This report describes progress in testing non-aqueous extraction methods for leaching Western ores of uranium and vanadium.

Abstract: "The accuracies which can be achieved in analog recording systems are for the most part tape limited. While reasonable variations in tape speed do not directly affect the accuracy, such variations result in improper tape tensioning, which in turn results in poor head-to-tape contact. The quality of the tape transport mechanism should be such that the error introduced by improper head- to tape contact is less than tape errors. Some additional equipment is necessary in setting up a tape recorder for a given experiment. The amplitude of the input pulse spectura to the recorder should be adjusted for optimum value and, if possible, the counting rate should be adjusted to obtain good tape utilization. An oscilloscope is probably adequate to satisfy both conditions."

From abstract: "Two samples, each containing an estimated 10 curies (2 mg) of polonium-210, were purified by vacuum distillation and evaporated onto oblique sections of X-ray targets made of copper. Four lines of the K series and ten lines of the L series of the X-ray spectrum of polonium were recorded with a one-meter transmission crystal spectrograph and a 25-centimeter Bragg spectrograph, respectively. Measured wavelengths agree approximately with values predicted by extrapolation of Moseley's law and with those claimed by Hulubei. Decay of polonium-210 (half life = 138 days) and growth of lead-206 (stable) were observed over a period of 180 days."

Report discussing a study regarding the time-dependent neutron flux for a pulsed subcritical assembly. From abstract: "A two-group analysis has been applied to the transient behavior of the thermal flux in a subcritical assembly which has been given a short burst of fast neutrons."

From introduction: "Analytical procedures for the determination of plutonium samples from the extraction and concentration plants utilize the carrying of the hydroxylamine-reduced trivulent plutonium by coprecipitation on lanthanum fluoride. Most other plutonium procedures also take advantage of the efficient carrying on lanthanum fluoride."

"This is a selected bibliography of books, journal articles and reports published on creep and relaxation in metals and ceramics from 1950 to March 1959. Particular attention has been paid to studies on or applicable to the consideration of creep and relaxation in beryllium oxide. Emphasis has alro been placed on studies of phenomenological materials behavior and high temperature studies."

None

The following report describes the results from studies based on the toxicity and metabolism of radioactive substances derived from uranium fission. Rats and mice were administered radioactive sodium and reactions and changes were studied.

This report follows an investigation on how hydrolysis products of tributyl phosphate (such as dibutyl and monobutyl phosphoric acids, orthophosphoric acid and butanol) effect the tributyl phosphate process for uranium recovery.

Work performed during the quarter is summarized by: direct measurement of fission gas pressure, loop operations, performance of UO2 fuel, UO2 grain growth and melting studies.

Report discussing a general introduction to heavy element chemistry.

Work performed during the quarter is summarized by direct measurement of fission gas pressure, loop operations, performance of UO2 fuel.

Introduction: The Transition Boiling Heat Transfer Program is sponsored jointly by the USAEC and Euroatom and is being conducted by the General Electric Company. The work commenced on this program February 11, 1963. The objective of this program is to perform basic investigation and measurement of the transition boiling regime in high pressure bulk boiling water flows, with particular emphasis i the high range of steam qualities.

The spontaneous fission rate of plutonium-240 has been redetermined and found to be 1.51 X 106 events/g/hr.

Technical report was prepared by the Health and Safety Laboratory (HASL) with the objective of presenting a current picture of the Strontium Program. Abstract: Strontium 90 levels in fallout, milk, canned fish and tap water are summarized for data available up to April 5, 1958. Original data submitted during the month of March are included as an appendix. Data are presented to show the amount of Strontium 90 in fallout at sampling stations within and outside the United States.

A research program is being conducted to obtain experimental data in the irradiation of plutonium-enriched fuel to confirm a theoretical model for predicting isotopic composition and reactivity changes in plutonium-enriched, light-water-moderated reactors. Quarterly progress: Work has begun in the Radioactive Materials Laboratory to sample the project fuel from the pins irradiated to 1800 and 5000 MWT/T. Some delay has been experienced due to preemption of the hot cells by priority work. Examination of the autoradiographs of the un-irradiated project fuel showed that in a volume of fuel approximately equivalent to a pellet there were 13 hot spots larger than 15 mils. Evaluation of these spots with the fuel analyzer showed that they contained about 14 mg of PuO2 or about 9% of the total present. The EPITHERMOS code is being modified to automatically normalize the epithermal scattering to the correct value for all moderators. Calibration of the flux wires has been made and the reduction of the data from the VBWR irradiation is nearly complete. A similar resonance activation was made in the water reflector of the Stanford Pool Reactor to obtain the relative activity in a well-defined pure water spectrum. Reduction of these data is also in progress.

From introduction: "Development of nuclear reactor cores having high power density, long fuel life, and low fabrication costs is the objective of this program sponsored by the AEC."

The ambient temperature of the Columbia River is of interest to the Aquatic Biology Operation since it provides a basis for controlling the temperatures in various experimental tanks which contain Columbia River organisms and since it provides some indication of whether conditions are favorable for the valuable species of fish living in the river. Since the start-up of the plant, temperatures of the river water have been taken in the several water treatment plants.

Basic Studies. It has been reported previously that mixed crystals of PuO2 and UO2 have a higher sintering rate than UO2 alone. However, results to the contrary were obtained on addition to 1/4, 1/2, 1, 2, 5, and 10 w/o PuO2 to PWR grade UO2. Pellets of the above concentrations were heated for one hour in hydrogen at 100 C intervals from 1000 to 1600C.

The Aircraft Reactor Experiment (ARE)was successfully concluded in November of 1954, and a detailed report of the operation was published the following year. At that time it was thought that an extensive examination of the reactor and system components after disassembly was warranted. It was realized, of course, that the level of radioactivity of the components would necessitate extensive delays in the examinations. Since examination of a few critical ARE samples showed nothing unexpected, much of the planned hot-cell inspection was postponed and complete examination of all but a few specimens was indefinitely suspended. The few examinations that were completed are described in this report, along with a description of the disassembly of the ARE system. Diagrams of the fuel system, sodium system, and off-gas system are presented in Figs. 1, 2, and 3 for reference use in visualizing the disassembly process.

A series of tests conducted in an attempt to reduce the observed O2 content of primary recirculation loop water to a value of <0.14ppm by the current loop method which is a combination of pressurizer degasification and venting flow.

Summary of miscellaneous updates related to the project. This includes information on the following: the declassification of a relevant paper, solubility measurements, static corrosion tests, various other tests involving bismuth, magnesium, uranium, protactinium, and thorium.

This is a report of work completed during the period January 1, 1962, to March 31, 1962. Work was done on fuel irradiation, activation studies and UO2 scattering experiment