacts thereby providing the ability to consistently evaluate images. The decomposition techniques used in this algorithm are based on the concepts of mathematical morphology. NLAD emulates the human capability of visually separating an image into different levels of resolution components, denoted as ''coarse'', ''fine'', and ''intermediate''. Very little resolution information overlaps any two of the component images. This method can easily determine and/or remove trends and noise from an image. NLAD has several additional advantages over conventional image processing algorithms, including no need for a transformation from one space to another, such as is done with Fourier transforms, and since only finite summations are required, the calculational effort is neither extensive nor complicated.
Date: July 5, 2006
Creator: Zaccaria, M. A.; Drudnoy, D. M. & Stasenko, J. E.
Object Type: Article
System: The UNT Digital Library
Measurement of the Spin of the Omega- Hyperon at Babar (open access)

Measurement of the Spin of the Omega- Hyperon at Babar

A measurement of the spin of the {Omega}{sup -} hyperon produced through the exclusive process {Xi}{sub c}{sup 0} {yields} {Omega}{sup -}K{sup +} is presented using a total integrated luminosity of 116 fb{sup -1} recorded with the BABAR detector at the e{sup +}e{sup -} asymmetric-energy B-Factory at SLAC. Under the assumption that the {Xi}{sub c}{sup 0} has spin 1/2, the angular distribution of the {Lambda} from {Omega}{sup -} {yields} {Lambda}K{sup -} decay is inconsistent with all half-integer {Omega}{sup -} spin values other than 3/2. Lower statistics data for the process {Omega}{sub c}{sup 0} {yields} {Omega}{sup -}{pi}{sup +} from a 230 fb{sup -1} sample are also found to be consistent with {Omega}{sup -} spin 3/2. If the {Xi}{sub c}{sup 0} spin were 3/2, an {Omega}{sup -} spin of 5/2 cannot be excluded.
Date: July 5, 2006
Creator: Aubert, B.
Object Type: Article
System: The UNT Digital Library
FUNCTIONALIZED LATERAL SURFACE COATED LASERS FOR CHEM-BIO DETECTION (open access)

FUNCTIONALIZED LATERAL SURFACE COATED LASERS FOR CHEM-BIO DETECTION

We present a class of compact, monolithic, photonic sensors consisting of multiple section edge emitting lasers with functionalized lateral surface coatings for low level detection of chemical or biological agents. Specifically, we discuss 8 {micro}m x 250 {micro}m Pd-coated H{sub 2} sensors and configurations to reduce the minimum detection limit from 138ppm for passive sensors to 1ppm for active sensors. Compared with conventional optical H{sub 2} sensors that use fiber gratings, surface plasmon resonances, or surface reflectance, our sensors offer the advantages of smaller size, wider dynamic range, monolithic integration of laser source and detector, and 2-D scalability to arrays of sensors that are functionalized to detect different agents.
Date: July 5, 2007
Creator: Goddard, L L; Bond, T C; Cole, G D & Behymer, E M
Object Type: Article
System: The UNT Digital Library
Resistive-Wall Instability in the Damping Rings of the ILC (open access)

Resistive-Wall Instability in the Damping Rings of the ILC

In the damping rings of the International Linear Collider (ILC), the resistive-wall instability is one of the dominant transverse instabilities. This instability directly influences the choice of material and aperture of the vacuum pipe, and the parameters of the transverse feedback system. This paper investigates the resistive-wall instabilities in an ILC damping ring under various conditions of beam pipe material, aperture, and fill pattern.
Date: July 5, 2006
Creator: Wang, L.; Bane, K .L. F.; Raubenheimer, T. & Ross, M.
Object Type: Article
System: The UNT Digital Library
A 30 ps Timing Resolution for Single Photons with Multi-pixel Burle MCP-PMT (open access)

A 30 ps Timing Resolution for Single Photons with Multi-pixel Burle MCP-PMT

We have achieved {approx}30 psec single-photoelectron and {approx}12ps for multi-photoelectron timing resolution with a new 64 pixel Burle MCP-PMT with 10 micron microchannel holes. We have also demonstrated that this detector works in a magnetic field of 15kG, and achieved a single-photoelectron timing resolution of better than 60 psec. The study is relevant for a new focusing DIRC RICH detector for particle identification at future Colliders such as the super B-factory or ILC, and for future TOF techniques. This study shows that a highly pixilated MCP-PMT can deliver excellent timing resolution.
Date: July 5, 2006
Creator: Va'vra, J.; Benitez, J.; Coleman, J.; Leith, D. W. G. S.; Mazaheri, G.; Ratcliff, B. et al.
Object Type: Article
System: The UNT Digital Library
Development of an Optimum Tracer Set for Apportioning Emissions of Individual Power Plants Using Highly Time-Resolved Measurements and Advanced Receptor Modeling (open access)

Development of an Optimum Tracer Set for Apportioning Emissions of Individual Power Plants Using Highly Time-Resolved Measurements and Advanced Receptor Modeling

In previous studies, 11 elements (Al, As, Cd, Cr, Cu, Fe, Mn, Ni, Pb, Se, and Zn) were determined in 30-minute aerosol samples collected with the University of Maryland Semicontinuous Elements in Aerosol Sampler (SEAS; Kidwell and Ondov, 2001, 2004; SEAS-II) in several locations in which air quality is influenced by emissions from coal- or oil-fired power plants. At this time resolution, plumes from stationary high temperature combustion sources are readily detected as large excursions in ambient concentrations of elements emitted by these sources (Pancras et al. ). Moreover, the time-series data contain intrinsic information on the lateral diffusion of the plume (e.g., {sigma}{sub y}), which Park et al. (2005 and 2006) have exploited in their Pseudo-Deterministic Receptor Model (PDRM), to calculate emission rates of SO{sub 2} and 11 elements (mentioned above) from four individual coal- and oil-fired power plants in the Tampa Bay area. In the current project, we proposed that the resolving power of source apportionment methods might be improved by expanding the set of maker species and that there exist some optimum set of marker species that could be used. The ultimate goal was to determine the utility of using additional elements to better identify and isolate …
Date: July 5, 2007
Creator: Ondov, John & Beachley, Gregory
Object Type: Report
System: The UNT Digital Library
Use of Optically Stimulated Luminescence Imaging Plates and Reader for Arms Control Applications (open access)

Use of Optically Stimulated Luminescence Imaging Plates and Reader for Arms Control Applications

Optically Stimulated Luminescence (OSL) technology has been pioneered at the Pacific Northwest National Laboratory (PNNL) for applications in personnel radiation dosimetry and commercially has become highly successful in replacing older technologies such as Thermoluminescence Dosimeters (TLDs) and film. OSL phosphors are used to measure radiation exposure by illuminating them with light after ionizing radiation exposure and measuring the amount of light emitted by the OSL phosphor. By using a two-dimensional plate of OSL material and raster scanning a light beam across the OSL plate a radiation pattern or image can be measured. The Arms Control community requires an electrons-free medium to measure the attributes of extent and symmetry on Pu pits in storage containers. OSL technology, used in the two-dimensional imaging mode, provides a means to measure these attributes with exposure times on the order of an hour. A special OSL reader has been built by PNNL to measure OSL imaging plates with a size of 20 cm by 30 cm. The reader uses 10 light emitting diode clusters with 10 corresponding photomultiplier tubes to measure an OSL imaging plate in less than 5 minutes. The resolution of each of the 10 measurement assemblies is 1 square-centimeter. A collimator assembly …
Date: July 5, 2001
Creator: Miller, Steven D.; Tomeraasen, Paul L.; Burghard, Brion J. & Traub, Richard J.
Object Type: Report
System: The UNT Digital Library
Single molecule study of a processivity clamp sliding on DNA (open access)

Single molecule study of a processivity clamp sliding on DNA

Using solution based single molecule spectroscopy, we study the motion of the polIII {beta}-subunit DNA sliding clamp ('{beta}-clamp') on DNA. Present in all cellular (and some viral) forms of life, DNA sliding clamps attach to polymerases and allow rapid, processive replication of DNA. In the absence of other proteins, the DNA sliding clamps are thought to 'freely slide' along the DNA; however, the abundance of positively charged residues along the inner surface may create favorable electrostatic contact with the highly negatively charged DNA. We have performed single-molecule measurements on a fluorescently labeled {beta}-clamp loaded onto freely diffusing plasmids annealed with fluorescently labeled primers of up to 90 bases. We find that the diffusion constant for 1D diffusion of the {beta}-clamp on DNA satisfies D {le} 10{sup -14} cm{sup 2}/s, much slower than the frictionless limit of D = 10{sup -10} cm{sup 2}/s. We find that the {beta} clamp remains at the 3-foot end in the presence of E. coli single-stranded binding protein (SSB), which would allow for a sliding clamp to wait for binding of the DNA polymerase. Replacement of SSB with Human RP-A eliminates this interaction; free movement of sliding clamp and poor binding of clamp loader to the …
Date: July 5, 2007
Creator: Laurence, T A; Kwon, Y; Johnson, A; Hollars, C; O?Donnell, M; Camarero, J A et al.
Object Type: Article
System: The UNT Digital Library
A Proposal for High-resolution X-ray Imaging of Intermodal Cargo Containers for Fissionable Materials (open access)

A Proposal for High-resolution X-ray Imaging of Intermodal Cargo Containers for Fissionable Materials

The sensitivity for identification of high-Z objects in elemental form in the massive cargo of intermodal containers with continuous bremsstrahlung radiation depends critically on discriminating the weak signal from uncollided photons from the very intense flux of scattered radiations that penetrate the cargo. We propose that this might be accomplished by rejection of detected events with E {le} 2-3 MeV that contain the majority of multiply-scattered photons along with a correction for single-scattered photons at higher energies. Monte Carlo simulations of radiographs with a 9-MeV bremsstrahlung spectrum demonstrate that rejection of detected events with E {le} 3 MeV removes the majority of signals from scattered photons emerging through cargo with Z {le} 30 and areal densities of at least 145 g cm{sup -2}. With analytical estimates of the single-scattered intensity at higher energies, accurate estimates of linear attenuation coefficients for shielded and unshielded uranium spheres with masses as small as 0.08 kg are found. The estimated maximum dose is generally so low that reasonable order tomography of interesting portions of a container should be possible.
Date: July 5, 2007
Creator: Quiter, B J; Prussin, S G; Pohl, B; Hall, J; Trebes, J; Stone, G et al.
Object Type: Article
System: The UNT Digital Library
SECONDARY ELECTRON EMISSION MEASUREMENTS FOR TIN COATING ON THE STAINLESS STEEL OF SNS ACCUMULATOR RING VACUUM CHAMBER. (open access)

SECONDARY ELECTRON EMISSION MEASUREMENTS FOR TIN COATING ON THE STAINLESS STEEL OF SNS ACCUMULATOR RING VACUUM CHAMBER.

BNL is responsible for the design and construction of the US Spallation Neutron Source (SNS) accumulator ring. Titanium Nitride (TiN) coating on the stainless steel vacuum chamber of the SNS accumulator ring is needed to reduce the secondary electron yield (SEY) and the undesirable resonant multiplication of electrons. The total SEY of TiN coated stainless steel material has been measured after coating samples were exposed to air and after electron and ion bombardment. We report here about TiN coating system setup at BNL and SEY measurements results at CERN, SLAC and KEK. We also present some simulation results of SNS accumulator ring electron-cloud effects using different SEY values.
Date: July 5, 2004
Creator: HE,P. HSEUH,H. C. TODD,R. J. ET AL.
Object Type: Article
System: The UNT Digital Library
RF TECHNIQUES FOR IMPROVED LUMINOSITY IN RHIC. (open access)

RF TECHNIQUES FOR IMPROVED LUMINOSITY IN RHIC.

The luminosity of the Relativistic Heavy Ion Collider has improved significantly [1] over the first three physics runs. A number of special rf techniques have been developed to facilitate higher luminosity. The techniques described herein include: an ultra low-noise rf source for the 197 MHz storage rf system, a frequency shift switch-on technique for transferring bunches from the acceleration to the storage system, synchronizing the rings during the energy ramp (including crossing the transition energy) to avoid incidental collisions, installation of dedicated 200 MHZ cavities to provide longitudinal Landau damping on the ramp, and the development of a bunch merging scheme in the Booster to increase the available bunch intensity from the injectors.
Date: July 5, 2004
Creator: BRENNAN,J. M. BLASKIEWICZ,J. BUTLER,J. DELONG,J. FISCHER,W. HAYES,T.
Object Type: Article
System: The UNT Digital Library
A Low Noise RF Source for RHIC (open access)

A Low Noise RF Source for RHIC

The Relativistic Heavy Ion Collider (RHIC) requires a low noise rf source to ensure that beam lifetime during a store is not limited by the rf system. The beam is particularly sensitive to noise from power line harmonics. Additionally, the rf source must be flexible enough to handle the frequency jump required for rebucketing (transferring bunches from the acceleration to the storage rf systems). This paper will describe the design of a Direct Digital Synthesizer (DDS) based system that provides both the noise performance and the flexibility required.
Date: July 5, 2004
Creator: Hayes, T.
Object Type: Article
System: The UNT Digital Library
Final Focus Shielding Designs for Modern Heavy-Ion Fusion Power Plant Designs (open access)

Final Focus Shielding Designs for Modern Heavy-Ion Fusion Power Plant Designs

Recent work in heavy-ion fusion accelerators and final focusing systems shows a trend towards less current per beam, and thus, a greater number of beams. Final focusing magnets are susceptible to nuclear heating, radiation damage, and neutron activation. The trend towards more beams, however, means that there can be less shielding for each magnet, Excessive levels of nuclear heating may lead to magnet quench or an intolerable recirculating power for magnet cooling. High levels of radiation damage may result in short magnet lifetimes and low reliability. Finally, neutron activation of the magnet components may lead to difficulties in maintenance, recycling, and waste disposal. The present work expands upon previous, three-dimensional magnet shielding calculations for a modified version of the HYLIFE-I1 IFE power plant design. We present key magnet results as a function of the number of beams.
Date: July 5, 2000
Creator: Latkowski, J. F. & Meier, W. R.
Object Type: Article
System: The UNT Digital Library
STOCHASTIC COOLING POWER REQUIREMENTS. (open access)

STOCHASTIC COOLING POWER REQUIREMENTS.

A practical obstacle for stochastic cooling in high-energy colliders like RHIC is the large amount of power needed for the cooling system. Based on the coasting-beam Fokker-Planck (F-P) equation, we analytically derived the optimum cooling rate and cooling power for a beam of uniform distribution and a cooling system of linear gain function. The results indicate that the usual back-of-envelope formula over-estimated the cooling power by a factor of the mixing factor M. On the other hand, the scaling laws derived from the coasting-beam Fokker-Planck approach agree with those derived from the bunched-beam Fokker-Planck approach if the peak beam intensity is used as the effective coasting-beam intensity. A longitudinal stochastic cooling system of 4-8 GHz bandwidth in RHIC can effectively counteract intrabeam scattering, preventing the beam from escaping the RF bucket becoming debunched around the ring.
Date: July 5, 2004
Creator: Wei, J.; Blaskiewicz, M. & Brennan, M.
Object Type: Article
System: The UNT Digital Library
ACCELERATION OF POLARIZED BEAMS USING MULTIPLE STRONG PARTIAL SIBERIAN SNAKES. (open access)

ACCELERATION OF POLARIZED BEAMS USING MULTIPLE STRONG PARTIAL SIBERIAN SNAKES.

Acceleration of polarized protons in the energy range of 5 to 25 GeV is particularly difficult since depolarizing spin resonances are strong enough to cause significant depolarization but full Siberian snakes cause intolerably large orbit excursions. Using a 20-30% partial Siberian snake both imperfection and intrinsic resonances can be overcome. Such a strong partial Siberian snake was designed for the Brookhaven AGS using a dual pitch helical superconducting dipole. Multiple strong partial snakes are also discussed for spin matching at beam injection and extraction.
Date: July 5, 2004
Creator: ROSER,T. AHRENS,L. BAI,M. ET AL.
Object Type: Article
System: The UNT Digital Library
Development of Components for Wavelength Division Multiplexing Over Parallel Optical Interconnects (open access)

Development of Components for Wavelength Division Multiplexing Over Parallel Optical Interconnects

Parallel optical interconnects based on multimode fiber ribbon cables are emerging as a robust, high-performance data link technology that enhances throughput by using parallel arrays of fibers. While this technology has primarily been implemented as single wavelength point-to-point links, it can be significantly enhanced by wavelength division multiplexing (WDM). WDM enables both increased point-to-point bandwidth as well as more complex interconnect topologies and routing approaches that are particularly attractive for massively parallel processing (MPP) systems. Exploiting the advantages of WDM interconnects requires multi-wavelength sources, a low loss routing fabric, and small footprint wavelength selective filter modules. The Lambda-connect project ({gamma}- Connect) at Lawrence Livermore National Laboratory is a technology development and proof-of-principle demonstration of the enabling hardware for WDM parallel optical interconnects for use in massively parallel processing systems and other high-performance data link applications. This dissertation demonstrates several key system components and technologies for {gamma}-Connect.
Date: July 5, 2001
Creator: Patel, R
Object Type: Report
System: The UNT Digital Library
A METHOD TO MEASURE THE FOCUSING PROPERTIES (R-MATRIX) OF A MAGNET. (open access)

A METHOD TO MEASURE THE FOCUSING PROPERTIES (R-MATRIX) OF A MAGNET.

In this paper we discuss, and study the feasibility of a method that may be used to measure the focusing properties of a magnet. This method may prove valuable when applied to ''non-conventional'' magnets that deviate from the usual dipole magnets or other multipole magnets (quadrupoles/sextupoles etc.) which are commonly used in a synchrotron or a beam line. In this category of ''non-conventional'' magnets, fall special magnets, which come under the name ''Snakes'', which are being used in synchrotron accelerators to introduce artificial spin resonances to help overcome the intrinsic and/or imperfection spin resonances which appear during the acceleration of polarized beams. This method of measuring the focusing properties of a magnet requires the use of ''low energy'' and ''high rigidity'' heavy-ions which may be obtained from the BNL Tandem accelerator. In brief the method consists on, injecting ''narrow-beamlets'' of heavy ions into a magnet and measuring the coordinates, of these ''narrow-beamlets'', at the entrance and exit of the magnet. From the measurement of the coordinates of the ''narrow-beamlets'' we can deduce information on the R matrix (first order transfer matrix elements) and higher order matrix elements that define the focusing properties of the magnet.
Date: July 5, 2004
Creator: TSOUPAS,N. THIEBERGER,P. BROWN,K. GASSNER,D. GLENN,W. AHRENS,L. ROSER,T. LEE,Y. Y. WEI,J.
Object Type: Article
System: The UNT Digital Library
Evaluation of the Radiochemistry of Near-Field Water Samples at the Nevada Test Site Applied to the Definition of a Hydrologic Source Term (open access)

Evaluation of the Radiochemistry of Near-Field Water Samples at the Nevada Test Site Applied to the Definition of a Hydrologic Source Term

Effective management of available groundwater resources and strategies for remediation of water impacted by past nuclear testing practices depend on knowledge about the migration of radionuclides in groundwater away from the sites of the explosions. A primary concern is to assess the relative mobilities of the different radionuclide species found near sites of underground nuclear tests and to determine the concentration, extent, and speed of this movement. Ultimately the long term transport behavior of radionuclides with half-lives long enough that they will persist for decades, their interaction with groundwater, and the resulting flux of these contaminants is of paramount importance. As part of a comprehensive approach to these assessments, more than three decades of site-specific sites studies have been undertaken at the Nevada Test Site (NTS) which have focused on the means responsible for the observed or suspected movement of radionuclides away from underground nuclear tests (RNM, 1983). More recently regional and local models of groundwater flow and radionuclide transport have been developed as part of a federal and state of Nevada program to assess the long-term effects of underground nuclear testing on human health and environment (e.g., U.S. DOE/NV, 1997a; Tompson et al., 1999; Pawloski et al., 2001). Necessary …
Date: July 5, 2002
Creator: Smith, D K
Object Type: Report
System: The UNT Digital Library
Nonlinear motion of coupled magnetic vortices in ferromagnetic/non-magnetic/ferromagnetic trilayer (open access)

Nonlinear motion of coupled magnetic vortices in ferromagnetic/non-magnetic/ferromagnetic trilayer

We have investigated a coupled motion of two vortex cores in ferromagnetic/nonmagnetic/ferromagnetic trilayer cynliders by means of micromagnetic simulation. Dynamic motion of two vortex with parallel and antiparallel relative chiralities of curling spins around the vortex cores have been examined after excitation by 1-ns pulsed external field. With systematic variation in non-magnetic spacer layer thickness from 0 to 20 nm, the coupling between two cores becomes significant as the spacer becomes thinner. Significant coupling leads to a nonlinear chaotic coupled motion of two vortex cores for the parallel chiralities and a faster coupled gyrotropic oscillation for the antiparallel chiralities.
Date: July 5, 2009
Creator: Jun, Su-Hyeong; Shim, Je-Ho; Oh, Suhk-Kun; Yu, Seong-Cho; Kim, Dong-Hyun; Mesler, Brooke et al.
Object Type: Article
System: The UNT Digital Library
Measurement of Tritium in Gas Phase Soil Moisture and Helium-3 in Soil Gas at the Hanford Townsite and 100 K Area (open access)

Measurement of Tritium in Gas Phase Soil Moisture and Helium-3 in Soil Gas at the Hanford Townsite and 100 K Area

In 1999, eight soil gas sampling points ranging in depth from 4.9 ft to 32 ft below ground surface (bgs) in two clusters were installed adjacent to well 699-41-1, south of the Hanford Townsite. Fifteen soil gas sampling points, ranging in depth from 7.0 ft to 10.4 ft bgs, were installed to the north and east of the 100-K East Reactor facility. Gas phase soil moisture samples were collected using silica gel traps from all eight sampling locations adjacent to well 699-41-1 and eight locations at the 100-K Area. Soil gas samples for helium-3 measurements were collected at all sampling points. No detectable tritium (<240 pCi/L) was found in the soil moisture samples from either the Hanford Townsite or 100-K Area sampling points. This behavior suggests that tritiated moisture from groundwater is not migrating upward to the sampling points and there are no large vadose zone sources of tritium at either location. Helium-3 analyses of the soil gas samples showed significant enrichments relative to ambient air helium-3 concentrations with a depth dependence consistent with a groundwater source from decay of tritium. Helium-3/helium-4 ratios (normalized to the abundances in ambient air) at the Hanford Townsite ranged from 1.012 at 5 feet …
Date: July 5, 2000
Creator: Olsen, Khris B.; Patton, Gregory W.; Poreda, R.; Dresel, P Evan & Evans, John C.
Object Type: Report
System: The UNT Digital Library
Collisional and Radiative Effects in Transient sub-Doppler Hole Burning: Double Resonance Measurements in CN (open access)

Collisional and Radiative Effects in Transient sub-Doppler Hole Burning: Double Resonance Measurements in CN

We report transient hole-burning and saturation recovery measurements in the CN radical with MHz frequency resolution and 20 ns time resolution. Narrow velocity groups of individual hyperfine levels of selected rotational states in CN (X{sup 2} {Sigma}{sup +}) are depleted and excited (A{sup 2}{pi}{sub i}) with a saturation laser and probed by a counterpropagating, frequency modulated probe beam. Recent work in our lab has used this method to measure and characterize the hyperfine splittings for a set of rotational, fine structure, and parity components of CN (A{sup 2}{pi}{sub i}, v=1). Extending this work, we report time and frequency dependence of the saturation signals following abrupt switching of the CW saturation beam on and off with an electro-optic amplitude modulator. Recovery of the unsaturated absorption following the turnoff of the saturation beam follows pressure-dependent kinetics, driven by collisions with the undissociated NCCN precursor with a rate coefficient of 2 x 10{sup -9} cm{sup 3} s{sup -1} molec{sup -1}. Similar recovery kinetics are observed for two-level saturation resonances, where the signal observed is a combination of X- and A-state kinetics, as well as for three-level crossover resonances, which can be chosen to probe selectively the holefilling in the X state or the …
Date: July 5, 2009
Creator: Hause,M.L.; Hall,G. & Sears, T.J.
Object Type: Article
System: The UNT Digital Library
A DFT and TDDFT Study of Alkylated Trimethylene-Bridged Bis(p-Phenylenediamines) (open access)

A DFT and TDDFT Study of Alkylated Trimethylene-Bridged Bis(p-Phenylenediamines)

The conclusions are: (1) LDA predicts fairly well the structures of {pi}-dimers. This has been reported before. Here we show that even the small difference between conformers can be described by LDA. Electron densities suggest a stronger bond is formed in LDA than B3LYP. (2) Though its good performance is possibly due to error cancelations, LDA may be used as a practical tool for large {pi}-dimer systems. (3) TDDFT once again does a good job for the optical transitions. The near-IR band shows a weak dependence on the functional, but a stronger one on the interplanar distance.
Date: July 5, 2009
Creator: Wu, Q.; Jalilov, A. & Nelson, S.
Object Type: Article
System: The UNT Digital Library
Atomistic Modeling of Wave Propagation in Nanocrystals (open access)

Atomistic Modeling of Wave Propagation in Nanocrystals

We present non-equilibrium molecular dynamics (MD) simulations of wave propagation in nanocrystals. We find that the width of the traveling wave front increases with grain size, d, as d{sup 1/2}. This width also decreases with the pressure behind the front. We extrapolate our results to micro-crystals and obtain reasonable agreement with experimental data. In addition, our extrapolation agrees with models that only take into account the various velocities of propagation along different crystalline orientations, without including grain boundary effects. Our results indicate that, even at the nanoscale, the role of grain boundaries as scattering centers or as sources of plasticity does not increase significantly the width of the traveling wave.
Date: July 5, 2005
Creator: Bringa, E; Caro, A; Victoria, M & Park, N
Object Type: Article
System: The UNT Digital Library