Multi-year search for a diffuse flxu of muon neutrinos with AMANDA-II (open access)

Multi-year search for a diffuse flxu of muon neutrinos with AMANDA-II

A search for TeV-PeV muon neutrinos from unresolved sources was performed on AMANDA-II data collected between 2000 and 2003 with an equivalent livetime of 807 days. This diffuse analysis sought to find an extraterrestrial neutrino flux from sources with non-thermal components. The signal is expected to have a harder spectrum than the atmospheric muon and neutrino backgrounds. Since no excess of events was seen in the data over the expected background, an upper limit of E{sup 2}{Phi}{sub 90%C.L.} < 7.4 x 10{sup -8} GeV cm{sup -2} s{sup -1} sr{sup -1} is placed on the diffuse flux of muon neutrinos with a {Phi} {proportional_to} E{sup -2} spectrum in the energy range 16 TeV to 2.5 PeV. This is currently the most sensitive {Phi} {proportional_to} E{sup -2} diffuse astrophysical neutrino limit. We also set upper limits for astrophysical and prompt neutrino models, all of which have spectra different than {Phi} {proportional_to} E{sup -2}.
Date: April 13, 2008
Creator: Collaboration, IceCube; Klein, Spencer; Achterberg, A. & Collaboration, IceCube
System: The UNT Digital Library
The silicon microstrip sensors of the ATLAS semiconductor tracker (open access)

The silicon microstrip sensors of the ATLAS semiconductor tracker

This paper describes the AC-coupled, single-sided, p-in-n silicon microstrip sensors used in the Semiconductor Tracker (SCT) of the ATLAS experiment at the CERN Large Hadron Collider (LHC). The sensor requirements, specifications and designs are discussed, together with the qualification and quality assurance procedures adopted for their production. The measured sensor performance is presented, both initially and after irradiation to the fluence anticipated after 10 years of LHC operation. The sensors are now successfully assembled within the detecting modules of the SCT, and the SCT tracker is completed and integrated within the ATLAS Inner Detector. Hamamatsu Photonics Ltd. supplied 92.2percent of the 15,392 installed sensors, with the remainder supplied by CiS.
Date: April 13, 2007
Creator: Collaboration, ATLAS SCT & Spieler, Helmuth G.
System: The UNT Digital Library
Shielding Calculations for NSLS-II Beamlines. (open access)

Shielding Calculations for NSLS-II Beamlines.

Brookhaven National Laboratory is in the process of designing a new Electron Synchrotron for scientific research using synchrotron radiation. This facility, called the 'National Synchrotron Light Source II' (NSLS-II), will provide x-ray radiation of ultra-high brightness and exceptional spatial and energy resolution. It will also provide advanced insertion devices, optics, detectors, and robotics, and a suite of scientific instruments designed to maximize the scientific output of the facility. The project scope includes the design, construction, installation, and commissioning of the following accelerators: a 200 MeV linac, a booster accelerator operating from 200 MeV to 3.0 GeV, the storage ring which stores 500 mA current of electrons at an energy of 3.0 GeV and 56 beamlines for experiments. It is planned to operate the facility primarily in a top-off mode, thereby maintaining the maximum variation in stored beam current to < 1%. Because of the very demanding requirements for beam emittance and synchrotron radiation brilliance, the beam life-time is expected to be quite low, on the order of 2 hours. Each of the 56 beamlines will be unique in terms of the source properties and configuration. The shielding designs for five representative beamlines are discussed in this paper.
Date: April 13, 2008
Creator: Job,P.K. & Casey, W.R.
System: The UNT Digital Library
A Filter-Fluorescer Diagnostic System (FFLEX) for the National Ignition Facility (NIF) (open access)

A Filter-Fluorescer Diagnostic System (FFLEX) for the National Ignition Facility (NIF)

An early Filter-Fluorescer Diagnostic System (FFLEX) is being fielded at the National Ignition Facility (NIF) at Lawrence Livermore National Laboratory (LLNL) to measure the amount of hard x-rays (20 < hv < 150 keV) generated in laser fusion experiments. From these measurements we hope to quantify the number of hot (20 to 50 keV) electrons produced in laser fusion experiments. The Measurement of hot electron production is important for ignition experiments because these electrons can preheat the fuel capsule. Hot electrons can also be employed in experimentation by preheating hydrodynamic packages or by driving plasmas out of equilibrium. The experimental apparatus, data collection, analysis and calibration issues are discussed. Expected data signal levels and rates are predicted and discussed.
Date: April 13, 2004
Creator: McDonald, J. W.; Kauffman, R. L.; Celeste, J. R.; Rhodes, M. A.; Lee, F. D.; Suter, L. J. et al.
System: The UNT Digital Library
Preliminary Performance Measurements for a Streak Camera with a Large-Format Direct-Coupled CCD Readout (open access)

Preliminary Performance Measurements for a Streak Camera with a Large-Format Direct-Coupled CCD Readout

Livermore's ICF Program has a large inventory of optical streak cameras built in the 1970s and 1980s. The cameras are still very functional, but difficult to maintain because many of their parts are obsolete including the original streak tube and image-intensifier tube. The University of Rochester's Laboratory for Laser Energetics is leading an effort to develop a fully automated, large-format streak camera that incorporates modern technology. Preliminary characterization of a prototype camera shows spatial resolution better than 20 lp/mm, temporal resolution of 12 ps, line-spread function of 40 {micro}m (fwhm), contrast transfer ratio (CTR) of 60% at 10 lp/mm, and system sensitivity of 16 CCD electrons per photoelectron. A dynamic range of 60 for a 2 ns window is determined from system noise, linearity and sensitivity measurements.
Date: April 13, 2004
Creator: Lerche, R. A.; McDonald, J. W.; Griffith, R. L.; de Dios, G. V.; Andrews, D. S.; Huey, A. W. et al.
System: The UNT Digital Library
Opto-electrical characterization and X-ray mapping of large-volume cadmium zinc telluride radiation detectors (open access)

Opto-electrical characterization and X-ray mapping of large-volume cadmium zinc telluride radiation detectors

Large-volume cadmium zinc telluride (CZT) radiation detectors would greatly improve radiation detection capabilities and, therefore, attract extensive scientific and commercial interests. CZT crystals with volumes as large as hundreds of centimeters can be achieved today due to improvements in the crystal growth technology. However, the poor performance of large-volume CZT detectors is still a challenging problem affecting the commercialization of CZT detectors and imaging arrays. We have employed Pockels effect measurements and synchrotron X-ray mapping techniques to investigate the performance-limiting factors for large-volume CZT detectors. Experimental results with the above characterization methods reveal the non-uniform distribution of internal electric field of large-volume CZT detectors, which help us to better understand the responsible mechanism for the insufficient carrier collection in large-volume CZT detectors.
Date: April 13, 2009
Creator: Yang, G.; Bolotnikov, A.E.; Camarda, G.S.; Cui, Y.; Hossain, A.; Yao, H.W. et al.
System: The UNT Digital Library
Measurements of the Total Charge-Changing Cross Sections for Collisions of Fast Ions with Target Gas Using High Current Experiment (open access)

Measurements of the Total Charge-Changing Cross Sections for Collisions of Fast Ions with Target Gas Using High Current Experiment

The sum of ionization and charge-exchange cross sections of several gas targets (H2, N2, He, Ne, Kr, Xe, Ar, and water vapor) impacted by 1MeV K+ beam are measured. In a high current ion beam, the self-electric field of the beam is high enough that ions produced from the gas ionization or charge exchange by the ion beam are quickly swept to the sides of accelerator. The flux of the expelled ions is measured by a retarding field analyzer. This allows accurate measuring of the total charge-changing cross sections (ionization plus charge exchange) of the beam interaction with gas. Cross sections for H2, He, and N2 are simulated using classical trajectory Monte Carlo (CTMC) method and compared with the experimental results, showing good agreement.
Date: April 13, 2009
Creator: Covo, Michel Kireeff; Molvik, Arthur W.; Kaganovich, Igor D.; Shnidman, Ariel & Vujic, Jasmina L.
System: The UNT Digital Library
Search for b\to u Transitions in \Bz \to \Dz \Kstarz Decays (open access)

Search for b\to u Transitions in \Bz \to \Dz \Kstarz Decays

We present a study of the decays B{sup 0} {yields} D{sup 0} K*{sup 0} and B{sup 0} {yields} {bar D}{sup 0} K*{sup 0} with K*{sup 0} {yields} K{sup +}{pi}{sup -}. The D{sup 0} and the {bar D}{sup 0} mesons are reconstructed in the final states f = K{sup +} {pi}{sup -}, K{sup +}{pi}{sup -}{pi}{sup 0}, K{sup +}{pi}{sup -}{pi}{sup +}{pi}{sup -} and their charge conjugates. Using a sample of 465 million B{bar B} pairs collected with the BABAR detector at PEP-II asymmetric-energy e{sup +}e{sup -} collider at SLAC, we measure the ratio R{sub ADS} {triple_bond} [{Lambda}({bar B}{sup 0} {yields} [f]{sub D}{bar K}*{sup 0}) + {Lambda}(B{sup 0} {yields} [{bar f}]{sub D}K*{sup 0})]/[{Lambda}({bar B}{sup 0} {yields} [{bar f}]{sub D}{bar K}*{sup 0}) + {Lambda}(B{sup 0} {yields} [f]{sub D}K*{sup 0})] for the three final states. We do not find significant evidence for a signal and set the following limits at 95% probability: R{sub ADS}(K{pi}) < 0.244, R{sub ADS}(K{pi}{pi}{sup 0}) < 0.181 and R{sub ADS}(K{pi}{pi}{pi}) < 0.391. From the combination of these three results, we find that the ratio r{sub S} between the b {yields} u and the b {yields} c amplitudes lies in the range [0.07; 0.41] at 95% probability.
Date: April 13, 2009
Creator: Aubert, B.; Bona, M.; Karyotakis, Y.; Lees, J. P.; Poireau, V.; Prencipe, E. et al.
System: The UNT Digital Library
Evidence for Nodal Superconductivity in LaFePO from Scanning SQUID Susceptometry (open access)

Evidence for Nodal Superconductivity in LaFePO from Scanning SQUID Susceptometry

We measure changes in the penetration depth {lambda} of the T{sub c} {approx} 6 K superconductor LaFePO. In the process scanning SQUID susceptometry is demonstrated as a technique for accurately measuring local temperature-dependent changes in {lambda}, making it ideal for studying early or difficult-to-grow materials. {lambda} of LaFePO is found to vary linearly with temperature from 0.36 to {approx} 2 K, with a slope of 143 {+-} 15 {angstrom}/K, suggesting line nodes in the superconducting order parameter. The linear dependence up to {approx} T{sub c}/3 is similar to the cuprate superconductors, indicating well-developed nodes.
Date: April 13, 2009
Creator: Hicks, Clifford W.; Lippman, Thomas M.; /Stanford U., Geballe Lab. /SLAC; Huber, Martin E.; /Colorado U., Denver; Analytis, James G. et al.
System: The UNT Digital Library
MODUTANK ENGINEERING EVALUATION/COST ANALYSIS (open access)

MODUTANK ENGINEERING EVALUATION/COST ANALYSIS

None
Date: April 13, 2009
Creator: FOSS, DL & CE, KENNEDY
System: The UNT Digital Library
A DISCIPLINED APPROACH TO ACCIDENT ANALYSIS DEVELOPMENT AND CONTROL SELECTION (open access)

A DISCIPLINED APPROACH TO ACCIDENT ANALYSIS DEVELOPMENT AND CONTROL SELECTION

The development and use of a Safety Input Review Committee (SIRC) process promotes consistent and disciplined Accident Analysis (AA) development to ensure that it accurately reflects facility design and operation; and that the credited controls are effective and implementable. Lessons learned from past efforts were reviewed and factored into the development of this new process. The implementation of the SIRC process has eliminated many of the problems previously encountered during Safety Basis (SB) document development. This process has been subsequently adopted for use by several Savannah River Site (SRS) facilities with similar results and expanded to support other analysis activities.
Date: April 13, 2007
Creator: Ortner, T & Mukesh Gupta, M
System: The UNT Digital Library
Efficient Schemes for Reducing Numerical Dispersion in ModelingMultiphase Transport through Porous and Fractured Media (open access)

Efficient Schemes for Reducing Numerical Dispersion in ModelingMultiphase Transport through Porous and Fractured Media

Numerical issues with modeling transport of chemicals or solute in realistic large-scale subsurface systems have been a serious concern, even with the continual progress made in both simulation algorithms and computer hardware in the past few decades. The problem remains and becomes even more difficult when dealing with chemical transport in a multiphase flow system using coarse, multidimensional regular or irregular grids, because of the known effects of numerical dispersion associated with moving plume fronts. We have investigated several total-variation-diminishing (TVD) or flux-limiter schemes by implementing and testing them in the T2R3D code, one of the TOUGH2 family of codes. The objectives of this paper are (1) to investigate the possibility of applying these TVD schemes, using multi-dimensional irregular unstructured grids, and (2) to help select more accurate spatial averaging methods for simulating chemical transport given a numerical grid or spatial discretization. We present an application example to show that such TVD schemes are able to effectively reduce numerical dispersion.
Date: April 13, 2006
Creator: Wu, Yu-Shu & Forsyth, Peter A.
System: The UNT Digital Library
Compact High-Current Heavy-Ion Injector (open access)

Compact High-Current Heavy-Ion Injector

To provide a compact high-brightness heavy-ion beam source for Heavy Ion Fusion (HIF), we have been experimenting with merging multi-beamlets in an injector which uses an RF plasma source. An array of converging beamlets was use to produce a beam with the envelope radius, convergence, and ellipticity matched to an electrostatic quadrupole (ESQ) channel. Experimental results were in good quantitative agreement with simulation and have demonstrated the feasibility of this concept. The size of a driver-scale injector system using this approach will be several times smaller than one designed using traditional single large-aperture beams. The success of this experiment has possible significant economical and technical impacts on the architecture of HIF drivers.
Date: April 13, 2006
Creator: Westenskow, G A; Grote, D P; Kwan, J W & Bieniosek, F
System: The UNT Digital Library
Topographic and Structural Effects on Dike Propagation and Eruption (open access)

Topographic and Structural Effects on Dike Propagation and Eruption

We have modeled magma flow in a dike rising in a crack whose strike runs from a highland or ridge to an adjacent lowland to determine the effect of topography on the flow, using a 3D hydromechanical code, FLAC3D (http://www.itascacg.com). The aperture, a, is calculated as a variable in a sheet of zones of fixed width d during the simulation as a function of model deformation. The permeability tensor of each zone is adjusted at each time step in response to the pressure in the cell according to the relationship k{sub ij} = {delta}{sub ij} {alpha}{sup 3}/12{mu}d, which is obtained by equating the flow through the layer of permeable zones from Darcy's law with Poiseuille's law under the same gradient. The fluid viscosity is {mu}, and the crack width is a We found a distinct tendency for the flow to be diverted away from the highland end of the strike toward the lowland. For the 4-km long strike length we modeled, eruption was offset between 500 and 1250 m toward the lowland from the center of the strike length. Separation of the geometric effect of the topography from the topographic overburden effect on lateral confining stresses at the crack indicates …
Date: April 13, 2006
Creator: Gaffney, E.
System: The UNT Digital Library
SOLID PHASE MICROEXTRACTION SAMPLING OF HIGH EXPLOSIVE RESIDUES IN THE PRESENCE OF RADIONUCLIDES AND RADIONUCLIDE SURROGATE METALS (open access)

SOLID PHASE MICROEXTRACTION SAMPLING OF HIGH EXPLOSIVE RESIDUES IN THE PRESENCE OF RADIONUCLIDES AND RADIONUCLIDE SURROGATE METALS

The Federal Bureau of Investigation (FBI) Laboratory currently does not have on site facilities for handling radioactive evidentiary materials and there are no established FBI methods or procedures for decontaminating high explosive (HE) evidence while maintaining evidentiary value. One experimental method for the isolation of HE residue involves using solid phase microextraction or SPME fibers to remove residue of interest. Due to their high affinity for organics, SPME fibers should have little affinity for most metals. However, no studies have measured the affinity of radionuclides for SPME fibers. The focus of this research was to examine the affinity of dissolved radionuclide ({sup 239/240}Pu, {sup 238}U, {sup 237}Np, {sup 85}Sr, {sup 133}Ba, {sup 137}Cs, {sup 60}Co and {sup 226}Ra) and stable radionuclide surrogate metals (Sr, Co, Ir, Re, Ni, Ba, Cs, Nb, Zr, Ru, and Nd) for SPME fibers at the exposure conditions that favor the uptake of HE residues. Our results from radiochemical and mass spectrometric analyses indicate these metals have little measurable affinity for these SPME fibers during conditions that are conducive to HE residue uptake with subsequent analysis by liquid or gas phase chromatography with mass spectrometric detection.
Date: April 13, 2007
Creator: Duff, M; S Crump, S; Robert02 Ray, R & Donna Beals, D
System: The UNT Digital Library
Proc. of the workshop on pushing the limits of RF superconductivity. (open access)

Proc. of the workshop on pushing the limits of RF superconductivity.

For three days in late September last year, some sixty experts in RF superconductivity from around the world came together at Argonne to discuss how to push the limits of RF superconductivity for particle accelerators. It was an intense workshop with in-depth presentations and ample discussions. There was added excitement due to the fact that, a few days before the workshop, the International Technology Recommendation Panel had decided in favor of superconducting technology for the International Linear Collider (ILC), the next major high-energy physics accelerator project. Superconducting RF technology is also important for other large accelerator projects that are either imminent or under active discussion at this time, such as the Rare Isotope Accelerator (RIA) for nuclear physics, energy recovery linacs (ERLs), and x-ray free-electron lasers. For these accelerators, the capability in maximum accelerating gradient and/or the Q value is essential to limit the length and/or operating cost of the accelerators. The technological progress of superconducting accelerators during the past two decades has been truly remarkable, both in low-frequency structures for acceleration of protons and ions as well as in high-frequency structures for electrons. The requirements of future accelerators demand an even higher level of performance. The topics of this …
Date: April 13, 2005
Creator: Kim, K-J., Eyberger, C., editors
System: The UNT Digital Library
Safeguards and Security Integration With Safety Analysis (open access)

Safeguards and Security Integration With Safety Analysis

The objective of this paper is to share the Savannah River Site lessons learned on Safeguards and Security (S&S) program integration with K-Area Complex (KAC) safety basis. The KAC Documented Safety Analysis (DSA), is managed by the Washington Savannah River Company (WSRC), and the S&S program, managed by Wackenhut Services, Incorporated--Savannah River Site (WSI-SRS). WSRC and WSI-SRS developed a contractual arrangement to recognize WSI-SRS requirements in the KAC safety analysis. Design Basis Threat 2003 (DBT03) security upgrades required physical modifications and operational changes which included the availability of weapons which could potentially impact the facility safety analysis. The KAC DSA did not previously require explicit linkage to the S&S program to satisfy the safety analysis. WSI-SRS have contractual requirements with the Department of Energy (DOE) which are separate from WSRC contract requirements. The lessons learned will include a discussion on planning, analysis, approval of the controls and implementation issues.
Date: April 13, 2007
Creator: Hearn, J. & James Lightner, J.
System: The UNT Digital Library
Tera-scalable Algorithms for Variable-Density Elliptic Hydrodynamics with Spectral Accuracy (open access)

Tera-scalable Algorithms for Variable-Density Elliptic Hydrodynamics with Spectral Accuracy

A hybrid spectral/compact solver for variable-density viscous incompressible flow is described. Parallelization strategies for the FFTs and band-diagonal matrices are discussed and compared. Transpose methods are found to be highly competitive with direct block parallel methods when the problem is scaled to tens of thousands of processors. Various mapping strategies for the IBM BlueGene/L torus configuration of processors are explored. By optimizing the communication, we have achieved virtually perfect scaling to 32768 nodes. Furthermore, communication rates come very close to the theoretical peak speed of the BlueGene/L network with sustained computation in the TeraFLOPS range.
Date: April 13, 2005
Creator: Cook, A. W.; Cabot, W. H.; Welcome, M. L.; Williams, P. L.; Miller, B. J.; de Supinski, B. R. et al.
System: The UNT Digital Library
Gamma motes for detection of radioactive materials in shipping containers (open access)

Gamma motes for detection of radioactive materials in shipping containers

Shipping containers can be effectively monitored for radiological materials using gamma (and neutron) motes in distributed mesh networks. The mote platform is ideal for collecting data for integration into operational management systems required for efficiently and transparently monitoring international trade. Significant reductions in size and power requirements have been achieved for room-temperature cadmium zinc telluride (CZT) gamma detectors. Miniaturization of radio modules and microcontroller units are paving the way for low-power, deeply-embedded, wireless sensor distributed mesh networks.
Date: April 13, 2007
Creator: McHugh, Harold; Quam, William; Weeks, Stephan & Sever, Brendan
System: The UNT Digital Library
Numerical simulation of leakage from a geologic disposal reservoirfor CO2, with transitions between super- and sub-criticalconditions (open access)

Numerical simulation of leakage from a geologic disposal reservoirfor CO2, with transitions between super- and sub-criticalconditions

The critical point of CO2 is at temperature and pressureconditions of Tcrit = 31.04oC, Pcrit = 73.82 bar. At lower (subcritical)temperatures and/or pressures, CO2 can exist in two different phases, aliquid and a gaseous state, as well as in two-phase mixtures of thesestates. Disposal of CO2 into brine formations would be made atsupercritical pressures. However, CO2 escaping from the storage reservoirmay migrate upwards towards regions with lower temperatures andpressures, where CO2 would be in subcritical conditions. An assessment ofthe fate of leaking CO2 requires a capability to model not onlysupercritical but also subcritical CO2, as well as phase changes betweenliquid and gaseous CO2 in sub-critical conditions. We have developed amethodology for numerically simulating the behavior of water-CO2 mixturesin permeable media under conditions that may include liquid, gaseous, andsupercritical CO2. This has been applied to simulations of leakage from adeep storage reservoir in which a rising CO2 plume undergoes transitionsfrom supercritical to subcritical conditions. We find strong coolingeffects when liquid CO2 rises to elevations where it begins to boil andevolve a gaseous CO2 phase. A three-phase zone forms (aqueous - liquid -gas), which over time becomes several hundred meters thick as decreasingtemperatures permit liquid CO2 to advance to shallower elevations. Fluidmobilities …
Date: April 13, 2003
Creator: Pruess, Karsten
System: The UNT Digital Library
Automatic registration of serial mammary gland sections (open access)

Automatic registration of serial mammary gland sections

We present two new methods for automatic registration of microscope images of consecutive tissue sections. They represent two possibilities for the first step in the 3-D reconstruction of histological structures from serially sectioned tissue blocks. The goal is to accurately align the sections in order to place every relevant shape contained in each image in front of its corresponding shape in the following section before detecting the structures of interest and rendering them in 3D. This is accomplished by finding the best rigid body transformation (translation and rotation) of the image being registered by maximizing a matching function based on the image content correlation. The first method makes use of the entire image information, whereas the second one uses only the information located at specific sites, as determined by the segmentation of the most relevant tissue structures. To reduce computing time, we use a multiresolution pyramidal approach that reaches the best registration transformation in increasing resolution steps. In each step, a subsampled version of the images is used. Both methods rely on a binary image which is a thresholded version of the Sobel gradients of the image (first method) or a set of boundaries manually or automatically obtained that define …
Date: April 13, 2004
Creator: Arganda-Carreras, Ignacio; Fernandez-Gonzalez, Rodrigo & Ortiz-de-Solorzano, Carlos
System: The UNT Digital Library
Anisotropic Ellipsoidal Smoothing of Volume Data (open access)

Anisotropic Ellipsoidal Smoothing of Volume Data

This paper describes a simple image processing algorithm for identifying and smoothing cell membranes in tomographic reconstructions of electron micrographs of frozen bacteria.
Date: April 13, 2005
Creator: Xue, Bai; Max, Nelson & Siegerist, Cristina
System: The UNT Digital Library
Electronic and Optical Properties of Energetic Particle-IrradiatedIn-rich InGaN (open access)

Electronic and Optical Properties of Energetic Particle-IrradiatedIn-rich InGaN

We have carried out a systematic study of the effects of irradiation on the electronic and optical properties of InGaN alloys over the entire composition range. High energy electrons, protons, and {sup 4}He{sup +} were used to produce displacement damage doses (D{sub d}) spanning over five orders of magnitude. The free electron concentrations in InN and In-rich InGaN increase with D{sub d} and finally saturate after a sufficiently high D{sub d}. The saturation of carrier density is attributed to the formation of native donors and the Fermi level pinning at the Fermi Stabilization Energy (E{sub FS}), as predicted by the amphoteric native defect model. Electrochemical capacitance-voltage (ECV) measurements reveal a surface electron accumulation whose concentration is determined by pinning at E{sub FS}.
Date: April 13, 2005
Creator: Li, S. X.; Yu, K. M.; Jones, R. E.; Wu, J.; Walukiewicz, W.; AgerIII, J. W. et al.
System: The UNT Digital Library
Effects of covalency on the p-shell photoemission of transition metals: MnO (open access)

Effects of covalency on the p-shell photoemission of transition metals: MnO

This article discusses the effects of covalency on the p-shell photoemission of transition metals. The treatment of covalency has not been included previously in ab initio theoretical studies of the 2p-shell XPS of transition-metal complexes. In this work, covalent interactions between the metal and ligands are treated on an equal footing with spin-orbit splittings.
Date: April 13, 2006
Creator: Bagus, Paul S. & Ilton, Eugene S.
System: The UNT Digital Library