This procedure is intended to be used as: 1. An instruction and guide for operation of the KER loops. 2. To aid in familiarization and understanding of the general operation of the loops. 3. To prevent lost time due to errors in loop operation. The procedure is not meant to be completely comprehensive in all details of loop operation.

Absolute differential cross sections for the reaction p + p - w+ + d were obtained by detecting meson-deuteron coincidences produced by passing the 340-Mev external proton beam of the Berkeley synchro-cyclotron through a liquid hydrogen target.

This quarterly progress details ongoing research at the Oak Ridge National Laboratory as a part of the Aircraft Nuclear Propulsion Project. Topics discussed include reactor theory and design, [part two is not included], materials research, and appendixes with information on analytical chemical studies.

Document HW-33176, "A Proposed Scope of the 100-K Sulfuric Acid Addition Facilities", presented the justification and bases for a sulfuric acid addition facility at the 183-K headhouses and included a system for adding the acid to the raw water. Since the issue of this document several factors to consider in such a system have been brought to light by experience gained both at K and at other areas. The alternate system presented here eliminates several of the troublesome points in the previously proposed system.

The following report discusses findings resulting from experiments on recycled carbon tetrachloride at various stages of the proposed purification process.

Abstract: This report deals with the development of a method using tracer technique for determining uranium extraction coefficients on solutions of low uranium concentration. It was found that extraction coefficients could be determined on systems containing as low as one part per million uranium using 1900 level uranium as the tracer. Results of several extraction series are presented in which aluminum nitrate is used as the salting agent and dibutyl carbitol the organic extractant.

By radiation dosimetry, we will mean the determination of the energy deposited per unit mass of irradiated material by ionizing radiation. Usually the material of interest in tissue and the results are to be applied to a radiobiological experiment, a radiotherapy treatment, or the protection of personnel from radiation hazards. The same methods, however, are applied to such engineering problems as the production of heat by reactor radiations, the use of radiation in chemical reactions or food processing, etc.

Technical report outlining the plan to develop the Brookhaven chemonuclear in-pile test loop because the interest in utilizing reactor radiation energy (fission-fragment recoil and neutron-gamma) for production of chemicals has developed to the point where a loop to study chemonuclear system in a reactor under dynamic conditions is necessary.

Technical report outlining cavity-type ionization chambers with graphite walls that are used to measure heat dissipation in the graphite reflector of the MTR mock-up. Studies the relationship between the ionization occurring in the chamber and the heat generated in the surrounding graphite medium. [From Abstract]

From abstract: This investigation was conducted in order to develop a process whereby the most abundant zirconium ore, namely zircon, could economically be put into solution and purified adequately for use in hafnium separation processes employing liquid-liquid extraction. Secondary aims concerned the preparation of pure zirconyl chloride, zirconyl nitrate, zirconyl sulfate, and zirconium oxide from the zircon ore.

The following report analyzes results from studies made while applying chelating agents to ion exchange separations of the elements americium and curium.

The countercurrent gas-liquid system BF3(g)—anisole·BF3(l) for the concentration of boron isotopes has been studied. The single-storage separation factor varies from 1.039 at 0°C to 1.029 at 30°C. Rate of exchange is rapid, and, with efficient contacting equipment, complete exchange may be obtained in less than 15 sec. A total separation of 1.525 has been realized in laboratory equipment. The critical-product reflux reaction is quite efficient. Only about 55 moles of BF3 remain in each million moles of effluent solvent under laboratory conditions. The vapor pressure of BF3 over the complex rises sharply as the temperature is increased. At 0°C the pressure is 150 mm Hg, and at 40°C the pressure has risen to 1800 mm Hg. From vapor-pressure measurements, an approximate upper limit of ΔH= -12kcal per mole of complex was calculated for the reaction [equation not transcribed]. Qualitative tests indicate good resistance of anisole to decomposition by BF3 under plant conditions. The uncatalyzed exchange of boron between BF3 and BCl3 was found to be too slow to be exploited in a countercurrent system. The single-stage, equilibrium separation factor for the Nitrox system is a function of acid concentration. At 26°C the factor ranges from 1.064 with 1 M acid …

This report examines the "vitamin B12 binding capacity of leukocytes obtained from three normal subjects and 19 persons with various hematologic disorders."

From introduction: "In this report we consider a few non-adiabatic processes. The types to be discussed will be limited because of two reasons: first, complete descriptions are available for some processes; second, as time goes on alternative injection methods undoubtedly will be discovered, so this list must necessarily be incomplete."

The following report provides the results of laboratory corrosion tests held to investigate the behavior of austenitic stainless steel, Type 347, in selected O.R.N.L. #1 Redox streams.

The corrosion resistance of four types of austenitic stainless steels to Purex process first and second acid concentrator bottoms was determined. Although the compositions of the two solutions were very similar, tests in simulated solutions of both compositions were conducted to strengthen the basis for the conclusions which were to be made.

The crystal structures of the normal fatty acids of low molecular weight have been rather neglected until recently. Formic acid and acetic acid occur in the solid as hydrogen-bonded linear polymers, while several acids with eleven or more carbon atoms per molecule exist in the solid as dimers. The melting points of these acids, when plotted against number of carbon atoms, fall on two rather similar curves for even and odd numbers of carbon atoms, respectively, each with a minimum near five carbon atoms. These facts and hope of explaining the melting-point behavior led us to examine the structures of propionic and butyric acid crystals. These crystals have different structures, but both contain dimers.

Apparent [Sigma] hyperon decay events in a large emulsion stack of 240 9" x 12" pellicles have been classified into those judged to have occurred at rest and those in flight. Of 36 decay events at rest, 21 secondaries were observed to be protons of about 1675 microns range. Of the events decaying in flight, 23 were decays into protons and 46 were decays into near-minimum secondaries. Attempts have been made to trace the tracks of 35 of the lightly ionizing secondaries; the results of this effort are summarized in a table.

The following report describes results from a study of three types of cement (Barytes, Brookhaven, and Portland) exposed in the ORNL Reactor for periods of seven and twenty-eight days.

The Turco 4501 process is recommended for the decontamination of the PRFR pilot leaching plant equipment. The caustic-tartrate-nitric acid process is recommended for the decontamination of the cell and the equipment exterior.

Abstract: "A description of the demand computer and its functions is given. Methods of testing and adjusting, and gain and response curves for the system and its parts are included."

Abstract: "The effect of variation in fuel element density upon f, p in a D2O cooled and moderated lattice of cylindrical fuel elements is investigated. The CP-3 lattice is chosen as a reference. The effect of a source term in the fuel element is considered. f, p are calculated as functions of "a", the ratio of the modified fuel element density to the original (fuel only) density. Curves showing f(a), p(a) are included. It is concluded that a 1 per cent decrease in the product, f(d), p(a) is not suffered until a=0.3. A 5 per cent decrease in k is estimated at a-0.4. The necessity of introducing the fuel element source term into the calculation after a has been decreased to about 0.6 is brought out."

From abstract: "The effects of a number of substances that depress protoheme formation and affect free protoporphyrin production in duck erythrocytes in vitro were measured."

Quarterly progress report describing work related to a study of radiation physics problems involved in the design of high-level cesium-137 gamma sources. It outlines work completed and ongoing goals for the project.