Research conducted as part of the Comprehensive Cooling Water Study (CCWS) has elucidated many factors that are important to fish population and community dynamics in a variety of habitats on the Savannah River Plant (SRP). Information gained from these studies is useful in predicting fish responses to SRP operations. The overall objective of the CCWS was (1) to determine the environmental effects of SRP cooling water withdrawals and discharges and (2) to determine the significance of the cooling water impacts on the environment. The purpose of this study was to: (1) examine the effects of thermal plumes on anadromous and resident fishes, including overwintering effects, in the SRP swamp and associated tributary streams; (2) assess fish spawning and locate nursery grounds on the SRP; (3) examine the level of use of the SRP by spawning fish from the Savannah River, this objective was shared with the Savannah River Laboratory, E.I. du Pont de Nemours and Company; and (4) determine impacts of cooling-water discharges on fish population and community attributes. Five studies were designed to address the above topics. The specific objectives and a summary of the findings of each study are presented.

At the conclusion of polarized proton commissioning in February 1986, protons with an average polarization of 45%, momentum of 21.7 GeV/c, and intensity of 2 x 10/sup 10/ protons per pulse, were extracted to an external polarimeter at the Brookhaven AGS. In order to maintain this polarization, five intrinsic and nearly forty imperfection depolarizing resonances had to be corrected. An apparent interaction between imperfection and intrinsic resonances occurring at very nearly the same energy was observed and the correction of imperfection resonances using ''beat'' magnetic harmonics discovered in the previous AGS commissioning run was further confirmed.

Modeling of glass degradation based on sound geochemical principles appears to be possible with revisions to EQ3/6. Realistic source terms for several repository scenarios may be generated with such a model. One scenario which appears very likely and which is also amenable to modeling using EQ3/6 is that in which an intact but perforated canister holds water in contact with waste glass. The water overflows continuously or periodically, allowing radionuclides to come in contact with repository rock. This isolated-type scenario will be the first realistic modeling effort because it limits complex interactions between rock and glass. However, EQ3/6 modeling should be possible even for very complicated scenarios if sufficient experimental data are available on rates and thermodynamics. This will be the limiting factor in progress toward modeling the complete system.

This paper discusses preliminary estimates of the release of radionuclides from waste packages containing glass-based waste forms under the expected conditions at Yucca Mountain. These estimates can be used to evaluate the contribution of waste package performance toward meeting repository regulatory restrictions on radionuclide release. Glass waste will be held in double stainless steel canisters. After failure of the container sometime after the 300 to 1000 year containment period, the open headspace in these cans will provide the only area where standing water can accumulate and react with the glass. A maximum release rate of 0.177 g/m{sup 2} x year or 1.3 grams per year was obtained. Normalized loss of 1.3 grams per year corresponds to 0.08 parts in 100,000 per year of the 1660 kg reference weight of DWPF glass.

Enhanced security measures against external threats (e.g., terrorists, criminals) have been implemented at most facilities that handle special nuclear material, classified information, or other assets critical to national security. Attention is not focussing on insider protection, and safeguards managers are attempting to provide balanced protection against insider and outsider threats. Potential insider threats include attempts by facility employees to steal special nuclear material (SNM), to cause a radiological hazard to the public, to sabotage critical facilities, or to steal property or classified information. This paper presents a report card on the status of insider protection at Department of Energy and Nuclear Regulatory Commission-licensed facilities, with emphasis on SNM theft. We discuss the general trends in insider protection and the limitations of protection measures currently in use. We also discuss the most critical needs for improved procedures, technology, analytical tools, and education for safeguards personnel.

As protection of DOE facilities against outsiders increases to acceptable levels, attention is shifting toward achieving comparable protection against insiders. Since threats and protection measures for insiders are substantially different from those for outsiders, new perspectives and approaches are needed. One such approach is the Safeguards Evaluation Method. This method helps in assessing safeguards vulnerabilities to theft or diversion of special nuclear meterial (SNM) by insiders. The Safeguards Evaluation Method-Insider Threat is a simple model that can be used by safeguards and security planners to evaluate safeguards and proposed upgrades at their own facilities. The method is used to evaluate the effectiveness of safeguards in both timely detection (in time to prevent theft) and late detection (after-the-fact). The method considers the various types of potential insider adversaries working alone or in collusion with other insiders. The approach can be used for a wide variety of facilities with various quantities and forms of SNM. An Evaluation Workbook provides documentation of the baseline assessment; this simplifies subsequent on-site appraisals. Quantitative evaluation is facilitated by an accompanying computer program. The method significantly increases an evaluation team's on-site analytical capabilities, thereby producing a more thorough and accurate safeguards evaluation.

The fission cross sections of /sup 238/Pu have been measured from 0.1 eV to 80 keV energy range using the Rensselaer Intense Neutron Spectrometer. The cross sections were normalized to the /sup 235/U ENDF/B-V data broadened to the resolution of the Rensselaer Intense Neutron Spectrometer system. The fission areas and widths were determined for the resolved low-energy resonances. The ENDF/B-V fission cross sections for the /sup 238/Pu isotope are, in general, not in good agreement with the measured cross sections and a new evaluation is recommended. The observations of structure in the unresolved fission cross sections is suggestive of the existence of intermediate structure. 18 refs., 1 fig., 1 tab.

A bounce-averaged Monte Carlo operator is presented that simulates bounce-averaged perturbative Lorentz pitch angle scattering of particles in toroidal plasmas, in particular a tokamak. In conjunction with bounce-averaged expressions for the deterministic motion, this operator allows a quick and inexpensive simulation on time scales long compared to a bounce time. An analytically tractable model of transport due to toroidal magnetic field ripple is described.

There are several ways to introduce processability to conjugated polymers, and one of them is discussed here. The basic approach involves the introduction of flexible centers in a conjugated backbone with a periodicity that allows the existence of conjugated sequences characterized by an electron mobility high enough to result in electronic conduction upon oxidation or reduction. The process consists of the use of AsF/sub 5/ as a polymerization catalyst, and AsF/sub 3/ as a non-conventional medium for the reaction. The Lewis acid coupling reactions, via which the polymerization occurs, result in soluble materials. Characteristics of the materials obtained by polymerizing acetylene and some aromatic compounds are discussed.

The physical properties of polyacetylene diblock copolymers containing polystyrene (PS) or polyisoprene (PI) blocks of various compositions are studied using electron spin resonance, resonance Raman scattering, and room temperature conductivity measurements. This study is performed to investigate the processability-conductivity correlation in these materials and their viability as conducting systems.

Two expert programs currently under development at the Los Alamos National Laboratory, PROCON and the Designer's Apprentice, are briefly described. Both codes define interface to simulations that provide a wide variety of information about the performance of complex devices. (BCS)

A magnetron with a circular anode aperture and a spherical dimple in the cathode has been operated. With this configuration, a normalized emittance (90%) of 0.1..pi..cm-mrad has been measured in both planes for an H/sup -/ current of >50 mA. Other than this symmetric emittance, the source performance is the same as with the typical anode slit and grooved cathode.

A ring magnetron D/sup -/ charge exchange ionizer has been built and tested. An H/sup -/ current of 500 ..mu..A was extracted with an estimated H/sup 0/ density in the ionizer of 10/sup 12/ cm/sup -3/. This exceeds the performance of ionizers presently in use on polarized H/sup -/ sources. The ionizer will soon be tested with a polarized atomic beam.

The AGS polarized H/sup -/ source (PONI-1) now produces currents of 25-40 ..mu..A, and has operated reliably during polarized physics runs. A new polarized source, having as its goal mA's of H-vector, is now under development. An atomic hydrogen beam has been cooled to about 20 K with a forward flux of approx.10/sup 19/ atoms/s/sr. A superconducting solenoid having a calculated acceptance angle of 0.1 sr for the cold H/sup 0/ beam, is now being built. An ionizer for the resulting polarized H/sup 0/ beam based on resonant charge exchange of H/sup 0/ with D/sup -/, is being tested. 500 ..mu..A of H/sup -/ have been produced by ionizing an unpolarized H/sup 0/ beam using this ionizer.

The AGS polarized H/sup -/ source presently produces 30 to 40 ..mu..A of vector H/sup -/ in 500 ..mu..s pulses, with a polarization of 70-75%. The source operates reliably and has been used for polarized physics runs the past two years. There is now a development program in progress which has as its goal an operational vector H/sup -/ source producing milliamperes of current for the AGS.

Test results from a full-length prototype of the drift chamber vertex detector for the Mark II SLC Upgrade detector are presented. The 22 cell jet chamber employs planes of grid wires above and below the sense wire plane to increase the electrostatic stability of the sense wires and to narrow the electron arrival time distribution. Two different grid designs have been investigated. The spatial resolution and pulse widths have been measured at a variety of operating points and for different timing schemes in a mixture of 92% CO/sub 2/ and 8% isobutane. Typical results at 3 atmospheres pressure give an average resolution over a 2 cm drift distance of 30 ..mu..m for both designs. Efficient double track detection is achieved for tracks separated by 500 ..mu..m for one design and by 1000 ..mu..m for the other.

Separate abstracts have been prepared for each of the three included papers. (MOW)

The mid-infrared interstellar emission spectrum with features at 3050, 1610, 1300, 1150, and 885 cm/sup -1/ (3.28, 6.2, 7.7, 8.7 and 11.3 microns) is discussed in terms of the Polycyclic Aromatic Hydrocarbon (PAH) hypothesis. This hypothesis is based on the suggestive, but inconclusive comparison between the interstellar emission spectrum with the infrared absorption and Raman spectra of a few PAHs. The fundamental vibrations of PAHs and PAH-like species which determine the ir and Raman properties are discussed. Interstellar ir band emission is due to relaxation from highly vibrationally excited PAHs which have been excited by ultraviolet photons. The excitation/emission process is described in general and the ir fluorescence from one PAH, chrysene, is traced in detail. Generally, there is sufficient energy to populate several vibrational levels in each mode. Molecular vibrational potentials are anharmonic and emission from these higher levels will fall at lower frequencies and produce weak features to the red of the stronger fundamentals. This process is also described and can account for some spectroscopic details of the interstellar emission spectra previously unexplained. Analysis of the interstellar spectrum shows that PAHs containing between 20 and 30 carbon atoms are responsible for the emission. 43 refs., 11 figs.

PAHs can have several forms in the interstellar medium. To assess the importance of each requires the availability of a collection of high quality, complete mid-ir interstellar emission spectra, a collection of laboratory spectra of PAH samples prepared under realistic conditions and a firm understanding of the microscopic emission mechanism. Given what we currently know about PAHs, the spectroscopic data suggests that there are at least two components which contribute to the interstellar emission spectrum: free molecule sized PAHs producing the narrow features and amorphous carbon particles (which are primarily made up of an irregular ''lattice'' of PAHs) contributing to the broad underlying components. An exact treatment of the ir fluorescence from highly vibrationally excited large molecules shows that species containing between 20 and 30 carbon atoms are responsible for the narrow features, although the spectra match more closely with the spectra of amorphous carbon particles. Since little is known about the spectroscopic properties of free PAHs and PAH clusters, much laboratory work is called for in conjunction with an observational program which focuses on the spatial characteristics of the spectra. In this way the distribution and evolution of carbon from molecule to particle can be traced. 38 refs., 9 …

Results of a TEM investigation of the microstructural changes produced by the room temperature implantation of energetic Kr/sup +/ ions into a glassy Ti-Cr thin film are reported. As in other metals, the Kr precipitates as solid crystallites. The precipitation of crystalline Kr is accompanied by ultrafine crystallization of the metal host around each Kr crystal. With increasing fluence, the Kr precipitates grow to a critical size at which they melt, and the adjacent fine metal crystals disappear. A new TEM imaging technique is described briefly which utilizes the small angle electron scattering fine structure and which in principle is capable of revealing all fine particles simultaneously.

The EBR-II rotating plug seals require frequent cleaning and maintenance to keep the plugs from sticking during fuel handling. Time consuming cleaning on the cover gas and air sides of the dip ring seal is required to remove oxidation and sodium reaction products that accumulate and stop plug rotation. Despite severely limited access, effective seal cleaning techniques have removed 11 800 lb (5 352 kg) of deposits from the seals since 1964. Temperature control modifications and repairs have also required major maintenance work. Suggested seal design recommendations could significantly reduce maintenance on future similar seals.

To produce energies of over 50 GeV for SLC, all klystron stations on the accelerator are being upgraded to produce 250 MeV energy contribution per station. This involves installing new, higher power, longer pulse klystrons, upgrading klystron modulators to provide these higher voltage, longer klystron beam pulses, and a new interlock and protection system. A new VAX based diagnostic system including automated microwave measurements, klystron beam monitors, and modulator performance checks is being implemented. Figure 1 shows a block diagram of the klystron-modulator system. To date, over half of the new klystrons have been installed and tested, the modulator upgrade program has converted 22 sectors (8 stations each) of modulators out of 30, and a four sector sampling of klystrons has been run at full SLC specs, namely 350 kV beam voltage, 3.5 microsecond pulse duration, peak output power in excess of 60 MW, and PRF of 120 pps. This paper discusses the klystron design, modulator design, interlock and diagnostic systems, and the results of the initial operation.

Several diagnostics measure the particle sources and losses in the Tandem Mirror Experiment-Upgrade (TMX-U) plasma. An absolutely calibrated high-speed (0.5 ms per frame) filtered (6561 A) video camera measures the total ionization source as a function of radius. An axial view of the plasma automatically integrates the axial variations within the depth of field of the system. Another camera, viewing the plasma radially, measures the axial source variations near the deuterium fueling source. Axial ion losses are measured by an array of Faraday cups that are equipped with grids for repelling electrons and are mounted at each end of the experiment. Unequal ion and electron (nonambipolar) radial losses are inferred from net current measurements on an array of grounded plates at each end. Any differences between the measured particle losses and sources may be attributed to ambipolar radial losses and/or azimuthal asymmetries in the particle-loss profiles. Methods of system calibration, along with details of computer data acquisition and processing of this relatively large set of data, are also presented. 6 refs., 1 fig.

Some properties of emittance, emittance distributions, and measurement techniques are reviewed. In comparing the results of measurements with several different types of H/sup -/ sources with each other and with emittance formulae, it is concluded that the emittance of surface-type sources is dominated by the effective ion temperature. Other effects, such as ion-optical distortions, may account for the emittance of volume-type sources.