We show that bonded hydrogen in a-Si:H is readily exchanged by atomic deuterium when exposed to a deuterium plasma discharge. The effective diffusion coefficient for the D,H exchange 10/sup -14/ cm/sup 2//sec at 160/sup 0/C, is comparable to that of interstitial hydrogen in c-Si.

Results of a TEM investigation of the microstructural changes produced by the room temperature implantation of energetic Kr/sup +/ ions into a glassy Ti-Cr thin film are reported. As in other metals, the Kr precipitates as solid crystallites. The precipitation of crystalline Kr is accompanied by ultrafine crystallization of the metal host around each Kr crystal. With increasing fluence, the Kr precipitates grow to a critical size at which they melt, and the adjacent fine metal crystals disappear. A new TEM imaging technique is described briefly which utilizes the small angle electron scattering fine structure and which in principle is capable of revealing all fine particles simultaneously.

One of the questions that must be answered in assessing the potential of pulsed microwave beams as directed energy weapons is, ''What is the maximum pulse energy (and/or peak power) that can be delivered from a source to a target.'' Atmospheric breakdown caused by the electromagnetic fields of the pulse sets one limit on energy propagation, and the breakdown threshold was the subject of fairly extensive investigation a number of years ago. The evolution of microwave source technology has extended the parameter range over which propagation needs to be understood, and additional issues that have not previously been investigated experimentally have assumed a new importance. A new generation of experiments is underway, planned, or proposed to investigate these issues. 13 refs.

In 4f compounds, there is a two-peaked structure associated with 4f photoemission spectroscopy, while most 5f compounds yield a single broad triangular-shaped 5f intensity. Evidence is presented from measurements on ternary alloys that show that at least part of the extra-5f intensity is due to the hitherto missing main peak (or d-screened f-hole peak) just as in the 4f systems. The remaining intensity is consistent with a band structure DOS. (The compounds used were URh/sub 3/B/sub x/, UPd/sub x/Rh/sub 3-x/, ThBe/sub 13/, UIr/sub 3/, and UBe/sub 13/.) (DLC)

The roles of energetic displacement cascades are ubiquitous in the fields of radiation damage and ion beam modifications of materials. These roles can be described on two time scales. For the first, which lasts approx. =10/sup -11/ s, small cascade volumes are characterized by large supersaturations of point defects and energy densities in excess of some tenths of eV's per atom. During this period, the system can be driven far from equilibrium with significant rearrangement of target atoms and the production of Frenkel pairs. Studies of ion beam mixing in conjunction with molecular dynamics computer simulations, have contributed largely toward understanding these dynamic cascade processes. At later times, the microstructure of the material evolves as cascades begin to overlap, or at elevated temperatures, point defects migrate away from their nascent cascades. It is shown how the primary state of damage in cascades influences this microstructural development. Examples involving radiation enhanced diffusion and ion-induced amorphization are discussed. 40 refs.

The sodium pumps for a liquid metal fast breeder reactor must be designed for exceptionally high reliability and long life. The principal adverse factor which tends to limit the primary pump life is cavitation which becomes potentially severe under off-design flow conditions caused by the requirement of two loop operations which resulted in a large operating flow range. This problem prompted an extensive study which included experimental investigations of scaled down and full size pumps. The investigations involved visual observations, acoustic signature recordings, and physical characteristic measurements of the model and full size impellers. The blade configuration of the model was modified several times. After each modification intensive testing was conducted with feedback to established design criteria. The results obtained from the final configuration showed excellent cavitation performance. This configuration was then machined on the full scale impeller and tested. The results confirmed acceptable performance in the entire range of operating conditions. This paper describes the test facilities erected for this study, discusses the experimental techniques employed, and presents the experimental techniques employed, and presents a sample of the experimental results.

The infrared, optical and x-ray continua from radio quiet active galactic nuclei (AGN) are explained by a compact non-thermal source surrounding a thermal ultraviolet emitter, presumably the accretion disk around a supermassive black hole. The ultraviolet source is observed as the ''big blue bump.'' The flat (..cap alpha.. approx. = .7) hard x-ray spectrum results from the scattering of thermal ultraviolet photons by the flat, low energy end of an electron distribution ''broken'' by Compton losses; the infrared through soft x-ray continuum is the synchrotron radiation of the steep, high energy end of the electron distribution. Quantitative fits to specific AGN result in models which satisfy the variability constraints but require electron (re)acceleration throughout the source. 11 refs., 1 fig.

In this paper the wakefields for the Stanford Linear Accelerator Center (SLAC) accelerating structure are first discussed, and then some considerations dealing with the longitudinal wakefields are described. The main focus is on the effects of the transverse wakefield on the beam, including the case when there is an energy variation along the bunch. The use of an energy spread to inhibit emittance growth in a linac, indeed to damp the oscillations of the core of the bunch to below the unperturbed betatron oscillations, (in a process that is similar to Landau Damping) is qualitatively detailed. The example of the SLC, including errors, is also in detail.

Recent developments in high reliability components for linear induction accelerators (LIA) make possible the use of these devices as economical power drives for very high gradient linear colliders. A particularly attractive realization of this ''two-beam accelerator'' approach is to configure the LIA as a monolithic relativistic klystron operating at 10 to 12 GHz with induction cells providing periodic reacceleration of the high current beam. Based upon a recent engineering design of a state-of-the-art, 10- to 20-MeV LIA at Lawrence Livermore National Laboratory, this paper presents an algorithm for scaling the cost of the relativistic klystron to the parameter regime of interest for the next generation high energy physics machines. The algorithm allows optimization of the collider luminosity with respect to cost by varying the characteristics (pulse length, drive current, repetition rate, etc.) of the klystron. It also allows us to explore cost sensitivities as a guide to research strategies for developing advanced accelerator technologies.

A well characterized binary mixture of normal (protonated) and perdeuterated monodisperse 1,2 polybutenes has been studied by small-angle neutron scattering (SANS). For scattering wavevectors q greater than the inverse radius-of-gyration R/sub g//sup -1/, the SANS intensity is quantitatively predicted by the random phase approximation (RPA) theory of deGennes over all measured values of the segment-segment interaction parameter Chi. In the region (Chi s-Chi)Chi s/sup -1/ > 0.5 the interaction parameter determined using the RPA theory for q > R/sub g//sup -1/ is greater than that calculated from the zero-angle intensity based on an Ornstein-Zernike plot, where Chi s represents the limit of single phase stability. These findings indicate a correlation between the critical fluctuation length xi and R/sub g/ which is not accounted for by the RPA theory.

We present predictions for the rapidity and transverse momentum distributions for inclusive production of bottom quarks at SSC energies, pp ..-->.. bX. Our computations are based on the simplest, lowest-order QCD mechanisms. To estimate uncertainties, we use three different choices for structure functions, G(x,Q), as well as different choices for the evolution scale Q.

A goal of the LLNL Laser Pantography (LP) program has been demonstrating processes in which a computer-steered and computer-modulated laser beam directly deposits or removes material onto or from a substrate such as a silicon wafer. Substantial advantages could accrue from a fully developed set of such processes, including: lower cost for prototyping and low volume manufacturing, faster fabrication, on-line repair, and customized computers. 7 refs., 10 figs.

This paper describes the distribution and chemistry of zeolites in tuffs and in fractures at Yucca Mountain. Samples used in this study were collected from continuously-cored exploratory drill holes. A variety of analytical techniques, including optical petrography, x-ray powder diffraction, electron microanalysis, and x-ray fluorescence, were used to characterize the distribution and chemistry of zeolites in these samples.

Shock waves amplify pre-existing turbulence. Shock tube and shock wave boundary layer interaction experiments provide qualitative confirmation. However, shock pressure, temperature, and rapid transit complicate direct measurement. Computational simulations supplement the experimental data base and help isolate the mechanisms responsible. Simulations and experiments, particularly under reflected shock wave conditions, significantly influence material mixing. In these pseudospectral Navier-Stokes simulations the shock wave is treated as either a moving (tracked or fitted) domain boundary. The simulations assist development of code mix models. Shock Mach number and pre-existing turbulence intensity initially emerge as key parameters. 20 refs., 8 figs.

For many geologic problems, subsurface observations are available only from a small number of irregularly distributed locations, for example from a handful of drill holes in the region of interest. These observations will be interpolated one way or another, for example by hand-drawn stratigraphic cross-sections, by trend-fitting techniques, or by simple averaging which ignores spatial correlation. In this paper we consider an interpolation technique for such situations which provides, in addition to point estimates, the error estimates which are lacking from other ad hoc methods. The proposed estimator is like a kriging estimator in form, but because direct estimation of the spatial covariance function is not possible the parameters of the estimator are selected by cross-validation. Its use in estimating subsurface stratigraphy at a candidate site for geologic waste repository provides an example.

Yucca Mountain, in southern Nevada, is being studied by the Nevada Nuclear Waste Storage Investigations (NNWSI) Project as a potential site for an underground high-level nuclear waste repository. The site is within Miocene volcanic rocks that are 1.5 to 4 km thick and range in age from 12.5 to 14 MY. Several holes have been drilled in Yucca Mountain for geologic and hydrologic studies. Drill hole USW G-4, the most recently cored hole within the potential repository block, was chosen for detailed study of fracture-filling minerals because it is closest to the planned NNWSI exploratory shaft. Drill hole USW G-4 was drilled to 914.7 m (3001 ft) and continuously cored from 6.7 m (22 ft) to total depth (TD). The drilling history, lithology of the core, and geophysical logs of the well were published earlier. Because manganese oxides in fractures may act as a natural barrier to radionuclide migration, it is important to determine exactly which manganese minerals are present, in what intervals they occur, and how extensive these fracture coatings are.

A simulator of reactive chemical transport has been constructed with the capabilities of treating variable temperatures and variable oxidation potentials within a single simulation. Homogeneous and heterogeneous chemical reactions are simulated at temperature-dependent equilibrium, and changes of oxidation states of multivalent elements can be simulated during transport. Chemical mass action relations for formation of complexes in the fluid phase are included explicitly within the partial differential equations of transport, and a special algorithm greatly simplifies treatment of reversible precipitation of solid phases. This approach allows direct solution of the complete set of governing equations for concentrations of all aqueous species and solids affected simultaneously by chemical and physical processes. Results of example simulations of transport, along a temperature gradient, of uranium solution species under conditions of varying pH and oxidation potential and with reversible precipitation of uraninite and coffinite are presented. The examples illustrate how inclusion of variable temperature and oxidation potential in numerical simulators can enhance understanding of the chemical mechanisms affecting migration of multivalent waste elements.

In this paper we analyze the transport of radionuclides through penetrations in nuclear waste containers. Penetrations may result from corrosion or cracks and may occur in the original container material, in degraded or corroded material, or in deposits of corrosion products. We do not consider how these penetrations occur or the characteristics of expected penetrations in waste containers. We are concerned only with the analytical formulation and solutions of equations to predict rates of mass transfer through penetrations of specified size and geometry. Expressions for the diffusive mass transfer rates through apertures are presented. We present numerical illustrations for steady-state mass-transfer rates through a circular hole, including concentration isopleths. The results are extended to multiple holes, including a criterion for hole spacing wherein superposition of single-hole solutions can be used. Results illustrated for holes in thin-walled containers show that significant mass transfer can occur even if a small fraction of the container area is perforated. We also illustrate the case of holes facing a water gap, instead of being in intimate contact with porous rock. In this case the radionuclide flux from many small holes approaches that from a bare waste cylinder.

A model has been constructed in which a small droplet is exploded by the absorption of energy from a high energy laser beam. The beam flux is so high that it is assumed that a plasma is formed. A single-fluid model of a plasma droplet interacting with laser radiation is used. Selfsimilarity is invoked to reduce the spherically symmetric problem involving hydrodynamics and Maxwell's equations to quadrature. It is shown analytically that the model reproduces in qualitative manner certain features observed experimentally.

The weak decays of beauty hadrons offer a unique opportunity at the SSC to study CP violation in a system other than the neutral kaons and provides a long lever arm for searching for new physics if a strategy can be found for triggering on and identifying these decays. We have determined that the decay sequence B ..-->.. J/psi + X followed by the decay of the J/psi ..-->.. ..mu../sup +/..mu../sup -/ presents an opportunity to both trigger on and to unambiguously distinguish b anti b events from the total cross section events.

The Nevada Nuclear Waste Storage Investigations project has completed a series of experiments that provide insight into groundwater chemistry and glass waste form performance in the presence of a gamma radiation field at 90{sup 0}C. Results from experiments done at 1 x 10{sup 3} and O R/hr are presented and compared to similar experiments done at 2 x 10{sup 5} and 1 x 10{sup 4} R/hr. The major effect of radiation is to lower the groundwater pH to a value near 6.4. The addition of glass to the system results in slightly more basic final pH, both in the presence and absence of radiation. However, there is essentially no difference in the extent of glass reaction, as measured by elemental release, as a function of dose rate or total dose, for reaction periods up to 278 days.

Gigawatt level virtual cathode sources have been proposed for several applications. These include microwave weapons and drivers for high-energy particle accelerators. Both of these require a microwave source with very high power output that is controllable in frequency and phase. A conventional virtual cathode oscillator will not meet these requirements. The addition of a resonant cavity surrounding the oscillating virtual cathode either alone or pumped with a low-power injection signal, causing it to operate as an amplifier, could greatly influence the performance of this type of source making it more practical for accelerator and weapon applications. The progress on an experiment to test these concepts will be discussed.

This paper reviews the status of experimental data and data evaluations for charged-particle reactions of interest in fusion-reactor design. In particular, the /sup 2/H(t,..cap alpha..)n, /sup 2/H(d,p)/sup 3/H, /sup 2/H(d,/sup 3/He)n, /sup 3/H(t,..cap alpha..)nn and /sup 3/He(d,p)/sup 4/He reactions at low energies are studied. Other secondary reactions are considered. The conclusion is that such cross sections are well known for the near and medium term, and that no crucial experimental lack exists. There is a serious lack of standard evaluations of these reactions, which should be in an internationally acceptable format and easily accessible. Support for generating such evaluations should be given serious consideration.

We have demonstrated that absolute values of bone lead concentrations can be established from well-known physical constants. The correlation between EDTA test results and tibial lead measured by three different groups using three different methods is found, after normalization to common units, to lie on a common curve that, on average, shows the bone lead to be directly proportional to the EDTA results. It appears possible to improve the sensitivity and accuracy of the K x-ray determinations by improved data analysis programs and by increased source intensity and source-detector geometry changes. A present, the method appears capable of measuring lead concentrations at the 5-ppM (wet mass) level with uncertainties of +- 30 to 50% in 20 to 30 minutes measuring time. The uncertainties decrease at higher concentration levels. Measurements of the lead distribution in bone specimens by microscopic techniques would be useful in defining the relative merits of using K or L lead x rays in the measurements. 9 refs., 7 figs., 2 tabs.