Progress report for the Piqua Reactor Operations Analysis Program describing observations and analyses at the Piqua Nuclear Power Facility (PNPF). The program goals are to monitor operations and collect data in order to ensure that the plant's operation is safe, to improve design and performance, to evaluate the performance and lifetime of the plant's components and systems, to evaluate plant safety and safeguards, and to disseminate all information to the scientific community.

To improve gamma discrimination and eliminate d-c cable leakage interference currents, mean square voltage fluctuation measurements have been made on neutron sensitive ion chambers.

Abstract: Progress is reported in several areas of development of fueled graphite containing coated particles for nonurged gas-cooled reactor systems. The sol-gel process has been modified for making spherical particles of both thorium-uranium carbide and thorium-uranium oxide suitable for coating. Equipment has been assembled and methods have been developed for deposition of pyrolytic-carbon coating under well-controlled conditions. Damage to coated particles during fabrication into a graphite matrix depends on the molding pressure and the volumetric content of coated particles. Vendor-supplied coated particles and fueled graphite spheres have been evaluated extensively in both in- and out-of-reactor tests. Duplex- and triplex-coasted particles have excellent fission-gas retention at 2050 degree F to burnups of 15 at. % burnup. Fueled graphite spheres containing coated particles have good irradiation performance, but the fission-gas release rates are somewhat higher than for unsupported coated particles. Fueled graphite spheres react with water vapor about as rapidly as do Speer Mod-2 and ATJ grades of graphite. The diffusion rates in pyrolytic carbon are the same for uranium, thorium, and protactinium. The diffusion rates in the direction parallel to the deposition plane are much higher than those in the perpendicular direction.

Abstract: "The Oak Ridge National Laboratory proposes to build an isochronous eight-sector proton cyclotron to provide an extracted beam in excess of 100 A at 810 MeV. The primary proton beam and the secondary meson and neutron beams will be used to investigate nuclear structure, and the interactions between elementary particles. Biomedical and Space-oriented research programs are also planned. Shielded research areas and an extensive beam transport and analysis system are provided. Theoretical and experimental studies have shown that the Mc2 Cyclotron is a practical concept; high extraction efficiencies can be obtained, and the residual radiation problems are manageable. The project would require less than seven years to complete, and would cost about $43,000,000."

One-region buckling measurements that were made on a series of D/sub 2/O- moderated lattices of heavy uranium metal tubes in the Process Development Pile at Savannah River Laboratory are presented. The purposes of these measurements are to provide normalization points for lattice bucklings and to extend the study of natural uranium- D/sub 2/O systems. The dependence of buckiing on the moderator-to-fuel ratio is studied for two types of lattices.

The purpose of this paper is to describe a few of the suggested advanced concepts for fast breeder reactors and to compare these with the standard approach as to their potential advantage. I have attempted to estimate the economic effect of full technical success with each of the proposed concepts. The proposed concepts include: (1) single sodium system, (2) steam-cooled core concept, (3) direct cycle reactor using potassium as reactor coolant and working fluid, (4) molten plutonium-fuel alloy circulated and cooled by a jet of sodium, (5) settled-bed core, (6) molten salt concept, and (7) paste-fuel system.

From American Nuclear Society Meeting, New York, Nov. 1963. The use of the asymptotic solution to the one-velocity transport equation is considered. The angular distribution for fast neutron elastic scattering by heavy elements is discussed. An exponential angular distribution on is assumed to simplify the decay length calculation. The diffusion length of 1 to 15 Mev neutrons in iron is calculated, as well as the vector flux angular dependence. The asymptotic solution for an arbitrary angular distribution of a plane delta -function source is also found. An isotropic source is investigated, and some applications of the model are examined.

Technical report describing the statistically designed empirical approach being used to choose a candidate Zr alloy optimum with respect to corrosion and hydriding rates in steam and having acceptable mechanical properties. The statistical techniques used and the reasons for their use are discussed in detail, with emphasis on the estimation of corrosion rates. Estimation of response surfaces is also considered.

Abstract: A stainless steel clad 9-rod assembly fabricated by The Babcock & Wilcox Company was irradiated in a boiling water loop of the General Electric Test Reactor. A post-irradiation examination revealed no significant dimensional changes on the fuel rods. the results of mass spectrometric analysis made of the pelletized UO2 fuel indicated a maximum burnup of 11,500 MWD/tonne was attained by Rod B-4 during the exposure.An x-ray diffraction examination of an unirradiated fuel sample revealed the presence of UN2 and U2N3 phases. Metallographic examination of the irradiated microstructures revealed similar second-phase particles.

Technical report describing that as part of the AEC Fuel Cycle Program, tests are being conducted to evaluate the significance of current fuel design limitations that do not permit the maximum fuel temperature to exceed the melting point of UO2. The reliability of prediction of the fuel rod operating conditions that will cause melting of the UO2 was evaluated by means of a calibration test conducted in the Vallecitos Boiling Water Reactor. Conclusions: (a) The central portion of the 3.15-cm diameter uranium dioxide fuel column melted. It appears that the UO2 was molten to a radius of 1.22 cm in the peak power region. The maximum extent of melting probably occurred during the peak power run when the kdT in this region of the rod reached 171 watts cm. The estimated radius of melting from metallographic examination indicates the kdT for sintered UO2 is 89 watts/cm. This supports a calculated estimate for sintered UO2 thermal conductivity published by D. R. deHalas and G. R. Horn. The results of the previous calibration run and subsequent experimental data by Lyons are also consistent with the value. This conclusion is contingent on the interpretation of the post-irradiation crystal structure of the UO2. Insufficient …

Summary: Data on equlaxed UO2 grain growth from "out of pile" experiments have been gathered from all known sources and analyzed to determine the relationship between the grain size developed and annealing temperature and between grain size and the time at temperature. On the basis of the analysis, an equation relating gain size to time and temperate has been selected that appears to best describe the data considered as a whole. The coefficients in this grain growth equation have been evaluated to indicate the variance between different investigations and/or different UO2 sinters. The general applicability and limitations of "out of pile" grain growth data for the determination of temperatures in the microstructures of irradiated UO2 are discussed. Specific recommendations are made for the conditions under which grain size can be reliably employed as a temperature indicator. The objective in undertaking this analysis on UO2 grain growth was to obtain a working relationship between UO2 grain size and annealing time and/or temperature, and also a measure of the potential variation in the relationship. The intended use of the results was the determination of temperatures based on the grain sized observed in the post-irradiation metallographic examination of AEC-Euratom High Performance UO2 Program …

Abstract: A core design study of a 10 Mwe fast ceramic reactor is presented. Local reactivity coefficients, safety criteria, accident analyses, and economics are considered. An attempt is made to find a new balance of characteristics by purely geometric devices, i.e., by exploring the sodium : fuel ratio and varying the height : diameter ratio of the core. The use of BeO in the core was also investigated.

From introduction: "This is the seventeenth in a series of quarterly reports which cover the progress and results from the conceptual designs, economic evaluations and research and development work performed by the General Electric Company as part of Contract AT(01-3)-189, Project Agreement No. 13."

The influence of the Doppler effect in the core disassembly process following a meltdown accident is examined with a Bethe-Tait type model in which the Doppler effect, as well as core disassembly, is considered in the reactor shutdown process. It is shown that a strong negative Doppler effect can radically reduce the explosive energy release in such an accident. (auth)

A measurement of the yield of the aerated, ferrous sulfate-sulfuric acid (Fricke) dosimeter for 14.6-Mev neutrons gave a value of GF /sub Fe/sup +5/= 11.5 plus or minus 1.8. G/sub Fe/ number of ferric ions produced per 100 ev deposited. The determination combined an analysis of the energy deposit by scattering and charged particle reactions with a determination of the neutron flux by two independent means: (1) a "long counter" method and (2) an activation technique. The result is in reasonable agreement with a prediction for G/sub Fe// sup plus or minus 5/ based on measured yields of the dosimeter to irradiations by monoenergetic charged particles.

From American Nuclear Society Meeting, New York, Nov. 1963. The need for control of the flow distribution and/or steam quality in boiling reactors is discussed. A quality control device is being developed which consists of an entrance venturi and an exit venturi for measuring the flow rates into and out of the channel, means for comparing the two flow rate signals, and a value for regulating the flow rate. This device can be used either as a constant quality device or as a controlled-quality device. Results are given of air-water studies of two-phase flow in a vertical venturi.

Introduction. Under AEC contract the Martin Company has followed up the design and construction of the PM-1 and PM-3A nuclear power plants with R&D efforts seeking improved plant efficiency, increased core life and higher operating power. The Advanced PM cores have evolved step by step, with the addition of degrees of freedom to design latitude. A first replacement core, Core 2, has been designed to achieve 50 percent greater life than PM-1 through relatively minor design changes. Core 3 realizes the potential extensive modifications in the fuel element and control element configurations. This paper outlines an analysis effort undertaken to define what may be called a performance profile over a range of configurations of interest for Core 3. It should be emphasized that this is a parametric or concept study and not a final design effort. The results of this study clearly indicate that a lifetime of 100 Mw-yr can be obtained from a 7 ft pressurized water core. If employed as a 10-Mw heat source for present PM equipment, this core has a lifetime approaching that of the plant equipment, 90,000 full-power hours. Core 3 will be suitable for applications demanding up to 40-Mw operating thermal power.

At the Chemonuclear Workshop held at Brookhaven National laboratory in November 1962 it was pointed out that the production of ozone from oxygen by a liquid phase fission fragment chemonuclear process appears to have reasonable economic potential. The maximum theoretical reaction yield for the formation of ozone from oxygen is a "G" value of 68 molecules for 100 ev based on heat of reaction data. The authors felt a "G" value of 15 to be reasonable for this study. the reactor system chosen has liquid oxygen as its moderator and the operating pressure and temperature were selected so as to allow boiling of the oxygen-ozone mixture. The total plant investment cost is estimated to be in the range of $100,000,000. Other system designs will be considered in the future.

The effects of competition between resonances of different isotopes were investigated. Flux and reaction rate calculations on a Pu/sup 239/-- U/sup 238/ system revealed that U/sup 238/ exhibits both self-shielding and interference effects, the latter becoming noticeable at enrichment of a few per cent. Gold activation was also found to be depressed by the presence of U, but was insensitive at low enrichment values, Investigation of the Pu/sup 239/ resonance integral showed an asymmetric effect involving both interference between potential and resonant scattering and interference with resonance absorption in another isotope. The interference scattering arising in each resonance level had a notable effect on the average change in the Doppler coefficient. (D.C.W.)

Abstract: To assess diffusion's importance, the temperature distribution in a cylindrical reactor is derived for a coolant with uniform properties and velocity, taking into account both radial and axial diffusion, for a cosine-J0 power distribution. The fractional temperature rise of the coolant is found to be [chemical formula] where E(z) = [sin(z) + sin(Z)]/2 sin(Z), z= π x/2′, x is the axial distance from the core center, -H and ′ are the core half-height and extrapolated half-height, -H≤x≤H; Fn = 1/J0(Pn)·[(Pn/2.405P)2-10, J1(Pn) = 0, P= R/R′ = core radius/extrapolated radius, ρ = r/R, r = radial distance from axis, 0≤r≤R; an = = βnH/Z, 2 Aβn + 1 =[1 + 4αβ(Pn/R)2]½, A = axial diffusivity /u, B = radial diffusivity /u, u = coolant axial velocity, and [chemical formula]. The expression is evaluated for a variety of values for all the parameters, and the results are discussed analytically and presented in tables and graphs. The effect is dependent upon the relative size of the diffusion eddies in comparison with the dimensions of the reactor. The eddy diffusivity is proportional to the size of the particles in the bed and is about ten times larger axially than radially. A small core …

In fast reactor safety studies, it is imperative to know the effects of temperature excursions on the fuel elements. Previous controlled out-of-pile experiments on the behavior of uranium fuel elements under meltdown or near-meltdown conditions have been performed using direct electrical resistance heating or furnace heating. As a step toward obtaining more complete information on reactivity effects accompanying fuel meltdown, the behavior of irradiated EBR II and Fermi A samples under transient nuclear heating in TREAT has been studied. The experiment results obtained indicate that effects of prior irradiation can produce significant effects upon reactivity changes produced by meltdown of metallic fast reactor fuel pins.

An essential part of establishing the acceptability of warm extruded Zircaloy-4 for the CVTR pressure tube application was the determination of irradiation effects on mechanical properties of the alloy. Representative specimens were irradiated in low temperature process water in the WTR for simulated two, three and five year exposure. The effects of this irradiation were then evaluated in terms of changes in tensile, impact and creep properties. The experiment results concluded that the irradiation-induced changes in mechanical proprieties will not introduce any operational hazard to the CVTR pressure tube under anticipated operating conditions.

Abstract. The determination of the infinite multiplication factor, k∞ , from measurement son a small test sample was investigated by both theoretical and experimental techniques. Theoretical relations were developed to calculate the error in the measurement due to a mismatch between the flux ratios in the critical assembly and those of the test sample. Experiments were carried out at the Hanford Laboratory of the General Electric Company with the PCTR, to obtain values of the multiplication factor for comparison with the theoretical results. Calculations with two-group theory gave results that agreed with the experimental results when the test sample, with natural uranium fuel, was surrounded by a buffer region of the same material. When this buffer region was loaded with highly enriched fuel, the errors in the measured values were not predicted by the two-group theory. Three-group theory relations were derived which gave calculated values in agreement with the experimental values and indicated that a mismatch of the epithermal neutron group leads to the measured differences in the value of k∞ for the two buffer types.

This study is part of a research into trace element physiology of fresh water snails. As an average, biological materials contain [approximately] o.0% (fresh weight) NaCl ; this means [approximately] 3540 mg Na/1 (in snails, 0.4% NaCl [approximately] ms/1). Under these conditions, the application of neutron activation plus gamma spectrum analysis for the study of most trace elements as a routine method, is difficult. We will narrow down the scope some more and consider only the interference between Na24 and Cu64.