Thomson-scattering based x-ray radiation sources, in which a laser beam is scattered off a relativistic electron beam resulting in a high-energy x-ray beam, are currently being developed by several groups around the world to enable studies of dynamic material properties which require temporal resolution on the order of tens of femtoseconds to tens of picoseconds. These sources offer pulses that are shorter than available from synchrotrons, more tunable than available from so-called Ka sources, and more penetrating and more directly probing than ultrafast lasers. Furthermore, Thomson-scattering sources can scale directly up to x-ray energies in the few MeV range, providing peak brightnesses far exceeding any other sources in this regime. This dissertation presents the development effort of one such source at Lawrence Livermore National Laboratory, the Picosecond Laser-Electron InterAction for the Dynamic Evaluation of Structures (PLEIADES) project, designed to target energies from 30 keV to 200 keV, with a peak brightness on the order of 10{sup 18} photons {center_dot} s{sup -1} {center_dot} mm{sup -2} {center_dot} mrad{sup -2} {center_dot} 0.01% bandwidth{sup -1}. A 10 TW Ti:Sapphire based laser system provides the photons for the interaction, and a 100 MeV accelerator with a 1.6 cell S-Band photoinjector at the front end provides …

It is well recognized that half the countries in the world will face significant fresh water shortages in the next 20 years, due largely to growing populations and increased agricultural and industrial demands (Gleick, 1997). These shortages will significantly limit economic growth, decrease the quality of life and human health for billions of people, and could potentially lead to violence and conflict over securing scarce supplies of water. In the Middle East, groundwater represents an important part of water supply in most locations, yet it is the least understood and one of the most fragile components of the entire water resource system. The occurrence of water underground contributes to the illusion of an infinite resource that is immune to anthropogenic activities. Nevertheless, as has been learned in the West, it can become highly impaired through the actions of man--through the disposal of human, animal, or industrial wastes, from excessive irrigation and fertilization practices in agriculture, or from simple overproduction and overexploitation--and can remain so for decades or even centuries. Finding solutions to groundwater resource and quality problems can be complex, time consuming, and costly. As is the case in many places in the world, but especially in the Middle East, …

Optical properties and electronic structures of disordered Ag{sub 1- x}In{sub x}(x = 0.0, 0.04, 0.08, 0.12) and Ni{sub 1-x}Cu{sub x} (x = 0.0, 0.1, 0.3, 0.4) alloys and ordered AuGa{sub 2}, PtGa{sub 2}, {beta}{prime}-NiAl, {beta}{prime}-CoAl, CeSn{sub 3}, and LaSn{sub 3} have been studied. The complex dielectric functions have been determined for Ag{sub 1-x}In{sub x}, Ni{sub 1-x}Cu{sub x}, AuGa{sub 2}, and PtGa{sub 2} in the 1.2--5.5 eV region and for CeSn{sub 3} and LaSn{sub 3} in the 1.5--4.5 eV region using spectroscopic ellipsometry. Self-consistent relativistic band calculations using the linearized-augmented-plane-wave method have been performed for AuGa{sub 2}, PtGa{sub 2}, {beta}{prime}-NiAl, {beta}{prime}-CoAl, CeSn{sub 3}, and LaSn{sub 3} to interpret the experimental optical spectra.

Abstract: And investigation of the interactions between 300-Mev neutrons and xenon was made by means of a cloud chamber in a pulsed magnetic field of 21,700 gauss placed in the neutron beam of the 184-inch Berkeley cyclotron. Eighty-seven negative pion events and 257 other stars were analyzed. In addition an experimental check was made on the energy of the incoming neutrons. Classification, identification, and angular and energy distributions of prongs associated with all events are presented. Interpretations of results are given.

The elastic scattering of C/sup 12/ ions from Ar, Fe, Ni, Ag/sup 107/ In, and Ta was measured as a function of angle, at a laboratory-system energy of 124.5 Mev with the Berkeley heavy-ion linear accelerator. The experimental equipment and techniques are discussed. The angular distributions show the same general behavior as previous heavy-ion elastic scattering experiments. The experimental data were analyzed with the semiclassical Blair model as modified by McIntyre. Very good agreement with experiment was obtained. The measurements were taken with 1% statistics in order to study the structure of the angular distributions in greater detail, because only by fitting the details in the structure was it possible to obtdin unambiguous sets of parameters. The parameters indicated a nuclear radius of 1.45A/sup 1/3/ x 10/sup -13/ cm, and a nearly constant surface thick ness of 1.6 x 10/sup -13/ cm. Total reaction cross sections were obtained. A rainbow-model analysis by Goldman of the data is given. Existing alpha - and heavy-ion scattering data were analyzed with the McIntyre model and compared with previous optical-model analyses of the same data. It was found that, by independent analysis, the two models give the same imaginary phase shifts for all partial …

SUBMITTED AS A DOCTORAL DISSERTATION IN COMPLETION OF REQUIREMENTS FOR THE DEGREE OF ED.D THROUGH WASHINGTON STATE UNIVERSITY. The overall purpose of this action research study was to explore the experiences of ten middle school science teachers involved in a three-year partnership program between scientists and teachers at a Department of Energy national laboratory, including the impact of the program on their professional development, and to improve the partnership program by developing a set of recommendations based on the study’s findings. This action research study relied on qualitative data including field notes recorded at the summer academies and data from two focus groups with teachers and scientists. Additionally, the participating teachers submitted written reflections in science notebooks, participated in open-ended telephone interviews that were transcribed verbatim, and wrote journal summaries to the Department of Energy at the end of the summer academy. The analysis of the data, collaboratively examined by the teachers, the scientists, and the science education specialist acting as co-researchers on the project, revealed five elements critical to the success of the professional development of science teachers. First, scientist-teacher partnerships are a unique contribution to the professional development of teachers of science that is not replicated in other …

An investigation of the interactions between 300-Mev neutrons and xenon was made by means of a cloud chamber in a pulsed magnetic field of 21,700 gauss placed in the neutron beam of the 184-inch Berkeley cyclotron. Eighty-seven negative pion events and 257 other stars were analyzed. In addition an experimental check was made on the energy of the incoming neutrons. Classification, identification, and angular and energy distributions of prongs associated with all events are presented. Interpretations of results are given.

This work is the result of the researchers carried out during a three years Ph.D. period in the BABAR experiment. The first chapter consists in an introduction to the theoretical aspects of the D{sup 0} meson lifetime determination and CP violation parameters, as well as an overview of the CP violation in the B sector, which is the main topic of the experiment. The description of the experimental apparatus follows with particular attention to the Silicon Vertex Tracker detector, the most critical detector for the determination of decay vertices and thus of lifetimes and time dependent CP violation asymmetries. In the fourth chapter the operation and running of the vertex detector is described, as a result from the experience as Operation Manager of the SVT, with particular attention to the safety of the device and the data quality assurance. The last chapter is dedicated to the determination of the D{sup 0} meson lifetime with the BABAR detector, which is the main data analysis carried out by the candidate. The analysis is characterized by the selection of an extremely pure sample of D{sup 0} mesons for which the decay flight length and proper time is reconstructed. The description of the unbinned …

Presented is a precise measurement of the {bar B}{sup 0} {yields} D*{sup +}{ell}{sup -}{bar {nu}}{sub {ell}} branching fraction using 81.47 fb{sup -1} of data collected with the BABAR detector at the PEP-II e{sup +}e{sup -} storage ring at the Stanford Linear Accelerator Center. The measurement was performed by partially reconstructing the D*{sup +} meson from {bar B}{sup 0} {yields} D*{sup +}{ell}{sup -}{bar {nu}}{sub {ell}} decays using only the soft pion of the D*{sup +} {yields} D{sup 0}{pi}{sup +} decay to reconstruct its four vector. The branching fraction was measured to be {Beta}({bar B}{sup 0} {yields} D*{sup +}{ell}{sup -}{bar {nu}}{sub {ell}}) = (4.91 {+-} 0.01{sub stat} {+-} 0.15{sub syst})%.

The D{sub J}{sup 0} is a family of four orbitally excited mesons: D*{sub 2}(2460){sup 0}, D{sub 1}(2420){sup 0}, D{sub 1}(j = 1/2){sup -}, and D*{sub 0}(j = 1/2){sup 0}. This dissertation presents the measurements of the inclusive branching fractions, {Beta}(B{sup -} {yields} D*{sup +}{pi}{sup -}{pi}{sup -}) and {Beta}(B{sup -} {yields} D{sup +}{pi}{sup -}{pi}{sup -}). The D{sub J}{sup 0} provides an intermediate resonance for those two modes. The data used for this analysis consists of Runs 1-5 with total integrated luminosity of 343.38 fb{sup -1}, which is corresponding to 383.92 million B{bar B} pairs, provided by the BABAR detector at the PEP-II asymmetric B Factory. The values presented are: {Beta}(B{sup -} {yields} D{sup +}{pi}{sup -}{pi}{sup -}) = (1.12 {+-} 0.02 {+-} 0.08) x 10{sup -3}; {Beta}(B{sup -} {yields} D*{sup +}{pi}{sup -}{pi}{sup -}) = (1.67 {+-} 0.03 {+-} 0.13) x 10{sup -3}.

In this work we presented measurements of CP violation and decay rates of B decays in final states not involving a charm quark in the final state. In particular, the time-dependent CP asymmetries of decays which proceed through b {yields} s elementary transition is a particularly sensitive probe of physics beyond the Standard Model. In fact, even if the precise measurements of CP conserving and CP violating processes show the success of the CKM picture of the flavour physics, the sector of b {yields} s transitions is still not strongly constrained and leaves room for new physics contributions. In particular, we considered the decays which have the cleanest theoretical prediction within the Standard Model: B{sup 0} {yields} {phi}K{sup 0} and B{sup 0} {yields} K{sub s}{sup 0}K{sub s}{sup 0}K{sub s}{sup 0} {beta}{sub eff}{sup SM} = 0.379. We examined the former with a completely new approach with respect to the past: the study of CP violation in the whole K{sup +}K{sup -}K{sup 0} phase space through a time-dependent Dalitz plot analysis. With this approach, we simultaneously measured the CP-violating asymmetries of the {phi}KJ{sup 0}, f{sub 0}(980)K{sup 0} resonant and K{sup +}K{sup -}K{sup 0} non-resonant contributions, avoiding one of the largest uncertainties which …

The rare decay B {yields} {pi}{ell}{sup +}{ell}{sup -} is the simplest manifestation of a b {yields} d{ell}{sup +}{ell}{sup -} flavor-changing neutral current (FCNC) process. This type of process only proceeds through penguin loop or box diagrams and is sensitive to physics at the electroweak scale. It can be used to constrain parameters of the Standard Model and its extensions. B {yields} {pi}{ell}{sup +}{ell}{sup -} events have not yet been observed; the branching fraction is expected to be an order of magnitude smaller than the measured branching fraction for the similar B {yields} K{ell}{sup +}{ell}{sup -} decay. Using 230 million B{bar B} meson pairs collected with the BABAR detector, we have done a search for the rare decay B {yields} {pi}{ell}{sup +}{ell}{sup -}. The data was produced in e+e? collision at the {Upsilon}(4S) resonance in the PEP-II collider between 1999 and 2004. Four exclusive B-meson decay modes have been reconstructed: B{sup +} {yields} {pi}{sup +}{ell}{sup +}{ell}{sup -} and B{sup 0} {yields} {pi}{sup 0}{ell}{sup +}{ell}{sup -}, where {ell}{sup +}{ell}{sup -} is either an electron pair (e{sup +}e{sup -}) or a muon pair ({mu}{sup +}{mu}{sup -}). We find no evidence for a signal, and we obtain upper limits on the branching fractions {Beta}. …

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This thesis reports measurements of the time-dependent CP asymmetries in fully reconstructed B{sup 0} {yields} (D{sup (*){-+}} and B{sup 0} {yields} D{sup {-+}} {rho}{sup {+-}}) decays in approximately 232 million {Upsilon}(4S) {yields} B{bar B} events, collected with the BABAR detector at the PEP-II asymmetric-energy B factory at the Stanford Linear Accelerator Center in California, as published in Ref. [14]. The phenomenon of CP violation allows one to distinguish between matter and antimatter, and, as such, is one of the essential ingredients needed to explain the apparent abundance of matter over antimatter in the universe. The Standard Model describes the observed elementary particles in terms of three generations of quarks and leptons, as well as the weak, electromagnetic, and strong interactions between them. In the Standard Model, CP violation is incorporated in the Cabibbo-Kobayashi-Maskawa (CKM) matrix, which describes the weak interactions between the quarks. The weak interactions between quarks are described by coupling constants that are functions of three real parameters and one irreducible complex phase. The magnitude of all CP violating effects in the Standard Model is related to this complex phase. The measurement of the CP violating phase of the CKM matrix is an important part of the present …

The authors report the results of a study of the exclusive charmless semileptonic decay, B{sup 0} {yields} {pi}{sup -}{ell}{sup +}{nu}, undertaken with approximately 227 million B{bar B} pairs collected at the {Upsilon}(4S) resonance with the BABAR detector. The analysis uses events in which the signal B decays are reconstructed with an innovative loose neutrino reconstruction technique. They obtain partial branching fractions in 12 bins of q{sup 2}, the momentum transfer squared, from which they extract the f{sub +}(q{sup 2}) form-factor shape and the total branching fraction {Beta}(B{sup 0} {yields} {pi}{sup -}{ell}{sup +}{nu}) = (1.46 {+-} 0.07{sub stat} {+-} 0.08{sub syst}) x 10{sup -4}. Based on a recent unquenched lattice QCD calculation of the form factor in the range q{sup 2} > 16 GeV{sup 2}/c{sup 4}, they find the magnitude of the CKM matrix element |V{sub ub}| to be (4.1 {+-} 0.2{sub stat} {+-} 0.2{sub syst{sub -0.4}{sup +0.6}FF}) x 10{sup -3}, where the last uncertainty is due to the normalization of the form factor.

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Note that the main goal of this thesis work is the measurement of the branching fractions, charge asymmetry, and Time-Dependent CP Violation in {eta}'K{sup 0} mode. All other measurements are reported here for completion because they are connected by similar physics arguments. They are part of the Milan analysis activity, done by undergraduate students. They should not be considered as done in this thesis work. The measurements of the two body-modes {eta}{eta}, {eta}{phi}, and {eta}'{phi} are used to determine a theoretical bound based on SU(3) flavor symmetry for the difference between SM prediction and the experimental measurements of CP violation parameters in b {yields} s loop-dominated modes. In general for this estimation we need to measure the branching fractions (or upper limits) of neutral B decays to two-body modes with {eta}', {eta}, {phi}, {omega}, {pi}{sup 0}, K{sup 0}, K*{sup 0} [13, 14, 15, 16]. There is an important issue related to the branching fractions of {eta}'K (charged and neutral) modes. Since the discover of B {yields} {eta}'K in 1997 [17] with high branching fraction (higher than expected), it was found that the corresponding mode with {eta} is suppressed. This fact was pointed out by Lipkin in 1991 [18]. In particular, …

The objective of this work is to investigate the thick diffusion limit of various spatial discretizations of the one-dimensional, steady-state, monoenergetic, discrete ordinates neutron transport equation. This work specifically addresses the two lowest order nodal methods, AHOT-N0 and AHOT-N1, as well as reconsiders the asymptotic limit of the Diamond Difference method. The asymptotic analyses of the AHOT-N0 and AHOT-N1 nodal methods show that AHOT-N0 does not possess the thick diffusion limit for cell edge or cell average fluxes except under very limiting conditions, which is to be expected considering the AHOT-N0 method limits to the Step method in the thick diffusion limit. The AHOT-N1 method, which uses a linear in-cell representation of the flux, was shown to possess the thick diffusion limit for both cell average and cell edge fluxes. The thick diffusion limit of the DD method, including the boundary conditions, was derived entirely in terms of cell average scalar fluxes. It was shown that, for vacuum boundaries, only when {sigma}{sub t}, h, and Q are constant and {sigma}{sub a} = 0 is the asymptotic limit of the DD method close to the finite-differenced diffusion equation in the system interior, and that the boundary conditions between the systems will …

In the last two decades, the field of nanoscience andnanotechnology has witnessed tremendous advancement in the synthesis andapplication of group II-VI colloidal nanocrystals. The synthesis based onhigh temperature decomposition of organometallic precursors has becomeone of the most successful methods of making group II-VI colloidalnanocrystals. This method is first demonstrated by Bawendi and coworkersin 1993 to prepare cadmium chalcogenide colloidal quantum dots and laterextended by others to prepare other group II-VI quantum dots as well asanisotropic shaped colloidal nanocrystals, such as nanorod and tetrapod.This dissertation focuses on the chemistry of this type of nanocrystalsynthesis. The synthesis of group II-VI nanocrystals was studied bycharacterizing the molecular structures of the precursors and productsand following their time evolution in the synthesis. Based on theseresults, a mechanism was proposed to account for the 2 reaction betweenthe precursors that presumably produces monomer for the growth ofnanocrystals. Theoretical study based on density functional theorycalculations revealed the detailed free energy landscape of the precursordecomposition and monomerformation pathway. Based on the proposedreaction mechanism, a new synthetic method was designed that uses wateras a novel reagent to control the diameter and the aspect ratio of CdSeand CdS nanorods.

Studies of colloidal nanocrystals and their assemblies are presented. Two of these studies concern the atomic-level structural characterization of the surfaces, interfaces, and interiors present in II-VI semiconductor nanorods. The third study investigates the crystallographic arrangement of cobalt nanocrystals in self-assembled aggregates. Crystallographically-aligned assemblies of colloidal CdSe nanorods are examined with linearly-polarized Se-EXAFS spectroscopy, which probes bonding along different directions in the nanorod. This orientation-specific probe is used, because it is expected that the presence of specific surfaces in a nanorod might cause bond relaxations specific to different crystallographic directions. Se-Se distances are found to be contracted along the long axis of the nanorod, while Cd-Se distances display no angular dependence, which is different from the bulk. Ab-initio density functional theory calculations upon CdSe nanowires indicate that relaxations on the rod surfaces cause these changes. ZnS/CdS-CdSe core-shell nanorods are studied with Se, Zn, Cd, and S X-ray absorption spectroscopy (XAS). It is hypothesized that there are two major factors influencing the core and shell structures of the nanorods: the large surface area-to-volume ratio, and epitaxial strain. The presence of the surface may induce bond rearrangements or relaxations to minimize surface energy; epitaxial strain might cause the core and shell lattices …

In the last two decades, the field of nanoscience andnanotechnology has witnessed tremendous advancement in the synthesis andapplication of group II-VI colloidal nanocrystals. The synthesis based onhigh temperature decomposition of organometallic precursors has becomeone of the most successful methods of making group II-VI colloidalnanocrystals. This methodis first demonstrated by Bawendi and coworkersin 1993 to prepare cadmium chalcogenide colloidal quantum dots and laterextended by others to prepare other group II-VI quantum dots as well asanisotropic shaped colloidal nanocrystals, such as nanorod and tetrapod.This dissertation focuses on the chemistry of this type of nanocrystalsynthesis. The synthesis of group II-VI nanocrystals was studied bycharacterizing the molecular structures of the precursors and productsand following their time evolution in the synthesis. Based on theseresults, a mechanism was proposed to account for the 2 reaction betweenthe precursors that presumably produces monomer for the growth ofnanocrystals. Theoretical study based on density functional theorycalculations revealed the detailed free energy landscape of the precursordecomposition and monomerformation pathway. Based on the proposedreaction mechanism, a new synthetic method was designed that uses wateras a novel reagent to control the diameter and the aspect ratio of CdSeand CdS nanorods.

Scientific computation is used for the simulation of increasingly complex phenomena, and generates data sets of ever increasing size, often on the order of terabytes. All of this data creates difficulties. Several problems that have been identified are (1) the inability to effectively handle the massive amounts of data created, (2) the inability to get the data off the computer and into storage fast enough, and (3) the inability of a remote user to easily obtain a rendered image of the data resulting from a simulation run. This dissertation presents several techniques that were developed to address these issues. The first is a prototype bin coder based on variable-to-variable length codes. The codes utilized are created through a process of parse tree leaf merging, rather than the common practice of leaf extension. This coder is very fast and its compression efficiency is comparable to other state-of-the-art coders. The second contribution is the Piecewise-Linear Haar (PLHaar) transform, a reversible n-bit to n-bit wavelet-like transform. PLHaar is simple to implement, ideal for environments where transform coefficients must be kept the same size as the original data, and is the only n-bit to n-bit transform suitable for both lossy and lossless coding.

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Photoconductive semiconductor switches (PCSS) have been investigated since the late 1970s. Some devices have been developed that withstand tens of kilovolts and others that switch hundreds of amperes. However, no single device has been developed that can reliably withstand both high voltage and switch high current. Yet, photoconductive switches still hold the promise of reliable high voltage and high current operation with subnanosecond risetimes. Particularly since good quality, bulk, single crystal, wide bandgap semiconductor materials have recently become available. In this chapter we will review the basic operation of PCSS devices, status of PCSS devices and properties of the wide bandgap semiconductors 4H-SiC, 6H-SiC and 2H-GaN.