The goal of Jefferson Lab experiment E01-004 (F?-2) was the measurement of the longitudinal and transverse cross sections via pion electroproduction from hydrogen and deuterium for the purpose of extracting the charged pion form factor using pole dominance. The data were taken at two values of Q2 (1.60 and 2.45 GeV/c)2. In order to attain full coverage in R?, charged pions were detected in parallel kinematics (along the direction of momentum transfer, q), and at ±3 degrees off the direction of momentum transfer. For each Q2 data were taken for two values of the virtual photon polarization, ?, respectively. All data were taken at a fixed center of mass energy, W=2.22 GeV. The longitudinal and transverse pieces of the cross section were separated using the Rosenbluth separation method.

In 2001, the D0 experiment entered a new era. Run II of the Tevatron at the Fermi National Accelerator Laboratory began, and the collider became the highest energy particle accelerator in the world. Accordingly, the D0 detector had already undergone a series of upgrades in order to fully exploit the physics now within reach. These included improvements to the tracking, calorimetry, muon detection and triggering capabilities. In the Standard Model, the Higgs boson is the last piece of the puzzle that remains to be discovered. The Higgs mechanism and consequently the Higgs boson is thought to be the fundamental ingredient by which particles acquire mass, and its existence (or lack of existence) is one of the most pressing issues in particle physics today. As such, one of the main goals of the Run II physics programme at D0 is to search for it. Armed with new accelerator capabilities, D0 will be able to impose tighter constraints on the mass of the Higgs, and perhaps even detect this elusive particle. If the Higgs does exist, it will be extremely difficult to find. One of the main challenges at a hadron-hadron collider is to reduce the large QCD background that masks the …

Run IIa of the D0 experiment at the Tevatron took place between Spring 2002 and Spring 2006, collecting approximately 1.2 fb{sup -1} of data. A fundamental principal of the D0 computing model is the utilization of globally distributed computing resources as part of a grid. In particular use is made of the 'SAMGrid'. The first part of this thesis describes the work undertaken at Imperial College on several D0 distributed computing projects. These included the deployment and development of parts of the SAMGrid software suite, and participation in the Winter 2003/2004 data reprocessing effort. One of the major goals of the D0 experiment is the observation of mixing in the B{sub s}{sup 0}-meson system. The measurement of the mixing frequency is important as it can be used to constrain the CKM matrix, which describes CP violation in the Standard Model. The second part of this thesis describes the development of an opposite side flavour tagging algorithm and its calibration using B{sup +} and B{sub d}{sup 0} meson decays. The application of this algorithm to an analysis of the B{sub s}{sup 0} meson system is then described, which lead to the world's first two-sided limit on the B{sub s}{sup 0} meson …

The D0 experiment is based at the Tevatron, which is currently the world's highest-energy accelerator. The detector comprises three major subsystems: the tracking system, the calorimeter and the muon detector. Jets, seen in the calorimeter, are the most common product of the proton-proton interactions at 2TeV. This thesis is divided into two parts. The first part focuses on jets and describes the derivation of a jet energy scale using p{bar p} {yields} (Z + jets) events as a cross-check of the official D0 jet energy scale (Versions 4.2 and 5.1) which is derived using p{bar p} {yields} {gamma} + jets events. Closure tests were also carried out on the jet energy calibration as a further verification. Jets from b-quarks are commonly produced at D0, readily identified and are a useful physics tool. These require a special correction in the case where the b-jet decays via a muon and a neutrino. Thus a semileptonic correction was also derived as an addition to the standard energy correction for jets. The search for the Higgs boson is one of the largest physics programs at D0. The second part of this thesis describes a search for the Standard Model Higgs boson in the ZH …

This dissertation presents the results of a research agenda aimed at improving integration and stability in nanocrystal-based solar cells through advances in active materials and device architectures. The introduction of 3-dimensional nanocrystals illustrates the potential for improving transport and percolation in hybrid solar cells and enables novel fabrication methods for optimizing integration in these systems. Fabricating cells by sequential deposition allows for solution-based assembly of hybrid composites with controlled and well-characterized dispersion and electrode contact. Hyperbranched nanocrystals emerge as a nearly ideal building block for hybrid cells, allowing the controlled morphologies targeted by templated approaches to be achieved in an easily fabricated solution-cast device. In addition to offering practical benefits to device processing, these approaches offer fundamental insight into the operation of hybrid solar cells, shedding light on key phenomena such as the roles of electrode-contact and percolation behavior in these cells. Finally, all-inorganic nanocrystal solar cells are presented as a wholly new cell concept, illustrating that donor-acceptor charge transfer and directed carrier diffusion can be utilized in a system with no organic components, and that nanocrystals may act as building blocks for efficient, stable, and low-cost thin-film solar cells.

Although the standard model of particle physics agrees perfectly with experimental data, it is unlikely the final theory describing particles and their interactions. New phenomena has been searched in the jets and missing transverse energy topology. Such phenomena may be due to the pair production of leptoquarks decaying into a quark and a neutrino or the pair production of stops decaying into a charm and a neutralino which is assumed to be the lightest supersymmetric particle. These searches have been performed with the D0 detector at hadronic collider TeVatron with a center of mass energy of 1.96 TeV. This kind of search needs a good understanding of the jet energy calibration. The determination of the relative jet energy scale has allowed them to reduce the systematic uncertainties on the jet energy measurement when comparing the data and the simulation. Moreover a new method has been developed in order to correct simulated jets for the differences observed in the jet energy scale, the jet energy resolution and the jet reconstruction efficiency between the data and the simulation. The data analysis, performed with an integrated luminosity of 310 pb{sup -1}, has not observed any excess. This result is interpreted in terms of …

This thesis presents a new determination of {Lambda}{sub QCD} from Next-to-Leading Order QCD fits to the Q{sup 2} dependence of neutrino-iron structure functions. This is the first measurement of {Lambda}{sub QCD} which uses a theoretical model that fully accounts for heavy quark production. Compared with previous neutrino measurements, the result has improved understanding of the largest systematic uncertainties on the muon and hadron energy scales. These improvements lead to one of the most precise determination of {alpha}{sub S} at moderate Q{sup 2}. NuTeV is a neutrino-iron deep inelastic scattering (DIS) experiment that collected data during 1996-97 at Fermilab. The key features of NuTeV include its sign-selected beam which produced separate high purity neutrino and antineutrino beams, and its continuous calibration beam which enabled NuTeV to considerably improve the knowledge of energy scales which have dominated uncertainties in the previous measurements.

The detector of the D0 experiment at the proton anti-proton collider Tevatron in Run II is discussed in detail. The performance of the collider and the experiment is presented. Standard model Higgs searches with integrated luminosities between 260 pb{sup -1} and 950 pb{sup -1} and their combination are performed. No deviation from SM background expectation has been observed. Sensitivity prospects at the Tevatron are shown.

We performed a search for Standard Model Higgs boson production in association with W boson (p{bar p} {yields} W{sup {+-}}H {yields} {ell}{nu}b{bar b}) in p{bar p} collisions at {radical}s = 1.96 TeV. The search uses the data collected between February 2002 and February 2006 at Collider Detector at Fermilab (CDF), which corresponds to an integrated luminosity of about 1 fb{sup -1}. The experimental final state of WH {yields} {ell}{nu}b{bar b} process is lepton (e{sup {+-}}/{mu}{sup {+-}}), missing transverse energy and two jets. The largest background in lepton+jets events is W+light flavor process, therefore the identification of jets as b-jets reduces this kind of background significantly. We used displaced SECondary VerTeX b-tagging (SECVTX) technique, which utilizes the signature that b-jets have secondary vertex displaced away from primary vertex because of the long life time of B-mesons. However, there is still much contamination in SECVTX b-tagged jets. Finite resolution of secondary vertex tracking measurements results in false tags, and c-jets are also identified as b-jets due to the long life time of D-mesons frequently. For the purpose of increasing the purity of the SECVTX b-tagged jets, we applied Neural Network to SECVTX tagged jets for the first time by using secondary vertex …

A first study of single diffractive central high-p{sub T} dijet events in p{bar p} collisions at center-of-mass energy {radical}s = 1.96 TeV is presented, using data recorded by the D0 detector at the Tevatron during RunIIa in 2002-2004. The total integrated luminosity corresponding to the data sample is 398 pb{sup -1}. A diffractive sample is selected using a rapidity gap approach. A precise definition of the rapidity gap constitutes the first part of the thesis. The rapidity gap is defined by means of two parts of the D0 detector--luminosity detectors and calorimeter. Luminosity detectors serve as a basic indicators of diffractive candidates and the calorimeter is used to confirm the low energy activity in the forward region (a rapidity gap). Presented studies of energy deposited in forward part of calorimeter by various types of events yield two rapidity gap definitions. Both of them use a fixed rapidity interval in calorimeter |{eta}| {element_of} [2.6,5.2] and introduce an upper limit on the energy deposited in this region. First definition, which corresponds to the lowest systematical errors, uses a limit of 10 GeV, an energy limit in the second definition is set to 3 GeV. This alternative definition corresponds to the lowest contamination …

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Supersymmetry is one of the most natural extensions of the Standard Model. At low energy it may consist in the Minimal Supersymmetric Standard Model which is the framework chosen to perform the search of the stop with 350 pb{sup -1} of data collected by D0 during the RunIIa period of the TeVatron. They selected the events with an electron, a muon, missing transverse energy and non-isolated tracks, signature for the stop decay in 3-body ({bar t} {yields} bl{bar {nu}}). Since no significant excess of signal is seen, the results are interpreted in terms of limit on the stop production cross-sections, in such a way that they extend the existing exclusion region in the parameter space (m{sub {bar t}},m{sub {bar {nu}}}) up to stop masses of 168 (140) GeV for sneutrino masses of 50 (94) GeV. Finally because of the crucial role of the electromagnetic calorimeter, a fine calibration was performed using Z {yields} e{sup +}e{sup -} events, which improved significantly the energy resolution.

This dissertation describes the development andimplementation of a visible/near infrared pump/mid-infrared probeapparatus. Chapter 1 describes the background and motivation ofinvestigating optically induced structural dynamics, paying specificattention to solvation and the excitation selection rules of highlysymmetric molecules such as carotenoids. Chapter 2 describes thedevelopment and construction of the experimental apparatus usedthroughout the remainder of this dissertation. Chapter 3 will discuss theinvestigation of DCM, a laser dye with a fluorescence signal resultingfrom a charge transfer state. By studying the dynamics of DCM and of itsmethyl deuterated isotopomer (an otherwise identical molecule), we areable to investigate the origins of the charge transfer state and provideevidence that it is of the controversial twisted intramolecular (TICT)type. Chapter 4 introduces the use of two-photon excitation to the S1state, combined with one-photon excitation to the S2 state of thecarotenoid beta-apo-8'-carotenal. These 2 investigations show evidencefor the formation of solitons, previously unobserved in molecular systemsand found only in conducting polymers Chapter 5 presents an investigationof the excited state dynamics of peridinin, the carotenoid responsiblefor the light harvesting of dinoflagellates. This investigation allowsfor a more detailed understanding of the importance of structuraldynamics of carotenoids in light harvesting.

In this thesis we present a new technique to analyze events containing two highly energetic leptons, as a probe of the Standard Model. The philosophy is to consider the data in a more global way, as opposed to the more traditional process dependent approach of extracting a given signal over the expected backgrounds by using various kinematical requirements. We use our global technique to simultaneously measure the cross sections of the main Standard Model processes; the t{bar t}, WW and Z {yields} {tau}{tau} production from p{bar p} collisions at {radical}s = 1.96 TeV in the CDF detector at Fermilab. We select events by requiring they contain two highly energetic leptons (e{mu}, ee, or {mu}{mu}), and make no other kinematic requirements, except for the ee and {mu}{mu} channels. We then use a likelihood fit of the data in the two-dimensional phase space defined by the missing transverse energy (E{sub T}) and the number of jets in the event (N{sub jet}), to the expected Standard Model distributions, to simultaneously extract the production cross-sections of the main process contributing to our dilepton sample.

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Modern sky surveys, such as the Sloan Digital Sky Survey (SDSS) and the Two-Micron All Sky Survey, have revolutionized how Astronomy is done. With millions of photometric and spectroscopic observations, global observational properties can be studied with unprecedented statistical significance. Low-mass stars dominate the local Milky Way, with tens of millions observed by SDSS within a few kpc. Thus, they make ideal tracers of the Galactic potential, and the thin and thick disks. In this thesis dissertation, I present my efforts to characterize the local low-mass stellar population, using a collection of observations from the Sloan Digital Sky Survey (SDSS). First, low-mass stellar template spectra were constructed from the co-addition of thousands of SDSS spectroscopic observations. These template spectra were used to quantify the observable changes introduced by chromospheric activity and metallicity. Furthermore, the average ugriz colors were measured as a function of spectral type. Next, the local kinematic structure of the Milky Way was quantified, using a special set of SDSS spectroscopic observations. Combining proper motions and radial velocities (measured using the spectral templates), along with distances, the full UVW space motions of over 7000 low-mass stars along one line of sight were computed. These stars were also separated …

W{sup {+-}} + b{bar b} events contain the associated production of a W{sup {+-}} boson, a pair of bottom quarks (b{bar b}), and any number of additional partons. This process is of much importance at hadron collider experiments due to its role as a background source in searches for Standard Model Higgs boson and single top-quark production. In this thesis the results are presented for a measurement of the b-jet cross-section in W{sup {+-}} + b{bar b} events containing 1 or 2 jets in 695 pb{sup -1} of {radical}s =1.96 TeV p{bar p} collisions at the CDF experiment. This is the first measurement of the cross-section of W{sup {+-}} b{bar b} performed in any experiment. The cross-section is defined to be proportional to the number of b-jets from W{sup {+-}} b{bar b} events with one or two jets, and a leptonically decaying W{sup {+-}} with decay products passing kinematics cuts (p{sub T}({ell}{sup {+-}}) {ge} 20.0 GeV, |{eta}({ell}{sup {+-}})| {le} 1.1, p{sub T}({nu}) {ge} 25.0 GeV). The invariant mass distribution of jets identified as containing a long-lived hadron is fit with components for bottom, charm, and light-flavor to find the fraction due to true b-decays. Background b-jet sources are subtracted to …

The lifetimes of the B{sup -}, B{sup 0} and B{sub s}{sup 0} mesons are measured using partially reconstructed semileptonic decays. Following semileptonic decay processes and their charge conjugates are used for this analysis: B{sup -}/B{sup 0} {yields} {ell}{sup -}{nu}D{sup 0}X; B{sup -}/B{sup 0} {yields} {ell}{sup -}{nu}D*{sup +}X; B{sub s}{sup 0} {yields} {ell}{sup -}{nu}D{sub s}{sup +}x, where {ell}{sup -} denotes either a muon or electron. The data are collected during 2002-2004 by the 8 GeV single lepton triggers in CDF Run II at the Fermilab Tevatron Collider. Corresponding integrated luminosity is about 260 and 360 pb{sup -1} used for the B{sup -}/B{sup 0} and B{sub s}{sup 0} lifetime analyses, respectively. With the single lepton triggers, events which contain a muon or electron with a transverse momentum greater than 8 GeV/c are selected. For these lepton candidates, further lepton identification cuts are applied to improve purity of the B semileptonic decay signal. After the lepton selection, three types of charm mesons associated with the lepton candidates are reconstructed. Following exclusive decay modes are used for the charm meson reconstruction: D{sup 0} {yields} K{sup -}{pi}{sup +}; D*{sup +} {yields} D{sup 0}{pi}{sub s}{sup +}, followed by D{sup 0} {yields} K{sup -}{pi}{sup +}; D{sub s}{sup …

Microfluidic reactors are investigated as a mechanism tocontrol the growth of semiconductor nanocrystals and characterize thestructural evolution of colloidal quantum dots. Due to their shortdiffusion lengths, low thermal masses, and predictable fluid dynamics,microfluidic devices can be used to quickly and reproducibly alterreaction conditions such as concentration, temperature, and reactiontime, while allowing for rapid reagent mixing and productcharacterization. These features are particularly useful for colloidalnanocrystal reactions, which scale poorly and are difficult to controland characterize in bulk fluids. To demonstrate the capabilities ofnanoparticle microreactors, a size series of spherical CdSe nanocrystalswas synthesized at high temperature in a continuous-flow, microfabricatedglass reactor. Nanocrystal diameters are reproducibly controlled bysystematically altering reaction parameters such as the temperature,concentration, and reaction time. Microreactors with finer control overtemperature and reagent mixing were designed to synthesize nanoparticlesof different shapes, such as rods, tetrapods, and hollow shells. The twomajor challenges observed with continuous flow reactors are thedeposition of particles on channel walls and the broad distribution ofresidence times that result from laminar flow. To alleviate theseproblems, I designed and fabricated liquid-liquid segmented flowmicroreactors in which the reaction precursors are encapsulated inflowing droplets suspended in an immiscible carrier fluid. The synthesisof CdSe nanocrystals in such microreactors exhibited reduced depositionand residence time …

In order to better understand the fundamental components that govern catalytic activity, two-dimensional model platinum nanocatalyst arrays have been designed and fabricated. These catalysts arrays are meant to model the interplay of the metal and support important to industrial heterogeneous catalytic reactions. Photolithography and sub-lithographic techniques such as electron beam lithography, size reduction lithography and nanoimprint lithography have been employed to create these platinum nanoarrays. Both in-situ and ex-situ surface science techniques and catalytic reaction measurements were used to correlate the structural parameters of the system to catalytic activity.

Many chemical reactions utilize organometallic complexes as catalysts. These complexes find use in reactions as varied as bond activation, polymerization, and isomerization. This thesis outlines the construction of a new ultrafast laser system with an emphasis on the generation of tunable mid-infrared pulses, data collection, and data analysis.

The shrinking of IC devices has followed the Moore's Law for over three decades, which states that the density of transistors on integrated circuits will double about every two years. This great achievement is obtained via continuous advance in lithography technology. With the adoption of complicated resolution enhancement technologies, such as the phase shifting mask (PSM), the optical proximity correction (OPC), optical lithography with wavelength of 193 nm has enabled 45 nm printing by immersion method. However, this achievement comes together with the skyrocketing cost of masks, which makes the production of low volume application-specific IC (ASIC) impractical. In order to provide an economical lithography approach for low to medium volume advanced IC fabrication, a maskless ion beam lithography method, called Maskless Micro-ion-beam Reduction Lithography (MMRL), has been developed in the Lawrence Berkeley National Laboratory. The development of the prototype MMRL system has been described by Dr. Vinh Van Ngo in his Ph.D. thesis. But the resolution realized on the prototype MMRL system was far from the design expectation. In order to improve the resolution of the MMRL system, the ion optical system has been investigated. By integrating a field-free limiting aperture into the optical column, reducing the electromagnetic interference …

Sum frequency generation (SFG) surface vibrational spectroscopy was used to characterize interfaces pertinent to current surface engineering applications, such as thin film polymers and novel catalysts. An array of advanced surface science techniques like scanning probe microscopy (SPM), x-ray photoelectron spectroscopy (XPS), gas chromatography (GC) and electron microscopy were used to obtain experimental measurements complementary to SFG data elucidating polymer and catalyst surface composition, surface structure, and surface mechanical behavior. Experiments reported in this dissertation concentrate on three fundamental questions: (1) How does the interfacial molecular structure differ from that of the bulk in real world applications? (2) How do differences in chemical environment affect interface composition or conformation? (3) How do these changes correlate to properties such as mechanical or catalytic performance? The density, surface energy and bonding at a solid interface dramatically alter the polymer configuration, physics and mechanical properties such as surface glass transition, adhesion and hardness. The enhanced sensitivity of SFG at the buried interface is applied to three systems: a series of acrylates under compression, the compositions and segregation behavior of binary polymer polyolefin blends, and the changes in surface structure of a hydrogel as a function of hydration. In addition, a catalytically active thin …

Our research focuses on taking advantage of the ability of scanning tunneling microscopy (STM) to operate at high-temperatures and high-pressures while still providing real-time atomic resolution images. We also utilize high-pressure x-ray photoelectron spectroscopy (HPXPS) to monitor systems under identical conditions thus giving us chemical information to compare and contrast with the structural and dynamic data provided by STM.